Articles | Volume 18, issue 23
https://doi.org/10.5194/acp-18-16829-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-16829-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
29 Nov 2018
Research article |
| 29 Nov 2018
| 29 Nov 2018
The influence of photochemical aging on light absorption of atmospheric black carbon and aerosol single-scattering albedo
Xuezhe Xu
Laboratory of Atmospheric Physico-Chemistry, Anhui Institute of
Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei, 230031, Anhui,
China
Graduate School, University of Science and Technology of
China, Hefei, 230026, Anhui, China
Laboratory of Atmospheric Physico-Chemistry, Anhui Institute of
Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei, 230031, Anhui,
China
Xiaodong Qian
Laboratory of Atmospheric Physico-Chemistry, Anhui Institute of
Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei, 230031, Anhui,
China
Graduate School, University of Science and Technology of
China, Hefei, 230026, Anhui, China
Shuo Wang
Laboratory of Atmospheric Physico-Chemistry, Anhui Institute of
Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei, 230031, Anhui,
China
Graduate School, University of Science and Technology of
China, Hefei, 230026, Anhui, China
Laboratory of Atmospheric Physico-Chemistry, Anhui Institute of
Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei, 230031, Anhui,
China
Qilei Zhang
Laboratory of Atmospheric Physico-Chemistry, Anhui Institute of
Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei, 230031, Anhui,
China
Graduate School, University of Science and Technology of
China, Hefei, 230026, Anhui, China
Weijun Zhang
CORRESPONDING AUTHOR
Laboratory of Atmospheric Physico-Chemistry, Anhui Institute of
Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei, 230031, Anhui,
China
Graduate School, University of Science and Technology of
China, Hefei, 230026, Anhui, China
School of Environmental Science
and Optoelectronic Technology, University of Science and Technology of China,
Hefei, 230026, Anhui, China
Dean S. Venables
School of Chemistry and Environmental
Research Institute, University College Cork, Cork, Ireland
Weidong Chen
Laboratoire de Physicochimie de l'Atmosphère, Université du
Littoral Côte d'Opale, 59140 Dunkerque, France
Yong Huang
Anhui Institute
of Meteorological Science, Hefei, 230031, Anhui, China
Shouxian
National Climatology Observatory, Shouxian, 232200, Anhui, China
Xueliang Deng
Anhui Institute
of Meteorological Science, Hefei, 230031, Anhui, China
Shouxian
National Climatology Observatory, Shouxian, 232200, Anhui, China
Biwen Wu
Anhui Institute
of Meteorological Science, Hefei, 230031, Anhui, China
Shouxian
National Climatology Observatory, Shouxian, 232200, Anhui, China
Xinfeng Lin
Shouxian
National Climatology Observatory, Shouxian, 232200, Anhui, China
Anhui Shouxian Meteorological Bureau, Shouxian, 232200, Anhui,
China
Sen Zhao
Shouxian
National Climatology Observatory, Shouxian, 232200, Anhui, China
Anhui Shouxian Meteorological Bureau, Shouxian, 232200, Anhui,
China
Yingxiang Tong
Shouxian
National Climatology Observatory, Shouxian, 232200, Anhui, China
Anhui Shouxian Meteorological Bureau, Shouxian, 232200, Anhui,
China
Viewed
Total article views: 4,340 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 26 Mar 2018)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 2,953 | 1,303 | 84 | 4,340 | 379 | 83 | 103 |
- HTML: 2,953
- PDF: 1,303
- XML: 84
- Total: 4,340
- Supplement: 379
- BibTeX: 83
- EndNote: 103
Total article views: 3,089 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 29 Nov 2018)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 2,179 | 842 | 68 | 3,089 | 219 | 70 | 87 |
- HTML: 2,179
- PDF: 842
- XML: 68
- Total: 3,089
- Supplement: 219
- BibTeX: 70
- EndNote: 87
Total article views: 1,251 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 26 Mar 2018)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 774 | 461 | 16 | 1,251 | 160 | 13 | 16 |
- HTML: 774
- PDF: 461
- XML: 16
- Total: 1,251
- Supplement: 160
- BibTeX: 13
- EndNote: 16
Viewed (geographical distribution)
Total article views: 4,340 (including HTML, PDF, and XML)
Thereof 4,193 with geography defined
and 147 with unknown origin.
