Articles | Volume 18, issue 9
https://doi.org/10.5194/acp-18-6187-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-6187-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Advanced source apportionment of carbonaceous aerosols by coupling offline AMS and radiocarbon size-segregated measurements over a nearly 2-year period
Athanasia Vlachou
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen
PSI, 5232, Switzerland
Kaspar R. Daellenbach
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen
PSI, 5232, Switzerland
Carlo Bozzetti
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen
PSI, 5232, Switzerland
Benjamin Chazeau
Aix-Marseille Université, CNRS, LCE, Marseille, France
Gary A. Salazar
Department of Chemistry and Biochemistry and Oeschger Centre for
Climate Change Research, University of Bern, 3012 Bern, Switzerland
Soenke Szidat
Department of Chemistry and Biochemistry and Oeschger Centre for
Climate Change Research, University of Bern, 3012 Bern, Switzerland
Jean-Luc Jaffrezo
Université Grenoble Alpes, CNRS, IRD, G-INP, IGE, 38000 Grenoble,
France
Christoph Hueglin
Swiss Federal Laboratories for Materials Science and Technology, Empa, 8600
Dübendorf, Switzerland
Urs Baltensperger
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen
PSI, 5232, Switzerland
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen
PSI, 5232, Switzerland
André S. H. Prévôt
CORRESPONDING AUTHOR
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen
PSI, 5232, Switzerland
Viewed
Total article views: 3,366 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 12 Dec 2017)
HTML | XML | Total | Supplement | BibTeX | EndNote | |
---|---|---|---|---|---|---|
2,041 | 1,225 | 100 | 3,366 | 442 | 69 | 98 |
- HTML: 2,041
- PDF: 1,225
- XML: 100
- Total: 3,366
- Supplement: 442
- BibTeX: 69
- EndNote: 98
Total article views: 2,758 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 03 May 2018)
HTML | XML | Total | Supplement | BibTeX | EndNote | |
---|---|---|---|---|---|---|
1,727 | 945 | 86 | 2,758 | 277 | 59 | 80 |
- HTML: 1,727
- PDF: 945
- XML: 86
- Total: 2,758
- Supplement: 277
- BibTeX: 59
- EndNote: 80
Total article views: 608 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 12 Dec 2017)
HTML | XML | Total | Supplement | BibTeX | EndNote | |
---|---|---|---|---|---|---|
314 | 280 | 14 | 608 | 165 | 10 | 18 |
- HTML: 314
- PDF: 280
- XML: 14
- Total: 608
- Supplement: 165
- BibTeX: 10
- EndNote: 18
Viewed (geographical distribution)
Total article views: 3,366 (including HTML, PDF, and XML)
Thereof 3,383 with geography defined
and -17 with unknown origin.
Total article views: 2,758 (including HTML, PDF, and XML)
Thereof 2,765 with geography defined
and -7 with unknown origin.
Total article views: 608 (including HTML, PDF, and XML)
Thereof 618 with geography defined
and -10 with unknown origin.
Country | # | Views | % |
---|
Country | # | Views | % |
---|
Country | # | Views | % |
---|
Total: | 0 |
HTML: | 0 |
PDF: | 0 |
XML: | 0 |
- 1
1
Total: | 0 |
HTML: | 0 |
PDF: | 0 |
XML: | 0 |
- 1
1
Total: | 0 |
HTML: | 0 |
PDF: | 0 |
XML: | 0 |
- 1
1
Cited
52 citations as recorded by crossref.
