Uncertainties of fluxes and <sup>13</sup>C  ∕ <sup>12</sup>C ratios of atmospheric reactive-gas emissions

Gromov, Sergey; Brenninkmeijer, Carl A. M.; Jöckel, Patrick

doi:https://doi.org/10.5194/acp-17-8525-2017

Articles | Volume 17, issue 13

https://doi.org/10.5194/acp-17-8525-2017

© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

Special issue:

The Modular Earth Submodel System (MESSy) (ACP/GMD inter-journal...

https://doi.org/10.5194/acp-17-8525-2017

© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

Articles | Volume 17, issue 13

Research article

|

13 Jul 2017

Research article |

| 13 Jul 2017

Uncertainties of fluxes and ¹³C  ∕ ¹²C ratios of atmospheric reactive-gas emissions

Sergey Gromov, Carl A. M. Brenninkmeijer, and Patrick Jöckel

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May 2017	37	8	11	56
Jun 2017	36	12	7	55
Jul 2017	151	56	2	209
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Short summary

We revisit the proxies/uncertainties for the ¹³C/¹²C ratios of emissions of reactive C into the atmosphere. Our main findings are (i) a factor of 2 less uncertain estimate of tropospheric CO surface sources δ¹³C, (ii) a confirmed disagreement between the bottom-up and top-down ¹³CO-inclusive emission estimates, and (iii) a novel estimate of the δ¹³C signatures of a range of NMHCs/VOCs to be used in modelling studies. Results are based on the EMAC model emission set-up evaluated for 2000.

Uncertainties of fluxes and ¹³C  ∕ ¹²C ratios of atmospheric reactive-gas emissions

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Uncertainties of fluxes and 13C ∕ 12C ratios of atmospheric reactive-gas emissions

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Uncertainties of fluxes and ¹³C  ∕ ¹²C ratios of atmospheric reactive-gas emissions