Articles | Volume 18, issue 16
https://doi.org/10.5194/acp-18-12241-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-12241-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Effectiveness of ammonia reduction on control of fine particle nitrate
Hongyu Guo
School of Earth and Atmospheric Sciences, Georgia Institute of
Technology, Atlanta, GA 30332, USA
Rene Otjes
Energy Research Centre of the Netherlands (ECN),
Petten, the Netherlands
Patrick Schlag
Institute for Marine and Atmospheric Research Utrecht (IMAU), Utrecht University, Utrecht, the Netherlands
Institute for Energy and Climate Research (IEK-8) – Troposphere,
Forschungszentrum Jülich, Jülich, Germany
now at: Institute of Physics, University of Sao Paulo, Sao Paulo, SP, Brazil
Astrid Kiendler-Scharr
Institute for Energy and Climate Research (IEK-8) – Troposphere,
Forschungszentrum Jülich, Jülich, Germany
Athanasios Nenes
School of Earth and Atmospheric Sciences, Georgia Institute of
Technology, Atlanta, GA 30332, USA
School of Chemical and Biomolecular Engineering, Georgia Institute
of Technology, Atlanta, GA 30332, USA
Institute for Chemical Engineering Sciences, Foundation for
Research and Technology – Hellas, Patras, 26504, Greece
Institute for Environmental Research and Sustainable Development,
National Observatory of Athens, Palea Penteli, Athens, 15236, Greece
School of Earth and Atmospheric Sciences, Georgia Institute of
Technology, Atlanta, GA 30332, USA
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- PM2.5 and water-soluble inorganic ion concentrations decreased faster in urban than rural areas in China Y. Zhang et al. 10.1016/j.jes.2021.09.031
- The complex chemical effects of COVID-19 shutdowns on air quality J. Kroll et al. 10.1038/s41557-020-0535-z
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- Importance of gas-particle partitioning of ammonia in haze formation in the rural agricultural environment J. Xu et al. 10.5194/acp-20-7259-2020
- Significant contrasts in aerosol acidity between China and the United States B. Zhang et al. 10.5194/acp-21-8341-2021
- Meteorological variations impeded the benefits of recent NOx mitigation in reducing atmospheric nitrate deposition in the Pearl River Delta region, Southeast China B. Zhong et al. 10.1016/j.envpol.2020.115076
- High efficiency of livestock ammonia emission controls in alleviating particulate nitrate during a severe winter haze episode in northern China Z. Xu et al. 10.5194/acp-19-5605-2019
- Initial Cost Barrier of Ammonia Control in Central China M. Zheng et al. 10.1029/2019GL084351
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- Ammonia emission abatement does not fully control reduced forms of nitrogen deposition J. Tan et al. 10.1073/pnas.1920068117
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- Review on Ammonia as a Potential Fuel: From Synthesis to Economics A. Valera-Medina et al. 10.1021/acs.energyfuels.0c03685
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- Response of fine aerosol nitrate chemistry to Clean Air Action in winter Beijing: Insights from the oxygen isotope signatures Z. Zhang et al. 10.1016/j.scitotenv.2020.141210
- Altering the substituents of salicylic acid to improve Berthelot reaction for ultrasensitive colorimetric detection of ammonium and atmospheric ammonia H. Yu et al. 10.1007/s00216-021-03485-3
- Spatioseasonal Variations of Atmospheric Ammonia Concentrations Over the United States: Comprehensive Model‐Observation Comparison A. Nair et al. 10.1029/2018JD030057
- Fine particle pH and its influencing factors during summer at Mt. Tai: Comparison between mountain and urban sites P. Liu et al. 10.1016/j.atmosenv.2021.118607
- Important Role of NO3 Radical to Nitrate Formation Aloft in Urban Beijing: Insights from Triple Oxygen Isotopes Measured at the Tower M. Fan et al. 10.1021/acs.est.1c02843
- Evaluation of the ammonia emission sensitivity of secondary inorganic aerosol concentrations measured by the national reference method J. Lim et al. 10.1016/j.atmosenv.2021.118903
- A review of aerosol chemistry in Asia: insights from aerosol mass spectrometer measurements W. Zhou et al. 10.1039/D0EM00212G
- Importance of NO3 radical in particulate nitrate formation in a southeast Chinese urban city: New constraints by δ15N-δ18O space of NO3- Z. Zhang et al. 10.1016/j.atmosenv.2021.118387
- An Odd Oxygen Framework for Wintertime Ammonium Nitrate Aerosol Pollution in Urban Areas: NO x and VOC Control as Mitigation Strategies C. Womack et al. 10.1029/2019GL082028
- Aerosol pH and liquid water content determine when particulate matter is sensitive to ammonia and nitrate availability A. Nenes et al. 10.5194/acp-20-3249-2020
- Partitioning of NH3-NH4+ in the Southeastern U.S. B. Cheng et al. 10.3390/atmos12121681
- Empirical Insights Into the Fate of Ammonia in Western U.S. Wildfire Smoke Plumes J. Lindaas et al. 10.1029/2020JD033730
- Aerosol water content enhancement leads to changes in the major formation mechanisms of nitrate and secondary organic aerosols in winter over the North China Plain C. Chen et al. 10.1016/j.envpol.2021.117625
- The acidity of atmospheric particles and clouds H. Pye et al. 10.5194/acp-20-4809-2020
- How alkaline compounds control atmospheric aerosol particle acidity V. Karydis et al. 10.5194/acp-21-14983-2021
Latest update: 06 Jun 2023
Short summary
Reduction in ammonia has been proposed as a way to lower fine particle mass and improve air quality, but gas-phase ammonia is linked to agricultural productivity. We assess the feasibility of ammonia control at a variety of locations through an aerosol thermodynamic analysis. We show that aerosol response to ammonia control is highly nonlinear and only becomes effective when ambient particle pH drops below approximately 3. Particle pH is a relevant aerosol air quality parameter.
Reduction in ammonia has been proposed as a way to lower fine particle mass and improve air...
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