Articles | Volume 17, issue 14
https://doi.org/10.5194/acp-17-8923-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Special issue:
https://doi.org/10.5194/acp-17-8923-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
25 Jul 2017
Research article |
| 25 Jul 2017
Evaporation of sulfate aerosols at low relative humidity
Georgios Tsagkogeorgas
CORRESPONDING AUTHOR
Leibniz Institute for Tropospheric Research, 04318 Leipzig, Germany
Pontus Roldin
Department of Physics, University of Helsinki, P.O. Box 64, 00014
Helsinki, Finland
Division of Nuclear Physics, Lund University, P.O. Box 118, 221 00
Lund, Sweden
Jonathan Duplissy
Department of Physics, University of Helsinki, P.O. Box 64, 00014
Helsinki, Finland
Helsinki Institute of Physics, University of Helsinki, P.O. Box 64,
00014 Helsinki, Finland
Linda Rondo
Institute for Atmospheric and Environmental Sciences, Goethe
University Frankfurt, 60438 Frankfurt am Main, Germany
Jasmin Tröstl
Paul Scherrer Institute, 5232 Villigen, Switzerland
Jay G. Slowik
Paul Scherrer Institute, 5232 Villigen, Switzerland
Sebastian Ehrhart
Institute for Atmospheric and Environmental Sciences, Goethe
University Frankfurt, 60438 Frankfurt am Main, Germany
now at: Atmospheric Chemistry Department, Max Planck Institute for
Chemistry, 55128 Mainz, Germany
Alessandro Franchin
Department of Physics, University of Helsinki, P.O. Box 64, 00014
Helsinki, Finland
Andreas Kürten
Institute for Atmospheric and Environmental Sciences, Goethe
University Frankfurt, 60438 Frankfurt am Main, Germany
Antonio Amorim
Fac. Ciencias & CENTRA, Universidade de Lisboa, Campo Grande,
1749–016 Lisbon, Portugal
Federico Bianchi
Department of Physics, University of Helsinki, P.O. Box 64, 00014
Helsinki, Finland
Jasper Kirkby
Institute for Atmospheric and Environmental Sciences, Goethe
University Frankfurt, 60438 Frankfurt am Main, Germany
CERN, 1211 Geneva, Switzerland
Tuukka Petäjä
Department of Physics, University of Helsinki, P.O. Box 64, 00014
Helsinki, Finland
Urs Baltensperger
Paul Scherrer Institute, 5232 Villigen, Switzerland
Michael Boy
Department of Physics, University of Helsinki, P.O. Box 64, 00014
Helsinki, Finland
Joachim Curtius
Institute for Atmospheric and Environmental Sciences, Goethe
University Frankfurt, 60438 Frankfurt am Main, Germany
Richard C. Flagan
California Institute of Technology, Pasadena, CA 91125, USA
Markku Kulmala
Department of Physics, University of Helsinki, P.O. Box 64, 00014
Helsinki, Finland
Helsinki Institute of Physics, University of Helsinki, P.O. Box 64,
00014 Helsinki, Finland
Neil M. Donahue
Center for Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA 15213, USA
Frank Stratmann
Leibniz Institute for Tropospheric Research, 04318 Leipzig, Germany
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10 citations as recorded by crossref.
- Towards understanding the characteristics of new particle formation in the Eastern Mediterranean R. Baalbaki et al. 10.5194/acp-21-9223-2021
- Measurement report: Insights into the chemical composition and origin of molecular clusters and potential precursor molecules present in the free troposphere over the southern Indian Ocean: observations from the Maïdo Observatory (2150 m a.s.l., Réunion) R. Salignat et al. 10.5194/acp-24-3785-2024
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- In situ observation of new particle formation (NPF) in the tropical tropopause layer of the 2017 Asian monsoon anticyclone – Part 2: NPF inside ice clouds R. Weigel et al. 10.5194/acp-21-13455-2021
- The evolution and dynamics of the Hunga Tonga–Hunga Ha'apai sulfate aerosol plume in the stratosphere B. Legras et al. 10.5194/acp-22-14957-2022
- Modelling studies of HOMs and their contributions to new particle formation and growth: comparison of boreal forest in Finland and a polluted environment in China X. Qi et al. 10.5194/acp-18-11779-2018
- Modeling of exhaust gas cleaning by acid pollutant conversion to aerosol particles T. Olenius et al. 10.1016/j.fuel.2020.120044
- Atmospheric clusters to nanoparticles: Recent progress and challenges in closing the gap in chemical composition J. Smith et al. 10.1016/j.jaerosci.2020.105733
- Can formaldehyde contribute to atmospheric new particle formation from sulfuric acid and water? C. Wang et al. 10.1016/j.atmosenv.2018.12.057
- Wet Adhesion of Soap Bubble Bridge between Two Curved Surfaces P. Xu et al. 10.1155/2022/3340078
Latest update: 28 Mar 2025
Short summary
The H2SO4 vapour pressure plays key role in Earth's and Venus' atmospheres. In regions where RH is low and stabilising bases are scarce, H2SO4 can evaporate from particles; however the H2SO4 vapour pressure at low RH is uncertain. To address this, we measured H2SO4 evaporation versus T and RH in the CLOUD chamber and constrained the equilibrium constants for dissociation and dehydration of H2SO4. This study is important for nucleation, particle growth and H2SO4 formation occurring in atmosphere.
The H2SO4 vapour pressure plays key role in Earth's and Venus' atmospheres. In regions where RH...
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