Articles | Volume 18, issue 8
https://doi.org/10.5194/acp-18-5483-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-5483-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
23 Apr 2018
Research article |
| 23 Apr 2018
High-resolution inversion of OMI formaldehyde columns to quantify isoprene emission on ecosystem-relevant scales: application to the southeast US
Jennifer Kaiser
CORRESPONDING AUTHOR
John A. Paulson School of Engineering and Applied Sciences, Harvard
University, Cambridge, MA, USA
Daniel J. Jacob
John A. Paulson School of Engineering and Applied Sciences, Harvard
University, Cambridge, MA, USA
Department of Earth and Planetary Sciences, Harvard University,
Cambridge, MA, USA
John A. Paulson School of Engineering and Applied Sciences, Harvard
University, Cambridge, MA, USA
Katherine R. Travis
John A. Paulson School of Engineering and Applied Sciences, Harvard
University, Cambridge, MA, USA
now at: Department of Civil and Environmental Engineering,
Massachusetts Institute of Technology, Cambridge, MA, USA
Jenny A. Fisher
Centre for Atmospheric Chemistry, School of Chemistry, University of
Wollongong, Wollongong, NSW, Australia
School of Earth and Environmental Sciences, University of Wollongong,
Wollongong, NSW, Australia
Gonzalo González Abad
Harvard–Smithsonian Center for Astrophysics, Cambridge, MA, USA
Lin Zhang
Laboratory for Climate and Ocean-Atmosphere Studies, Department of
Atmospheric and Oceanic Sciences, School of Physics, Peking University,
Beijing 100871, People's Republic of China
Xuesong Zhang
Department of Physics, University of Toronto, Toronto, Ontario, Canada
Alan Fried
Institute for Arctic and Alpine Research, University of Colorado,
Boulder, CO, USA
John D. Crounse
Division of Geological and Planetary Sciences, California Institute of
Technology, Pasadena, CA, USA
Jason M. Clair
Division of Geological and Planetary Sciences, California Institute of
Technology, Pasadena, CA, USA
now at: Atmospheric Chemistry and Dynamics Laboratory, NASA
Goddard Space Flight Center, Greenbelt, MD, USA
now at: Joint Center for Earth Systems Technology, University
of Maryland Baltimore County, Baltimore, MD, USA
Armin Wisthaler
Institute for Ion Physics and Applied Physics, University of
Innsbruck, Innsbruck, Austria
Department of Chemistry, University of Oslo, Oslo, Norway
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- Next‐Generation Isoprene Measurements From Space: Detecting Daily Variability at High Resolution K. Wells et al. 10.1029/2021JD036181
- Comparative assessment of TROPOMI and OMI formaldehyde observations and validation against MAX-DOAS network column measurements I. De Smedt et al. 10.5194/acp-21-12561-2021
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- Towards a satellite formaldehyde – in situ hybrid estimate for organic aerosol abundance J. Liao et al. 10.5194/acp-19-2765-2019
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- Chinese Regulations Are Working—Why Is Surface Ozone Over Industrialized Areas Still High? Applying Lessons From Northeast US Air Quality Evolution X. Chen et al. 10.1029/2021GL092816
- Multipollutant modeling of ozone, reactive nitrogen and HAPs across the continental US with CMAQ-CB6 D. Luecken et al. 10.1016/j.atmosenv.2018.11.060
- Long-term MAX-DOAS measurements of NO<sub>2</sub>, HCHO, and aerosols and evaluation of corresponding satellite data products over Mohali in the Indo-Gangetic Plain V. Kumar et al. 10.5194/acp-20-14183-2020
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- A long-term estimation of biogenic volatile organic compound (BVOC) emission in China from 2001–2016: the roles of land cover change and climate variability H. Wang et al. 10.5194/acp-21-4825-2021
- Satellite Formaldehyde to Support Model Evaluation M. Harkey et al. 10.1029/2020JD032881
- Algorithm theoretical baseline for formaldehyde retrievals from S5P TROPOMI and from the QA4ECV project I. De Smedt et al. 10.5194/amt-11-2395-2018
36 citations as recorded by crossref.
