Articles | Volume 17, issue 14
https://doi.org/10.5194/acp-17-9081-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-9081-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
27 Jul 2017
Research article |
| 27 Jul 2017
Global atmospheric chemistry – which air matters
Department of Earth System Science, University of California,
Irvine, CA 92697-3100, USA
Xin Zhu
Department of Earth System Science, University of California,
Irvine, CA 92697-3100, USA
Clare M. Flynn
Department of Earth System Science, University of California,
Irvine, CA 92697-3100, USA
Sarah A. Strode
NASA Goddard Space Flight Center,
Greenbelt, MD, USA
Universities Space Research Association (USRA),
GESTAR, Columbia, MD, USA
Jose M. Rodriguez
NASA Goddard Space Flight Center,
Greenbelt, MD, USA
Stephen D. Steenrod
NASA Goddard Space Flight Center,
Greenbelt, MD, USA
Universities Space Research Association (USRA),
GESTAR, Columbia, MD, USA
Junhua Liu
NASA Goddard Space Flight Center,
Greenbelt, MD, USA
Universities Space Research Association (USRA),
GESTAR, Columbia, MD, USA
Jean-Francois Lamarque
Atmospheric Chemistry, Observations and
Modeling Laboratory, National Center for Atmospheric Research, Boulder, CO
80301, USA
Arlene M. Fiore
Department of Earth and Environmental Sciences and
Lamont-Doherty Earth Observatory of Columbia University, Palisades, NY,
USA
Larry W. Horowitz
Geophysical Fluid Dynamics Laboratory, National Oceanic and
Atmospheric Administration, Princeton, NJ, USA
Jingqiu Mao
Geophysical
Institute and Department of Chemistry, University of Alaska Fairbanks,
Fairbanks, AK, USA
Lee T. Murray
Department of Earth and Environmental
Sciences, University of Rochester, Rochester, NY 14627-0221, USA
Drew T. Shindell
Nicholas School of the Environment, Duke University, Durham, NC,
USA
Steven C. Wofsy
School of Engineering and Applied Sciences, Harvard
University, Cambridge, MA 02138, USA
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- Cloud impacts on photochemistry: building a climatology of photolysis rates from the Atmospheric Tomography mission S. Hall et al. 10.5194/acp-18-16809-2018
- Forecasting carbon monoxide on a global scale for the ATom-1 aircraft mission: insights from airborne and satellite observations and modeling S. Strode et al. 10.5194/acp-18-10955-2018
- H2O2 and CH3OOH (MHP) in the Remote Atmosphere: 1. Global Distribution and Regional Influences H. Allen et al. 10.1029/2021JD035701
- A round Earth for climate models M. Prather & J. Hsu 10.1073/pnas.1908198116
- Tropospheric Ozone Assessment Report A. Archibald et al. 10.1525/elementa.2020.034
- GISS‐E2.1: Configurations and Climatology M. Kelley et al. 10.1029/2019MS002025
- Sea spray aerosol concentration modulated by sea surface temperature S. Liu et al. 10.1073/pnas.2020583118
- Lifetimes and timescales of tropospheric ozone M. Prather & X. Zhu 10.1525/elementa.2023.00112
- Resetting tropospheric OH and CH 4 lifetime with ultraviolet H 2 O absorption M. Prather & L. Zhu 10.1126/science.adn0415
- HCOOH in the Remote Atmosphere: Constraints from Atmospheric Tomography (ATom) Airborne Observations X. Chen et al. 10.1021/acsearthspacechem.1c00049
- Global Measurements of Brown Carbon and Estimated Direct Radiative Effects L. Zeng et al. 10.1029/2020GL088747
- A multi-model assessment of the Global Warming Potential of hydrogen M. Sand et al. 10.1038/s43247-023-00857-8
- Anthropogenic, biogenic, and photochemical influences on surface formaldehyde and its significant decadal (2006–2017) decrease in the Lewiston-Clarkston valley of the northwestern United States R. Li et al. 10.1016/j.chemosphere.2023.140962
