Articles | Volume 18, issue 23
https://doi.org/10.5194/acp-18-17259-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-17259-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
06 Dec 2018
Research article |
| 06 Dec 2018
| 06 Dec 2018
Airborne and ground-based observations of ammonium-nitrate-dominated aerosols in a shallow boundary layer during intense winter pollution episodes in northern Utah
Alessandro Franchin
CORRESPONDING AUTHOR
NOAA Earth System Research Laboratory (ESRL) Chemical Sciences
Division, 325 Broadway, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences (CIRES),
University of Colorado, Boulder, CO 80309, USA
Dorothy L. Fibiger
NOAA Earth System Research Laboratory (ESRL) Chemical Sciences
Division, 325 Broadway, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences (CIRES),
University of Colorado, Boulder, CO 80309, USA
now at: California Air Resources Board, Monitoring and
Laboratory Division, Sacramento, CA 95811, USA
Lexie Goldberger
University of Washington, Department of Atmospheric Sciences,
Seattle, WA 98195, USA
now at: Pacific Northwest National Laboratory, Richland, WA 99354,
USA
Erin E. McDuffie
NOAA Earth System Research Laboratory (ESRL) Chemical Sciences
Division, 325 Broadway, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences (CIRES),
University of Colorado, Boulder, CO 80309, USA
Alexander Moravek
Department of Chemistry, University of Toronto, Toronto, ON M5S 3H6,
Canada
Caroline C. Womack
NOAA Earth System Research Laboratory (ESRL) Chemical Sciences
Division, 325 Broadway, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences (CIRES),
University of Colorado, Boulder, CO 80309, USA
Erik T. Crosman
University of Utah, Department of Atmospheric Sciences, Salt Lake
City, UT 84112, USA
Kenneth S. Docherty
Jacobs Technology, Inc., RTP, NC 27709, Durham, NC 27709, USA
William P. Dube
NOAA Earth System Research Laboratory (ESRL) Chemical Sciences
Division, 325 Broadway, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences (CIRES),
University of Colorado, Boulder, CO 80309, USA
Sebastian W. Hoch
University of Utah, Department of Atmospheric Sciences, Salt Lake
City, UT 84112, USA
Ben H. Lee
University of Washington, Department of Atmospheric Sciences,
Seattle, WA 98195, USA
Russell Long
Environmental Protection Agency (EPA), Durham, NC 27709, USA
Jennifer G. Murphy
Department of Chemistry, University of Toronto, Toronto, ON M5S 3H6,
Canada
Joel A. Thornton
University of Washington, Department of Atmospheric Sciences,
Seattle, WA 98195, USA
Steven S. Brown
NOAA Earth System Research Laboratory (ESRL) Chemical Sciences
Division, 325 Broadway, Boulder, CO 80305, USA
Munkhbayar Baasandorj
University of Utah, Department of Atmospheric Sciences, Salt Lake
City, UT 84112, USA
Ann M. Middlebrook
NOAA Earth System Research Laboratory (ESRL) Chemical Sciences
Division, 325 Broadway, Boulder, CO 80305, USA
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Cited
34 citations as recorded by crossref.
