Articles | Volume 18, issue 10
https://doi.org/10.5194/acp-18-7669-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-7669-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
01 Jun 2018
Research article |
| 01 Jun 2018
| 01 Jun 2018
Strong impacts on aerosol indirect effects from historical oxidant changes
Inger Helene Hafsahl Karset
CORRESPONDING AUTHOR
University of Oslo, Department of Geosciences, Section for Meteorology and Oceanography, Oslo, Norway
Terje Koren Berntsen
University of Oslo, Department of Geosciences, Section for Meteorology and Oceanography, Oslo, Norway
CICERO Center for International Climate Research, Oslo, Norway
Trude Storelvmo
University of Oslo, Department of Geosciences, Section for Meteorology and Oceanography, Oslo, Norway
Kari Alterskjær
CICERO Center for International Climate Research, Oslo, Norway
Alf Grini
Norwegian Meteorological Institute, Oslo, Norway
Dirk Olivié
Norwegian Meteorological Institute, Oslo, Norway
Alf Kirkevåg
Norwegian Meteorological Institute, Oslo, Norway
Øyvind Seland
Norwegian Meteorological Institute, Oslo, Norway
Trond Iversen
Norwegian Meteorological Institute, Oslo, Norway
Michael Schulz
Norwegian Meteorological Institute, Oslo, Norway
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- Continued Rise in Health Burden from Ambient PM2.5 in India under SSP Scenarios Until 2100 despite Decreasing Concentrations Y. Wang et al. 10.1021/acs.est.4c02264
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- Implementing a sectional scheme for early aerosol growth from new particle formation in the Norwegian Earth System Model v2: comparison to observations and climate impacts S. Blichner et al. 10.5194/gmd-14-3335-2021
- Chemistry-albedo feedbacks offset up to a third of forestation’s CO 2 removal benefits J. Weber et al. 10.1126/science.adg6196
- Large difference in aerosol radiative effects from BVOC-SOA treatment in three Earth system models M. Sporre et al. 10.5194/acp-20-8953-2020
- Tropospheric ozone in CMIP6 simulations P. Griffiths et al. 10.5194/acp-21-4187-2021
- Evaluation of SO2, SO42− and an updated SO2 dry deposition parameterization in the United Kingdom Earth System Model C. Hardacre et al. 10.5194/acp-21-18465-2021
- Future tropospheric ozone budget and distribution over east Asia under a net-zero scenario X. Hou et al. 10.5194/acp-23-15395-2023
- Multidecadal increases in global tropospheric ozone derived from ozonesonde and surface site observations: can models reproduce ozone trends? A. Christiansen et al. 10.5194/acp-22-14751-2022
- On the Changing Role of the Stratosphere on the Tropospheric Ozone Budget: 1979–2010 P. Griffiths et al. 10.1029/2019GL086901
- Chemistry-driven changes strongly influence climate forcing from vegetation emissions J. Weber et al. 10.1038/s41467-022-34944-9
- BVOC–aerosol–climate feedbacks investigated using NorESM M. Sporre et al. 10.5194/acp-19-4763-2019
- Assessment of pre-industrial to present-day anthropogenic climate forcing in UKESM1 F. O'Connor et al. 10.5194/acp-21-1211-2021
- Apportionment of the Pre‐Industrial to Present‐Day Climate Forcing by Methane Using UKESM1: The Role of the Cloud Radiative Effect F. O’Connor et al. 10.1029/2022MS002991
- Atmospheric isoprene measurements reveal larger-than-expected Southern Ocean emissions V. Ferracci et al. 10.1038/s41467-024-46744-4
- Ozone air concentration trend attributes assist hours-ahead forecasts from univariate recorded data avoiding exogenous data inputs D. Wood 10.1016/j.uclim.2022.101382
- A production-tagged aerosol module for Earth system models, OsloAero5.3 – extensions and updates for CAM5.3-Oslo A. Kirkevåg et al. 10.5194/gmd-11-3945-2018
- Modelled surface climate response to effusive Icelandic volcanic eruptions: sensitivity to season and size T. Zoëga et al. 10.5194/acp-25-2989-2025
- Olfaction in the Anthropocene: NO 3 negatively affects floral scent and nocturnal pollination J. Chan et al. 10.1126/science.adi0858
- Atmospheric nanoparticle growth D. Stolzenburg et al. 10.1103/RevModPhys.95.045002
- Description and evaluation of aerosol in UKESM1 and HadGEM3-GC3.1 CMIP6 historical simulations J. Mulcahy et al. 10.5194/gmd-13-6383-2020
- Year-round measurement of atmospheric volatile organic compounds using sequential sampling in Dronning Maud Land, East-Antarctica P. Van Overmeiren et al. 10.1016/j.atmosenv.2023.120074
Saved (final revised paper)
Latest update: 14 Jul 2025
Short summary
This study highlights the role of oxidants in modeling of the preindustrial-to-present-day aerosol indirect effects. We argue that the aerosol precursor gases should be exposed to oxidants of its era to get a more correct representation of secondary aerosol formation. Our global model simulations show that the total aerosol indirect effect changes from −1.32 to −1.07 W m−2 when the precursor gases in the preindustrial simulation are exposed to preindustrial instead of present-day oxidants.
This study highlights the role of oxidants in modeling of the preindustrial-to-present-day...
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