Articles | Volume 18, issue 2
https://doi.org/10.5194/acp-18-635-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-635-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Exploring the observational constraints on the simulation of brown carbon
Department of Civil and Environmental Engineering, Massachusetts
Institute of Technology, Cambridge, MA, USA
now at: School of Engineering and Applied Sciences, Harvard
University, Cambridge, MA, USA
Colette L. Heald
Department of Civil and Environmental Engineering, Massachusetts
Institute of Technology, Cambridge, MA, USA
Department of Earth, Atmospheric and Planetary Sciences, Massachusetts
Institute of Technology, Cambridge, MA, USA
Jiumeng Liu
Atmospheric Sciences and Global Change Division, Pacific Northwest
National Laboratory, Richland, WA, USA
Rodney J. Weber
School of Earth and Atmospheric Sciences, Georgia Institute of
Technology, Atlanta, GA, USA
Pedro Campuzano-Jost
Department of Chemistry, University of Colorado Boulder, Boulder, CO,
USA
Cooperative Institute for Research in Environmental Sciences,
University of Colorado Boulder, Boulder, CO, USA
Jose L. Jimenez
Department of Chemistry, University of Colorado Boulder, Boulder, CO,
USA
Cooperative Institute for Research in Environmental Sciences,
University of Colorado Boulder, Boulder, CO, USA
Joshua P. Schwarz
Chemical Sciences Division, Earth System Research Laboratory, National
Oceanic and Atmospheric Administration, Boulder, CO, USA
Anne E. Perring
Cooperative Institute for Research in Environmental Sciences,
University of Colorado Boulder, Boulder, CO, USA
Chemical Sciences Division, Earth System Research Laboratory, National
Oceanic and Atmospheric Administration, Boulder, CO, USA
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- Seasonal variation of water-soluble brown carbon in Qingdao, China: Impacts from marine and terrestrial emissions Y. Zhan et al. 10.1016/j.envres.2022.113144
- Aging of Atmospheric Brown Carbon Aerosol R. Hems et al. 10.1021/acsearthspacechem.0c00346
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- Global Measurements of Brown Carbon and Estimated Direct Radiative Effects L. Zeng et al. 10.1029/2020GL088747
- The Direct Radiative Forcing Impact of Agriculture‐Emitted Black Carbon Associated With India's Green Revolution X. Liu et al. 10.1029/2021EF001975
- Photochemical evolution of the molecular composition of dissolved organic carbon and dissolved brown carbon from wood smoldering R. Zhao et al. 10.1016/j.envint.2024.108629
- Composition of Size-Resolved Aged Boreal Fire Aerosols: Brown Carbon, Biomass Burning Tracers, and Reduced Nitrogen R. Di Lorenzo et al. 10.1021/acsearthspacechem.7b00137
- Shortwave absorption by wildfire smoke dominated by dark brown carbon R. Chakrabarty et al. 10.1038/s41561-023-01237-9
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Latest update: 20 Nov 2024
Short summary
Brown carbon (BrC) contributes significantly to uncertainty in estimating the global direct radiative effect (DRE) of aerosols. We develop a global model simulation of BrC and test it against BrC absorption measurements from two aircraft campaigns in the continental United States. We suggest that BrC DRE has been overestimated previously due to the lack of observational constraints from direct measurements and omission of the effects of photochemical whitening.
Brown carbon (BrC) contributes significantly to uncertainty in estimating the global direct...
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