Articles | Volume 18, issue 18
https://doi.org/10.5194/acp-18-13411-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-13411-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
21 Sep 2018
Research article |
| 21 Sep 2018
| 21 Sep 2018
Exploration of the influence of environmental conditions on secondary organic aerosol formation and organic species properties using explicit simulations: development of the VBS-GECKO parameterization
Victor Lannuque
LISA, UMR CNRS 7583, IPSL, Université Paris Est Créteil and Université Paris Diderot, 94010 Créteil CEDEX, France
INERIS, National Institute for Industrial Environment and Risks, Parc Technologique ALATA, 60550 Verneuil-en-Halatte, France
Agence de l'Environnement et de la Maîtrise de l'Energie, 20 avenue du Grésillé – BP 90406, 49004 Angers CEDEX 01, France
Marie Camredon
CORRESPONDING AUTHOR
LISA, UMR CNRS 7583, IPSL, Université Paris Est Créteil and Université Paris Diderot, 94010 Créteil CEDEX, France
Florian Couvidat
INERIS, National Institute for Industrial Environment and Risks, Parc Technologique ALATA, 60550 Verneuil-en-Halatte, France
Alma Hodzic
National Center for Atmospheric Research, Boulder, CO, USA
Laboratoire d'Aérologie, Observatoire Midi-Pyrénées, Université Paul Sabatier, CNRS, Toulouse, France
Richard Valorso
LISA, UMR CNRS 7583, IPSL, Université Paris Est Créteil and Université Paris Diderot, 94010 Créteil CEDEX, France
Sasha Madronich
National Center for Atmospheric Research, Boulder, CO, USA
Bertrand Bessagnet
INERIS, National Institute for Industrial Environment and Risks, Parc Technologique ALATA, 60550 Verneuil-en-Halatte, France
Bernard Aumont
CORRESPONDING AUTHOR
LISA, UMR CNRS 7583, IPSL, Université Paris Est Créteil and Université Paris Diderot, 94010 Créteil CEDEX, France
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Cited
26 citations as recorded by crossref.
- Nonlinear behavior of organic aerosol in biomass burning plumes: a microphysical model analysis I. Konovalov et al. 10.5194/acp-19-12091-2019
- Opinion: Challenges and needs of tropospheric chemical mechanism development B. Ervens et al. 10.5194/acp-24-13317-2024
- SSH-Aerosol v1.1: A Modular Box Model to Simulate the Evolution of Primary and Secondary Aerosols K. Sartelet et al. 10.3390/atmos11050525
- A Scheme for Representing Aromatic Secondary Organic Aerosols in Chemical Transport Models: Application to Source Attribution of Organic Aerosols Over South Korea During the KORUS‐AQ Campaign J. Brewer et al. 10.1029/2022JD037257
- Influence of the NO/NO2 Ratio on Oxidation Product Distributions under High-NO Conditions K. Nihill et al. 10.1021/acs.est.0c07621
- Contrast in Secondary Organic Aerosols between the Present Day and the Preindustrial Period: The Importance of Nontraditional Sources and the Changed Atmospheric Oxidation Capability Y. Yang et al. 10.1007/s00376-024-3281-0
- Modelling molecular composition of SOA from toluene photo-oxidation at urban and street scales K. Sartelet et al. 10.1039/D4EA00049H
- Gas–particle partitioning of toluene oxidation products: an experimental and modeling study V. Lannuque et al. 10.5194/acp-23-15537-2023
- How does tropospheric VOC chemistry affect climate? An investigation of preindustrial control simulations using the Community Earth System Model version 2 N. Stanton & N. Tandon 10.5194/acp-23-9191-2023
- Polarity on adsorption and photocatalytic performances of N-GR/TiO2 towards gaseous acetaldehyde and ethylene X. Dai et al. 10.1016/j.apsusc.2019.04.221
- Transfer Learning Approach to Multitarget Temperature-Dependent Reaction Rate Prediction E. Al Ibrahim & A. Farooq 10.1021/acs.jpca.2c00713
- Future changes in isoprene-epoxydiol-derived secondary organic aerosol (IEPOX SOA) under the Shared Socioeconomic Pathways: the importance of physicochemical dependency D. Jo et al. 10.5194/acp-21-3395-2021
