Articles | Volume 18, issue 13
https://doi.org/10.5194/acp-18-9845-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-9845-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
12 Jul 2018
Research article |
| 12 Jul 2018
| 12 Jul 2018
Morphological transformation of soot: investigation of microphysical processes during the condensation of sulfuric acid and limonene ozonolysis product vapors
Xiangyu Pei
Department of Chemistry and Molecular Biology, University of
Gothenburg, Gothenburg, 41296, Sweden
Mattias Hallquist
Department of Chemistry and Molecular Biology, University of
Gothenburg, Gothenburg, 41296, Sweden
Axel C. Eriksson
Division of Nuclear Physics, Department of Physics, Lund University,
Lund, 22100, Sweden
Ergonomics and Aerosol Technology, Lund University, Lund, 22100,
Sweden
Joakim Pagels
Ergonomics and Aerosol Technology, Lund University, Lund, 22100,
Sweden
Neil M. Donahue
Center for Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA 15213, USA
Thomas Mentel
Institute for Energy and Climate Research, IEK-8: Troposphere, Forschungszentrum Jülich, 52425 Jülich, Germany
Birgitta Svenningsson
Division of Nuclear Physics, Department of Physics, Lund University,
Lund, 22100, Sweden
William Brune
Department of Meteorology and Atmospheric Science, Pennsylvania State
University, University Park, PA 16802, USA
Ravi Kant Pathak
CORRESPONDING AUTHOR
Department of Chemistry and Molecular Biology, University of
Gothenburg, Gothenburg, 41296, Sweden
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- Absorption closure in highly aged biomass burning smoke J. Taylor et al. 10.5194/acp-20-11201-2020
- Investigation of RH effect on uncommon limonene ozonolysis products and SOA formation in indoor air with real time measurement techniques K. Pytel & B. Zabiegała 10.1016/j.chemosphere.2023.140854
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- Characterization, sources, and atmospheric transformation of a few key short-lived climate pollutants (SLCPs) at a rural super-site in the Indo-Gangetic Plain (IGP) of India J. Prakash et al. 10.1039/D1EA00083G
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- Characterization of Propane Fueled Flames: A Significant Source of Brown Carbon J. Prakash et al. 10.3390/atmos13081270
- Laboratory studies of ice nucleation onto bare and internally mixed soot–sulfuric acid particles K. Gao et al. 10.5194/acp-22-5331-2022
- Quantification and physical analysis of nanoparticle emissions from a marine engine using different fuels and a laboratory wet scrubber L. Santos et al. 10.1039/D2EM00054G
- Coated soot particles with tunable, well-controlled properties generated in the laboratory with a miniCAST BC and a micro smog chamber M. Ess et al. 10.1016/j.jaerosci.2021.105820
- Characterization of tandem aerosol classifiers for selecting particles: implication for eliminating the multiple charging effect Y. Song et al. 10.5194/amt-15-3513-2022
- A shape model of internally mixed soot particles derived from artificial surface tension H. Ishimoto et al. 10.5194/amt-12-107-2019
- Effect of organic coatings derived from the OH-initiated oxidation of amines on soot morphology and cloud activation C. Chen et al. 10.1016/j.atmosres.2020.104905
- Rapid transformation of ambient absorbing aerosols from West African biomass burning H. Wu et al. 10.5194/acp-21-9417-2021
- Coating material-dependent differences in modelled lidar-measurable quantities for heavily coated soot particles F. Kanngiesser & M. Kahnert 10.1364/OE.27.036368
- Mechanisms of soot-aggregate restructuring and compaction J. Corbin et al. 10.1080/02786826.2022.2137385
- A Review of the Representation of Aerosol Mixing State in Atmospheric Models R. Stevens & A. Dastoor 10.3390/atmos10040168
- Changes in CCN activity of ship exhaust particles induced by fuel sulfur content reduction and wet scrubbing L. Santos et al. 10.1039/D2EA00081D
- Quantifying the Fractal Dimension and Morphology of Individual Atmospheric Soot Aggregates Y. Pang et al. 10.1029/2021JD036055
- A review of measurement techniques for aerosol effective density L. Peng et al. 10.1016/j.scitotenv.2021.146248
- More Than Emissions and Chemistry: Fire Size, Dilution, and Background Aerosol Also Greatly Influence Near‐Field Biomass Burning Aerosol Aging A. Hodshire et al. 10.1029/2018JD029674
- Role of Secondary Organic Matter on Soot Particle Toxicity in Reconstituted Human Bronchial Epithelia Exposed at the Air–Liquid Interface Z. Leni et al. 10.1021/acs.est.2c03692
- Modelling optical properties of atmospheric black carbon aerosols M. Kahnert & F. Kanngießer 10.1016/j.jqsrt.2020.106849
- Intercomparison of equivalent black carbon (eBC) and elemental carbon (EC) concentrations with three-year continuous measurement in Beijing, China X. Liu et al. 10.1016/j.envres.2022.112791
- An optical soot sizing method without prior morphology parameters J. Zeng et al. 10.1016/j.combustflame.2024.113295
- Light scattering matrix for soot aerosol: Comparisons between experimental measurements and numerical simulations J. Liu et al. 10.1016/j.jqsrt.2020.106946
- Amplification of black carbon light absorption induced by atmospheric aging: temporal variation at seasonal and diel scales in urban Guangzhou J. Sun et al. 10.5194/acp-20-2445-2020
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Saved (final revised paper)
Latest update: 14 Dec 2024
Short summary
The findings in this study show that morphological transformation of soot occurs via two key complementary and sequential processes, i.e., void filling in the particle and its diameter growth. To quantify the state of morphological transformation, i.e., the utilization of material for filling and growth during the condensation processes, a framework was developed which can further be utilized to quantify the effect of condensed material on the optical and hygroscopic properties of soot.
The findings in this study show that morphological transformation of soot occurs via two key...
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