- Constraining Emissions of Volatile Organic Compounds Over the Indian Subcontinent Using Space‐Based Formaldehyde Measurements S. Chaliyakunnel et al. 10.1029/2019JD031262
- Vertical Transport, Entrainment, and Scavenging Processes Affecting Trace Gases in a Modeled and Observed SEAC 4 RS Case Study G. Cuchiara et al. 10.1029/2019JD031957
- Formaldehyde evolution in US wildfire plumes during the Fire Influence on Regional to Global Environments and Air Quality experiment (FIREX-AQ) J. Liao et al. 10.5194/acp-21-18319-2021
- Next‐Generation Isoprene Measurements From Space: Detecting Daily Variability at High Resolution K. Wells et al. 10.1029/2021JD036181
- Comparative assessment of TROPOMI and OMI formaldehyde observations and validation against MAX-DOAS network column measurements I. De Smedt et al. 10.5194/acp-21-12561-2021
- High-resolution biogenic global emission inventory for the time period 2000–2019 for air quality modelling K. Sindelarova et al. 10.5194/essd-14-251-2022
- Changes in the ozone chemical regime over the contiguous United States inferred by the inversion of NOx and VOC emissions using satellite observation J. Jung et al. 10.1016/j.atmosres.2022.106076
- Towards a satellite formaldehyde – in situ hybrid estimate for organic aerosol abundance J. Liao et al. 10.5194/acp-19-2765-2019
- Ground ozone variations at an urban and a rural station in Beijing from 2006 to 2017: Trend, meteorological influences and formation regimes N. Cheng et al. 10.1016/j.jclepro.2019.06.204
- Quantifying Emissions of CO and NO x Using Observations From MOPITT, OMI, TES, and OSIRIS X. Zhang et al. 10.1029/2018JD028670
- Chinese Regulations Are Working—Why Is Surface Ozone Over Industrialized Areas Still High? Applying Lessons From Northeast US Air Quality Evolution X. Chen et al. 10.1029/2021GL092816
- Multipollutant modeling of ozone, reactive nitrogen and HAPs across the continental US with CMAQ-CB6 D. Luecken et al. 10.1016/j.atmosenv.2018.11.060
- Long-term MAX-DOAS measurements of NO<sub>2</sub>, HCHO, and aerosols and evaluation of corresponding satellite data products over Mohali in the Indo-Gangetic Plain V. Kumar et al. 10.5194/acp-20-14183-2020
- Formaldehyde Generation in Photooxidation of Isoprene on Iron Oxide Nanoclusters S. Lv et al. 10.1021/acs.jpcc.8b12471
- Spatial Variation of Surface O 3 Responses to Drought Over the Contiguous United States During Summertime: Role of Precursor Emissions and Ozone Chemistry W. Li et al. 10.1029/2021JD035607
- Spatiotemporal variations and pollution sources of HCHO over Jiangsu-Zhejiang-Shanghai based on OMI T. Ju et al. 10.1007/s11869-021-01076-w
- Satellite isoprene retrievals constrain emissions and atmospheric oxidation K. Wells et al. 10.1038/s41586-020-2664-3
- Hybrid Mass Balance/4D‐Var Joint Inversion of NO x and SO 2 Emissions in East Asia Z. Qu et al. 10.1029/2018JD030240
- Isoprene versus Monoterpenes as Gas-Phase Organic Acid Precursors in the Atmosphere M. Link et al. 10.1021/acsearthspacechem.1c00093
- Development of a reduced-complexity plant canopy physics surrogate model for use in chemical transport models: a case study with GEOS-Chem v12.3.0 S. Silva et al. 10.5194/gmd-13-2569-2020
- Measured and modelled ozone photochemical production in the Baltimore-Washington airshed L. Hembeck et al. 10.1016/j.aeaoa.2019.100017
- Top-down estimates of anthropogenic VOC emissions in South Korea using formaldehyde vertical column densities from aircraft during the KORUS-AQ campaign H. Kwon et al. 10.1525/elementa.2021.00109
- Observations of Integral Formaldehyde Content in the Lower Troposphere in Urban Agglomerations of Moscow and Tomsk Using the Method of Differential Optical Absorption Spectroscopy I. Bruchkouski et al. 10.1134/S1024856019030047
- Assessing the Iterative Finite Difference Mass Balance and 4D‐Var Methods to Derive Ammonia Emissions Over North America Using Synthetic Observations C. Li et al. 10.1029/2018JD030183
- Impacts of global NO<sub><i>x</i></sub> inversions on NO<sub>2</sub> and ozone simulations Z. Qu et al. 10.5194/acp-20-13109-2020
- Global and regional impacts of land cover changes on isoprene emissions derived from spaceborne data and the MEGAN model B. Opacka et al. 10.5194/acp-21-8413-2021
- On the sources and sinks of atmospheric VOCs: an integrated analysis of recent aircraft campaigns over North America X. Chen et al. 10.5194/acp-19-9097-2019
- New constraints on biogenic emissions using satellite-based estimates of carbon monoxide fluxes H. Worden et al. 10.5194/acp-19-13569-2019
- Space‐Based Constraints on Terrestrial Glyoxal Production S. Silva et al. 10.1029/2018JD029311
- Comprehensive isoprene and terpene gas-phase chemistry improves simulated surface ozone in the southeastern US R. Schwantes et al. 10.5194/acp-20-3739-2020
- Airborne formaldehyde and volatile organic compound measurements over the Daesan petrochemical complex on Korea’s northwest coast during the Korea-United States Air Quality study A. Fried et al. 10.1525/elementa.2020.121
- Review on plant terpenoid emissions worldwide and in China W. Yang et al. 10.1016/j.scitotenv.2021.147454
- A meteorologically adjusted ensemble Kalman filter approach for inversing daily emissions: A case study in the Pearl River Delta, China G. Jia et al. 10.1016/j.jes.2021.08.048
- A new model mechanism for atmospheric oxidation of isoprene: global effects on oxidants, nitrogen oxides, organic products, and secondary organic aerosol K. Bates & D. Jacob 10.5194/acp-19-9613-2019
- A long-term estimation of biogenic volatile organic compound (BVOC) emission in China from 2001–2016: the roles of land cover change and climate variability H. Wang et al. 10.5194/acp-21-4825-2021
- Satellite Formaldehyde to Support Model Evaluation M. Harkey et al. 10.1029/2020JD032881
1 citations as recorded by crossref.
Latest update: 28 Mar 2023
Short summary
Isoprene emissions from vegetation have a large effect on atmospheric chemistry and air quality. Here we use the adjoint of GEOS-Chem in an inversion of OMI formaldehyde observations to produce top-down estimates of isoprene emissions in the southeast US during the summer of 2013. We find that MEGAN v2.1 is biased high on average by 40 %. Our downward correction of isoprene emissions leads to a small reduction in modeled surface O3 and decreases the contribution of isoprene to organic aerosol.
Isoprene emissions from vegetation have a large effect on atmospheric chemistry and air quality....
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