Articles | Volume 17, issue 14
https://doi.org/10.5194/acp-17-8887-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-8887-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
24 Jul 2017
Research article |
| 24 Jul 2017
Modeling the role of highly oxidized multifunctional organic molecules for the growth of new particles over the boreal forest region
Emilie Öström
CORRESPONDING AUTHOR
Division of Nuclear Physics, Lund University, Lund, P.O. Box 118, 221 00, Sweden
Centre for Environmental and Climate Research, Lund University, Lund, P.O. Box 118, 221 00, Sweden
Zhou Putian
Department of Physics, University of Helsinki, Helsinki, P.O. Box 64, 00014, Finland
Guy Schurgers
Department of Geosciences and Natural Resource Management, University of Copenhagen, Copenhagen, 1350, Denmark
Mikhail Mishurov
Department of Physical Geography and Ecosystem Science, Lund University, Lund, 223 62, Sweden
Niku Kivekäs
Finnish Meteorological Institute, Helsinki, P.O. Box 503, 00101, Finland
Heikki Lihavainen
Finnish Meteorological Institute, Helsinki, P.O. Box 503, 00101, Finland
Mikael Ehn
Department of Physics, University of Helsinki, Helsinki, P.O. Box 64, 00014, Finland
Matti P. Rissanen
Department of Physics, University of Helsinki, Helsinki, P.O. Box 64, 00014, Finland
Theo Kurtén
Department of Chemistry, University of Helsinki, Helsinki, P.O. Box 55, 00014, Finland
Michael Boy
Department of Physics, University of Helsinki, Helsinki, P.O. Box 64, 00014, Finland
Erik Swietlicki
Division of Nuclear Physics, Lund University, Lund, P.O. Box 118, 221 00, Sweden
Pontus Roldin
Division of Nuclear Physics, Lund University, Lund, P.O. Box 118, 221 00, Sweden
Department of Physics, University of Helsinki, Helsinki, P.O. Box 64, 00014, Finland
Viewed
Total article views: 3,506 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 09 Dec 2016)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 2,143 | 1,219 | 144 | 3,506 | 425 | 78 | 138 |
- HTML: 2,143
- PDF: 1,219
- XML: 144
- Total: 3,506
- Supplement: 425
- BibTeX: 78
- EndNote: 138
Total article views: 2,652 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 24 Jul 2017)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 1,643 | 902 | 107 | 2,652 | 285 | 61 | 97 |
- HTML: 1,643
- PDF: 902
- XML: 107
- Total: 2,652
- Supplement: 285
- BibTeX: 61
- EndNote: 97
Total article views: 854 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 09 Dec 2016)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 500 | 317 | 37 | 854 | 140 | 17 | 41 |
- HTML: 500
- PDF: 317
- XML: 37
- Total: 854
- Supplement: 140
- BibTeX: 17
- EndNote: 41
Viewed (geographical distribution)
Total article views: 3,506 (including HTML, PDF, and XML)
Thereof 3,498 with geography defined
and 8 with unknown origin.
Total article views: 2,652 (including HTML, PDF, and XML)
Thereof 2,658 with geography defined
and -6 with unknown origin.
Total article views: 854 (including HTML, PDF, and XML)
Thereof 840 with geography defined
and 14 with unknown origin.
| Country | # | Views | % |
|---|
| Country | # | Views | % |
|---|
| Country | # | Views | % |
|---|
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
Cited
25 citations as recorded by crossref.
