Articles | Volume 18, issue 10
https://doi.org/10.5194/acp-18-7669-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-7669-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
01 Jun 2018
Research article |
| 01 Jun 2018
| 01 Jun 2018
Strong impacts on aerosol indirect effects from historical oxidant changes
Inger Helene Hafsahl Karset
CORRESPONDING AUTHOR
University of Oslo, Department of Geosciences, Section for Meteorology and Oceanography, Oslo, Norway
Terje Koren Berntsen
University of Oslo, Department of Geosciences, Section for Meteorology and Oceanography, Oslo, Norway
CICERO Center for International Climate Research, Oslo, Norway
Trude Storelvmo
University of Oslo, Department of Geosciences, Section for Meteorology and Oceanography, Oslo, Norway
Kari Alterskjær
CICERO Center for International Climate Research, Oslo, Norway
Alf Grini
Norwegian Meteorological Institute, Oslo, Norway
Dirk Olivié
Norwegian Meteorological Institute, Oslo, Norway
Alf Kirkevåg
Norwegian Meteorological Institute, Oslo, Norway
Øyvind Seland
Norwegian Meteorological Institute, Oslo, Norway
Trond Iversen
Norwegian Meteorological Institute, Oslo, Norway
Michael Schulz
Norwegian Meteorological Institute, Oslo, Norway
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- Evaluation of SO2, SO42− and an updated SO2 dry deposition parameterization in the United Kingdom Earth System Model C. Hardacre et al. 10.5194/acp-21-18465-2021
- Future tropospheric ozone budget and distribution over east Asia under a net-zero scenario X. Hou et al. 10.5194/acp-23-15395-2023
- Multidecadal increases in global tropospheric ozone derived from ozonesonde and surface site observations: can models reproduce ozone trends? A. Christiansen et al. 10.5194/acp-22-14751-2022
- On the Changing Role of the Stratosphere on the Tropospheric Ozone Budget: 1979–2010 P. Griffiths et al. 10.1029/2019GL086901
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- Description and evaluation of aerosol in UKESM1 and HadGEM3-GC3.1 CMIP6 historical simulations J. Mulcahy et al. 10.5194/gmd-13-6383-2020
- Year-round measurement of atmospheric volatile organic compounds using sequential sampling in Dronning Maud Land, East-Antarctica P. Van Overmeiren et al. 10.1016/j.atmosenv.2023.120074
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Saved (final revised paper)
Latest update: 29 Jul 2025
Short summary
This study highlights the role of oxidants in modeling of the preindustrial-to-present-day aerosol indirect effects. We argue that the aerosol precursor gases should be exposed to oxidants of its era to get a more correct representation of secondary aerosol formation. Our global model simulations show that the total aerosol indirect effect changes from −1.32 to −1.07 W m−2 when the precursor gases in the preindustrial simulation are exposed to preindustrial instead of present-day oxidants.
This study highlights the role of oxidants in modeling of the preindustrial-to-present-day...
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