Articles | Volume 18, issue 18
https://doi.org/10.5194/acp-18-13511-2018
https://doi.org/10.5194/acp-18-13511-2018
Research article
 | 
24 Sep 2018
Research article |  | 24 Sep 2018

Shortwave radiative impact of liquid–liquid phase separation in brown carbon aerosols

Mehrnoush M. Fard, Ulrich K. Krieger, and Thomas Peter

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Short summary
Atmospheric aerosol particles may undergo liquid–liquid phase separation (LLPS) when exposed to varying relative humidity, with an aqueous organic phase enclosing an aqueous inorganic phase below a threshold of relative humidity. Brown carbon (BrC) compounds will redistribute to the organic phase upon LLPS. We use numerical modeling to study the shortwave radiative impact of LLPS containing BrC and conclude that it is not significant for atmospheric aerosol.
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