- Organic aerosol source apportionment in Zurich using an extractive electrospray ionization time-of-flight mass spectrometer (EESI-TOF-MS) – Part 1: Biogenic influences and day–night chemistry in summer G. Stefenelli et al. 10.5194/acp-19-14825-2019
- Radiocarbon isotope technique as a powerful tool in tracking anthropogenic emissions of carbonaceous air pollutants and greenhouse gases: A review G. Zhang et al. 10.1016/j.fmre.2021.03.007
- Indoor-outdoor relationship of submicron particulate matter in mechanically ventilated building: Chemical composition, sources and infiltration factor I. Garbarienė et al. 10.1016/j.buildenv.2022.109429
- Polyols and glucose particulate species as tracers of primary biogenic organic aerosols at 28 French sites A. Samaké et al. 10.5194/acp-19-3357-2019
- Organic aerosol sources in the Milan metropolitan area – Receptor modelling based on field observations and air quality modelling K. Daellenbach et al. 10.1016/j.atmosenv.2023.119799
- Development of a versatile source apportionment analysis based on positive matrix factorization: a case study of the seasonal variation of organic aerosol sources in Estonia A. Vlachou et al. 10.5194/acp-19-7279-2019
- A European aerosol phenomenology - 7: High-time resolution chemical characteristics of submicron particulate matter across Europe M. Bressi et al. 10.1016/j.aeaoa.2021.100108
- Is biomass burning always a dominant contributor of fine aerosols in upper northern Thailand? W. Song et al. 10.1016/j.envint.2022.107466
- Sources of particulate-matter air pollution and its oxidative potential in Europe K. Daellenbach et al. 10.1038/s41586-020-2902-8
- Contributions of fossil and non-fossil fractions to total carbon in urban aerosols in Bratislava (Slovakia) I. Kontul et al. 10.1016/j.jenvrad.2024.107512
- Organic aerosol source apportionment by using rolling positive matrix factorization: Application to a Mediterranean coastal city B. Chazeau et al. 10.1016/j.aeaoa.2022.100176
- Oxidative stress-induced inflammation in susceptible airways by anthropogenic aerosol Z. Leni et al. 10.1371/journal.pone.0233425
- Source Apportionment of Brown Carbon Absorption by Coupling Ultraviolet–Visible Spectroscopy with Aerosol Mass Spectrometry V. Moschos et al. 10.1021/acs.estlett.8b00118
- Time-dependent source apportionment of submicron organic aerosol for a rural site in an alpine valley using a rolling positive matrix factorisation (PMF) window G. Chen et al. 10.5194/acp-21-15081-2021
- Nonnegligible biogenic organic aerosol and the correlations with light absorption at three high altitude locations in the Qinghai–Tibetan Plateau C. Zhu et al. 10.1016/j.atmosenv.2022.119394
- Yields and molecular composition of gas-phase and secondary organic aerosol from the photooxidation of the volatile consumer product benzyl alcohol: formation of highly oxygenated and hydroxy nitro-aromatic compounds M. Jaoui et al. 10.5194/acp-23-4637-2023
- Source apportionment of fine particulate matter in a Middle Eastern Metropolis, Tehran-Iran, using PMF with organic and inorganic markers S. Esmaeilirad et al. 10.1016/j.scitotenv.2019.135330
- Indication of primary biogenic contribution to BrC over a high altitude location in the southeastern Tibet C. Zhu et al. 10.1016/j.atmosenv.2020.117462
- Comparison of five methodologies to apportion organic aerosol sources during a PM pollution event D. Srivastava et al. 10.1016/j.scitotenv.2020.143168
- Quantitative chemical assay of nanogram-level particulate matter using aerosol mass spectrometry: characterization of particles collected from uncrewed atmospheric measurement platforms C. Niedek et al. 10.5194/amt-16-955-2023
- Organic aerosol sources in Krakow, Poland, before implementation of a solid fuel residential heating ban R. Casotto et al. 10.1016/j.scitotenv.2022.158655