- How Atmospheric Chemistry and Transport Drive Surface Variability of N2O and CFC‐11 D. Ruiz et al. 10.1029/2020JD033979
- On the Chemical Pathways Influencing the Effective Global Warming Potential of Commercial Hydrofluoroolefin Gases G. Salierno 10.1002/cssc.202400280
- Gravitational separation of Ar∕N<sub>2</sub> and age of air in the lowermost stratosphere in airborne observations and a chemical transport model B. Birner et al. 10.5194/acp-20-12391-2020
- Assessing Uncertainties and Approximations in Solar Heating of the Climate System J. Hsu & M. Prather 10.1029/2020MS002131
- Atlantic Multidecadal Variability and the U.K. ACSIS Program R. Sutton et al. 10.1175/BAMS-D-16-0266.1
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- Global atmospheric CO<sub>2</sub> inverse models converging on neutral tropical land exchange, but disagreeing on fossil fuel and atmospheric growth rate B. Gaubert et al. 10.5194/bg-16-117-2019
- Description and evaluation of the UKCA stratosphere–troposphere chemistry scheme (StratTrop vn 1.0) implemented in UKESM1 A. Archibald et al. 10.5194/gmd-13-1223-2020
- Fast time response measurements of particle size distributions in the 3–60 nm size range with the nucleation mode aerosol size spectrometer C. Williamson et al. 10.5194/amt-11-3491-2018
- Deconstruction of tropospheric chemical reactivity using aircraft measurements: the Atmospheric Tomography Mission (ATom) data M. Prather et al. 10.5194/essd-15-3299-2023
- Heterogeneity and chemical reactivity of the remote troposphere defined by aircraft measurements H. Guo et al. 10.5194/acp-21-13729-2021
- How well can global chemistry models calculate the reactivity of short-lived greenhouse gases in the remote troposphere, knowing the chemical composition M. Prather et al. 10.5194/amt-11-2653-2018
- The IAGOS NO<sub><i>x</i></sub> instrument – design, operation and first results from deployment aboard passenger aircraft F. Berkes et al. 10.5194/amt-11-3737-2018
- Implementation and evaluation of updated photolysis rates in the EMEP MSC-W chemistry-transport model using Cloud-J v7.3e W. van Caspel et al. 10.5194/gmd-16-7433-2023
- Ozone solvatochromism in selected solvents F. Cataldo 10.1016/j.molliq.2018.07.021
- Heterogeneity and chemical reactivity of the remote troposphere defined by aircraft measurements – corrected H. Guo et al. 10.5194/acp-23-99-2023
30 citations as recorded by crossref.
- Global-scale distribution of ozone in the remote troposphere from the ATom and HIPPO airborne field missions I. Bourgeois et al. 10.5194/acp-20-10611-2020
- Cloud impacts on photochemistry: building a climatology of photolysis rates from the Atmospheric Tomography mission S. Hall et al. 10.5194/acp-18-16809-2018
- Forecasting carbon monoxide on a global scale for the ATom-1 aircraft mission: insights from airborne and satellite observations and modeling S. Strode et al. 10.5194/acp-18-10955-2018
- H2O2 and CH3OOH (MHP) in the Remote Atmosphere: 1. Global Distribution and Regional Influences H. Allen et al. 10.1029/2021JD035701
- A round Earth for climate models M. Prather & J. Hsu 10.1073/pnas.1908198116
- Tropospheric Ozone Assessment Report A. Archibald et al. 10.1525/elementa.2020.034
- GISS‐E2.1: Configurations and Climatology M. Kelley et al. 10.1029/2019MS002025
- Sea spray aerosol concentration modulated by sea surface temperature S. Liu et al. 10.1073/pnas.2020583118
- Lifetimes and timescales of tropospheric ozone M. Prather & X. Zhu 10.1525/elementa.2023.00112
- Resetting tropospheric OH and CH 4 lifetime with ultraviolet H 2 O absorption M. Prather & L. Zhu 10.1126/science.adn0415
- HCOOH in the Remote Atmosphere: Constraints from Atmospheric Tomography (ATom) Airborne Observations X. Chen et al. 10.1021/acsearthspacechem.1c00049