Total article views: 3,089 (including HTML, PDF, and XML)
Thereof 2,956 with geography defined
and 133 with unknown origin.
Total article views: 1,251 (including HTML, PDF, and XML)
Thereof 1,237 with geography defined
and 14 with unknown origin.
| Country | # | Views | % |
|---|
| Country | # | Views | % |
|---|
| Country | # | Views | % |
|---|
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
Cited
40 citations as recorded by crossref.
- In situ optical and microphysical properties of tropospheric aerosols in the Canadian High Arctic from 2016 to 2019 A. Vicente-Luis et al. 10.1016/j.atmosenv.2021.118254
- Effects of Polyoxymethylene Dimethyl Ether (PODEn) Blended Fuel on Diesel Engine Emission: Insight from Soot-Particle Aerosol Mass Spectrometry and Aethalometer Measurements M. Ma et al. 10.2139/ssrn.4197569
- Amplification of black carbon light absorption induced by atmospheric aging: temporal variation at seasonal and diel scales in urban Guangzhou J. Sun et al. 10.5194/acp-20-2445-2020
- Exploring the Drivers and Photochemical Impact of the Positive Correlation between Single Scattering Albedo and Aerosol Optical Depth in the Troposphere W. Wang et al. 10.1021/acs.estlett.1c00300
- Photochemical evolution of the molecular composition of dissolved organic carbon and dissolved brown carbon from wood smoldering R. Zhao et al. 10.1016/j.envint.2024.108629
- Quantifying the effects of the microphysical hygroscopic restructuring of soot on ensemble optical properties and satellite aerosol optical depth retrievals K. Chang et al. 10.1016/j.scitotenv.2024.177821
- Filter-based absorption enhancement measurement for internally mixed black carbon particles over southern China Y. Fu et al. 10.1016/j.scitotenv.2020.144194
- Absorption closure in highly aged biomass burning smoke J. Taylor et al. 10.5194/acp-20-11201-2020
- Estimating mass-absorption cross-section of ambient black carbon aerosols: Theoretical, empirical, and machine learning models H. Li & A. May 10.1080/02786826.2022.2114311
- Enhancing Our Vision of Aerosols: Progress in Scattering Phase Function Measurements Y. Bian & C. Zhao 10.1007/s40726-024-00292-z
- A review of quantification methods for light absorption enhancement of black carbon aerosol Y. Kong et al. 10.1016/j.scitotenv.2024.171539
- High contributions of fossil fuel sources to char-EC/soot-EC at a high-altitude site: Direct radiative effects and transport pathway H. Liu et al. 10.1016/j.fuel.2023.130632
- Absorption enhancement of black carbon particles in a Mediterranean city and countryside: effect of particulate matter chemistry, ageing and trend analysis J. Yus-Díez et al. 10.5194/acp-22-8439-2022
- Secondary inorganic aerosol dominated the light absorption enhancement of black carbon aerosol in Wuhan, Central China H. Zheng et al. 10.1016/j.atmosenv.2022.119288
- Unmanned-aerial-vehicle-borne cavity enhanced albedometer: a powerful tool for simultaneous in-situ measurement of aerosol light scattering and absorption vertical profiles J. Zhou et al. 10.1364/OE.493696
- Photocatalytic O2 activation carried out by organic aerosol: A case study of 1, 8-naphthalic anhydride T. Dong et al. 10.1016/j.apcatb.2024.123889
- Broadband spectrum characteristics and radiative effects of primary brown carbon from wood pyrolysis Q. Liu et al. 10.1016/j.scitotenv.2023.163500
- Spatiotemporal Distribution of Major Aerosol Types over China Based on MODIS Products between 2008 and 2017 Q. Chen et al. 10.3390/atmos11070703
- Optical Modeling of Black Carbon With Different Coating Materials: The Effect of Coating Configurations J. Luo et al. 10.1029/2019JD031701