- Urban Oxidation Flow Reactor Measurements Reveal Significant Secondary Organic Aerosol Contributions from Volatile Emissions of Emerging Importance R. Shah et al. 10.1021/acs.est.9b06531
- Characterization of the PM2.5 aerosol fraction monitored at a suburban site in south-eastern Italy by integrating isotopic techniques and ion beam analysis S. Romano et al. 10.3389/fenvs.2022.971204
- Contribution of fossil and biomass-derived secondary organic carbon to winter water-soluble organic aerosols in Delhi, India H. Bhowmik et al. 10.1016/j.scitotenv.2023.168655
- Characterizing the Sources of Ambient PM10 Organic Aerosol in Urban and Rural Catalonia, Spain M. in 't Veld et al. 10.2139/ssrn.4463228
- Development of graphitization method for low carbon aerosol filter samples with Automated Graphitization System AGE-3 L. Butkus et al. 10.1016/j.apradiso.2022.110461
- An optimised organic carbon ∕ elemental carbon (OC ∕ EC) fraction separation method for radiocarbon source apportionment applied to low-loaded Arctic aerosol filters M. Rauber et al. 10.5194/amt-16-825-2023
- Source-specific light absorption by carbonaceous components in the complex aerosol matrix from yearly filter-based measurements V. Moschos et al. 10.5194/acp-21-12809-2021
- Atomic Spectrometry Update – a review of advances in environmental analysis J. Bacon et al. 10.1039/C8JA90044B
- Long-term sub-micrometer aerosol chemical composition in the boreal forest: inter- and intra-annual variability L. Heikkinen et al. 10.5194/acp-20-3151-2020
- Source apportionment of atmospheric PM<sub>10</sub> oxidative potential: synthesis of 15 year-round urban datasets in France S. Weber et al. 10.5194/acp-21-11353-2021
- Quantification of fossil and non-fossil sources to the reduction of carbonaceous aerosols in the Yangtze River Delta, China: Insights from radiocarbon analysis during 2014–2019 M. Yu et al. 10.1016/j.atmosenv.2022.119421
- A 1-year aerosol chemical speciation monitor (ACSM) source analysis of organic aerosol particle contributions from anthropogenic sources after long-range transport at the TROPOS research station Melpitz S. Atabakhsh et al. 10.5194/acp-23-6963-2023
- Impact of anthropogenic and biogenic sources on the seasonal variation in the molecular composition of urban organic aerosols: a field and laboratory study using ultra-high-resolution mass spectrometry K. Daellenbach et al. 10.5194/acp-19-5973-2019
- Complex plant-derived organic aerosol as ice-nucleating particles – more than the sums of their parts? I. Steinke et al. 10.5194/acp-20-11387-2020
- Characterisation of urban aerosol size distribution by radiocarbon and PIXE analyses in a middle-European urban environment for source identification: a pilot study A. Angyal et al. 10.1007/s11356-024-34215-8
- Abundant Biogenic Oxygenated Organic Aerosol in Atmospheric Coarse Particles: Plausible Sources and Atmospheric Implications X. Huang et al. 10.1021/acs.est.9b06311
- Accurate observation of black and brown carbon in atmospheric fine particles via a versatile aerosol concentration enrichment system (VACES) H. Kang et al. 10.1016/j.scitotenv.2022.155817
- Source apportionment of carbonaceous aerosols in Beijing with radiocarbon and organic tracers: insight into the differences between urban and rural sites S. Hou et al. 10.5194/acp-21-8273-2021
- Composition and Sources of Organic Aerosol in Two Megacities in Western China Using Complementary Mass Spectrometric and Statistical Techniques T. Cui et al. 10.1021/acsestair.4c00051
- Real-time measurement and source apportionment of elements in Delhi's atmosphere P. Rai et al. 10.1016/j.scitotenv.2020.140332
- Sources and formation of carbonaceous aerosols in Xi'an, China: primary emissions and secondary formation constrained by radiocarbon H. Ni et al. 10.5194/acp-19-15609-2019
