Articles | Volume 19, issue 16
https://doi.org/10.5194/acp-19-10981-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-10981-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
29 Aug 2019
Research article |
| 29 Aug 2019
| 29 Aug 2019
Relative importance of gas uptake on aerosol and ground surfaces characterized by equivalent uptake coefficients
Max Planck Institute for Chemistry, Mainz, 55118, Germany
now at: Chemical Science Division, Earth System Research
Laboratory, National Oceanic and Atmospheric Administration (NOAA), Boulder,
Colorado 80305, USA
Max Planck Institute for Chemistry, Mainz, 55118, Germany
Max Planck Institute for Chemistry, Mainz, 55118, Germany
Nan Ma
Center for Air Pollution and Climate Change Research (APCC),
Institute for Environmental and Climate Research (ECI), Jinan University,
Guangzhou, 511443, China
Ulrich Pöschl
Max Planck Institute for Chemistry, Mainz, 55118, Germany
Max Planck Institute for Chemistry, Mainz, 55118, Germany
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- Urban aerosol chemistry at a land–water transition site during summer – Part 1: Impact of agricultural and industrial ammonia emissions N. Balasus et al. 10.5194/acp-21-13051-2021
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- Organic acid evaporation kinetics from aqueous aerosols: implications for aerosol buffering capacity in the atmosphere K. Angle et al. 10.1039/D2EA00092J
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- Ozone Chemistry and Photochemistry at the Surface of Icelandic Volcanic Dust: Insights from Elemental Speciation Analysis M. Abou-Ghanem et al. 10.1021/acsearthspacechem.0c00363
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- Emerging investigator series: ozone uptake by urban road dust and first evidence for chlorine activation during ozone uptake by agro-based anti-icer: implications for wintertime air quality in high-latitude urban environments M. Abou-Ghanem et al. 10.1039/D1EM00393C
- Kinetics study of heterogeneous reactions of O3 and SO2 with sea salt single droplets using micro-FTIR spectroscopy: Potential for formation of sulfate aerosol in atmospheric environment X. He & Y. Zhang 10.1016/j.saa.2020.118219
- New Multiphase Chemical Processes Influencing Atmospheric Aerosols, Air Quality, and Climate in the Anthropocene H. Su et al. 10.1021/acs.accounts.0c00246
- Extensive field evidence for the release of HONO from the photolysis of nitrate aerosols S. Andersen et al. 10.1126/sciadv.add6266
- Contribution of Vehicle Emission and NO2 Surface Conversion to Nitrous Acid (HONO) in Urban Environments: Implications from Tests in a Tunnel S. Li et al. 10.1021/acs.est.1c00405
- Simultaneous formation of sulfate and nitrate via co-uptake of SO2 and NO2 by aqueous NaCl droplets: combined effect of nitrate photolysis and chlorine chemistry R. Zhang & C. Chan 10.5194/acp-23-6113-2023
- Dust-Dominated Coarse Particles as a Medium for Rapid Secondary Organic and Inorganic Aerosol Formation in Highly Polluted Air W. Xu et al. 10.1021/acs.est.0c07243
- Investigating the sources of atmospheric nitrous acid (HONO) in the megacity of Beijing, China R. Gu et al. 10.1016/j.scitotenv.2021.152270
- Mixing state and distribution of iodine-containing particles in Arctic Ocean during summertime L. Wang et al. 10.1016/j.scitotenv.2022.155030
- Differences in airborne stability of SARS-CoV-2 variants of concern is impacted by alkalinity of surrogates of respiratory aerosol A. Haddrell et al. 10.1098/rsif.2023.0062
20 citations as recorded by crossref.