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- Global Nitrogen Cycle: Critical Enzymes, Organisms, and Processes for Nitrogen Budgets and Dynamics X. Zhang et al. 10.1021/acs.chemrev.9b00613
- Nitrate pollution deterioration in winter driven by surface ozone increase Z. Zhang et al. 10.1038/s41612-024-00667-5
- High efficiency of nitric acid controls in alleviating particulate nitrate in livestock and urban areas in South Korea H. Kim et al. 10.1039/D2EA00051B
- Increased night-time oxidation over China despite widespread decrease across the globe H. Wang et al. 10.1038/s41561-022-01122-x
- On the contribution of nocturnal heterogeneous reactive nitrogen chemistry to particulate matter formation during wintertime pollution events in Northern Utah E. McDuffie et al. 10.5194/acp-19-9287-2019
- Elucidating HONO formation mechanism and its essential contribution to OH during haze events X. Zhang et al. 10.1038/s41612-023-00371-w
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- Secondary aerosol formation drives atmospheric particulate matter pollution over megacities (Beijing and Seoul) in East Asia Y. Qiu et al. 10.1016/j.atmosenv.2023.119702
- Abundant nitrogen oxide and weakly acidic environment synergistically promote daytime particulate nitrate pollution Y. Wei et al. 10.1016/j.jhazmat.2023.131655
- Assessing PM2.5 model performance for the conterminous U.S. with comparison to model performance statistics from 2007-2015 J. Kelly et al. 10.1016/j.atmosenv.2019.116872
- An Odd Oxygen Framework for Wintertime Ammonium Nitrate Aerosol Pollution in Urban Areas: NOx and VOC Control as Mitigation Strategies C. Womack et al. 10.1029/2019GL082028
- A Satellite-Based Indicator for Diagnosing Particulate Nitrate Sensitivity to Precursor Emissions: Application to East Asia, Europe, and North America R. Dang et al. 10.1021/acs.est.4c08082
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- Twenty-Year Review of Outdoor Air Quality in Utah, USA C. Flowerday et al. 10.3390/atmos14101496
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- Human Health and Economic Costs of Air Pollution in Utah: An Expert Assessment I. Errigo et al. 10.3390/atmos11111238
- Wintertime haze and ozone at Dinosaur National Monument A. Prenni et al. 10.1080/10962247.2022.2048922
- Wintertime Particulate Matter Decrease Buffered by Unfavorable Chemical Processes Despite Emissions Reductions in China D. Leung et al. 10.1029/2020GL087721
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- Reactive nitrogen and total organic carbon calibration techniques for the Aerodyne aerosol mass spectrometer D. Price et al. 10.1080/02786826.2023.2218462
- Wintertime spatial distribution of ammonia and its emission sources in the Great Salt Lake region A. Moravek et al. 10.5194/acp-19-15691-2019
- The proceeded ammonia release from ammonium nitrate owing to sodium malonate addition: Dependence of RH, acidity and surfactant W. Wang et al. 10.1016/j.jaerosci.2023.106315
- Impact of aerosol-boundary layer interactions on PM2.5 pollution during cold air pool events in a semi-arid urban basin M. Zhang et al. 10.1016/j.scitotenv.2024.171225
- Box Model Applications for Secondary Inorganic Aerosol: A Review Focused on Nitrate Formation S. Park 10.5572/KOSAE.2024.40.1.1
- Diagnosing the Sensitivity of Particulate Nitrate to Precursor Emissions Using Satellite Observations of Ammonia and Nitrogen Dioxide R. Dang et al. 10.1029/2023GL105761
- An Observational Based Modeling of the Surface Layer Particulate Nitrate in the North China Plain During Summertime Z. Tan et al. 10.1029/2021JD035623
- Particulate nitrate photolysis in the atmosphere M. Gen et al. 10.1039/D1EA00087J
34 citations as recorded by crossref.
- Midlatitude Ozone Depletion and Air Quality Impacts from Industrial Halogen Emissions in the Great Salt Lake Basin C. Womack et al. 10.1021/acs.est.2c05376
- Global Nitrogen Cycle: Critical Enzymes, Organisms, and Processes for Nitrogen Budgets and Dynamics X. Zhang et al. 10.1021/acs.chemrev.9b00613
- Nitrate pollution deterioration in winter driven by surface ozone increase Z. Zhang et al. 10.1038/s41612-024-00667-5
- High efficiency of nitric acid controls in alleviating particulate nitrate in livestock and urban areas in South Korea H. Kim et al. 10.1039/D2EA00051B
- Increased night-time oxidation over China despite widespread decrease across the globe H. Wang et al. 10.1038/s41561-022-01122-x
- On the contribution of nocturnal heterogeneous reactive nitrogen chemistry to particulate matter formation during wintertime pollution events in Northern Utah E. McDuffie et al. 10.5194/acp-19-9287-2019
- Elucidating HONO formation mechanism and its essential contribution to OH during haze events X. Zhang et al. 10.1038/s41612-023-00371-w