- Light absorption enhancement of black carbon and its impact factors during winter in a megacity of the Sichuan Basin, China Y. Lan et al. 10.1016/j.scitotenv.2024.170374
- A Review of the Representation of Aerosol Mixing State in Atmospheric Models R. Stevens & A. Dastoor 10.3390/atmos10040168
- Absorption enhancement of black carbon and the contribution of brown carbon to light absorption in the summer of Nanjing, China F. Cui et al. 10.1016/j.apr.2020.12.008
- Black Carbon Involved Photochemistry Enhances the Formation of Sulfate in the Ambient Atmosphere: Evidence From In Situ Individual Particle Investigation G. Zhang et al. 10.1029/2021JD035226
- Retrieval of refractive index and water content for the coating materials of aged black carbon aerosol based on optical properties: a theoretical analysis J. Liu et al. 10.5194/acp-24-12341-2024
- Moisture-induced secondary inorganic aerosol formation dominated the light absorption enhancement of refractory black carbon at an urban site in northwest China Z. Chen et al. 10.1016/j.atmosenv.2023.120113
- Effects of polyoxymethylene dimethyl ether (PODEn) blended fuel on diesel engine emission: Insight from soot-particle aerosol mass spectrometry and aethalometer measurements M. Ma et al. 10.1016/j.aeaoa.2023.100216
- Effect of urban submicron particles on single scattering albedo: the case study of high pollution event J. Pauraite et al. 10.1016/j.jqsrt.2022.108075
- Simultaneous measurements of the relative-humidity-dependent aerosol light extinction, scattering, absorption, and single-scattering albedo with a humidified cavity-enhanced albedometer J. Zhou et al. 10.5194/amt-13-2623-2020
- Real-time retrieval of aerosol chemical composition using effective density and the imaginary part of complex refractive index S. Wang et al. 10.1016/j.atmosenv.2020.117959
- Mixing state of refractory black carbon in fog and haze at rural sites in winter on the North China Plain Y. Zhang et al. 10.5194/acp-21-17631-2021
- Mass Absorption Efficiency of PM1 in Mexico City during ACU15 C. Prieto et al. 10.3390/atmos14010100
- Seasonal variations in fire conditions are important drivers in the trend of aerosol optical properties over the south-eastern Atlantic H. Che et al. 10.5194/acp-22-8767-2022
- Black Carbon over Wuhan, China: Seasonal Variations in Its Optical Properties, Radiative Forcing and Contribution to Atmospheric Aerosols Y. Ma et al. 10.3390/rs13183620
- Seasonal variation and source analyses of aerosol optical properties in Nanjing, China F. Cui et al. 10.1016/j.apr.2021.101117
- Higher absorption enhancement of black carbon in summer shown by 2-year measurements at the high-altitude mountain site of Pic du Midi Observatory in the French Pyrenees S. Tinorua et al. 10.5194/acp-24-1801-2024
- Aging of biomass burning emissions in the Indo-Gangetic Plain outflow: Implications for black carbon light-absorption enhancement S. Kompalli et al. 10.1016/j.atmosres.2023.106949
- An improved representation of aerosol mixing state for air quality–weather interactions R. Stevens et al. 10.5194/acp-22-13527-2022
- Effect of Photooxidation on Size Distribution, Light Absorption, and Molecular Compositions of Smoke Particles from Rice Straw Combustion R. Zhao et al. 10.2139/ssrn.4095686
- Impact of aerosol-boundary layer interactions on PM2.5 pollution during cold air pool events in a semi-arid urban basin M. Zhang et al. 10.1016/j.scitotenv.2024.171225
- Cloud droplet activation of black carbon particles coated with organic compounds of varying solubility M. Dalirian et al. 10.5194/acp-18-12477-2018
39 citations as recorded by crossref.