- Development and evaluation of an improved offline aerosol mass spectrometry technique C. Vasilakopoulou et al. 10.5194/amt-16-2837-2023
- Chemical composition and sources of organic aerosol on the Adriatic coast in Croatia R. Casotto et al. 10.1016/j.aeaoa.2022.100159
- Local incomplete combustion emissions define the PM2.5 oxidative potential in Northern India D. Bhattu et al. 10.1038/s41467-024-47785-5
- Using highly time-resolved online mass spectrometry to examine biogenic and anthropogenic contributions to organic aerosol in Beijing A. Mehra et al. 10.1039/D0FD00080A
- A 1-year characterization of organic aerosol composition and sources using an extractive electrospray ionization time-of-flight mass spectrometer (EESI-TOF) L. Qi et al. 10.5194/acp-20-7875-2020
- Sources of organic aerosols in Europe: a modeling study using CAMx with modified volatility basis set scheme J. Jiang et al. 10.5194/acp-19-15247-2019
- A comprehensive characterization of ice nucleation by three different types of cellulose particles immersed in water N. Hiranuma et al. 10.5194/acp-19-4823-2019
- Arabitol, mannitol, and glucose as tracers of primary biogenic organic aerosol: the influence of environmental factors on ambient air concentrations and spatial distribution over France A. Samaké et al. 10.5194/acp-19-11013-2019
- Characterizing the sources of ambient PM10 organic aerosol in urban and rural Catalonia, Spain M. in 't Veld et al. 10.1016/j.scitotenv.2023.166440
- Insights into organic-aerosol sources via a novel laser-desorption/ionization mass spectrometry technique applied to one year of PM<sub>10</sub> samples from nine sites in central Europe K. Daellenbach et al. 10.5194/acp-18-2155-2018
51 citations as recorded by crossref.
- Organic aerosol source apportionment in Zurich using an extractive electrospray ionization time-of-flight mass spectrometer (EESI-TOF-MS) – Part 1: Biogenic influences and day–night chemistry in summer G. Stefenelli et al. 10.5194/acp-19-14825-2019
- Radiocarbon isotope technique as a powerful tool in tracking anthropogenic emissions of carbonaceous air pollutants and greenhouse gases: A review G. Zhang et al. 10.1016/j.fmre.2021.03.007
- Indoor-outdoor relationship of submicron particulate matter in mechanically ventilated building: Chemical composition, sources and infiltration factor I. Garbarienė et al. 10.1016/j.buildenv.2022.109429
- Polyols and glucose particulate species as tracers of primary biogenic organic aerosols at 28 French sites A. Samaké et al. 10.5194/acp-19-3357-2019
- Organic aerosol sources in the Milan metropolitan area – Receptor modelling based on field observations and air quality modelling K. Daellenbach et al. 10.1016/j.atmosenv.2023.119799
- Development of a versatile source apportionment analysis based on positive matrix factorization: a case study of the seasonal variation of organic aerosol sources in Estonia A. Vlachou et al. 10.5194/acp-19-7279-2019
- A European aerosol phenomenology - 7: High-time resolution chemical characteristics of submicron particulate matter across Europe M. Bressi et al. 10.1016/j.aeaoa.2021.100108
- Is biomass burning always a dominant contributor of fine aerosols in upper northern Thailand? W. Song et al. 10.1016/j.envint.2022.107466
- Sources of particulate-matter air pollution and its oxidative potential in Europe K. Daellenbach et al. 10.1038/s41586-020-2902-8
- Contributions of fossil and non-fossil fractions to total carbon in urban aerosols in Bratislava (Slovakia) I. Kontul et al. 10.1016/j.jenvrad.2024.107512
- Organic aerosol source apportionment by using rolling positive matrix factorization: Application to a Mediterranean coastal city B. Chazeau et al. 10.1016/j.aeaoa.2022.100176
