Articles | Volume 18, issue 8
Atmos. Chem. Phys., 18, 6095–6120, 2018
https://doi.org/10.5194/acp-18-6095-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Atmos. Chem. Phys., 18, 6095–6120, 2018
https://doi.org/10.5194/acp-18-6095-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article 02 May 2018
Research article | 02 May 2018
The atmospheric impacts of monoterpene ozonolysis on global stabilised Criegee intermediate budgets and SO2 oxidation: experiment, theory and modelling
Mike J. Newland et al.
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Cited
19 citations as recorded by crossref.
- Quantification of the role of stabilized Criegee intermediates in the formation of aerosols in limonene ozonolysis Y. Gong & Z. Chen 10.5194/acp-21-813-2021
- Trends in stabilisation of Criegee intermediates from alkene ozonolysis M. Newland et al. 10.1039/D0CP00897D
- Importance of Hydroxyl Radical Chemistry in Isoprene Suppression of Particle Formation from α-Pinene Ozonolysis Y. Wang et al. 10.1021/acsearthspacechem.0c00294
- Quantitative constraints on autoxidation and dimer formation from direct probing of monoterpene-derived peroxy radical chemistry Y. Zhao et al. 10.1073/pnas.1812147115
- Unimolecular decay dynamics of Criegee intermediates: Energy-resolved rates, thermal rates, and their atmospheric impact T. Stephenson & M. Lester 10.1080/0144235X.2020.1688530
- Accretion Product Formation from Ozonolysis and OH Radical Reaction of α-Pinene: Mechanistic Insight and the Influence of Isoprene and Ethylene T. Berndt et al. 10.1021/acs.est.8b02210
- Rapid unimolecular reaction of stabilized Criegee intermediates and implications for atmospheric chemistry B. Long et al. 10.1038/s41467-019-09948-7
- Criegee intermediates: production, detection and reactivity R. Chhantyal-Pun et al. 10.1080/0144235X.2020.1792104
- Anthropogenic Effects on Biogenic Secondary Organic Aerosol Formation L. Xu et al. 10.1007/s00376-020-0284-3
- Sulfur Dioxide Modifies Aerosol Particle Formation and Growth by Ozonolysis of Monoterpenes and Isoprene C. Stangl et al. 10.1029/2018JD030064
- Evaluated kinetic and photochemical data for atmospheric chemistry: Volume VII – Criegee intermediates R. Cox et al. 10.5194/acp-20-13497-2020
- Growth of Aitken mode ammonium sulfate particles by α-pinene ozonolysis J. Krasnomowitz et al. 10.1080/02786826.2019.1568381
- Theoretical Study on Criegee Intermediate’s Role in Ozonolysis of Acrylic Acid X. Lin et al. 10.1021/acs.jpca.8b11671
- New particle formation from the reactions of ozone with indene and styrene L. Bracco et al. 10.1039/C9CP00912D
- Evidence and evolution of Criegee intermediates, hydroperoxides and secondary organic aerosols formedviaozonolysis of α-pinene A. Bagchi et al. 10.1039/C9CP06306D
- Impact of Criegee Intermediate Reactions with Peroxy Radicals on Tropospheric Organic Aerosol R. Chhantyal-Pun et al. 10.1021/acsearthspacechem.0c00147
- Impacts of the Degradation of 2,3,3,3-Tetrafluoropropene into Trifluoroacetic Acid from Its Application in Automobile Air Conditioners in China, the United States, and Europe Z. Wang et al. 10.1021/acs.est.7b05960
- Ozonolysis of <i>α</i>-phellandrene – Part 2: Compositional analysis of secondary organic aerosol highlights the role of stabilised Criegee intermediates F. Mackenzie-Rae et al. 10.5194/acp-18-4673-2018
- Criegee intermediates and their impacts on the troposphere M. Khan et al. 10.1039/C7EM00585G
16 citations as recorded by crossref.
