Articles | Volume 18, issue 11
https://doi.org/10.5194/acp-18-7933-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-7933-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
06 Jun 2018
Research article |
| 06 Jun 2018
| 06 Jun 2018
High-resolution modeling of gaseous methylamines over a polluted region in China: source-dependent emissions and implications of spatial variations
Jingbo Mao
Shanghai Key Laboratory of Atmospheric Particle Pollution
and Prevention, Department of Environmental Science and Engineering,
Fudan University, Shanghai 200438, China
Institute of Atmospheric Sciences, Fudan University,
Shanghai 200438, China
Shanghai Key Laboratory of Atmospheric Particle Pollution
and Prevention, Department of Environmental Science and Engineering,
Fudan University, Shanghai 200438, China
Atmospheric Sciences Research Center, State University of
New York, 251 Fuller Road, Albany, New York 12203, USA
Yan Zhang
CORRESPONDING AUTHOR
Shanghai Key Laboratory of Atmospheric Particle Pollution
and Prevention, Department of Environmental Science and Engineering,
Fudan University, Shanghai 200438, China
Shanghai Institute of Eco-Chongming (SIEC), No.3663 Northern
Zhongshan Road, Shanghai 200062, China
Institute of Atmospheric Sciences, Fudan University,
Shanghai 200438, China
Data Institute for Carbon Emission and Environmental
Pollution, Fudan University, Shanghai 200433, China
Jingyu An
Shanghai Academy of Environmental Sciences, Shanghai 200233,
China
Shanghai Key Laboratory of Atmospheric Particle Pollution
and Prevention, Department of Environmental Science and Engineering,
Fudan University, Shanghai 200438, China
Jun Zheng
School of Environmental Science and Engineering, Nanjing
University of Information Science and Technology, Nanjing 210044,
China
Lei Yao
Shanghai Key Laboratory of Atmospheric Particle Pollution
and Prevention, Department of Environmental Science and Engineering,
Fudan University, Shanghai 200438, China
Atmospheric Sciences Research Center, State University of
New York, 251 Fuller Road, Albany, New York 12203, USA
Weichun Ma
Shanghai Key Laboratory of Atmospheric Particle Pollution
and Prevention, Department of Environmental Science and Engineering,
Fudan University, Shanghai 200438, China
Qi Yu
Shanghai Key Laboratory of Atmospheric Particle Pollution
and Prevention, Department of Environmental Science and Engineering,
Fudan University, Shanghai 200438, China
Cheng Huang
Shanghai Academy of Environmental Sciences, Shanghai 200233,
China
Shanghai Academy of Environmental Sciences, Shanghai 200233,
China
Limin Chen
Shanghai Key Laboratory of Atmospheric Particle Pollution
and Prevention, Department of Environmental Science and Engineering,
Fudan University, Shanghai 200438, China
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40 citations as recorded by crossref.
- Characterization of Particle Size Distributions and Water-Soluble Ions in Particulate Matter Measured at a Broiler Farm P. Silva et al. 10.3390/agriculture13071284
- Rapid sulfuric acid–dimethylamine nucleation enhanced by nitric acid in polluted regions L. Liu et al. 10.1073/pnas.2108384118
- Trimethylamine from Subtropical Forests Rival Total Farmland Emissions in China Y. Chang et al. 10.1021/acs.est.4c00622
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- Chemical composition and sources of amines in PM2.5 in an urban site of PRD, China S. Huang et al. 10.1016/j.envres.2022.113261
- Contribution of marine biological emissions to gaseous methylamines in the atmosphere: An emission inventory based on multi-source data sets Q. Zhang et al. 10.1016/j.scitotenv.2023.165285
- Influence of atmospheric conditions on sulfuric acid-dimethylamine-ammonia-based new particle formation H. Li et al. 10.1016/j.chemosphere.2019.125554
- Secondary Inorganic Ions Characteristics in PM2.5 Along Offshore and Coastal Areas of the Megacity Shanghai J. Sun et al. 10.1029/2021JD035139
- The atmospheric importance of methylamine additions to Criegee intermediates H. Mull et al. 10.1039/D0CP03781H
- A dynamic parameterization of sulfuric acid–dimethylamine nucleation and its application in three-dimensional modeling Y. Li et al. 10.5194/acp-23-8789-2023
- Large contributions of anthropogenic sources to amines in fine particles at a coastal area in northern China in winter Z. Liu et al. 10.1016/j.scitotenv.2022.156281
- Characteristics and sources of aerosol aminiums over the eastern coast of China: insights from the integrated observations in a coastal city, adjacent island and surrounding marginal seas S. Zhou et al. 10.5194/acp-19-10447-2019
- Photodissociation dynamics of methylamine in the blue edge of the A-band. II. The NH2 + CH3 channel J. Cachón et al. 10.1063/5.0159855
- Unexpected Catalytic Influence of Atmospheric Pollutants on the Formation of Environmentally Persistent Free Radicals L. Wang et al. 10.2139/ssrn.4054575
