Articles | Volume 17, issue 8
https://doi.org/10.5194/acp-17-5459-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-5459-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
28 Apr 2017
Research article |
| 28 Apr 2017
Secondary organic aerosol formation in biomass-burning plumes: theoretical analysis of lab studies and ambient plumes
Qijing Bian
Department of Atmospheric Science, Colorado State University, Fort
Collins, CO, USA
Shantanu H. Jathar
Department of Mechanical Engineering, Colorado State University, Fort
Collins, CO, USA
John K. Kodros
Department of Atmospheric Science, Colorado State University, Fort
Collins, CO, USA
Kelley C. Barsanti
Department of Chemical and Environmental Engineering and College of
Engineering, Center for Environmental Research and Technology (CE-CERT),
University of California, Riverside, CA, USA
Lindsay E. Hatch
Department of Chemical and Environmental Engineering and College of
Engineering, Center for Environmental Research and Technology (CE-CERT),
University of California, Riverside, CA, USA
Andrew A. May
Department of Civil, Environmental and Geodetic Engineering, the Ohio
State University, Columbus, OH, USA
Sonia M. Kreidenweis
Department of Atmospheric Science, Colorado State University, Fort
Collins, CO, USA
Jeffrey R. Pierce
CORRESPONDING AUTHOR
Department of Atmospheric Science, Colorado State University, Fort
Collins, CO, USA
Department of Physics and Atmospheric Science, Dalhousie University,
Halifax, NS, Canada
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- Biomass burning in the northern peninsular Southeast Asia: Aerosol chemical profile and potential exposure S. Pani et al. 10.1016/j.atmosres.2019.03.031
- Transformation and ageing of biomass burning carbonaceous aerosol over tropical South America from aircraft in situ measurements during SAMBBA W. Morgan et al. 10.5194/acp-20-5309-2020
- Measurements of I/SVOCs in biomass-burning smoke using solid-phase extraction disks and two-dimensional gas chromatography L. Hatch et al. 10.5194/acp-18-17801-2018
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- NEIVAv1.0: Next-generation Emissions InVentory expansion of Akagi et al. (2011) version 1.0 S. Binte Shahid et al. 10.5194/gmd-17-7679-2024
- Emission and Evolution of Submicron Organic Aerosol in Smoke from Wildfires in the Western United States L. Garofalo et al. 10.1021/acsearthspacechem.9b00125
- Criteria-Based Identification of Important Fuels for Wildland Fire Emission Research A. Watts et al. 10.3390/atmos11060640
- Aging Effects on Biomass Burning Aerosol Mass and Composition: A Critical Review of Field and Laboratory Studies A. Hodshire et al. 10.1021/acs.est.9b02588
- Effects of Atmospheric Processing on the Oxidative Potential of Biomass Burning Organic Aerosols J. Wong et al. 10.1021/acs.est.9b01034
- Precursors and formation of secondary organic aerosols from wildfires in the Euro-Mediterranean region M. Majdi et al. 10.5194/acp-19-5543-2019
- Simulating the forest fire plume dispersion, chemistry, and aerosol formation using SAM-ASP version 1.0 C. Lonsdale et al. 10.5194/gmd-13-4579-2020
- Nonlinear behavior of organic aerosol in biomass burning plumes: a microphysical model analysis I. Konovalov et al. 10.5194/acp-19-12091-2019
- Evolution of Organic Aerosol From Wood Smoke Influenced by Burning Phase and Solar Radiation S. Li et al. 10.1029/2021JD034534
- An extensive assessment on the distribution pattern of organic contaminants in the aerosols samples in the Middle East M. Orif et al. 10.1515/chem-2022-0260
- Major secondary aerosol formation in southern African open biomass burning plumes V. Vakkari et al. 10.1038/s41561-018-0170-0
- Investigation of levoglucosan decay in wood smoke smog-chamber experiments: The importance of aerosol loading, temperature, and vapor wall losses in interpreting results V. Pratap et al. 10.1016/j.atmosenv.2018.11.020
- Effects of near-source coagulation of biomass burning aerosols on global predictions of aerosol size distributions and implications for aerosol radiative effects E. Ramnarine et al. 10.5194/acp-19-6561-2019
- Effects of photochemical aging on the molecular composition of organic aerosols derived from agricultural biomass burning in whole combustion process L. Li et al. 10.1016/j.scitotenv.2024.174152
- Impact of the Atmospheric Photochemical Evolution of the Organic Component of Biomass Burning Aerosol on Its Radiative Forcing Efficiency: A Box Model Analysis T. Zhuravleva et al. 10.3390/atmos12121555
- Secondary aerosol formation during the dark oxidation of residential biomass burning emissions J. Kodros et al. 10.1039/D2EA00031H
- Multi-day photochemical evolution of organic aerosol from biomass burning emissions A. Dearden et al. 10.1039/D3EA00111C
- Photochemical model evaluation of 2013 California wild fire air quality impacts using surface, aircraft, and satellite data K. Baker et al. 10.1016/j.scitotenv.2018.05.048
