Articles | Volume 18, issue 21
https://doi.org/10.5194/acp-18-16099-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-16099-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
08 Nov 2018
Research article |
| 08 Nov 2018
| 08 Nov 2018
Is there an aerosol signature of chemical cloud processing?
NOAA/ESRL/Chemical Sciences Division, Boulder, CO, USA
CIRES, University of Colorado, Boulder, CO, USA
now at: Université Clermont Auvergne, CNRS, SIGMA Clermont, Institut de Chimie de Clermont-Ferrand, Clermont-Ferrand, France
Department of Chemical and Environmental Engineering, University of Arizona, Tucson, AZ, USA
Department of Hydrology and Atmospheric Sciences, University of Arizona, Tucson, AZ, USA
Abdulmonam M. Aldhaif
Department of Chemical and Environmental Engineering, University of Arizona, Tucson, AZ, USA
Taylor Shingler
Science Systems and Applications, Inc., Hampton, VA, USA
NASA Langley Research Center, Hampton, VA, USA
Ewan Crosbie
Science Systems and Applications, Inc., Hampton, VA, USA
NASA Langley Research Center, Hampton, VA, USA
Luke Ziemba
NASA Langley Research Center, Hampton, VA, USA
Pedro Campuzano-Jost
CIRES, University of Colorado, Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
Jose L. Jimenez
CIRES, University of Colorado, Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
Armin Wisthaler
Department of Chemistry, University of Oslo, Oslo, Norway
Institute for Ion Physics and Applied Physics, University of Innsbruck, Innsbruck, Austria
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Saved (preprint)
Latest update: 17 Apr 2025
Short summary
The paper presents a new framework that can be used to identify emission scenarios in which aerosol populations are most likely modified by chemical processes in clouds. We show that in neither very polluted nor in very clean air masses is this the case. Only if the ratio of possible aerosol mass precursors (sulfur dioxide, some organics) and preexisting aerosol mass is sufficiently high will aerosol particles show substantially modified physicochemical properties upon cloud processing.
The paper presents a new framework that can be used to identify emission scenarios in which...
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