Articles | Volume 18, issue 3
https://doi.org/10.5194/acp-18-2199-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-2199-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
15 Feb 2018
Research article |
| 15 Feb 2018
| 15 Feb 2018
Bulk and molecular-level characterization of laboratory-aged biomass burning organic aerosol from oak leaf and heartwood fuels
Claire F. Fortenberry
Department of Energy, Environmental, and Chemical Engineering, Washington University in Saint Louis, Saint Louis, MO 63130, USA
Michael J. Walker
Department of Energy, Environmental, and Chemical Engineering, Washington University in Saint Louis, Saint Louis, MO 63130, USA
Yaping Zhang
Department of Energy, Environmental, and Chemical Engineering, Washington University in Saint Louis, Saint Louis, MO 63130, USA
Dhruv Mitroo
Department of Energy, Environmental, and Chemical Engineering, Washington University in Saint Louis, Saint Louis, MO 63130, USA
now at: Department of Atmospheric Sciences, Rosenstiel School of Marine and Atmospheric Sciences, University of Miami, Miami, FL 33149, USA
William H. Brune
Department of Meteorology and Atmospheric Science, Pennsylvania State University, State College, PA 16801, USA
Brent J. Williams
CORRESPONDING AUTHOR
Department of Energy, Environmental, and Chemical Engineering, Washington University in Saint Louis, Saint Louis, MO 63130, USA
Viewed
Total article views: 3,545 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 05 Jul 2017)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 2,230 | 1,246 | 69 | 3,545 | 575 | 55 | 90 |
- HTML: 2,230
- PDF: 1,246
- XML: 69
- Total: 3,545
- Supplement: 575
- BibTeX: 55
- EndNote: 90
Total article views: 2,699 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 15 Feb 2018)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 1,700 | 943 | 56 | 2,699 | 378 | 49 | 75 |
- HTML: 1,700
- PDF: 943
- XML: 56
- Total: 2,699
- Supplement: 378
- BibTeX: 49
- EndNote: 75
Total article views: 846 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 05 Jul 2017)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 530 | 303 | 13 | 846 | 197 | 6 | 15 |
- HTML: 530
- PDF: 303
- XML: 13
- Total: 846
- Supplement: 197
- BibTeX: 6
- EndNote: 15
Viewed (geographical distribution)
Total article views: 3,545 (including HTML, PDF, and XML)
Thereof 3,544 with geography defined
and 1 with unknown origin.
Total article views: 2,699 (including HTML, PDF, and XML)
Thereof 2,705 with geography defined
and -6 with unknown origin.
Total article views: 846 (including HTML, PDF, and XML)
Thereof 839 with geography defined
and 7 with unknown origin.
| Country | # | Views | % |
|---|
| Country | # | Views | % |
|---|
| Country | # | Views | % |
|---|
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
Cited
30 citations as recorded by crossref.
- Contribution of Charge-Transfer Complexes to Absorptivity of Primary Brown Carbon Aerosol A. Trofimova et al. 10.1021/acsearthspacechem.9b00116
- Amplification of black carbon light absorption induced by atmospheric aging: temporal variation at seasonal and diel scales in urban Guangzhou J. Sun et al. 10.5194/acp-20-2445-2020
- Biomass Burning Markers and Residential Burning in the WINTER Aircraft Campaign A. Sullivan et al. 10.1029/2017JD028153
- Secondary organic aerosols produced from photochemical oxidation of secondarily evaporated biomass burning organic gases: Chemical composition, toxicity, optical properties, and climate effect Z. Fang et al. 10.1016/j.envint.2021.106801
- Polar semivolatile organic compounds in biomass-burning emissions and their chemical transformations during aging in an oxidation flow reactor D. Sengupta et al. 10.5194/acp-20-8227-2020
- A new oxidation flow reactor for the measurements of secondary aerosol formation: Characterisation and a case study C. Wu et al. 10.1016/j.atmosenv.2023.119886
