Articles | Volume 19, issue 16
https://doi.org/10.5194/acp-19-10981-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-10981-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Relative importance of gas uptake on aerosol and ground surfaces characterized by equivalent uptake coefficients
Max Planck Institute for Chemistry, Mainz, 55118, Germany
now at: Chemical Science Division, Earth System Research
Laboratory, National Oceanic and Atmospheric Administration (NOAA), Boulder,
Colorado 80305, USA
Max Planck Institute for Chemistry, Mainz, 55118, Germany
Max Planck Institute for Chemistry, Mainz, 55118, Germany
Nan Ma
Center for Air Pollution and Climate Change Research (APCC),
Institute for Environmental and Climate Research (ECI), Jinan University,
Guangzhou, 511443, China
Ulrich Pöschl
Max Planck Institute for Chemistry, Mainz, 55118, Germany
Max Planck Institute for Chemistry, Mainz, 55118, Germany
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- Secondary Brown Carbon Aerosol Resists Bleaching by Ozone under Acidic Conditions K. Jansen et al. 10.1021/acs.jpca.4c02356
- The Significant Role of New Particle Composition and Morphology on the HNO3-Driven Growth of Particles down to Sub-10 nm Y. Li et al. 10.1021/acs.est.3c09454
- Multi-process atmospheric particle number size distribution over the Bohai Sea: Insights from cruise and onboard unmanned aerial vehicle observations Z. Liu et al. 10.1016/j.atmosenv.2024.120726
- Exploring dust heterogeneous chemistry over China: Insights from field observation and GEOS-Chem simulation R. Tian et al. 10.1016/j.scitotenv.2021.149307
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- Rapid hydrolysis of NO2 at High Ionic Strengths of Deliquesced Aerosol Particles M. Gen et al. 10.1021/acs.est.3c08810
- Contribution of Vehicle Emission and NO2 Surface Conversion to Nitrous Acid (HONO) in Urban Environments: Implications from Tests in a Tunnel S. Li et al. 10.1021/acs.est.1c00405
- A systematic review of reactive nitrogen simulations with chemical transport models in China H. Zhang et al. 10.1016/j.atmosres.2024.107586
- Dust-Dominated Coarse Particles as a Medium for Rapid Secondary Organic and Inorganic Aerosol Formation in Highly Polluted Air W. Xu et al. 10.1021/acs.est.0c07243
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- Differences in airborne stability of SARS-CoV-2 variants of concern is impacted by alkalinity of surrogates of respiratory aerosol A. Haddrell et al. 10.1098/rsif.2023.0062
- Improving the representation of HONO chemistry in CMAQ and examining its impact on haze over China S. Zhang et al. 10.5194/acp-21-15809-2021
- Modeling particulate nitrate in China: Current findings and future directions X. Xie et al. 10.1016/j.envint.2022.107369
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- Organic acid evaporation kinetics from aqueous aerosols: implications for aerosol buffering capacity in the atmosphere K. Angle et al. 10.1039/D2EA00092J
- The Impact of Agroecosystems on Nitrous Acid (HONO) Emissions during Spring and Autumn in the North China Plain J. Zeng et al. 10.3390/toxics12050331
- Nitrous acid budgets in the coastal atmosphere: potential daytime marine sources X. Zhong et al. 10.5194/acp-23-14761-2023
- Efficient Nitrate Formation in Fog Events Implicates Fog Interstitial Aerosols as Significant Drivers of Atmospheric Chemistry W. Xu et al. 10.1021/acs.est.4c09078
- The seasonal variations and potential sources of nitrous acid (HONO) in the rural North China Plain Y. Song et al. 10.1016/j.envpol.2022.119967
- Ozone Chemistry and Photochemistry at the Surface of Icelandic Volcanic Dust: Insights from Elemental Speciation Analysis M. Abou-Ghanem et al. 10.1021/acsearthspacechem.0c00363
- Emerging investigator series: ozone uptake by urban road dust and first evidence for chlorine activation during ozone uptake by agro-based anti-icer: implications for wintertime air quality in high-latitude urban environments M. Abou-Ghanem et al. 10.1039/D1EM00393C
- Kinetics study of heterogeneous reactions of O3 and SO2 with sea salt single droplets using micro-FTIR spectroscopy: Potential for formation of sulfate aerosol in atmospheric environment X. He & Y. Zhang 10.1016/j.saa.2020.118219
- New Multiphase Chemical Processes Influencing Atmospheric Aerosols, Air Quality, and Climate in the Anthropocene H. Su et al. 10.1021/acs.accounts.0c00246
- Extensive field evidence for the release of HONO from the photolysis of nitrate aerosols S. Andersen et al. 10.1126/sciadv.add6266
- Simultaneous formation of sulfate and nitrate via co-uptake of SO2 and NO2 by aqueous NaCl droplets: combined effect of nitrate photolysis and chlorine chemistry R. Zhang & C. Chan 10.5194/acp-23-6113-2023
Latest update: 09 Dec 2024
Short summary
Aerosols and the ground provide two kinds of surfaces for multiphase reactions in the planetary boundary layer. However, the relative importance of these two surfaces for gas uptake has not been quantified. We compare the uptake fluxes of aerosols and the ground surface for reactive trace gases under various conditions. More studies regarding O3 uptake on liquid organic aerosols and H2O2 uptakes on various aerosols are needed considering their potential important roles in atmospheric chemistry.
Aerosols and the ground provide two kinds of surfaces for multiphase reactions in the planetary...
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