Evaporation of sulfate aerosols at low relative humidity

Tsagkogeorgas, Georgios; Roldin, Pontus; Duplissy, Jonathan; Rondo, Linda; Tröstl, Jasmin; Slowik, Jay G.; Ehrhart, Sebastian; Franchin, Alessandro; Kürten, Andreas; Amorim, Antonio; Bianchi, Federico; Kirkby, Jasper; Petäjä, Tuukka; Baltensperger, Urs; Boy, Michael; Curtius, Joachim; Flagan, Richard C.; Kulmala, Markku; Donahue, Neil M.; Stratmann, Frank

doi:https://doi.org/10.5194/acp-17-8923-2017

Articles | Volume 17, issue 14

Atmos. Chem. Phys., 17, 8923–8938, 2017

https://doi.org/10.5194/acp-17-8923-2017

© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

Special issue: The CERN CLOUD experiment (ACP/AMT inter-journal SI)

Atmos. Chem. Phys., 17, 8923–8938, 2017

https://doi.org/10.5194/acp-17-8923-2017

© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

Articles | Volume 17, issue 14

Research article 25 Jul 2017

Research article | 25 Jul 2017

Evaporation of sulfate aerosols at low relative humidity

Georgios Tsagkogeorgas et al.

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Dec 2016	66	25	2	93
Jan 2017	43	38	2	83
Feb 2017	32	20	3	55
Mar 2017	45	37	8	90
Apr 2017	45	35	9	89
May 2017	45	16	7	68
Jun 2017	31	8	4	43
Jul 2017	128	41	3	172
Aug 2017	95	53	3	151
Sep 2017	44	38	2	84
Oct 2017	25	27	1	53
Nov 2017	19	15	0	34
Dec 2017	33	18	0	51
Jan 2018	17	10	1	28
Feb 2018	9	7	0	16
Mar 2018	17	18	1	36
Apr 2018	18	11	0	29
May 2018	11	18	1	30
Jun 2018	13	19	1	33
Jul 2018	11	11	1	23
Aug 2018	17	9	1	27
Sep 2018	11	11	3	25
Oct 2018	20	10	3	33
Nov 2018	16	8	3	27
Dec 2018	13	4	1	18
Jan 2019	5	5	3	13
Feb 2019	16	7	3	26
Mar 2019	8	6	2	16
Apr 2019	10	6	0	16
May 2019	11	10	6	27
Jun 2019	8	5	2	15
Jul 2019	6	4	2	12
Aug 2019	11	6	2	19
Sep 2019	11	4	4	19
Oct 2019	6	8	8	22
Nov 2019	10	9	3	22
Dec 2019	6	7	5	18
Jan 2020	10	4	2	16
Feb 2020	10	5	7	22
Mar 2020	4	4	7	15
Apr 2020	5	10	1	16
May 2020	9	12	6	27
Jun 2020	11	13	5	29
Jul 2020	17	23	11	51
Aug 2020	20	9	12	41
Sep 2020	19	13	3	35
Oct 2020	9	10	4	23
Nov 2020	6	12	8	26
Dec 2020	8	19	7	34
Jan 2021	17	23	15	55
Feb 2021	13	14	12	39
Mar 2021	15	24	7	46
Apr 2021	12	28	14	54
May 2021	7	9	18	34
Jun 2021	9	16	11	36
Jul 2021	8	13	1	22
Aug 2021	13	16	0	29
Sep 2021	15	31	1	47
Oct 2021	6	43	3	52
Nov 2021	11	20	1	32
Dec 2021	16	14	2	32
Jan 2022	11	14	5	30

Cumulative views and downloads (calculated since 16 Dec 2016)

Month	HTML	PDF	XML	Total
Dec 2016	66	25	2	93
Jan 2017	43	38	2	83
Feb 2017	32	20	3	55
Mar 2017	45	37	8	90
Apr 2017	45	35	9	89
May 2017	45	16	7	68
Jun 2017	31	8	4	43
Jul 2017	128	41	3	172
Aug 2017	95	53	3	151
Sep 2017	44	38	2	84
Oct 2017	25	27	1	53
Nov 2017	19	15	0	34
Dec 2017	33	18	0	51
Jan 2018	17	10	1	28
Feb 2018	9	7	0	16
Mar 2018	17	18	1	36
Apr 2018	18	11	0	29
May 2018	11	18	1	30
Jun 2018	13	19	1	33
Jul 2018	11	11	1	23
Aug 2018	17	9	1	27
Sep 2018	11	11	3	25
Oct 2018	20	10	3	33
Nov 2018	16	8	3	27
Dec 2018	13	4	1	18
Jan 2019	5	5	3	13
Feb 2019	16	7	3	26
Mar 2019	8	6	2	16
Apr 2019	10	6	0	16
May 2019	11	10	6	27
Jun 2019	8	5	2	15
Jul 2019	6	4	2	12
Aug 2019	11	6	2	19
Sep 2019	11	4	4	19
Oct 2019	6	8	8	22
Nov 2019	10	9	3	22
Dec 2019	6	7	5	18
Jan 2020	10	4	2	16
Feb 2020	10	5	7	22
Mar 2020	4	4	7	15
Apr 2020	5	10	1	16
May 2020	9	12	6	27
Jun 2020	11	13	5	29
Jul 2020	17	23	11	51
Aug 2020	20	9	12	41
Sep 2020	19	13	3	35
Oct 2020	9	10	4	23
Nov 2020	6	12	8	26
Dec 2020	8	19	7	34
Jan 2021	17	23	15	55
Feb 2021	13	14	12	39
Mar 2021	15	24	7	46
Apr 2021	12	28	14	54
May 2021	7	9	18	34
Jun 2021	9	16	11	36
Jul 2021	8	13	1	22
Aug 2021	13	16	0	29
Sep 2021	15	31	1	47
Oct 2021	6	43	3	52
Nov 2021	11	20	1	32
Dec 2021	16	14	2	32
Jan 2022	11	14	5	30

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Short summary

The H₂SO₄ vapour pressure plays key role in Earth's and Venus' atmospheres. In regions where RH is low and stabilising bases are scarce, H₂SO₄ can evaporate from particles; however the H₂SO₄ vapour pressure at low RH is uncertain. To address this, we measured H₂SO₄ evaporation versus T and RH in the CLOUD chamber and constrained the equilibrium constants for dissociation and dehydration of H₂SO₄. This study is important for nucleation, particle growth and H₂SO₄ formation occurring in atmosphere.

Article

Evaporation of sulfate aerosols at low relative humidity

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