Articles | Volume 18, issue 8
https://doi.org/10.5194/acp-18-5483-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-5483-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
23 Apr 2018
Research article |
| 23 Apr 2018
| 23 Apr 2018
High-resolution inversion of OMI formaldehyde columns to quantify isoprene emission on ecosystem-relevant scales: application to the southeast US
Jennifer Kaiser
CORRESPONDING AUTHOR
John A. Paulson School of Engineering and Applied Sciences, Harvard
University, Cambridge, MA, USA
Daniel J. Jacob
John A. Paulson School of Engineering and Applied Sciences, Harvard
University, Cambridge, MA, USA
Department of Earth and Planetary Sciences, Harvard University,
Cambridge, MA, USA
John A. Paulson School of Engineering and Applied Sciences, Harvard
University, Cambridge, MA, USA
Katherine R. Travis
John A. Paulson School of Engineering and Applied Sciences, Harvard
University, Cambridge, MA, USA
now at: Department of Civil and Environmental Engineering,
Massachusetts Institute of Technology, Cambridge, MA, USA
Jenny A. Fisher
Centre for Atmospheric Chemistry, School of Chemistry, University of
Wollongong, Wollongong, NSW, Australia
School of Earth and Environmental Sciences, University of Wollongong,
Wollongong, NSW, Australia
Gonzalo González Abad
Harvard–Smithsonian Center for Astrophysics, Cambridge, MA, USA
Lin Zhang
Laboratory for Climate and Ocean-Atmosphere Studies, Department of
Atmospheric and Oceanic Sciences, School of Physics, Peking University,
Beijing 100871, People's Republic of China
Xuesong Zhang
Department of Physics, University of Toronto, Toronto, Ontario, Canada
Alan Fried
Institute for Arctic and Alpine Research, University of Colorado,
Boulder, CO, USA
John D. Crounse
Division of Geological and Planetary Sciences, California Institute of
Technology, Pasadena, CA, USA
Jason M. St. Clair
Division of Geological and Planetary Sciences, California Institute of
Technology, Pasadena, CA, USA
now at: Atmospheric Chemistry and Dynamics Laboratory, NASA
Goddard Space Flight Center, Greenbelt, MD, USA
now at: Joint Center for Earth Systems Technology, University
of Maryland Baltimore County, Baltimore, MD, USA
Armin Wisthaler
Institute for Ion Physics and Applied Physics, University of
Innsbruck, Innsbruck, Austria
Department of Chemistry, University of Oslo, Oslo, Norway
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- Changes in the ozone chemical regime over the contiguous United States inferred by the inversion of NOx and VOC emissions using satellite observation J. Jung et al. 10.1016/j.atmosres.2022.106076
- Global Formaldehyde Products From the Ozone Mapping and Profiler Suite (OMPS) Nadir Mappers on Suomi NPP and NOAA‐20 C. Nowlan et al. 10.1029/2022EA002643
- Ground ozone variations at an urban and a rural station in Beijing from 2006 to 2017: Trend, meteorological influences and formation regimes N. Cheng et al. 10.1016/j.jclepro.2019.06.204
- Quantifying Emissions of CO and NOx Using Observations From MOPITT, OMI, TES, and OSIRIS X. Zhang et al. 10.1029/2018JD028670
- Chinese Regulations Are Working—Why Is Surface Ozone Over Industrialized Areas Still High? Applying Lessons From Northeast US Air Quality Evolution X. Chen et al. 10.1029/2021GL092816
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- Evaluating the Impact of Chemical Complexity and Horizontal Resolution on Tropospheric Ozone Over the Conterminous US With a Global Variable Resolution Chemistry Model R. Schwantes et al. 10.1029/2021MS002889
- Role of chemical production and depositional losses on formaldehyde in the Community Regional Atmospheric Chemistry Multiphase Mechanism (CRACMM) T. Skipper et al. 10.5194/acp-24-12903-2024
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- Source and variability of formaldehyde in the Fenwei Plain: An integrated multi-source satellite and emission inventory study L. Li et al. 10.1016/j.jes.2024.02.030
- Airborne formaldehyde and volatile organic compound measurements over the Daesan petrochemical complex on Korea’s northwest coast during the Korea-United States Air Quality study A. Fried et al. 10.1525/elementa.2020.121
- MAX-DOAS Measurements of Tropospheric NO2 and HCHO Vertical Profiles at the Longfengshan Regional Background Station in Northeastern China S. Liu et al. 10.3390/s23063269
- A meteorologically adjusted ensemble Kalman filter approach for inversing daily emissions: A case study in the Pearl River Delta, China G. Jia et al. 10.1016/j.jes.2021.08.048
- A new model mechanism for atmospheric oxidation of isoprene: global effects on oxidants, nitrogen oxides, organic products, and secondary organic aerosol K. Bates & D. Jacob 10.5194/acp-19-9613-2019
- Optimizing the Isoprene Emission Model MEGAN With Satellite and Ground‐Based Observational Constraints C. DiMaria et al. 10.1029/2022JD037822
- Satellite Formaldehyde to Support Model Evaluation M. Harkey et al. 10.1029/2020JD032881
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Latest update: 07 May 2025
Short summary
Isoprene emissions from vegetation have a large effect on atmospheric chemistry and air quality. Here we use the adjoint of GEOS-Chem in an inversion of OMI formaldehyde observations to produce top-down estimates of isoprene emissions in the southeast US during the summer of 2013. We find that MEGAN v2.1 is biased high on average by 40 %. Our downward correction of isoprene emissions leads to a small reduction in modeled surface O3 and decreases the contribution of isoprene to organic aerosol.
Isoprene emissions from vegetation have a large effect on atmospheric chemistry and air quality....
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