Articles | Volume 19, issue 15
https://doi.org/10.5194/acp-19-10405-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-10405-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
15 Aug 2019
Research article |
| 15 Aug 2019
| 15 Aug 2019
High contributions of fossil sources to more volatile organic aerosol
Haiyan Ni
Centre for Isotope Research (CIO), Energy and Sustainability Research Institute Groningen (ESRIG), University of Groningen, Groningen, 9747 AG, the Netherlands
State Key Laboratory of Loess and Quaternary Geology, Key Laboratory of Aerosol Chemistry and Physics, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an, 710061, China
CAS Center for Excellence in Quaternary Science and Global Change, Chinese Academy of Sciences, Xi'an, 710061, China
University of Chinese Academy of Sciences, Beijing, 100049, China
Ru-Jin Huang
CORRESPONDING AUTHOR
State Key Laboratory of Loess and Quaternary Geology, Key Laboratory of Aerosol Chemistry and Physics, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an, 710061, China
CAS Center for Excellence in Quaternary Science and Global Change, Chinese Academy of Sciences, Xi'an, 710061, China
Junji Cao
State Key Laboratory of Loess and Quaternary Geology, Key Laboratory of Aerosol Chemistry and Physics, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an, 710061, China
CAS Center for Excellence in Quaternary Science and Global Change, Chinese Academy of Sciences, Xi'an, 710061, China
Wenting Dai
State Key Laboratory of Loess and Quaternary Geology, Key Laboratory of Aerosol Chemistry and Physics, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an, 710061, China
CAS Center for Excellence in Quaternary Science and Global Change, Chinese Academy of Sciences, Xi'an, 710061, China
Jiamao Zhou
State Key Laboratory of Loess and Quaternary Geology, Key Laboratory of Aerosol Chemistry and Physics, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an, 710061, China
CAS Center for Excellence in Quaternary Science and Global Change, Chinese Academy of Sciences, Xi'an, 710061, China
Haoyue Deng
Centre for Isotope Research (CIO), Energy and Sustainability Research Institute Groningen (ESRIG), University of Groningen, Groningen, 9747 AG, the Netherlands
Anita Aerts-Bijma
Centre for Isotope Research (CIO), Energy and Sustainability Research Institute Groningen (ESRIG), University of Groningen, Groningen, 9747 AG, the Netherlands
Harro A. J. Meijer
Centre for Isotope Research (CIO), Energy and Sustainability Research Institute Groningen (ESRIG), University of Groningen, Groningen, 9747 AG, the Netherlands
Ulrike Dusek
Centre for Isotope Research (CIO), Energy and Sustainability Research Institute Groningen (ESRIG), University of Groningen, Groningen, 9747 AG, the Netherlands
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Cited
9 citations as recorded by crossref.
- Source apportionment of carbonaceous aerosols in Beijing with radiocarbon and organic tracers: insight into the differences between urban and rural sites S. Hou et al. 10.5194/acp-21-8273-2021
- Identifying the sources of PM2.5 at a COALESCE site in the Brahmaputra Valley Region using dispersion normalized PMF A. Qadri et al. 10.1016/j.atmosenv.2024.120501
- Seasonal characteristics of organic aerosol chemical composition and volatility in Stuttgart, Germany W. Huang et al. 10.5194/acp-19-11687-2019
- Variabilities of δ13C and carbonaceous components in ambient PM2.5 in Northeast India: Insights into sources and atmospheric processes A. Qadri et al. 10.1016/j.envres.2022.113801
- 13C signatures of aerosol organic and elemental carbon from major combustion sources in China compared to worldwide estimates P. Yao et al. 10.1016/j.scitotenv.2021.151284
- Organic aerosol volatility and viscosity in the North China Plain: contrast between summer and winter W. Xu et al. 10.5194/acp-21-5463-2021
- Measurement report: dual-carbon isotopic characterization of carbonaceous aerosol reveals different primary and secondary sources in Beijing and Xi'an during severe haze events H. Ni et al. 10.5194/acp-20-16041-2020
- Dual carbon isotope-based brown carbon aerosol characteristics at a high-altitude site in the northeastern Himalayas: Role of biomass burning M. Devaprasad et al. 10.1016/j.scitotenv.2023.169451
- Organic aerosol formation and aging processes in Beijing constrained by size-resolved measurements of radiocarbon and stable isotopic 13C H. Ni et al. 10.1016/j.envint.2021.106890
9 citations as recorded by crossref.
- Source apportionment of carbonaceous aerosols in Beijing with radiocarbon and organic tracers: insight into the differences between urban and rural sites S. Hou et al. 10.5194/acp-21-8273-2021
- Identifying the sources of PM2.5 at a COALESCE site in the Brahmaputra Valley Region using dispersion normalized PMF A. Qadri et al. 10.1016/j.atmosenv.2024.120501
- Seasonal characteristics of organic aerosol chemical composition and volatility in Stuttgart, Germany W. Huang et al. 10.5194/acp-19-11687-2019
- Variabilities of δ13C and carbonaceous components in ambient PM2.5 in Northeast India: Insights into sources and atmospheric processes A. Qadri et al. 10.1016/j.envres.2022.113801
- 13C signatures of aerosol organic and elemental carbon from major combustion sources in China compared to worldwide estimates P. Yao et al. 10.1016/j.scitotenv.2021.151284
- Organic aerosol volatility and viscosity in the North China Plain: contrast between summer and winter W. Xu et al. 10.5194/acp-21-5463-2021
- Measurement report: dual-carbon isotopic characterization of carbonaceous aerosol reveals different primary and secondary sources in Beijing and Xi'an during severe haze events H. Ni et al. 10.5194/acp-20-16041-2020
- Dual carbon isotope-based brown carbon aerosol characteristics at a high-altitude site in the northeastern Himalayas: Role of biomass burning M. Devaprasad et al. 10.1016/j.scitotenv.2023.169451
- Organic aerosol formation and aging processes in Beijing constrained by size-resolved measurements of radiocarbon and stable isotopic 13C H. Ni et al. 10.1016/j.envint.2021.106890
Latest update: 23 Nov 2024
Short summary
We apply radiocarbon source apportionment of more volatile organic carbon (mvOC) to winter aerosol samples from six Chinese cities. We find a consistently larger contribution of fossil sources to mvOC than to secondary or total organic carbon. Fossil mvOC concentrations are strongly correlated with primary fossil OC but not with secondary fossil OC. The variability in nonfossil mvOC seems to be related to both primary and secondary biomass burning sources.
We apply radiocarbon source apportionment of more volatile organic carbon (mvOC) to winter...
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