- Diesel soot aging in urban plumes within hours under cold dark and humid conditions A. Eriksson et al. 10.1038/s41598-017-12433-0
- Multi-year statistical and modeling analysis of submicrometer aerosol number size distributions at a rain forest site in Amazonia L. Varanda Rizzo et al. 10.5194/acp-18-10255-2018
- Theoretical study of the reaction of organic peroxyl radicals with alkenes and their accretion products involved in the atmospheric nucleation B. Dong et al. 10.1016/j.atmosenv.2024.120718
- Relative-humidity-dependent organic aerosol thermodynamics via an efficient reduced-complexity model K. Gorkowski et al. 10.5194/acp-19-13383-2019
- Modelling studies of HOMs and their contributions to new particle formation and growth: comparison of boreal forest in Finland and a polluted environment in China X. Qi et al. 10.5194/acp-18-11779-2018
- Highly Oxygenated Organic Molecules (HOM) from Gas-Phase Autoxidation Involving Peroxy Radicals: A Key Contributor to Atmospheric Aerosol F. Bianchi et al. 10.1021/acs.chemrev.8b00395
- Global simulations of monoterpene-derived peroxy radical fates and the distributions of highly oxygenated organic molecules (HOMs) and accretion products R. Xu et al. 10.5194/acp-22-5477-2022
- Natural Marine Precursors Boost Continental New Particle Formation and Production of Cloud Condensation Nuclei R. de Jonge et al. 10.1021/acs.est.4c01891
- New particle formation from agricultural recycling of organic waste products R. Ciuraru et al. 10.1038/s41612-021-00160-3
- Probing autoxidation of oleic acid at air-water interface: A neglected and significant pathway for secondary organic aerosols formation J. He et al. 10.1016/j.envres.2022.113232
- An aldehyde as a rapid source of secondary aerosol precursors: theoretical and experimental study of hexanal autoxidation S. Barua et al. 10.5194/acp-23-10517-2023
- Secondary aerosol formation in marine Arctic environments: a model measurement comparison at Ny-Ålesund C. Xavier et al. 10.5194/acp-22-10023-2022
- Aerosol characteristics and particle production in the upper troposphere over the Amazon Basin M. Andreae et al. 10.5194/acp-18-921-2018
- Overview: Recent advances in the understanding of the northern Eurasian environments and of the urban air quality in China – a Pan-Eurasian Experiment (PEEX) programme perspective H. Lappalainen et al. 10.5194/acp-22-4413-2022
- Estimation of biogenic VOC emissions and their corresponding impact on ozone and secondary organic aerosol formation in China K. Wu et al. 10.1016/j.atmosres.2019.104656
- Implementation of the sectional aerosol module SALSA2.0 into the PALM model system 6.0: model development and first evaluation M. Kurppa et al. 10.5194/gmd-12-1403-2019
- The role of highly oxygenated organic molecules in the Boreal aerosol-cloud-climate system P. Roldin et al. 10.1038/s41467-019-12338-8
- Combined Smog Chamber/Oxidation Flow Reactor Study on Aging of Secondary Organic Aerosol from Photooxidation of Aromatic Hydrocarbons T. Chen et al. 10.1021/acs.est.3c04089
- Aerosol mass yields of selected biogenic volatile organic compounds – a theoretical study with nearly explicit gas-phase chemistry C. Xavier et al. 10.5194/acp-19-13741-2019
- Chemical ionization mass spectrometry: Developments and applications for on-line characterization of atmospheric aerosols and trace gases Y. Zhang et al. 10.1016/j.trac.2023.117353
- Atmospheric clusters to nanoparticles: Recent progress and challenges in closing the gap in chemical composition J. Smith et al. 10.1016/j.jaerosci.2020.105733
- Interactions between the atmosphere, cryosphere, and ecosystems at northern high latitudes M. Boy et al. 10.5194/acp-19-2015-2019
- Multi-generation OH oxidation as a source for highly oxygenated organic molecules from aromatics O. Garmash et al. 10.5194/acp-20-515-2020
- Implementing detailed nucleation predictions in the Earth system model EC-Earth3.3.4: sulfuric acid–ammonia nucleation C. Svenhag et al. 10.5194/gmd-17-4923-2024
- Gas-to-Particle Partitioning of Cyclohexene- and α-Pinene-Derived Highly Oxygenated Dimers Evaluated Using COSMOtherm N. Hyttinen et al. 10.1021/acs.jpca.0c11328
25 citations as recorded by crossref.
