Articles | Volume 18, issue 16
https://doi.org/10.5194/acp-18-12329-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-12329-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
27 Aug 2018
Research article |
| 27 Aug 2018
| 27 Aug 2018
Mercury distribution in the upper troposphere and lowermost stratosphere according to measurements by the IAGOS-CARIBIC observatory: 2014–2016
Franz Slemr
CORRESPONDING AUTHOR
Max-Planck-Institut für Chemie (MPI), Air Chemistry Division, Hahn-Meitner-Weg 1, 55128 Mainz, Germany
Andreas Weigelt
Helmholtz-Zentrum Geesthacht (HZG), Institute of Coastal Research, Max-Planck-Str. 1, 21502 Geesthacht, Germany
now at: Bundesamt für Seeschifffahrt und Hydrographie (BSH), Wüstland 2, 22589 Hamburg, Germany
Ralf Ebinghaus
Helmholtz-Zentrum Geesthacht (HZG), Institute of Coastal Research, Max-Planck-Str. 1, 21502 Geesthacht, Germany
Johannes Bieser
Helmholtz-Zentrum Geesthacht (HZG), Institute of Coastal Research, Max-Planck-Str. 1, 21502 Geesthacht, Germany
Carl A. M. Brenninkmeijer
Max-Planck-Institut für Chemie (MPI), Air Chemistry Division, Hahn-Meitner-Weg 1, 55128 Mainz, Germany
Armin Rauthe-Schöch
Max-Planck-Institut für Chemie (MPI), Air Chemistry Division, Hahn-Meitner-Weg 1, 55128 Mainz, Germany
now at: Deutscher Wetterdienst, Global Precipitation Climatology Centre, Frankfurter Straße 135, 63067 Offenbach/Main, Germany
Markus Hermann
Leibniz-Institut für Troposphärenforschung (Tropos), Permoserstr. 15, 04318 Leipzig, Germany
Bengt G. Martinsson
University of Lund, Division of Nuclear Physics, P.O. Box 118, 22100 Lund, Sweden
Peter van Velthoven
Royal Netherlands Meteorological Institute (KNMI), P.O. Box 201, 3730 AE, de Bilt, the Netherlands
Harald Bönisch
Institute of Meteorology and Climate Research (IMK), Karlsruhe Institute of Technology, Hermann-von-Helmholtz-Platz, 76344 Eggenstein-Leopoldshafen, Germany
Marco Neumaier
Institute of Meteorology and Climate Research (IMK), Karlsruhe Institute of Technology, Hermann-von-Helmholtz-Platz, 76344 Eggenstein-Leopoldshafen, Germany
Andreas Zahn
Institute of Meteorology and Climate Research (IMK), Karlsruhe Institute of Technology, Hermann-von-Helmholtz-Platz, 76344 Eggenstein-Leopoldshafen, Germany
Helmut Ziereis
Deutsches Zentrum für Luft- und Raumfahrt (DLR), Institut für Physik der Atmosphäre, 82230 Wessling, Germany
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Cited
20 citations as recorded by crossref.
- Reductive Adsorption of Atmospheric Oxidized Mercury on Ice: Insights from Density Functional Calculations Y. Yi et al. 10.1021/acsearthspacechem.1c00269
- Near-global mapping of TGM based on aircraft measurements from intercontinental flights D. Custódio & R. Ebinghaus 10.1016/j.atmosenv.2022.119354
- BrHgO• + CO: Analogue of OH + CO and Reduction Path for Hg(II) in the Atmosphere D. Khiri et al. 10.1021/acsearthspacechem.0c00171
- Where there is smoke there is mercury: Assessing boreal forest fire mercury emissions using aircraft and highlighting uncertainties associated with upscaling emissions estimates D. McLagan et al. 10.5194/acp-21-5635-2021
- The 3D biogeochemical marine mercury cycling model MERCY v2.0 – linking atmospheric Hg to methylmercury in fish J. Bieser et al. 10.5194/gmd-16-2649-2023
- The Chemistry of Mercury in the Stratosphere A. Saiz‐Lopez et al. 10.1029/2022GL097953
- Recent advances in understanding and measurement of Hg in the environment: Surface-atmosphere exchange of gaseous elemental mercury (Hg0) J. Sommar et al. 10.1016/j.scitotenv.2020.137648
- Mercury biogeochemical cycling: A synthesis of recent scientific advances M. Gustin et al. 10.1016/j.scitotenv.2020.139619
- Dissociation of Mercuric Oxides Drives Anomalous Isotope Fractionation during Net Photo-oxidation of Mercury Vapor in Air G. Sun et al. 10.1021/acs.est.2c02722
- Atmospheric mercury sources in a coastal-urban environment: a case study in Boston, Massachusetts, USA H. Angot et al. 10.1039/D1EM00253H
- Improved Mechanistic Model of the Atmospheric Redox Chemistry of Mercury V. Shah et al. 10.1021/acs.est.1c03160
- 4D dispersion of total gaseous mercury derived from a mining source: identification of criteria to assess risks related to high concentrations of atmospheric mercury J. Esbrí et al. 10.5194/acp-20-12995-2020
- Photochemistry of oxidized Hg(I) and Hg(II) species suggests missing mercury oxidation in the troposphere A. Saiz-Lopez et al. 10.1073/pnas.1922486117
- Effects of temperature and relative humidity on the partitioning of atmospheric oxidized mercury at a high-altitude mountain background site in Taiwan L. Nguyen et al. 10.1016/j.atmosenv.2021.118572
- Earth system modeling of mercury using CESM2 – Part 1: Atmospheric model CAM6-Chem/Hg v1.0 P. Zhang & Y. Zhang 10.5194/gmd-15-3587-2022
- Atmospheric mercury in the Southern Hemisphere – Part 2: Source apportionment analysis at Cape Point station, South Africa J. Bieser et al. 10.5194/acp-20-10427-2020
- Soil–atmosphere exchange flux of total gaseous mercury (TGM) at subtropical and temperate forest catchments J. Zhou et al. 10.5194/acp-20-16117-2020
- Intercomparison of in-situ aircraft and satellite aerosol measurements in the stratosphere O. Sandvik et al. 10.1038/s41598-019-52089-6
- Natural Background and the Anthropogenic Enrichment of Mercury in the Southern Florida Environment: A Review with a Discussion on Public Health T. Missimer et al. 10.3390/ijerph21010118
- Event-Based Atmospheric Precipitation Uncovers Significant Even and Odd Hg Isotope Anomalies Associated with the Circumpolar Vortex S. Yuan et al. 10.1021/acs.est.2c02613
20 citations as recorded by crossref.
