Articles | Volume 18, issue 15
https://doi.org/10.5194/acp-18-10985-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-10985-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
07 Aug 2018
Research article |
| 07 Aug 2018
| 07 Aug 2018
Establishing the impact of model surfactants on cloud condensation nuclei activity of sea spray aerosol mimics
Sara D. Forestieri
Department of Civil and Environmental Engineering, University of California, Davis, CA, USA
now at: California Air Resources Board, Sacramento, CA, USA
Sean M. Staudt
Department of Chemistry, University of Wisconsin, Madison, WI, USA
Thomas M. Kuborn
Department of Chemistry, University of Wisconsin, Madison, WI, USA
Katharine Faber
Department of Chemistry, Carleton College, Northfield, MN, USA
Christopher R. Ruehl
California Air Resources Board, Sacramento, CA, USA
Timothy H. Bertram
Department of Chemistry, University of Wisconsin, Madison, WI, USA
Department of Civil and Environmental Engineering, University of California, Davis, CA, USA
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- Hygroscopic growth and CCN activity of secondary organic aerosol produced from dark ozonolysis of γ-terpinene H. Bouzidi et al. 10.1016/j.scitotenv.2022.153010
- Key drivers of cloud response to surface-active organics S. Lowe et al. 10.1038/s41467-019-12982-0
- Cloud condensation nuclei activity of internally mixed particle populations at a remote marine free troposphere site in the North Atlantic Ocean Z. Cheng et al. 10.1016/j.scitotenv.2023.166865
- Heterogeneous reaction and condensation growth observation of NaCl/dicarboxylic acids nanoparticles by aerosol time-of-flight mass spectrometer with water-based particle size amplifier Z. Xie et al. 10.1016/j.atmosenv.2020.118162
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- Insights into the behavior of nonanoic acid and its conjugate base at the air/water interface through a combined experimental and theoretical approach M. Luo et al. 10.1039/D0SC02354J
- Insights into the Headgroup and Chain Length Dependence of Surface Characteristics of Organic-Coated Sea Spray Aerosols S. Cheng et al. 10.1021/acsearthspacechem.8b00212
- Effects of surface tension time-evolution for CCN activation of a complex organic surfactant J. Lin et al. 10.1039/C9EM00426B
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- Effect of Sodium Dodecyl Benzene Sulfonate on the Production of Cloud Condensation Nuclei from Breaking Waves S. Hartery et al. 10.1021/acsearthspacechem.2c00230
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- Size-Resolved Surface-Active Substances of Atmospheric Aerosol: Reconsideration of the Impact on Cloud Droplet Formation A. Kroflič et al. 10.1021/acs.est.8b02381
50 citations as recorded by crossref.
- Cloud droplet activation of organic–salt mixtures predicted from two model treatments of the droplet surface J. Lin et al. 10.1039/C8EM00345A
- Surfactant Charge Modulates Structure and Stability of Lipase-Embedded Monolayers at Marine-Relevant Aerosol Surfaces M. Luo et al. 10.1021/acs.langmuir.9b00689
- Chemical transformation of a long-chain alkyl organosulfate via heterogeneous OH oxidation: a case study of sodium dodecyl sulfate S. Madeleine Ng et al. 10.1039/D2EA00026A
- The effect of hydrophobic glassy organic material on the cloud condensation nuclei activity of particles with different morphologies A. Tandon et al. 10.5194/acp-19-3325-2019
- Ocean Aerobiology A. Alsante et al. 10.3389/fmicb.2021.764178
- Optical trapping and light scattering in atmospheric aerosol science A. Rafferty et al. 10.1039/D2CP05301B
- Atomic Force Microscopy: An Emerging Tool in Measuring the Phase State and Surface Tension of Individual Aerosol Particles H. Lee & A. Tivanski 10.1146/annurev-physchem-090419-110133
- Cloud condensation nuclei activity of six pollenkitts and the influence of their surface activity N. Prisle et al. 10.5194/acp-19-4741-2019
- Constraints on the Role of Laplace Pressure in Multiphase Reactions and Viscosity of Organic Aerosols S. Petters 10.1029/2022GL098959
- Technical note: The role of evolving surface tension in the formation of cloud droplets J. Davies et al. 10.5194/acp-19-2933-2019
- Cloud condensation nuclei activation properties of Mediterranean pollen types considering organic chemical composition and surface tension effects A. Casans et al. 10.1016/j.atmosenv.2023.119961
- Marine Polymer-Gels’ Relevance in the Atmosphere as Aerosols and CCN M. Orellana et al. 10.3390/gels7040185
- Sea spray aerosol organic enrichment, water uptake and surface tension effects L. Cravigan et al. 10.5194/acp-20-7955-2020
- Snowpack-stored atmospheric surface-active contaminants traced with snowmelt water surface film rheology S. Pogorzelski et al. 10.1007/s11356-020-10874-1
- Water activity and surface tension of aqueous ammonium sulfate and D-glucose aerosol nanoparticles E. Mikhailov et al. 10.5194/acp-24-2971-2024
- Night-Time Oxidation of a Monolayer Model for the Air–Water Interface of Marine Aerosols—A Study by Simultaneous Neutron Reflectometry and in Situ Infra-Red Reflection Absorption Spectroscopy (IRRAS) B. Woden et al. 10.3390/atmos9120471
- Molecular dynamics simulations demonstrate that non-ideal mixing dominates subsaturation organic aerosol hygroscopicity D. Roston 10.1039/D1CP00245G
