Articles | Volume 18, issue 13
https://doi.org/10.5194/acp-18-9845-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-9845-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Morphological transformation of soot: investigation of microphysical processes during the condensation of sulfuric acid and limonene ozonolysis product vapors
Xiangyu Pei
Department of Chemistry and Molecular Biology, University of
Gothenburg, Gothenburg, 41296, Sweden
Mattias Hallquist
Department of Chemistry and Molecular Biology, University of
Gothenburg, Gothenburg, 41296, Sweden
Axel C. Eriksson
Division of Nuclear Physics, Department of Physics, Lund University,
Lund, 22100, Sweden
Ergonomics and Aerosol Technology, Lund University, Lund, 22100,
Sweden
Joakim Pagels
Ergonomics and Aerosol Technology, Lund University, Lund, 22100,
Sweden
Neil M. Donahue
Center for Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA 15213, USA
Thomas Mentel
Institute for Energy and Climate Research, IEK-8: Troposphere, Forschungszentrum Jülich, 52425 Jülich, Germany
Birgitta Svenningsson
Division of Nuclear Physics, Department of Physics, Lund University,
Lund, 22100, Sweden
William Brune
Department of Meteorology and Atmospheric Science, Pennsylvania State
University, University Park, PA 16802, USA
Ravi Kant Pathak
CORRESPONDING AUTHOR
Department of Chemistry and Molecular Biology, University of
Gothenburg, Gothenburg, 41296, Sweden
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- More Than Emissions and Chemistry: Fire Size, Dilution, and Background Aerosol Also Greatly Influence Near‐Field Biomass Burning Aerosol Aging A. Hodshire et al. 10.1029/2018JD029674
- Role of Secondary Organic Matter on Soot Particle Toxicity in Reconstituted Human Bronchial Epithelia Exposed at the Air–Liquid Interface Z. Leni et al. 10.1021/acs.est.2c03692
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- Intercomparison of equivalent black carbon (eBC) and elemental carbon (EC) concentrations with three-year continuous measurement in Beijing, China X. Liu et al. 10.1016/j.envres.2022.112791
- An optical soot sizing method without prior morphology parameters J. Zeng et al. 10.1016/j.combustflame.2024.113295
- Light scattering matrix for soot aerosol: Comparisons between experimental measurements and numerical simulations J. Liu et al. 10.1016/j.jqsrt.2020.106946
- Amplification of black carbon light absorption induced by atmospheric aging: temporal variation at seasonal and diel scales in urban Guangzhou J. Sun et al. 10.5194/acp-20-2445-2020
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Saved (final revised paper)
Latest update: 16 Aug 2024
Short summary
The findings in this study show that morphological transformation of soot occurs via two key complementary and sequential processes, i.e., void filling in the particle and its diameter growth. To quantify the state of morphological transformation, i.e., the utilization of material for filling and growth during the condensation processes, a framework was developed which can further be utilized to quantify the effect of condensed material on the optical and hygroscopic properties of soot.
The findings in this study show that morphological transformation of soot occurs via two key...
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