- Quantification of the role of stabilized Criegee intermediates in the formation of aerosols in limonene ozonolysis Y. Gong & Z. Chen 10.5194/acp-21-813-2021
- Trends in stabilisation of Criegee intermediates from alkene ozonolysis M. Newland et al. 10.1039/D0CP00897D
- Importance of Hydroxyl Radical Chemistry in Isoprene Suppression of Particle Formation from α-Pinene Ozonolysis Y. Wang et al. 10.1021/acsearthspacechem.0c00294
- Quantitative constraints on autoxidation and dimer formation from direct probing of monoterpene-derived peroxy radical chemistry Y. Zhao et al. 10.1073/pnas.1812147115
- Unimolecular decay dynamics of Criegee intermediates: Energy-resolved rates, thermal rates, and their atmospheric impact T. Stephenson & M. Lester 10.1080/0144235X.2020.1688530
- Accretion Product Formation from Ozonolysis and OH Radical Reaction of α-Pinene: Mechanistic Insight and the Influence of Isoprene and Ethylene T. Berndt et al. 10.1021/acs.est.8b02210
- Rapid unimolecular reaction of stabilized Criegee intermediates and implications for atmospheric chemistry B. Long et al. 10.1038/s41467-019-09948-7
- Criegee intermediates: production, detection and reactivity R. Chhantyal-Pun et al. 10.1080/0144235X.2020.1792104
- Anthropogenic Effects on Biogenic Secondary Organic Aerosol Formation L. Xu et al. 10.1007/s00376-020-0284-3
- Sulfur Dioxide Modifies Aerosol Particle Formation and Growth by Ozonolysis of Monoterpenes and Isoprene C. Stangl et al. 10.1029/2018JD030064
- Evaluated kinetic and photochemical data for atmospheric chemistry: Volume VII – Criegee intermediates R. Cox et al. 10.5194/acp-20-13497-2020
- Growth of Aitken mode ammonium sulfate particles by α-pinene ozonolysis J. Krasnomowitz et al. 10.1080/02786826.2019.1568381
- Theoretical Study on Criegee Intermediate’s Role in Ozonolysis of Acrylic Acid X. Lin et al. 10.1021/acs.jpca.8b11671
- New particle formation from the reactions of ozone with indene and styrene L. Bracco et al. 10.1039/C9CP00912D
- Evidence and evolution of Criegee intermediates, hydroperoxides and secondary organic aerosols formedviaozonolysis of α-pinene A. Bagchi et al. 10.1039/C9CP06306D
- Impact of Criegee Intermediate Reactions with Peroxy Radicals on Tropospheric Organic Aerosol R. Chhantyal-Pun et al. 10.1021/acsearthspacechem.0c00147
3 citations as recorded by crossref.
- Impacts of the Degradation of 2,3,3,3-Tetrafluoropropene into Trifluoroacetic Acid from Its Application in Automobile Air Conditioners in China, the United States, and Europe Z. Wang et al. 10.1021/acs.est.7b05960
- Ozonolysis of <i>α</i>-phellandrene – Part 2: Compositional analysis of secondary organic aerosol highlights the role of stabilised Criegee intermediates F. Mackenzie-Rae et al. 10.5194/acp-18-4673-2018
- Criegee intermediates and their impacts on the troposphere M. Khan et al. 10.1039/C7EM00585G
Latest update: 06 Mar 2021
Short summary
Stabilised Criegee intermediates (SCIs) are formed in the reaction of alkenes with ozone, both of which are ubiquitous throughout the troposphere. We determine the fate and global distribution of SCI from monoterpene ozonolysis. One major fate of SCI is reaction with H2O, but for a fraction of SCIs, unimolecular reactions dominate. Concentrations of SCIs are high enough regionally to play a key role in the conversion of sulfur dioxide to aerosol, affecting air quality and climate.
Stabilised Criegee intermediates (SCIs) are formed in the reaction of alkenes with ozone, both...
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