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Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
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The paper presents a new framework that can be used to identify emission scenarios in which aerosol populations are most likely modified by chemical processes in clouds. We show that in neither very polluted nor in very clean air masses is this the case. Only if the ratio of possible aerosol mass precursors (sulfur dioxide, some organics) and preexisting aerosol mass is sufficiently high will aerosol particles show substantially modified physicochemical properties upon cloud processing.
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ACP | Articles | Volume 18, issue 21
Atmos. Chem. Phys., 18, 16099–16119, 2018
https://doi.org/10.5194/acp-18-16099-2018
Atmos. Chem. Phys., 18, 16099–16119, 2018
https://doi.org/10.5194/acp-18-16099-2018

Research article 08 Nov 2018

Research article | 08 Nov 2018

Is there an aerosol signature of chemical cloud processing?

Barbara Ervens et al.

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Short summary
The paper presents a new framework that can be used to identify emission scenarios in which aerosol populations are most likely modified by chemical processes in clouds. We show that in neither very polluted nor in very clean air masses is this the case. Only if the ratio of possible aerosol mass precursors (sulfur dioxide, some organics) and preexisting aerosol mass is sufficiently high will aerosol particles show substantially modified physicochemical properties upon cloud processing.
Citation
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Final-revised paper
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