- The relationship between Brown haze, atmospheric boundary layer structure, and air pollution in an urban area of complex coastal terrain H. Marley et al. 10.1016/j.apr.2021.101057
- Secondary aerosol formation drives atmospheric particulate matter pollution over megacities (Beijing and Seoul) in East Asia Y. Qiu et al. 10.1016/j.atmosenv.2023.119702
- Abundant nitrogen oxide and weakly acidic environment synergistically promote daytime particulate nitrate pollution Y. Wei et al. 10.1016/j.jhazmat.2023.131655
- Assessing PM2.5 model performance for the conterminous U.S. with comparison to model performance statistics from 2007-2015 J. Kelly et al. 10.1016/j.atmosenv.2019.116872
- An Odd Oxygen Framework for Wintertime Ammonium Nitrate Aerosol Pollution in Urban Areas: NOx and VOC Control as Mitigation Strategies C. Womack et al. 10.1029/2019GL082028
- A Satellite-Based Indicator for Diagnosing Particulate Nitrate Sensitivity to Precursor Emissions: Application to East Asia, Europe, and North America R. Dang et al. 10.1021/acs.est.4c08082
- The formation and mitigation of nitrate pollution: comparison between urban and suburban environments S. Yang et al. 10.5194/acp-22-4539-2022
- A case study of heavy PM2.5 secondary formation by N2O5 nocturnal chemistry in Seoul, Korea in January 2018: Model performance and error analysis H. Jo et al. 10.1016/j.atmosres.2021.105951
- An ensemble-based model of PM2.5 concentration across the contiguous United States with high spatiotemporal resolution Q. Di et al. 10.1016/j.envint.2019.104909
- The role of coarse aerosol particles as a sink of HNO<sub>3</sub> in wintertime pollution events in the Salt Lake Valley A. Hrdina et al. 10.5194/acp-21-8111-2021
- Twenty-Year Review of Outdoor Air Quality in Utah, USA C. Flowerday et al. 10.3390/atmos14101496
- Development and evaluation of processes affecting simulation of diel fine particulate matter variation in the GEOS-Chem model Y. Li et al. 10.5194/acp-23-12525-2023
- Human Health and Economic Costs of Air Pollution in Utah: An Expert Assessment I. Errigo et al. 10.3390/atmos11111238
- Wintertime haze and ozone at Dinosaur National Monument A. Prenni et al. 10.1080/10962247.2022.2048922
- Wintertime Particulate Matter Decrease Buffered by Unfavorable Chemical Processes Despite Emissions Reductions in China D. Leung et al. 10.1029/2020GL087721
- Airborne flux measurements of ammonia over the southern Great Plains using chemical ionization mass spectrometry S. Schobesberger et al. 10.5194/amt-16-247-2023
- Summary of PM2.5 measurement artifacts associated with the Teledyne T640 PM Mass Monitor under controlled chamber experimental conditions using polydisperse ammonium sulfate aerosols and biomass smoke R. Long et al. 10.1080/10962247.2023.2171156
- Analysis of Wintertime Nitrate Formation in Seoul Using Box Model Simulations M. Yeo et al. 10.5572/KOSAE.2024.40.4.427
- Tracking ammonia morning peak, sources and transport with 1 Hz measurements at a rural site in North China Plain Y. He et al. 10.1016/j.atmosenv.2020.117630
- Reactive nitrogen and total organic carbon calibration techniques for the Aerodyne aerosol mass spectrometer D. Price et al. 10.1080/02786826.2023.2218462
- Wintertime spatial distribution of ammonia and its emission sources in the Great Salt Lake region A. Moravek et al. 10.5194/acp-19-15691-2019
- The proceeded ammonia release from ammonium nitrate owing to sodium malonate addition: Dependence of RH, acidity and surfactant W. Wang et al. 10.1016/j.jaerosci.2023.106315
- Impact of aerosol-boundary layer interactions on PM2.5 pollution during cold air pool events in a semi-arid urban basin M. Zhang et al. 10.1016/j.scitotenv.2024.171225
- Box Model Applications for Secondary Inorganic Aerosol: A Review Focused on Nitrate Formation S. Park 10.5572/KOSAE.2024.40.1.1
- Diagnosing the Sensitivity of Particulate Nitrate to Precursor Emissions Using Satellite Observations of Ammonia and Nitrogen Dioxide R. Dang et al. 10.1029/2023GL105761
- An Observational Based Modeling of the Surface Layer Particulate Nitrate in the North China Plain During Summertime Z. Tan et al. 10.1029/2021JD035623
- Particulate nitrate photolysis in the atmosphere M. Gen et al. 10.1039/D1EA00087J
Latest update: 14 Dec 2024
Short summary
We present the results of aerosol and trace gas measurements from airborne and ground-based platforms. The measurements took place in January–February 2017 in northern Utah as part of the Utah Winter Fine Particulate Study (UWFPS). We characterized the chemical composition of PM1 on a regional scale, also probing the vertical dimension. We used a thermodynamic model to study the effectiveness of limiting total ammonium or total nitrate as a strategy to control aerosol concentrations.
We present the results of aerosol and trace gas measurements from airborne and ground-based...
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