- Secondary organic aerosol formation from the laboratory oxidation of biomass burning emissions C. Lim et al. 10.5194/acp-19-12797-2019
- Six global biomass burning emission datasets: intercomparison and application in one global aerosol model X. Pan et al. 10.5194/acp-20-969-2020
- Links between the optical properties and chemical compositions of brown carbon chromophores in different environments: Contributions and formation of functionalized aromatic compounds X. Li et al. 10.1016/j.scitotenv.2021.147418
- Dilution impacts on smoke aging: evidence in Biomass Burning Observation Project (BBOP) data A. Hodshire et al. 10.5194/acp-21-6839-2021
- Atmospheric aging enhances the ice nucleation ability of biomass-burning aerosol L. Jahl et al. 10.1126/sciadv.abd3440
- Optical properties of biomass burning aerosol during the 2021 Oregon fire season: comparison between wild and prescribed fires A. Marsavin et al. 10.1039/D2EA00118G
- Differential response of human lung epithelial cells to particulate matter in fresh and photochemically aged biomass-burning smoke K. Atwi et al. 10.1016/j.atmosenv.2021.118929
- Insights into the aging of biomass burning aerosol from satellite observations and 3D atmospheric modeling: evolution of the aerosol optical properties in Siberian wildfire plumes I. Konovalov et al. 10.5194/acp-21-357-2021
- Tracing the Relative Significance of Primary versus Secondary Organic Aerosols from Biomass Burning Plumes over Coastal Ocean Using Sugar Compounds and Stable Carbon Isotopes S. Bikkina et al. 10.1021/acsearthspacechem.9b00140
- Spatiotemporal variation characteristics of global fires and their emissions H. Fan et al. 10.5194/acp-23-7781-2023
- Volatile Organic Compounds from Logwood Combustion: Emissions and Transformation under Dark and Photochemical Aging Conditions in a Smog Chamber A. Hartikainen et al. 10.1021/acs.est.7b06269
- Aerosol Mass and Optical Properties, Smoke Influence on O3, and High NO3 Production Rates in a Western U.S. City Impacted by Wildfires V. Selimovic et al. 10.1029/2020JD032791
- Constraining nucleation, condensation, and chemistry in oxidation flow reactors using size-distribution measurements and aerosol microphysical modeling A. Hodshire et al. 10.5194/acp-18-12433-2018
- Widespread biomass burning smoke throughout the remote troposphere G. Schill et al. 10.1038/s41561-020-0586-1
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- Introductory lecture: air quality in megacities L. Molina 10.1039/D0FD00123F
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- More Than Emissions and Chemistry: Fire Size, Dilution, and Background Aerosol Also Greatly Influence Near‐Field Biomass Burning Aerosol Aging A. Hodshire et al. 10.1029/2018JD029674
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- Radiative Forcing of Smoke Aerosol Taking into Account the Photochemical Evolution of Its Organic Component: Impact of Illumination Conditions and Surface Albedo T. Zhuravleva et al. 10.1134/S1024856023010219
- Dilution and photooxidation driven processes explain the evolution of organic aerosol in wildfire plumes A. Akherati et al. 10.1039/D1EA00082A
- Cloud processing and weeklong ageing affect biomass burning aerosol properties over the south-eastern Atlantic H. Che et al. 10.1038/s43247-022-00517-3
- Relationships between atmospheric mercury and optical properties of spring outflow aerosols from Southeast Asia L. Nguyen et al. 10.1016/j.apr.2021.101178
- Formation of secondary organic aerosol from wildfire emissions enhanced by long-time ageing Y. He et al. 10.1038/s41561-023-01355-4
- Computational simulation of the dynamics of secondary organic aerosol formation in an environmental chamber A. Sunol et al. 10.1080/02786826.2018.1427209
- Biomass burning in the northern peninsular Southeast Asia: Aerosol chemical profile and potential exposure S. Pani et al. 10.1016/j.atmosres.2019.03.031
- Transformation and ageing of biomass burning carbonaceous aerosol over tropical South America from aircraft in situ measurements during SAMBBA W. Morgan et al. 10.5194/acp-20-5309-2020
- Measurements of I/SVOCs in biomass-burning smoke using solid-phase extraction disks and two-dimensional gas chromatography L. Hatch et al. 10.5194/acp-18-17801-2018
Latest update: 18 Apr 2025
Short summary
In this paper, we perform simulations of the evolution of biomass-burning organic aerosol in laboratory smog-chamber experiments and ambient plumes. We find that in smog-chamber experiments, vapor wall losses lead to a large reduction in the apparent secondary organic aerosol formation. In ambient plumes, fire size and meteorology regulate the plume dilution rate, primary organic aerosol evaporation rate, and secondary organic aerosol formation rate.
In this paper, we perform simulations of the evolution of biomass-burning organic aerosol in...
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