- Discovery of a Potent Source of Gaseous Amines in Urban China Y. Chang et al. 10.1021/acs.estlett.1c00229
- Nonagricultural emissions enhance dimethylamine and modulate urban atmospheric nucleation Y. Chang et al. 10.1016/j.scib.2023.05.033
- Piperazine Enhancing Sulfuric Acid-Based New Particle Formation: Implications for the Atmospheric Fate of Piperazine F. Ma et al. 10.1021/acs.est.9b02117
- Spatial Inhomogeneity of New Particle Formation in the Urban and Mountainous Atmospheres of the North China Plain during the 2022 Winter Olympics D. Shang et al. 10.3390/atmos14091395
- Quantum chemical modeling of atmospheric molecular clusters involving inorganic acids and methanesulfonic acid M. Engsvang et al. 10.1063/5.0152517
- Global variability in atmospheric new particle formation mechanisms B. Zhao et al. 10.1038/s41586-024-07547-1
- Intense formation of secondary ultrafine particles from Amazonian vegetation fires and their invigoration of deep clouds and precipitation M. Shrivastava et al. 10.1016/j.oneear.2024.05.015
- The catalytic effects of H2O, basic and acidic catalysts on the gas‐phase hydrolysis mechanism of carbonyl fluoride (CF2O) Y. Lu et al. 10.1002/qua.26657
- Atmospheric new particle formation in China B. Chu et al. 10.5194/acp-19-115-2019
- New particle formation (NPF) events in China urban clusters given by sever composite pollution background Q. Zhang et al. 10.1016/j.chemosphere.2020.127842
- Autoxidation mechanism for atmospheric oxidation of tertiary amines: Implications for secondary organic aerosol formation F. Ma et al. 10.1016/j.chemosphere.2020.129207
- Nitric Acid and Organic Acids Suppress the Role of Methanesulfonic Acid in Atmospheric New Particle Formation Y. Knattrup et al. 10.1021/acs.jpca.3c04393
- Spatial and temporal distribution characteristics and ozone formation potentials of volatile organic compounds from three typical functional areas in China H. Luo et al. 10.1016/j.envres.2020.109141
- Influence of atmospheric conditions on the role of trifluoroacetic acid in atmospheric sulfuric acid–dimethylamine nucleation L. Liu et al. 10.5194/acp-21-6221-2021
- Trifluoroacetaldehyde aminolysis catalyzed by a single water molecule: An important sink pathway for trifluoroacetaldehyde and a potential pathway for secondary organic aerosol growth Z. Dong et al. 10.1016/j.atmosenv.2021.118242
- Different characteristics and source contributions to aerosol aminiums over a coastal city and adjacent marginal seas Z. Xu et al. 10.1071/EN21070
- Competitive Uptake of Dimethylamine and Trimethylamine against Ammonia on Acidic Particles in Marine Atmospheres D. Chen et al. 10.1021/acs.est.1c08713
- Unexpected catalytic influence of atmospheric pollutants on the formation of environmentally persistent free radicals L. Wang et al. 10.1016/j.chemosphere.2022.134854
- OH Kinetics with a Range of Nitrogen-Containing Compounds: N-Methylformamide, t-Butylamine, and N-Methyl-propane Diamine T. Speak et al. 10.1021/acs.jpca.1c08104
- Mechanism and predictive model development of reaction rate constants for N-center radicals with O2 C. Liu et al. 10.1016/j.chemosphere.2019.124411
- Mapping gaseous dimethylamine, trimethylamine, ammonia, and their particulate counterparts in marine atmospheres of China's marginal seas – Part 1: Differentiating marine emission from continental transport D. Chen et al. 10.5194/acp-21-16413-2021
- Nonagricultural Emissions Dominate Urban Atmospheric Amines as Revealed by Mobile Measurements Y. Chang et al. 10.1029/2021GL097640
- Simulating the impacts of ship emissions on coastal air quality: Importance of a high-resolution emission inventory relative to cruise- and land-based observations J. Mao et al. 10.1016/j.scitotenv.2020.138454
- Computational chemistry of cluster: Understanding the mechanism of atmospheric new particle formation at the molecular level X. Zhang et al. 10.1016/j.chemosphere.2022.136109
- Reducing chemical complexity in representation of new-particle formation: evaluation of simplification approaches T. Olenius et al. 10.1039/D2EA00174H
Latest update: 20 Nov 2024
Short summary
A few pptv of gaseous amines have been observed to affect particle nucleation and growth, and it is necessary to understand the sources and concentrations of atmospheric amines. This study presents the source-dependent amines to ammonia emission ratios and simulates methylamines concentrations in a polluted region in China with WRF-Chem. The performance of simulations based on source-dependent ratios is much better than those based on fixed ratios that have been assumed in all previous studies.
A few pptv of gaseous amines have been observed to affect particle nucleation and growth, and it...
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