- Improving the representation of HONO chemistry in CMAQ and examining its impact on haze over China S. Zhang et al. 10.5194/acp-21-15809-2021
- Model bias in simulating major chemical components of PM<sub>2.5</sub> in China R. Miao et al. 10.5194/acp-20-12265-2020
- Primary sources of HONO vary during the daytime: Insights based on a field campaign D. Chen et al. 10.1016/j.scitotenv.2023.166605
- Urban aerosol chemistry at a land–water transition site during summer – Part 1: Impact of agricultural and industrial ammonia emissions N. Balasus et al. 10.5194/acp-21-13051-2021
- Modeling particulate nitrate in China: Current findings and future directions X. Xie et al. 10.1016/j.envint.2022.107369
- Organic acid evaporation kinetics from aqueous aerosols: implications for aerosol buffering capacity in the atmosphere K. Angle et al. 10.1039/D2EA00092J
- The seasonal variations and potential sources of nitrous acid (HONO) in the rural North China Plain Y. Song et al. 10.1016/j.envpol.2022.119967
- Exploring dust heterogeneous chemistry over China: Insights from field observation and GEOS-Chem simulation R. Tian et al. 10.1016/j.scitotenv.2021.149307
- Ozone Chemistry and Photochemistry at the Surface of Icelandic Volcanic Dust: Insights from Elemental Speciation Analysis M. Abou-Ghanem et al. 10.1021/acsearthspacechem.0c00363
- The Seasonal Variations and Potential Sources of Nitrous Acid (Hono) in the Rural North China Plain Y. Song et al. 10.2139/ssrn.4112814
- Emerging investigator series: ozone uptake by urban road dust and first evidence for chlorine activation during ozone uptake by agro-based anti-icer: implications for wintertime air quality in high-latitude urban environments M. Abou-Ghanem et al. 10.1039/D1EM00393C
- Kinetics study of heterogeneous reactions of O3 and SO2 with sea salt single droplets using micro-FTIR spectroscopy: Potential for formation of sulfate aerosol in atmospheric environment X. He & Y. Zhang 10.1016/j.saa.2020.118219
- New Multiphase Chemical Processes Influencing Atmospheric Aerosols, Air Quality, and Climate in the Anthropocene H. Su et al. 10.1021/acs.accounts.0c00246
- Extensive field evidence for the release of HONO from the photolysis of nitrate aerosols S. Andersen et al. 10.1126/sciadv.add6266
- Contribution of Vehicle Emission and NO2 Surface Conversion to Nitrous Acid (HONO) in Urban Environments: Implications from Tests in a Tunnel S. Li et al. 10.1021/acs.est.1c00405
- Simultaneous formation of sulfate and nitrate via co-uptake of SO2 and NO2 by aqueous NaCl droplets: combined effect of nitrate photolysis and chlorine chemistry R. Zhang & C. Chan 10.5194/acp-23-6113-2023
- Dust-Dominated Coarse Particles as a Medium for Rapid Secondary Organic and Inorganic Aerosol Formation in Highly Polluted Air W. Xu et al. 10.1021/acs.est.0c07243
- Investigating the sources of atmospheric nitrous acid (HONO) in the megacity of Beijing, China R. Gu et al. 10.1016/j.scitotenv.2021.152270
- Mixing state and distribution of iodine-containing particles in Arctic Ocean during summertime L. Wang et al. 10.1016/j.scitotenv.2022.155030
- Differences in airborne stability of SARS-CoV-2 variants of concern is impacted by alkalinity of surrogates of respiratory aerosol A. Haddrell et al. 10.1098/rsif.2023.0062
Latest update: 03 Dec 2023
Short summary
Aerosols and the ground provide two kinds of surfaces for multiphase reactions in the planetary boundary layer. However, the relative importance of these two surfaces for gas uptake has not been quantified. We compare the uptake fluxes of aerosols and the ground surface for reactive trace gases under various conditions. More studies regarding O3 uptake on liquid organic aerosols and H2O2 uptakes on various aerosols are needed considering their potential important roles in atmospheric chemistry.
Aerosols and the ground provide two kinds of surfaces for multiphase reactions in the planetary...
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