Articles | Volume 18, issue 8
Atmos. Chem. Phys., 18, 6095–6120, 2018
https://doi.org/10.5194/acp-18-6095-2018
Atmos. Chem. Phys., 18, 6095–6120, 2018
https://doi.org/10.5194/acp-18-6095-2018

Research article 02 May 2018

Research article | 02 May 2018

The atmospheric impacts of monoterpene ozonolysis on global stabilised Criegee intermediate budgets and SO2 oxidation: experiment, theory and modelling

Mike J. Newland et al.

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Short summary
Stabilised Criegee intermediates (SCIs) are formed in the reaction of alkenes with ozone, both of which are ubiquitous throughout the troposphere. We determine the fate and global distribution of SCI from monoterpene ozonolysis. One major fate of SCI is reaction with H2O, but for a fraction of SCIs, unimolecular reactions dominate. Concentrations of SCIs are high enough regionally to play a key role in the conversion of sulfur dioxide to aerosol, affecting air quality and climate.
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