Articles | Volume 18, issue 21
https://doi.org/10.5194/acp-18-16099-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-16099-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
08 Nov 2018
Research article |
| 08 Nov 2018
| 08 Nov 2018
Is there an aerosol signature of chemical cloud processing?
NOAA/ESRL/Chemical Sciences Division, Boulder, CO, USA
CIRES, University of Colorado, Boulder, CO, USA
now at: Université Clermont Auvergne, CNRS, SIGMA Clermont, Institut de Chimie de Clermont-Ferrand, Clermont-Ferrand, France
Department of Chemical and Environmental Engineering, University of Arizona, Tucson, AZ, USA
Department of Hydrology and Atmospheric Sciences, University of Arizona, Tucson, AZ, USA
Abdulmonam M. Aldhaif
Department of Chemical and Environmental Engineering, University of Arizona, Tucson, AZ, USA
Taylor Shingler
Science Systems and Applications, Inc., Hampton, VA, USA
NASA Langley Research Center, Hampton, VA, USA
Ewan Crosbie
Science Systems and Applications, Inc., Hampton, VA, USA
NASA Langley Research Center, Hampton, VA, USA
Luke Ziemba
NASA Langley Research Center, Hampton, VA, USA
Pedro Campuzano-Jost
CIRES, University of Colorado, Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
Jose L. Jimenez
CIRES, University of Colorado, Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
Armin Wisthaler
Department of Chemistry, University of Oslo, Oslo, Norway
Institute for Ion Physics and Applied Physics, University of Innsbruck, Innsbruck, Austria
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32 citations as recorded by crossref.
- The effect of clouds and precipitation on the aerosol concentrations and composition in a boreal forest environment S. Isokääntä et al. 10.5194/acp-22-11823-2022
- Source apportionment of soot particles and aqueous-phase processing of black carbon coatings in an urban environment R. Farley et al. 10.5194/acp-23-15039-2023
- Biomass burning and marine aerosol processing over the southeast Atlantic Ocean: a TEM single-particle analysis C. Dang et al. 10.5194/acp-22-9389-2022
- Fog/cloud processing of atmospheric aerosols from a single particle perspective: A review of field observations G. Zhang et al. 10.1016/j.atmosenv.2024.120536
- Temperature-dependent aqueous OH kinetics of C2–C10 linear and terpenoid alcohols and diols: new rate coefficients, structure–activity relationship, and atmospheric lifetimes B. Witkowski et al. 10.5194/acp-24-663-2024
- An emerging aerosol climatology via remote sensing over Metro Manila, the Philippines G. Lorenzo et al. 10.5194/acp-23-10579-2023
- An automated size and time-resolved aerosol collector platform integrated with environmental sensors to study the vertical profile of aerosols Z. Cheng et al. 10.1039/D2EA00097K
- Interfacial Dark Aging Is an Overlooked Source of Aqueous Secondary Organic Aerosol F. Zhang et al. 10.3390/atmos13020188
- Measurement report: Closure analysis of aerosol–cloud composition in tropical maritime warm convection E. Crosbie et al. 10.5194/acp-22-13269-2022
- Chemical characteristics of cloud water and the impacts on aerosol properties at a subtropical mountain site in Hong Kong SAR T. Li et al. 10.5194/acp-20-391-2020
- Atmospheric Research Over the Western North Atlantic Ocean Region and North American East Coast: A Review of Past Work and Challenges Ahead A. Sorooshian et al. 10.1029/2019JD031626
- Large contribution to secondary organic aerosol from isoprene cloud chemistry H. Lamkaddam et al. 10.1126/sciadv.abe2952
- CCN measurements at the Princess Elisabeth Antarctica research station during three austral summers P. Herenz et al. 10.5194/acp-19-275-2019
- Long-range aerosol transport and impacts on size-resolved aerosol composition in Metro Manila, Philippines R. Braun et al. 10.5194/acp-20-2387-2020
- Vertical Gradient of Size-Resolved Aerosol Compositions over the Arctic Reveals Cloud Processed Aerosol in-Cloud and above Cloud N. Lata et al. 10.1021/acs.est.2c09498
- Understanding the Evolution of Smoke Mass Extinction Efficiency Using Field Campaign Measurements P. Saide et al. 10.1029/2022GL099175
- Detrainment Dominates CCN Concentrations Around Non‐Precipitating Convective Clouds Over the Amazon R. Braga et al. 10.1029/2022GL100411
- An annual time series of weekly size-resolved aerosol properties in the megacity of Metro Manila, Philippines C. Stahl et al. 10.1038/s41597-020-0466-y
- Size-resolved composition and morphology of particulate matter during the southwest monsoon in Metro Manila, Philippines M. Cruz et al. 10.5194/acp-19-10675-2019
- Impacts of Cloud‐Processing on Ice Nucleation of Soot Particles Internally Mixed With Sulfate and Organics K. Gao & Z. Kanji 10.1029/2022JD037146
- Diverse sources and aging change the mixing state and ice nucleation properties of aerosol particles over the western Pacific and Southern Ocean J. Xue et al. 10.5194/acp-24-7731-2024
- High-altitude aerosol chemical characterization and source identification: insights from the CALISHTO campaign O. Zografou et al. 10.5194/acp-24-8911-2024
- Characterizing Weekly Cycles of Particulate Matter in a Coastal Megacity: The Importance of a Seasonal, Size‐Resolved, and Chemically Speciated Analysis M. Hilario et al. 10.1029/2020JD032614
- Improvement of inorganic aerosol component in PM2.5 by constraining aqueous-phase formation of sulfate in cloud with satellite retrievals: WRF-Chem simulations T. Sha et al. 10.1016/j.scitotenv.2021.150229
- Chemical Signatures of Seasonally Unique Anthropogenic Influences on Organic Aerosol Composition in the Central Amazon E. Franklin et al. 10.1021/acs.est.2c07260
- Aerosol–cloud impacts on aerosol detrainment and rainout in shallow maritime tropical clouds G. Leung et al. 10.5194/acp-23-5263-2023
- Is There a Relationship between Lake Urmia Saline Lakebed Emissions and Wet Deposition Composition in the Caucasus Region? H. Ahmady-Birgani et al. 10.1021/acsearthspacechem.1c00320
- Influence of open ocean biogeochemistry on aerosol and clouds: Recent findings and perspectives K. Sellegri et al. 10.1525/elementa.2023.00058
- Anomalous Noble Gas Solubility in Liquid Cloud Water: Possible Implications for Noble Gas Temperatures and Cloud Physics C. Hall et al. 10.1029/2020WR029306
- Classification of Clouds Sampled at the Puy de Dôme Station (France) Based on Chemical Measurements and Air Mass History Matrices P. Renard et al. 10.3390/atmos11070732
- Impact of Aerosol-Cloud Cycling on Aqueous Secondary Organic Aerosol Formation W. Tsui et al. 10.3390/atmos10110666
- Differences in fine particle chemical composition on clear and cloudy days A. Christiansen et al. 10.5194/acp-20-11607-2020
Saved (preprint)
Latest update: 21 Nov 2024
Short summary
The paper presents a new framework that can be used to identify emission scenarios in which aerosol populations are most likely modified by chemical processes in clouds. We show that in neither very polluted nor in very clean air masses is this the case. Only if the ratio of possible aerosol mass precursors (sulfur dioxide, some organics) and preexisting aerosol mass is sufficiently high will aerosol particles show substantially modified physicochemical properties upon cloud processing.
The paper presents a new framework that can be used to identify emission scenarios in which...
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