- Diesel soot aging in urban plumes within hours under cold dark and humid conditions A. Eriksson et al. 10.1038/s41598-017-12433-0
- Multi-year statistical and modeling analysis of submicrometer aerosol number size distributions at a rain forest site in Amazonia L. Varanda Rizzo et al. 10.5194/acp-18-10255-2018
- Theoretical study of the reaction of organic peroxyl radicals with alkenes and their accretion products involved in the atmospheric nucleation B. Dong et al. 10.1016/j.atmosenv.2024.120718
- Relative-humidity-dependent organic aerosol thermodynamics via an efficient reduced-complexity model K. Gorkowski et al. 10.5194/acp-19-13383-2019
- Modelling studies of HOMs and their contributions to new particle formation and growth: comparison of boreal forest in Finland and a polluted environment in China X. Qi et al. 10.5194/acp-18-11779-2018
- Highly Oxygenated Organic Molecules (HOM) from Gas-Phase Autoxidation Involving Peroxy Radicals: A Key Contributor to Atmospheric Aerosol F. Bianchi et al. 10.1021/acs.chemrev.8b00395
- Global simulations of monoterpene-derived peroxy radical fates and the distributions of highly oxygenated organic molecules (HOMs) and accretion products R. Xu et al. 10.5194/acp-22-5477-2022
- Natural Marine Precursors Boost Continental New Particle Formation and Production of Cloud Condensation Nuclei R. de Jonge et al. 10.1021/acs.est.4c01891
- New particle formation from agricultural recycling of organic waste products R. Ciuraru et al. 10.1038/s41612-021-00160-3
- Probing autoxidation of oleic acid at air-water interface: A neglected and significant pathway for secondary organic aerosols formation J. He et al. 10.1016/j.envres.2022.113232
- An aldehyde as a rapid source of secondary aerosol precursors: theoretical and experimental study of hexanal autoxidation S. Barua et al. 10.5194/acp-23-10517-2023
- Secondary aerosol formation in marine Arctic environments: a model measurement comparison at Ny-Ålesund C. Xavier et al. 10.5194/acp-22-10023-2022
- Aerosol characteristics and particle production in the upper troposphere over the Amazon Basin M. Andreae et al. 10.5194/acp-18-921-2018
- Overview: Recent advances in the understanding of the northern Eurasian environments and of the urban air quality in China – a Pan-Eurasian Experiment (PEEX) programme perspective H. Lappalainen et al. 10.5194/acp-22-4413-2022
- Estimation of biogenic VOC emissions and their corresponding impact on ozone and secondary organic aerosol formation in China K. Wu et al. 10.1016/j.atmosres.2019.104656
- Implementation of the sectional aerosol module SALSA2.0 into the PALM model system 6.0: model development and first evaluation M. Kurppa et al. 10.5194/gmd-12-1403-2019
- The role of highly oxygenated organic molecules in the Boreal aerosol-cloud-climate system P. Roldin et al. 10.1038/s41467-019-12338-8
- Combined Smog Chamber/Oxidation Flow Reactor Study on Aging of Secondary Organic Aerosol from Photooxidation of Aromatic Hydrocarbons T. Chen et al. 10.1021/acs.est.3c04089
- Aerosol mass yields of selected biogenic volatile organic compounds – a theoretical study with nearly explicit gas-phase chemistry C. Xavier et al. 10.5194/acp-19-13741-2019
- Chemical ionization mass spectrometry: Developments and applications for on-line characterization of atmospheric aerosols and trace gases Y. Zhang et al. 10.1016/j.trac.2023.117353
- Atmospheric clusters to nanoparticles: Recent progress and challenges in closing the gap in chemical composition J. Smith et al. 10.1016/j.jaerosci.2020.105733
- Interactions between the atmosphere, cryosphere, and ecosystems at northern high latitudes M. Boy et al. 10.5194/acp-19-2015-2019
- Multi-generation OH oxidation as a source for highly oxygenated organic molecules from aromatics O. Garmash et al. 10.5194/acp-20-515-2020
- Implementing detailed nucleation predictions in the Earth system model EC-Earth3.3.4: sulfuric acid–ammonia nucleation C. Svenhag et al. 10.5194/gmd-17-4923-2024
- Gas-to-Particle Partitioning of Cyclohexene- and α-Pinene-Derived Highly Oxygenated Dimers Evaluated Using COSMOtherm N. Hyttinen et al. 10.1021/acs.jpca.0c11328
Latest update: 25 Dec 2024
Short summary
We used a model to study how biogenic volatile organic compounds (BVOCs) emitted from the boreal forest contribute to the formation and growth of particles in the atmosphere. Some of these particles are important climate forcers, acting as seeds for cloud droplet fomation. We implemented a new gas chemistry mechanism that describes how the BVOCs are oxidized and form low-volatility highly oxidized organic molecules. With the new mechanism we are able to accurately predict the particle growth.
We used a model to study how biogenic volatile organic compounds (BVOCs) emitted from the boreal...
Altmetrics
Final-revised paper
Preprint