- Implementation of a parallel reduction algorithm in the GENerator of reduced Organic Aerosol mechanisms (GENOA v2.0): Application to multiple monoterpene aerosol precursors Z. Wang et al. 10.1016/j.jaerosci.2023.106248
- Toward Emulating an Explicit Organic Chemistry Mechanism With Random Forest Models C. Mouchel‐Vallon & A. Hodzic 10.1029/2022JD038227
- IL-assisted synthesis of defect-rich polyaniline/NH2-MIL-125 nanohybrids with strengthened interfacial contact for ultra-fast photocatalytic degradation of acetaldehyde under high humidity S. Shah et al. 10.1016/j.cej.2021.128590
- Elucidating gas–surface interactions relevant to atmospheric particle growth using combined temperature programmed desorption and temperature-dependent uptake K. Johnson et al. 10.1039/D4CP02528H
- Secondary organic aerosol formation from camphene oxidation: measurements and modeling Q. Li et al. 10.5194/acp-22-3131-2022
- Linking gas, particulate, and toxic endpoints to air emissions in the Community Regional Atmospheric Chemistry Multiphase Mechanism (CRACMM) H. Pye et al. 10.5194/acp-23-5043-2023
- Neural Network Emulation of the Formation of Organic Aerosols Based on the Explicit GECKO‐A Chemistry Model J. Schreck et al. 10.1029/2021MS002974
- Derivation of atmospheric reaction mechanisms for volatile organic compounds by the SAPRC mechanism generation system (MechGen) W. Carter et al. 10.5194/acp-25-199-2025
- Atmospheric Chemistry in a Box or a Bag G. Hidy 10.3390/atmos10070401
- Modeling organic aerosol over Europe in summer conditions with the VBS-GECKO parameterization: sensitivity to secondary organic compound properties and IVOC (intermediate-volatility organic compound) emissions V. Lannuque et al. 10.5194/acp-20-4905-2020
- Biogenic secondary organic aerosol sensitivity to organic aerosol simulation schemes in climate projections A. Cholakian et al. 10.5194/acp-19-13209-2019
- Volatility Parametrization of Low-Volatile Components of Ambient Organic Aerosols Based on Molecular Formulas X. Yang et al. 10.1021/acs.est.3c02073
- GENerator of reduced Organic Aerosol mechanism (GENOA v1.0): an automatic generation tool of semi-explicit mechanisms Z. Wang et al. 10.5194/gmd-15-8957-2022
- Impact of organic molecular structure on the estimation of atmospherically relevant physicochemical parameters G. Isaacman-VanWertz & B. Aumont 10.5194/acp-21-6541-2021
26 citations as recorded by crossref.
- Nonlinear behavior of organic aerosol in biomass burning plumes: a microphysical model analysis I. Konovalov et al. 10.5194/acp-19-12091-2019
- Opinion: Challenges and needs of tropospheric chemical mechanism development B. Ervens et al. 10.5194/acp-24-13317-2024
- SSH-Aerosol v1.1: A Modular Box Model to Simulate the Evolution of Primary and Secondary Aerosols K. Sartelet et al. 10.3390/atmos11050525
- A Scheme for Representing Aromatic Secondary Organic Aerosols in Chemical Transport Models: Application to Source Attribution of Organic Aerosols Over South Korea During the KORUS‐AQ Campaign J. Brewer et al. 10.1029/2022JD037257
- Influence of the NO/NO2 Ratio on Oxidation Product Distributions under High-NO Conditions K. Nihill et al. 10.1021/acs.est.0c07621
- Contrast in Secondary Organic Aerosols between the Present Day and the Preindustrial Period: The Importance of Nontraditional Sources and the Changed Atmospheric Oxidation Capability Y. Yang et al. 10.1007/s00376-024-3281-0
- Modelling molecular composition of SOA from toluene photo-oxidation at urban and street scales K. Sartelet et al. 10.1039/D4EA00049H
- Gas–particle partitioning of toluene oxidation products: an experimental and modeling study V. Lannuque et al. 10.5194/acp-23-15537-2023