- Hygroscopic growth and CCN activity of secondary organic aerosol produced from dark ozonolysis of γ-terpinene H. Bouzidi et al. 10.1016/j.scitotenv.2022.153010
- Key drivers of cloud response to surface-active organics S. Lowe et al. 10.1038/s41467-019-12982-0
- Cloud condensation nuclei activity of internally mixed particle populations at a remote marine free troposphere site in the North Atlantic Ocean Z. Cheng et al. 10.1016/j.scitotenv.2023.166865
- Heterogeneous reaction and condensation growth observation of NaCl/dicarboxylic acids nanoparticles by aerosol time-of-flight mass spectrometer with water-based particle size amplifier Z. Xie et al. 10.1016/j.atmosenv.2020.118162
- Surface tension of single suspended aerosol microdroplets Y. Tong et al. 10.1016/j.cclet.2023.109062
- Model for estimating activity coefficients in binary and ternary ionic surfactant solutions S. Calderón et al. 10.1007/s10874-020-09407-4
- In situ measurements of human cough aerosol hygroscopicity R. Groth et al. 10.1098/rsif.2021.0209
- Comparison of six approaches to predicting droplet activation of surface active aerosol – Part 2: Strong surfactants S. Vepsäläinen et al. 10.5194/acp-23-15149-2023
- Aqueous Radical Initiated Oxidation of an Organic Monolayer at the Air–Water Interface as a Proxy for Thin Films on Atmospheric Aerosol Studied with Neutron Reflectometry S. Jones et al. 10.1021/acs.jpca.3c03846
- Physicochemical Mixing State of Sea Spray Aerosols: Morphologies Exhibit Size Dependence H. Lee et al. 10.1021/acsearthspacechem.0c00153
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- Morphology and hygroscopicity of nanoplastics in sea spray S. Petters et al. 10.1039/D3CP03793B
- Understanding the Interfacial Behavior of Typical Perfluorocarboxylic Acids at Surfactant‐Coated Aqueous Interfaces S. Cheng et al. 10.1029/2019JD032182
- A thermodynamic framework for bulk–surface partitioning in finite-volume mixed organic–inorganic aerosol particles and cloud droplets R. Schmedding & A. Zuend 10.5194/acp-23-7741-2023
- Emerging investigator series: surfactants, films, and coatings on atmospheric aerosol particles: a review K. Wokosin et al. 10.1039/D2EA00003B
- Comparison of six approaches to predicting droplet activation of surface active aerosol – Part 1: moderately surface active organics S. Vepsäläinen et al. 10.5194/acp-22-2669-2022
- A Monolayer Partitioning Scheme for Droplets of Surfactant Solutions J. Malila & N. Prisle 10.1029/2018MS001456
- Solubility and Activity Coefficients of Atmospheric Surfactants in Aqueous Solution Evaluated Using COSMOtherm G. Michailoudi et al. 10.1021/acs.jpca.9b09780
- Insights into the behavior of nonanoic acid and its conjugate base at the air/water interface through a combined experimental and theoretical approach M. Luo et al. 10.1039/D0SC02354J
- Insights into the Headgroup and Chain Length Dependence of Surface Characteristics of Organic-Coated Sea Spray Aerosols S. Cheng et al. 10.1021/acsearthspacechem.8b00212
- Effects of surface tension time-evolution for CCN activation of a complex organic surfactant J. Lin et al. 10.1039/C9EM00426B
- The surface tension of surfactant-containing, finite volume droplets B. Bzdek et al. 10.1073/pnas.1915660117
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- Constraining the Effect of Surfactants on the Hygroscopic Growth of Model Sea Spray Aerosol Particles R. Bramblett & A. Frossard 10.1021/acs.jpca.2c04539
- Ocean flux of salt, sulfate, and organic components to atmospheric aerosol L. Russell et al. 10.1016/j.earscirev.2023.104364
- Establishing a model organic film of low volatile compound mixture on aqueous aerosol surface S. Li et al. 10.1016/j.atmosenv.2018.11.052
- A Lagrangian particle-based numerical model for surfactant-laden droplets at macroscales M. Denys et al. 10.1063/5.0101930
- A predictive thermodynamic framework of cloud droplet activation for chemically unresolved aerosol mixtures, including surface tension, non-ideality, and bulk–surface partitioning N. Prisle 10.5194/acp-21-16387-2021
- Exploring the Nanostructures Accessible to an Organic Surfactant Atmospheric Aerosol Proxy A. Milsom et al. 10.1021/acs.jpca.2c04611
- Cloud droplet activation of secondary organic aerosol is mainly controlled by molecular weight, not water solubility J. Wang et al. 10.5194/acp-19-941-2019
- Investigating Carbonaceous Aerosol and Its Absorption Properties From Fires in the Western United States (WE‐CAN) and Southern Africa (ORACLES and CLARIFY) T. Carter et al. 10.1029/2021JD034984
- Emerging investigator series: exploring the surface properties of aqueous aerosols coated with mixed surfactants J. Li et al. 10.1039/C8EM00419F
Latest update: 24 Apr 2024
Short summary
Our work establishes how surface tension reduction influences droplet growth and activation of simple sea spray mimics (NaCl coated with fatty acids). Fatty acids can substantially reduce droplet surface tension near activation but have limited impact on activation. Coating of NaCl by palmitic acid (a wax) impedes water uptake, but this impedance is removed if oleic acid (a liquid) is mixed in. The properties that surface-active compounds need to impact activation are theoretically examined.
Our work establishes how surface tension reduction influences droplet growth and activation of...
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