- Global Measurements of Brown Carbon and Estimated Direct Radiative Effects L. Zeng et al. 10.1029/2020GL088747
- A multi-model assessment of the Global Warming Potential of hydrogen M. Sand et al. 10.1038/s43247-023-00857-8
- Anthropogenic, biogenic, and photochemical influences on surface formaldehyde and its significant decadal (2006–2017) decrease in the Lewiston-Clarkston valley of the northwestern United States R. Li et al. 10.1016/j.chemosphere.2023.140962
- How Atmospheric Chemistry and Transport Drive Surface Variability of N2O and CFC‐11 D. Ruiz et al. 10.1029/2020JD033979
- On the Chemical Pathways Influencing the Effective Global Warming Potential of Commercial Hydrofluoroolefin Gases G. Salierno 10.1002/cssc.202400280
- Gravitational separation of Ar∕N<sub>2</sub> and age of air in the lowermost stratosphere in airborne observations and a chemical transport model B. Birner et al. 10.5194/acp-20-12391-2020
- Assessing Uncertainties and Approximations in Solar Heating of the Climate System J. Hsu & M. Prather 10.1029/2020MS002131
- Atlantic Multidecadal Variability and the U.K. ACSIS Program R. Sutton et al. 10.1175/BAMS-D-16-0266.1
- Evaluation of the interactive stratospheric ozone (O3v2) module in the E3SM version 1 Earth system model Q. Tang et al. 10.5194/gmd-14-1219-2021
- Global atmospheric CO<sub>2</sub> inverse models converging on neutral tropical land exchange, but disagreeing on fossil fuel and atmospheric growth rate B. Gaubert et al. 10.5194/bg-16-117-2019
- Description and evaluation of the UKCA stratosphere–troposphere chemistry scheme (StratTrop vn 1.0) implemented in UKESM1 A. Archibald et al. 10.5194/gmd-13-1223-2020
- Fast time response measurements of particle size distributions in the 3–60 nm size range with the nucleation mode aerosol size spectrometer C. Williamson et al. 10.5194/amt-11-3491-2018
- Deconstruction of tropospheric chemical reactivity using aircraft measurements: the Atmospheric Tomography Mission (ATom) data M. Prather et al. 10.5194/essd-15-3299-2023
- Heterogeneity and chemical reactivity of the remote troposphere defined by aircraft measurements H. Guo et al. 10.5194/acp-21-13729-2021
- How well can global chemistry models calculate the reactivity of short-lived greenhouse gases in the remote troposphere, knowing the chemical composition M. Prather et al. 10.5194/amt-11-2653-2018
- The IAGOS NO<sub><i>x</i></sub> instrument – design, operation and first results from deployment aboard passenger aircraft F. Berkes et al. 10.5194/amt-11-3737-2018
- Implementation and evaluation of updated photolysis rates in the EMEP MSC-W chemistry-transport model using Cloud-J v7.3e W. van Caspel et al. 10.5194/gmd-16-7433-2023
- Ozone solvatochromism in selected solvents F. Cataldo 10.1016/j.molliq.2018.07.021
- Heterogeneity and chemical reactivity of the remote troposphere defined by aircraft measurements – corrected H. Guo et al. 10.5194/acp-23-99-2023
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Latest update: 26 Jul 2024
Short summary
We present a new approach for comparing atmospheric chemistry models with measurements based on what these models are used to do, i.e., calculate changes in ozone and methane, prime greenhouse gases. This method anticipates a new type of measurements from the NASA Atmospheric Tomography (ATom) mission. In comparing the mixture of species within air parcels, we focus on those responsible for key chemical changes and weight these parcels by their chemical reactivity.
We present a new approach for comparing atmospheric chemistry models with measurements based on...
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