Articles | Volume 18, issue 2
https://doi.org/10.5194/acp-18-1045-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-1045-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
26 Jan 2018
Research article |
| 26 Jan 2018
| 26 Jan 2018
Hygroscopicity of organic surrogate compounds from biomass burning and their effect on the efflorescence of ammonium sulfate in mixed aerosol particles
Ting Lei
State Key Laboratory for Structural Chemistry of Unstable and Stable Species, CAS Research/Education Center for Excellence in Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing, 100190, China
Multiphase Department, Max Planck Institute for Chemistry, Mainz 55128, Germany
Andreas Zuend
Department of Atmospheric and Oceanic Sciences, McGill University, Montreal, Quebec, Canada
Yafang Cheng
Multiphase Department, Max Planck Institute for Chemistry, Mainz 55128, Germany
Institute for Environmental and Climate Research, Jinan University, Guangzhou, China
Multiphase Department, Max Planck Institute for Chemistry, Mainz 55128, Germany
Institute for Environmental and Climate Research, Jinan University, Guangzhou, China
Weigang Wang
State Key Laboratory for Structural Chemistry of Unstable and Stable Species, CAS Research/Education Center for Excellence in Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing, 100190, China
State Key Laboratory for Structural Chemistry of Unstable and Stable Species, CAS Research/Education Center for Excellence in Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing, 100190, China
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- Significant impact of water-soluble organic matter on hygroscopicity of fine particles under low relative humidity condition J. Tao et al. 10.1016/j.scitotenv.2023.167980
- Hygroscopic Properties of Water-Soluble Counterpart of Ultrafine Particles from Agriculture Crop-Residue Burning in Patiala, Northwestern India A. Alang et al. 10.3390/atmos15070835
- Measurement of atmospheric nanoparticles: Bridging the gap between gas-phase molecules and larger particles C. Peng et al. 10.1016/j.jes.2022.03.006
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- Advances in analysis of atmospheric ultrafine particles and application in air quality, climate, and health research T. Lei et al. 10.1016/j.scitotenv.2024.175045
- Hygroscopicity of organic compounds as a function of organic functionality, water solubility, molecular weight, and oxidation level S. Han et al. 10.5194/acp-22-3985-2022
- Hygroscopicity of aerosol particles composed of surfactant SDS and its internal mixture with ammonium sulfate at relative humidities up to 99.9% C. Zhang et al. 10.1016/j.atmosenv.2023.119625
- Photochemical Oxidation of Water-Soluble Organic Carbon (WSOC) on Mineral Dust and Enhanced Organic Ammonium Formation T. Wang et al. 10.1021/acs.est.0c04616
- Secondary Organic Aerosol from Biomass Burning Phenolic Compounds and Nitrate Radicals can be Highly Viscous over a Wide Relative Humidity Range S. Nikkho et al. 10.1021/acs.est.4c06235
- Strong Acids or Bases Displaced by Weak Acids or Bases in Aerosols: Reactions Driven by the Continuous Partitioning of Volatile Products into the Gas Phase Z. Chen et al. 10.1021/acs.accounts.1c00318
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- Effect of mixing structure on the water uptake of mixtures of ammonium sulfate and phthalic acid particles W. Wang et al. 10.5194/acp-21-2179-2021
- Surfactant effect on the hygroscopicity of aerosol particles at relative humidity ranging from 80% to 99.5%: Internally mixed adipic acid-ammonium sulfate particles C. Zhang et al. 10.1016/j.atmosenv.2021.118725
- Hygroscopicity of Secondary Brown Carbon Aerosol from Aqueous Photo-Oxidation of Phenolic Precursors K. Betz et al. 10.1021/acsearthspacechem.2c00132
- Important Oxidants and Their Impact on the Environmental Effects of Aerosols M. Ge et al. 10.1021/acs.jpca.0c10236
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- Development of aerosol optical properties for improving the MESSy photolysis module in the GEM-MACH v2.4 air quality model and application for calculating photolysis rates in a biomass burning plume M. Majdzadeh et al. 10.5194/gmd-15-219-2022
- Modelling the gas–particle partitioning and water uptake of isoprene-derived secondary organic aerosol at high and low relative humidity D. Amaladhasan et al. 10.5194/acp-22-215-2022
- Quantitative description of surface tension for nanodroplets containing ammonium sulfate and its application to the particle hygroscopicity prediction C. Zhang et al. 10.1063/5.0245540
- Quantitative description of self-, Maxwell–Stefan, and Fick diffusion coefficients in sucrose and citric acid solution based on molecular dynamics simulations H. Bao et al. 10.1063/5.0268503
- Hygroscopic behavior of inorganic–organic aerosol systems including ammonium sulfate, dicarboxylic acids, and oligomer H. Bouzidi et al. 10.1016/j.atmosenv.2020.117481
- Hygroscopic properties of NaCl nanoparticles on the surface: a scanning force microscopy study X. Wang et al. 10.1039/D0CP00155D
- A database for deliquescence and efflorescence relative humidities of compounds with atmospheric relevance C. Peng et al. 10.1016/j.fmre.2021.11.021
26 citations as recorded by crossref.