- In situ optical and microphysical properties of tropospheric aerosols in the Canadian High Arctic from 2016 to 2019 A. Vicente-Luis et al. 10.1016/j.atmosenv.2021.118254
- Effects of Polyoxymethylene Dimethyl Ether (PODEn) Blended Fuel on Diesel Engine Emission: Insight from Soot-Particle Aerosol Mass Spectrometry and Aethalometer Measurements M. Ma et al. 10.2139/ssrn.4197569
- Amplification of black carbon light absorption induced by atmospheric aging: temporal variation at seasonal and diel scales in urban Guangzhou J. Sun et al. 10.5194/acp-20-2445-2020
- Exploring the Drivers and Photochemical Impact of the Positive Correlation between Single Scattering Albedo and Aerosol Optical Depth in the Troposphere W. Wang et al. 10.1021/acs.estlett.1c00300
- Photochemical evolution of the molecular composition of dissolved organic carbon and dissolved brown carbon from wood smoldering R. Zhao et al. 10.1016/j.envint.2024.108629
- Quantifying the effects of the microphysical hygroscopic restructuring of soot on ensemble optical properties and satellite aerosol optical depth retrievals K. Chang et al. 10.1016/j.scitotenv.2024.177821
- Filter-based absorption enhancement measurement for internally mixed black carbon particles over southern China Y. Fu et al. 10.1016/j.scitotenv.2020.144194
- Absorption closure in highly aged biomass burning smoke J. Taylor et al. 10.5194/acp-20-11201-2020
- Estimating mass-absorption cross-section of ambient black carbon aerosols: Theoretical, empirical, and machine learning models H. Li & A. May 10.1080/02786826.2022.2114311
- Enhancing Our Vision of Aerosols: Progress in Scattering Phase Function Measurements Y. Bian & C. Zhao 10.1007/s40726-024-00292-z
- A review of quantification methods for light absorption enhancement of black carbon aerosol Y. Kong et al. 10.1016/j.scitotenv.2024.171539
- High contributions of fossil fuel sources to char-EC/soot-EC at a high-altitude site: Direct radiative effects and transport pathway H. Liu et al. 10.1016/j.fuel.2023.130632
- Absorption enhancement of black carbon particles in a Mediterranean city and countryside: effect of particulate matter chemistry, ageing and trend analysis J. Yus-Díez et al. 10.5194/acp-22-8439-2022
- Secondary inorganic aerosol dominated the light absorption enhancement of black carbon aerosol in Wuhan, Central China H. Zheng et al. 10.1016/j.atmosenv.2022.119288
- Unmanned-aerial-vehicle-borne cavity enhanced albedometer: a powerful tool for simultaneous in-situ measurement of aerosol light scattering and absorption vertical profiles J. Zhou et al. 10.1364/OE.493696
- Photocatalytic O2 activation carried out by organic aerosol: A case study of 1, 8-naphthalic anhydride T. Dong et al. 10.1016/j.apcatb.2024.123889
- Broadband spectrum characteristics and radiative effects of primary brown carbon from wood pyrolysis Q. Liu et al. 10.1016/j.scitotenv.2023.163500
- Spatiotemporal Distribution of Major Aerosol Types over China Based on MODIS Products between 2008 and 2017 Q. Chen et al. 10.3390/atmos11070703
- Optical Modeling of Black Carbon With Different Coating Materials: The Effect of Coating Configurations J. Luo et al. 10.1029/2019JD031701
- Light absorption enhancement of black carbon and its impact factors during winter in a megacity of the Sichuan Basin, China Y. Lan et al. 10.1016/j.scitotenv.2024.170374
- A Review of the Representation of Aerosol Mixing State in Atmospheric Models R. Stevens & A. Dastoor 10.3390/atmos10040168
- Absorption enhancement of black carbon and the contribution of brown carbon to light absorption in the summer of Nanjing, China F. Cui et al. 10.1016/j.apr.2020.12.008
