Simulating secondary organic aerosol from anthropogenic and biogenic precursors: comparison to outdoor chamber experiments, effect of oligomerization on SOA formation and reactive uptake of aldehydes
Florian Couvidat,Marta G. Vivanco,and Bertrand Bessagnet
Institut National de l'Environnement Industriel et des Risques, Verneuil-en-Halatte, France
Marta G. Vivanco
Centro de Investigaciones Energéticas, Medioambientales y Tecnológicas (CIEMAT), Departamento de Medio Ambiente,
Av. Complutense 40, 28040-Madrid, Spain
Bertrand Bessagnet
Institut National de l'Environnement Industriel et des Risques, Verneuil-en-Halatte, France
now at: Hangzhou Futuris Environmental Technology Co. Ltd, Zhejiang Overseas High-Level
Talent Innovation Park, No. 998 WenYi Road, 311121, Hangzhou, Zhejiang, China
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Several new parameterizations and mechanisms for SOA formation are developed based on available experimental results. To evaluate the parameterizations, a box model was developed to simulate SOA formation from monoterpenes and aromatics in the environmental chamber EUPHORE. This box model takes oligomerization, nonideality of the aerosol, multiphase partitioning, aging, vapor wall losses and particle-phase diffusion into account. All these phenomena are rarely taken into account together.
Several new parameterizations and mechanisms for SOA formation are developed based on available...