- Reductive Adsorption of Atmospheric Oxidized Mercury on Ice: Insights from Density Functional Calculations Y. Yi et al. 10.1021/acsearthspacechem.1c00269
- Near-global mapping of TGM based on aircraft measurements from intercontinental flights D. Custódio & R. Ebinghaus 10.1016/j.atmosenv.2022.119354
- BrHgO• + CO: Analogue of OH + CO and Reduction Path for Hg(II) in the Atmosphere D. Khiri et al. 10.1021/acsearthspacechem.0c00171
- Where there is smoke there is mercury: Assessing boreal forest fire mercury emissions using aircraft and highlighting uncertainties associated with upscaling emissions estimates D. McLagan et al. 10.5194/acp-21-5635-2021
- The 3D biogeochemical marine mercury cycling model MERCY v2.0 – linking atmospheric Hg to methylmercury in fish J. Bieser et al. 10.5194/gmd-16-2649-2023
- The Chemistry of Mercury in the Stratosphere A. Saiz‐Lopez et al. 10.1029/2022GL097953
- Recent advances in understanding and measurement of Hg in the environment: Surface-atmosphere exchange of gaseous elemental mercury (Hg0) J. Sommar et al. 10.1016/j.scitotenv.2020.137648
- Mercury biogeochemical cycling: A synthesis of recent scientific advances M. Gustin et al. 10.1016/j.scitotenv.2020.139619
- Dissociation of Mercuric Oxides Drives Anomalous Isotope Fractionation during Net Photo-oxidation of Mercury Vapor in Air G. Sun et al. 10.1021/acs.est.2c02722
- Atmospheric mercury sources in a coastal-urban environment: a case study in Boston, Massachusetts, USA H. Angot et al. 10.1039/D1EM00253H
- Improved Mechanistic Model of the Atmospheric Redox Chemistry of Mercury V. Shah et al. 10.1021/acs.est.1c03160
- 4D dispersion of total gaseous mercury derived from a mining source: identification of criteria to assess risks related to high concentrations of atmospheric mercury J. Esbrí et al. 10.5194/acp-20-12995-2020
- Photochemistry of oxidized Hg(I) and Hg(II) species suggests missing mercury oxidation in the troposphere A. Saiz-Lopez et al. 10.1073/pnas.1922486117
- Effects of temperature and relative humidity on the partitioning of atmospheric oxidized mercury at a high-altitude mountain background site in Taiwan L. Nguyen et al. 10.1016/j.atmosenv.2021.118572
- Earth system modeling of mercury using CESM2 – Part 1: Atmospheric model CAM6-Chem/Hg v1.0 P. Zhang & Y. Zhang 10.5194/gmd-15-3587-2022
- Atmospheric mercury in the Southern Hemisphere – Part 2: Source apportionment analysis at Cape Point station, South Africa J. Bieser et al. 10.5194/acp-20-10427-2020
- Soil–atmosphere exchange flux of total gaseous mercury (TGM) at subtropical and temperate forest catchments J. Zhou et al. 10.5194/acp-20-16117-2020
- Intercomparison of in-situ aircraft and satellite aerosol measurements in the stratosphere O. Sandvik et al. 10.1038/s41598-019-52089-6
- Natural Background and the Anthropogenic Enrichment of Mercury in the Southern Florida Environment: A Review with a Discussion on Public Health T. Missimer et al. 10.3390/ijerph21010118
- Event-Based Atmospheric Precipitation Uncovers Significant Even and Odd Hg Isotope Anomalies Associated with the Circumpolar Vortex S. Yuan et al. 10.1021/acs.est.2c02613
Latest update: 26 Jul 2024
Short summary
Total and elemental mercury were measured in the upper troposphere and lower stratosphere onboard a passenger aircraft. Their concentrations in the upper troposphere were comparable implying low concentrations of oxidized mercury in this region. Large scale seasonally dependent influence of emissions from biomass burning was also observed. Their distributions in the lower stratosphere implies a long stratospheric lifetime, which precludes significant mercury oxidation by ozone.
Total and elemental mercury were measured in the upper troposphere and lower stratosphere...
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