- Oxidative stress-induced inflammation in susceptible airways by anthropogenic aerosol Z. Leni et al. 10.1371/journal.pone.0233425
- Source Apportionment of Brown Carbon Absorption by Coupling Ultraviolet–Visible Spectroscopy with Aerosol Mass Spectrometry V. Moschos et al. 10.1021/acs.estlett.8b00118
- Time-dependent source apportionment of submicron organic aerosol for a rural site in an alpine valley using a rolling positive matrix factorisation (PMF) window G. Chen et al. 10.5194/acp-21-15081-2021
- Nonnegligible biogenic organic aerosol and the correlations with light absorption at three high altitude locations in the Qinghai–Tibetan Plateau C. Zhu et al. 10.1016/j.atmosenv.2022.119394
- Yields and molecular composition of gas-phase and secondary organic aerosol from the photooxidation of the volatile consumer product benzyl alcohol: formation of highly oxygenated and hydroxy nitro-aromatic compounds M. Jaoui et al. 10.5194/acp-23-4637-2023
- Source apportionment of fine particulate matter in a Middle Eastern Metropolis, Tehran-Iran, using PMF with organic and inorganic markers S. Esmaeilirad et al. 10.1016/j.scitotenv.2019.135330
- Indication of primary biogenic contribution to BrC over a high altitude location in the southeastern Tibet C. Zhu et al. 10.1016/j.atmosenv.2020.117462
- Comparison of five methodologies to apportion organic aerosol sources during a PM pollution event D. Srivastava et al. 10.1016/j.scitotenv.2020.143168
- Quantitative chemical assay of nanogram-level particulate matter using aerosol mass spectrometry: characterization of particles collected from uncrewed atmospheric measurement platforms C. Niedek et al. 10.5194/amt-16-955-2023
- Organic aerosol sources in Krakow, Poland, before implementation of a solid fuel residential heating ban R. Casotto et al. 10.1016/j.scitotenv.2022.158655
- Urban Oxidation Flow Reactor Measurements Reveal Significant Secondary Organic Aerosol Contributions from Volatile Emissions of Emerging Importance R. Shah et al. 10.1021/acs.est.9b06531
- Characterization of the PM2.5 aerosol fraction monitored at a suburban site in south-eastern Italy by integrating isotopic techniques and ion beam analysis S. Romano et al. 10.3389/fenvs.2022.971204
- Contribution of fossil and biomass-derived secondary organic carbon to winter water-soluble organic aerosols in Delhi, India H. Bhowmik et al. 10.1016/j.scitotenv.2023.168655
- Characterizing the Sources of Ambient PM10 Organic Aerosol in Urban and Rural Catalonia, Spain M. in 't Veld et al. 10.2139/ssrn.4463228
- Development of graphitization method for low carbon aerosol filter samples with Automated Graphitization System AGE-3 L. Butkus et al. 10.1016/j.apradiso.2022.110461
- An optimised organic carbon ∕ elemental carbon (OC ∕ EC) fraction separation method for radiocarbon source apportionment applied to low-loaded Arctic aerosol filters M. Rauber et al. 10.5194/amt-16-825-2023
- Source-specific light absorption by carbonaceous components in the complex aerosol matrix from yearly filter-based measurements V. Moschos et al. 10.5194/acp-21-12809-2021
- Atomic Spectrometry Update – a review of advances in environmental analysis J. Bacon et al. 10.1039/C8JA90044B
- Long-term sub-micrometer aerosol chemical composition in the boreal forest: inter- and intra-annual variability L. Heikkinen et al. 10.5194/acp-20-3151-2020
- Source apportionment of atmospheric PM<sub>10</sub> oxidative potential: synthesis of 15 year-round urban datasets in France S. Weber et al. 10.5194/acp-21-11353-2021
- Quantification of fossil and non-fossil sources to the reduction of carbonaceous aerosols in the Yangtze River Delta, China: Insights from radiocarbon analysis during 2014–2019 M. Yu et al. 10.1016/j.atmosenv.2022.119421