- Quantifying the relative importance of major tracers for fine particles released from biofuel combustion in households in the rural North China Plain J. Tao et al. 10.1016/j.envpol.2020.115764
- Chemical composition of PM<sub>2.5</sub> in October 2017 Northern California wildfire plumes Y. Liang et al. 10.5194/acp-21-5719-2021
- Improving thermal desorption aerosol gas chromatography using a dual-trap design H. Ren et al. 10.1016/j.chroma.2019.04.045
- Development, Demonstration, and Evaluation of Routine Monitoring of Aerosol Carbon, Oxygen, and Sulfur Content P. Kumar et al. 10.1021/acsestair.3c00059
- Physical and chemical characterization of aerosol in fresh and aged emissions from open combustion of biomass fuels C. Bhattarai et al. 10.1080/02786826.2018.1498585
- Quantifying the Light-Absorption Properties and Molecular Composition of Brown Carbon Aerosol from Sub-Saharan African Biomass Combustion V. Moschos et al. 10.1021/acs.est.3c09378
- Emission factors for polycyclic aromatic hydrocarbons from laboratory biomass-burning and their chemical transformations during aging in an oxidation flow reactor D. Sengupta et al. 10.1016/j.scitotenv.2023.161857
- Changes in Physicochemical Properties of Organic Aerosol During Photochemical Aging of Cooking and Burning Emissions W. Xu et al. 10.1029/2022JD037911
- Airborne extractive electrospray mass spectrometry measurements of the chemical composition of organic aerosol D. Pagonis et al. 10.5194/amt-14-1545-2021
- A searchable database and mass spectral comparison tool for the Aerosol Mass Spectrometer (AMS) and the Aerosol Chemical Speciation Monitor (ACSM) S. Jeon et al. 10.5194/amt-16-6075-2023
- Radical chemistry in oxidation flow reactors for atmospheric chemistry research Z. Peng & J. Jimenez 10.1039/C9CS00766K
- Secondary organic aerosol formation and aging from ambient air in an oxidation flow reactor during wintertime in Beijing, China W. Xu et al. 10.1016/j.envres.2022.112751
- Influence of the vapor wall loss on the degradation rate constants in chamber experiments of levoglucosan and other biomass burning markers A. Bertrand et al. 10.5194/acp-18-10915-2018
- Comprehensive analysis of emissions from wood and cow dung burning using chemometrics and two-dimensional gas chromatography M. Loebel Roson et al. 10.1016/j.chemosphere.2024.143445
- Polyols and glucose particulate species as tracers of primary biogenic organic aerosols at 28 French sites A. Samaké et al. 10.5194/acp-19-3357-2019
- Insights Into Formation and Aging of Secondary Organic Aerosol From Oxidation Flow Reactors: A Review Z. Zhang et al. 10.1007/s40726-024-00309-7
- Evolution of the chemical fingerprint of biomass burning organic aerosol during aging A. Bertrand et al. 10.5194/acp-18-7607-2018
- Quantifying the Chemical Composition and Real-Time Mass Loading of Nanoplastic Particles in the Atmosphere Using Aerosol Mass Spectrometry S. Niu et al. 10.1021/acs.est.3c10286
- Dimensionality-reduction techniques for complex mass spectrometric datasets: application to laboratory atmospheric organic oxidation experiments A. Koss et al. 10.5194/acp-20-1021-2020
- Recent advances in mass spectrometry techniques for atmospheric chemistry research on molecular‐level W. Zhang et al. 10.1002/mas.21857
- Quartz filter-based thermal desorption gas chromatography mass spectrometry for in-situ molecular level measurement of ambient organic aerosols H. Ren et al. 10.1016/j.chroma.2019.01.010
- Evaluation of the Oxidation Flow Reactor for particulate matter emission limit certification J. Cao et al. 10.1016/j.atmosenv.2019.117086
- Real-time chemical characterization of primary and aged biomass burning aerosols derived from sub-Saharan African biomass fuels in smoldering fires M. James et al. 10.1039/D4EA00110A
- Liquid chromatographic isolation of individual carbohydrates from environmental matrices for stable carbon analysis and radiocarbon dating A. Nouara et al. 10.1016/j.aca.2019.03.028
29 citations as recorded by crossref.