- Black Carbon Involved Photochemistry Enhances the Formation of Sulfate in the Ambient Atmosphere: Evidence From In Situ Individual Particle Investigation G. Zhang et al. 10.1029/2021JD035226
- Retrieval of refractive index and water content for the coating materials of aged black carbon aerosol based on optical properties: a theoretical analysis J. Liu et al. 10.5194/acp-24-12341-2024
- Moisture-induced secondary inorganic aerosol formation dominated the light absorption enhancement of refractory black carbon at an urban site in northwest China Z. Chen et al. 10.1016/j.atmosenv.2023.120113
- Effects of polyoxymethylene dimethyl ether (PODEn) blended fuel on diesel engine emission: Insight from soot-particle aerosol mass spectrometry and aethalometer measurements M. Ma et al. 10.1016/j.aeaoa.2023.100216
- Effect of urban submicron particles on single scattering albedo: the case study of high pollution event J. Pauraite et al. 10.1016/j.jqsrt.2022.108075
- Simultaneous measurements of the relative-humidity-dependent aerosol light extinction, scattering, absorption, and single-scattering albedo with a humidified cavity-enhanced albedometer J. Zhou et al. 10.5194/amt-13-2623-2020
- Real-time retrieval of aerosol chemical composition using effective density and the imaginary part of complex refractive index S. Wang et al. 10.1016/j.atmosenv.2020.117959
- Mixing state of refractory black carbon in fog and haze at rural sites in winter on the North China Plain Y. Zhang et al. 10.5194/acp-21-17631-2021
- Mass Absorption Efficiency of PM1 in Mexico City during ACU15 C. Prieto et al. 10.3390/atmos14010100
- Seasonal variations in fire conditions are important drivers in the trend of aerosol optical properties over the south-eastern Atlantic H. Che et al. 10.5194/acp-22-8767-2022
- Black Carbon over Wuhan, China: Seasonal Variations in Its Optical Properties, Radiative Forcing and Contribution to Atmospheric Aerosols Y. Ma et al. 10.3390/rs13183620
- Seasonal variation and source analyses of aerosol optical properties in Nanjing, China F. Cui et al. 10.1016/j.apr.2021.101117
- Higher absorption enhancement of black carbon in summer shown by 2-year measurements at the high-altitude mountain site of Pic du Midi Observatory in the French Pyrenees S. Tinorua et al. 10.5194/acp-24-1801-2024
- Aging of biomass burning emissions in the Indo-Gangetic Plain outflow: Implications for black carbon light-absorption enhancement S. Kompalli et al. 10.1016/j.atmosres.2023.106949
- An improved representation of aerosol mixing state for air quality–weather interactions R. Stevens et al. 10.5194/acp-22-13527-2022
- Effect of Photooxidation on Size Distribution, Light Absorption, and Molecular Compositions of Smoke Particles from Rice Straw Combustion R. Zhao et al. 10.2139/ssrn.4095686
- Impact of aerosol-boundary layer interactions on PM2.5 pollution during cold air pool events in a semi-arid urban basin M. Zhang et al. 10.1016/j.scitotenv.2024.171225
1 citations as recorded by crossref.
Saved (final revised paper)
Saved (preprint)
Latest update: 14 Dec 2024
Short summary
We report the direct field measurement of size-resolved mixing state, Eabs, and aerosol single-scattering albedo (SSA) at λ = 532 nm at a rural site in east China in summer. Parameterization of Eabs and SSA captures much of the influence of black carbon (BC) coating and particle absorption. The results show that absorption amplification depends on the coating thickness and the absorption of coating materials, and photochemistry plays role in modifying the absorption of BC-containing particles.
We report the direct field measurement of size-resolved mixing state, Eabs, and aerosol...
Altmetrics
Final-revised paper
Preprint