Articles | Volume 18, issue 2
https://doi.org/10.5194/acp-18-635-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-635-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
19 Jan 2018
Research article |
| 19 Jan 2018
Exploring the observational constraints on the simulation of brown carbon
Department of Civil and Environmental Engineering, Massachusetts
Institute of Technology, Cambridge, MA, USA
now at: School of Engineering and Applied Sciences, Harvard
University, Cambridge, MA, USA
Colette L. Heald
Department of Civil and Environmental Engineering, Massachusetts
Institute of Technology, Cambridge, MA, USA
Department of Earth, Atmospheric and Planetary Sciences, Massachusetts
Institute of Technology, Cambridge, MA, USA
Jiumeng Liu
Atmospheric Sciences and Global Change Division, Pacific Northwest
National Laboratory, Richland, WA, USA
Rodney J. Weber
School of Earth and Atmospheric Sciences, Georgia Institute of
Technology, Atlanta, GA, USA
Pedro Campuzano-Jost
Department of Chemistry, University of Colorado Boulder, Boulder, CO,
USA
Cooperative Institute for Research in Environmental Sciences,
University of Colorado Boulder, Boulder, CO, USA
Jose L. Jimenez
Department of Chemistry, University of Colorado Boulder, Boulder, CO,
USA
Cooperative Institute for Research in Environmental Sciences,
University of Colorado Boulder, Boulder, CO, USA
Joshua P. Schwarz
Chemical Sciences Division, Earth System Research Laboratory, National
Oceanic and Atmospheric Administration, Boulder, CO, USA
Anne E. Perring
Cooperative Institute for Research in Environmental Sciences,
University of Colorado Boulder, Boulder, CO, USA
Chemical Sciences Division, Earth System Research Laboratory, National
Oceanic and Atmospheric Administration, Boulder, CO, USA
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- Enhancement in Particulate Organic Nitrogen and Light Absorption of Humic-Like Substances over Tibetan Plateau Due to Long-Range Transported Biomass Burning Emissions Y. Wang et al. 10.1021/acs.est.9b06152
- Aqueous Photoreactions of Wood Smoke Brown Carbon R. Hems et al. 10.1021/acsearthspacechem.0c00117
- A Review of the Representation of Aerosol Mixing State in Atmospheric Models R. Stevens & A. Dastoor 10.3390/atmos10040168
- Impact of the Atmospheric Photochemical Evolution of the Organic Component of Biomass Burning Aerosol on Its Radiative Forcing Efficiency: A Box Model Analysis T. Zhuravleva et al. 10.3390/atmos12121555
Saved (final revised paper)
Latest update: 30 May 2023
Short summary
Brown carbon (BrC) contributes significantly to uncertainty in estimating the global direct radiative effect (DRE) of aerosols. We develop a global model simulation of BrC and test it against BrC absorption measurements from two aircraft campaigns in the continental United States. We suggest that BrC DRE has been overestimated previously due to the lack of observational constraints from direct measurements and omission of the effects of photochemical whitening.
Brown carbon (BrC) contributes significantly to uncertainty in estimating the global direct...
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