- A 1-year aerosol chemical speciation monitor (ACSM) source analysis of organic aerosol particle contributions from anthropogenic sources after long-range transport at the TROPOS research station Melpitz S. Atabakhsh et al. 10.5194/acp-23-6963-2023
- Impact of anthropogenic and biogenic sources on the seasonal variation in the molecular composition of urban organic aerosols: a field and laboratory study using ultra-high-resolution mass spectrometry K. Daellenbach et al. 10.5194/acp-19-5973-2019
- Complex plant-derived organic aerosol as ice-nucleating particles – more than the sums of their parts? I. Steinke et al. 10.5194/acp-20-11387-2020
- Characterisation of urban aerosol size distribution by radiocarbon and PIXE analyses in a middle-European urban environment for source identification: a pilot study A. Angyal et al. 10.1007/s11356-024-34215-8
- Abundant Biogenic Oxygenated Organic Aerosol in Atmospheric Coarse Particles: Plausible Sources and Atmospheric Implications X. Huang et al. 10.1021/acs.est.9b06311
- Accurate observation of black and brown carbon in atmospheric fine particles via a versatile aerosol concentration enrichment system (VACES) H. Kang et al. 10.1016/j.scitotenv.2022.155817
- Source apportionment of carbonaceous aerosols in Beijing with radiocarbon and organic tracers: insight into the differences between urban and rural sites S. Hou et al. 10.5194/acp-21-8273-2021
- Composition and Sources of Organic Aerosol in Two Megacities in Western China Using Complementary Mass Spectrometric and Statistical Techniques T. Cui et al. 10.1021/acsestair.4c00051
- Real-time measurement and source apportionment of elements in Delhi's atmosphere P. Rai et al. 10.1016/j.scitotenv.2020.140332
- Sources and formation of carbonaceous aerosols in Xi'an, China: primary emissions and secondary formation constrained by radiocarbon H. Ni et al. 10.5194/acp-19-15609-2019
- Development and evaluation of an improved offline aerosol mass spectrometry technique C. Vasilakopoulou et al. 10.5194/amt-16-2837-2023
- Chemical composition and sources of organic aerosol on the Adriatic coast in Croatia R. Casotto et al. 10.1016/j.aeaoa.2022.100159
- Local incomplete combustion emissions define the PM2.5 oxidative potential in Northern India D. Bhattu et al. 10.1038/s41467-024-47785-5
- Using highly time-resolved online mass spectrometry to examine biogenic and anthropogenic contributions to organic aerosol in Beijing A. Mehra et al. 10.1039/D0FD00080A
- A 1-year characterization of organic aerosol composition and sources using an extractive electrospray ionization time-of-flight mass spectrometer (EESI-TOF) L. Qi et al. 10.5194/acp-20-7875-2020
- Sources of organic aerosols in Europe: a modeling study using CAMx with modified volatility basis set scheme J. Jiang et al. 10.5194/acp-19-15247-2019
- A comprehensive characterization of ice nucleation by three different types of cellulose particles immersed in water N. Hiranuma et al. 10.5194/acp-19-4823-2019
- Arabitol, mannitol, and glucose as tracers of primary biogenic organic aerosol: the influence of environmental factors on ambient air concentrations and spatial distribution over France A. Samaké et al. 10.5194/acp-19-11013-2019
- Characterizing the sources of ambient PM10 organic aerosol in urban and rural Catalonia, Spain M. in 't Veld et al. 10.1016/j.scitotenv.2023.166440
Latest update: 12 Dec 2024
Short summary
Carbonaceous aerosols are related to adverse human health effects, which depend on the aerosol chemical composition and size. Here, we combine aerosol mass spectrometry and radiocarbon measurements of size-resolved samples collected over a long term to identify the origins of primary and secondary carbonaceous aerosols in the fine and coarse modes.
Carbonaceous aerosols are related to adverse human health effects, which depend on the aerosol...
Altmetrics
Final-revised paper
Preprint