- Chip-Based Dark-filed Microscopy for Sensing the Dynamical Changes of Single Aerosol Nanoparticles Z. Fan et al. 10.1109/JSTQE.2023.3239389
- The effect of clouds and precipitation on the aerosol concentrations and composition in a boreal forest environment S. Isokääntä et al. 10.5194/acp-22-11823-2022
- Significant impact of water-soluble organic matter on hygroscopicity of fine particles under low relative humidity condition J. Tao et al. 10.1016/j.scitotenv.2023.167980
- Hygroscopic Properties of Water-Soluble Counterpart of Ultrafine Particles from Agriculture Crop-Residue Burning in Patiala, Northwestern India A. Alang et al. 10.3390/atmos15070835
- Measurement of atmospheric nanoparticles: Bridging the gap between gas-phase molecules and larger particles C. Peng et al. 10.1016/j.jes.2022.03.006
- Microscopic mechanism of the interaction between water and formic acid-sodium chloride aerosol C. Zhang et al. 10.1016/j.powtec.2018.11.105
- Advances in analysis of atmospheric ultrafine particles and application in air quality, climate, and health research T. Lei et al. 10.1016/j.scitotenv.2024.175045
- Hygroscopicity of organic compounds as a function of organic functionality, water solubility, molecular weight, and oxidation level S. Han et al. 10.5194/acp-22-3985-2022
- Hygroscopicity of aerosol particles composed of surfactant SDS and its internal mixture with ammonium sulfate at relative humidities up to 99.9% C. Zhang et al. 10.1016/j.atmosenv.2023.119625
- Photochemical Oxidation of Water-Soluble Organic Carbon (WSOC) on Mineral Dust and Enhanced Organic Ammonium Formation T. Wang et al. 10.1021/acs.est.0c04616
- Secondary Organic Aerosol from Biomass Burning Phenolic Compounds and Nitrate Radicals can be Highly Viscous over a Wide Relative Humidity Range S. Nikkho et al. 10.1021/acs.est.4c06235
- Strong Acids or Bases Displaced by Weak Acids or Bases in Aerosols: Reactions Driven by the Continuous Partitioning of Volatile Products into the Gas Phase Z. Chen et al. 10.1021/acs.accounts.1c00318
- Size-dependent hygroscopicity of levoglucosan and D-glucose aerosol nanoparticles T. Lei et al. 10.5194/acp-23-4763-2023
- In Situ Quantitative Observation of Hygroscopic Growth of Single Nanoparticle Aerosol by Surface Plasmon Resonance Microscopy Z. Xie et al. 10.1021/acs.analchem.0c00431
- Effect of mixing structure on the water uptake of mixtures of ammonium sulfate and phthalic acid particles W. Wang et al. 10.5194/acp-21-2179-2021
- Surfactant effect on the hygroscopicity of aerosol particles at relative humidity ranging from 80% to 99.5%: Internally mixed adipic acid-ammonium sulfate particles C. Zhang et al. 10.1016/j.atmosenv.2021.118725
- Hygroscopicity of Secondary Brown Carbon Aerosol from Aqueous Photo-Oxidation of Phenolic Precursors K. Betz et al. 10.1021/acsearthspacechem.2c00132
- Important Oxidants and Their Impact on the Environmental Effects of Aerosols M. Ge et al. 10.1021/acs.jpca.0c10236
- Nano-hygroscopicity tandem differential mobility analyzer (nano-HTDMA) for investigating hygroscopic properties of sub-10 nm aerosol nanoparticles T. Lei et al. 10.5194/amt-13-5551-2020
- Development of aerosol optical properties for improving the MESSy photolysis module in the GEM-MACH v2.4 air quality model and application for calculating photolysis rates in a biomass burning plume M. Majdzadeh et al. 10.5194/gmd-15-219-2022
- Modelling the gas–particle partitioning and water uptake of isoprene-derived secondary organic aerosol at high and low relative humidity D. Amaladhasan et al. 10.5194/acp-22-215-2022
- Quantitative description of surface tension for nanodroplets containing ammonium sulfate and its application to the particle hygroscopicity prediction C. Zhang et al. 10.1063/5.0245540
- Quantitative description of self-, Maxwell–Stefan, and Fick diffusion coefficients in sucrose and citric acid solution based on molecular dynamics simulations H. Bao et al. 10.1063/5.0268503
- Hygroscopic behavior of inorganic–organic aerosol systems including ammonium sulfate, dicarboxylic acids, and oligomer H. Bouzidi et al. 10.1016/j.atmosenv.2020.117481
- Hygroscopic properties of NaCl nanoparticles on the surface: a scanning force microscopy study X. Wang et al. 10.1039/D0CP00155D
- A database for deliquescence and efflorescence relative humidities of compounds with atmospheric relevance C. Peng et al. 10.1016/j.fmre.2021.11.021
Discussed (preprint)
Latest update: 11 Jul 2025
Short summary
Measurements and thermodynamic equilibrium predictions for organic–inorganic aerosols related to components from biomass burning emissions demonstrate a diversity of hygroscopic growth and shrinking behavior, which we observed using a hygroscopicity tandem differential mobility analyzer (HTDMA). Controlled laboratory experiments with single solutes and/or with mixed organic–inorganic systems of known phase state will be useful to constrain model parameters of thermodynamic equilibrium models.
Measurements and thermodynamic equilibrium predictions for organic–inorganic aerosols related to...
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