- Contribution of Charge-Transfer Complexes to Absorptivity of Primary Brown Carbon Aerosol A. Trofimova et al. 10.1021/acsearthspacechem.9b00116
- Amplification of black carbon light absorption induced by atmospheric aging: temporal variation at seasonal and diel scales in urban Guangzhou J. Sun et al. 10.5194/acp-20-2445-2020
- Biomass Burning Markers and Residential Burning in the WINTER Aircraft Campaign A. Sullivan et al. 10.1029/2017JD028153
- Secondary organic aerosols produced from photochemical oxidation of secondarily evaporated biomass burning organic gases: Chemical composition, toxicity, optical properties, and climate effect Z. Fang et al. 10.1016/j.envint.2021.106801
- Polar semivolatile organic compounds in biomass-burning emissions and their chemical transformations during aging in an oxidation flow reactor D. Sengupta et al. 10.5194/acp-20-8227-2020
- A new oxidation flow reactor for the measurements of secondary aerosol formation: Characterisation and a case study C. Wu et al. 10.1016/j.atmosenv.2023.119886
- Quantifying the relative importance of major tracers for fine particles released from biofuel combustion in households in the rural North China Plain J. Tao et al. 10.1016/j.envpol.2020.115764
- Chemical composition of PM<sub>2.5</sub> in October 2017 Northern California wildfire plumes Y. Liang et al. 10.5194/acp-21-5719-2021
- Improving thermal desorption aerosol gas chromatography using a dual-trap design H. Ren et al. 10.1016/j.chroma.2019.04.045
- Development, Demonstration, and Evaluation of Routine Monitoring of Aerosol Carbon, Oxygen, and Sulfur Content P. Kumar et al. 10.1021/acsestair.3c00059
- Physical and chemical characterization of aerosol in fresh and aged emissions from open combustion of biomass fuels C. Bhattarai et al. 10.1080/02786826.2018.1498585
- Quantifying the Light-Absorption Properties and Molecular Composition of Brown Carbon Aerosol from Sub-Saharan African Biomass Combustion V. Moschos et al. 10.1021/acs.est.3c09378
- Emission factors for polycyclic aromatic hydrocarbons from laboratory biomass-burning and their chemical transformations during aging in an oxidation flow reactor D. Sengupta et al. 10.1016/j.scitotenv.2023.161857
- Changes in Physicochemical Properties of Organic Aerosol During Photochemical Aging of Cooking and Burning Emissions W. Xu et al. 10.1029/2022JD037911
- Airborne extractive electrospray mass spectrometry measurements of the chemical composition of organic aerosol D. Pagonis et al. 10.5194/amt-14-1545-2021
- A searchable database and mass spectral comparison tool for the Aerosol Mass Spectrometer (AMS) and the Aerosol Chemical Speciation Monitor (ACSM) S. Jeon et al. 10.5194/amt-16-6075-2023
- Radical chemistry in oxidation flow reactors for atmospheric chemistry research Z. Peng & J. Jimenez 10.1039/C9CS00766K
- Secondary organic aerosol formation and aging from ambient air in an oxidation flow reactor during wintertime in Beijing, China W. Xu et al. 10.1016/j.envres.2022.112751
- Influence of the vapor wall loss on the degradation rate constants in chamber experiments of levoglucosan and other biomass burning markers A. Bertrand et al. 10.5194/acp-18-10915-2018
- Comprehensive analysis of emissions from wood and cow dung burning using chemometrics and two-dimensional gas chromatography M. Loebel Roson et al. 10.1016/j.chemosphere.2024.143445
- Polyols and glucose particulate species as tracers of primary biogenic organic aerosols at 28 French sites A. Samaké et al. 10.5194/acp-19-3357-2019
- Insights Into Formation and Aging of Secondary Organic Aerosol From Oxidation Flow Reactors: A Review Z. Zhang et al. 10.1007/s40726-024-00309-7
- Evolution of the chemical fingerprint of biomass burning organic aerosol during aging A. Bertrand et al. 10.5194/acp-18-7607-2018
- Quantifying the Chemical Composition and Real-Time Mass Loading of Nanoplastic Particles in the Atmosphere Using Aerosol Mass Spectrometry S. Niu et al. 10.1021/acs.est.3c10286
- Dimensionality-reduction techniques for complex mass spectrometric datasets: application to laboratory atmospheric organic oxidation experiments A. Koss et al. 10.5194/acp-20-1021-2020
- Recent advances in mass spectrometry techniques for atmospheric chemistry research on molecular‐level W. Zhang et al. 10.1002/mas.21857
- Quartz filter-based thermal desorption gas chromatography mass spectrometry for in-situ molecular level measurement of ambient organic aerosols H. Ren et al. 10.1016/j.chroma.2019.01.010
- Evaluation of the Oxidation Flow Reactor for particulate matter emission limit certification J. Cao et al. 10.1016/j.atmosenv.2019.117086
- Real-time chemical characterization of primary and aged biomass burning aerosols derived from sub-Saharan African biomass fuels in smoldering fires M. James et al. 10.1039/D4EA00110A
Latest update: 14 Dec 2024
Short summary
In these laboratory studies, two types of biomass burning organic aerosol (BBOA) were generated in a combustion chamber and treated in a flow reactor to mimic atmospheric oxidation. Complementary bulk and molecular chemical measurements show that while many species deplete with oxidation, oxidized BBOA markers are enhanced. The results provide insight into the complex chemical evolution of BBOA over nearly 10 days of atmospheric photochemistry, informing future laboratory and field studies.
In these laboratory studies, two types of biomass burning organic aerosol (BBOA) were generated...
Altmetrics
Final-revised paper
Preprint