- How does tropospheric VOC chemistry affect climate? An investigation of preindustrial control simulations using the Community Earth System Model version 2 N. Stanton & N. Tandon 10.5194/acp-23-9191-2023
- Polarity on adsorption and photocatalytic performances of N-GR/TiO2 towards gaseous acetaldehyde and ethylene X. Dai et al. 10.1016/j.apsusc.2019.04.221
- Transfer Learning Approach to Multitarget Temperature-Dependent Reaction Rate Prediction E. Al Ibrahim & A. Farooq 10.1021/acs.jpca.2c00713
- Future changes in isoprene-epoxydiol-derived secondary organic aerosol (IEPOX SOA) under the Shared Socioeconomic Pathways: the importance of physicochemical dependency D. Jo et al. 10.5194/acp-21-3395-2021
- Implementation of a parallel reduction algorithm in the GENerator of reduced Organic Aerosol mechanisms (GENOA v2.0): Application to multiple monoterpene aerosol precursors Z. Wang et al. 10.1016/j.jaerosci.2023.106248
- Toward Emulating an Explicit Organic Chemistry Mechanism With Random Forest Models C. Mouchel‐Vallon & A. Hodzic 10.1029/2022JD038227
- IL-assisted synthesis of defect-rich polyaniline/NH2-MIL-125 nanohybrids with strengthened interfacial contact for ultra-fast photocatalytic degradation of acetaldehyde under high humidity S. Shah et al. 10.1016/j.cej.2021.128590
- Elucidating gas–surface interactions relevant to atmospheric particle growth using combined temperature programmed desorption and temperature-dependent uptake K. Johnson et al. 10.1039/D4CP02528H
- Secondary organic aerosol formation from camphene oxidation: measurements and modeling Q. Li et al. 10.5194/acp-22-3131-2022
- Linking gas, particulate, and toxic endpoints to air emissions in the Community Regional Atmospheric Chemistry Multiphase Mechanism (CRACMM) H. Pye et al. 10.5194/acp-23-5043-2023
- Neural Network Emulation of the Formation of Organic Aerosols Based on the Explicit GECKO‐A Chemistry Model J. Schreck et al. 10.1029/2021MS002974
- Derivation of atmospheric reaction mechanisms for volatile organic compounds by the SAPRC mechanism generation system (MechGen) W. Carter et al. 10.5194/acp-25-199-2025
- Atmospheric Chemistry in a Box or a Bag G. Hidy 10.3390/atmos10070401
- Modeling organic aerosol over Europe in summer conditions with the VBS-GECKO parameterization: sensitivity to secondary organic compound properties and IVOC (intermediate-volatility organic compound) emissions V. Lannuque et al. 10.5194/acp-20-4905-2020
- Biogenic secondary organic aerosol sensitivity to organic aerosol simulation schemes in climate projections A. Cholakian et al. 10.5194/acp-19-13209-2019
- Volatility Parametrization of Low-Volatile Components of Ambient Organic Aerosols Based on Molecular Formulas X. Yang et al. 10.1021/acs.est.3c02073
- GENerator of reduced Organic Aerosol mechanism (GENOA v1.0): an automatic generation tool of semi-explicit mechanisms Z. Wang et al. 10.5194/gmd-15-8957-2022
- Impact of organic molecular structure on the estimation of atmospherically relevant physicochemical parameters G. Isaacman-VanWertz & B. Aumont 10.5194/acp-21-6541-2021
Latest update: 04 Apr 2025
Short summary
Large uncertainties remain in understanding the influence of atmospheric environmental conditions on secondary organic aerosol (SOA) formation, evolution and properties. In this article, the GECKO-A modelling tool has been used in a box model under various environmental conditions to (i) explore the sensitivity of SOA formation and properties to changes on physical and chemical conditions and (ii) develop a volatility-basis-set-type parameterization for air quality models.
Large uncertainties remain in understanding the influence of atmospheric environmental...
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