Articles | Volume 17, issue 6
https://doi.org/10.5194/acp-17-4229-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-4229-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Evaluation of the absorption Ångström exponents for traffic and wood burning in the Aethalometer-based source apportionment using radiocarbon measurements of ambient aerosol
Peter Zotter
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen PSI, Switzerland
now at: Lucerne University of Applied Sciences and Arts, School of
Engineering and Architecture, Bioenergy Research, Technikumstrasse 21, 6048 Horw, Switzerland
Hanna Herich
Laboratory for Air Pollution and Environmental Technology, Swiss
Federal Laboratories for Materials Science and Technology (Empa),
Überlandstrasse 129, 8600 Dübendorf, Switzerland
now at: Kanton St.Gallen, Amt für Umwelt und Energie, 9001 St. Gallen, Switzerland
Martin Gysel
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen PSI, Switzerland
Imad El-Haddad
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen PSI, Switzerland
Yanlin Zhang
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen PSI, Switzerland
Department of Chemistry and Biochemistry, University of Bern, Bern,
Switzerland
Oeschger Centre for Climate Change Research, University of Bern, Bern,
Switzerland
Laboratory of Radiochemistry and Environmental Chemistry, Paul
Scherrer Institute (PSI), 5232 Villigen PSI, Switzerland
now at: Yale-NUIST Center on Atmospheric Environment, Nanjing
University of Information Science and Technology, 210044, Nanjing, China
Griša Močnik
Research and Development Department, Aerosol d.o.o., Ljubljana, Slovenia
Condensed Matter Physics Department, Jožef Stefan Institute,
Ljubljana, Slovenia
Christoph Hüglin
Laboratory for Air Pollution and Environmental Technology, Swiss
Federal Laboratories for Materials Science and Technology (Empa),
Überlandstrasse 129, 8600 Dübendorf, Switzerland
Urs Baltensperger
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen PSI, Switzerland
Sönke Szidat
Department of Chemistry and Biochemistry, University of Bern, Bern,
Switzerland
Oeschger Centre for Climate Change Research, University of Bern, Bern,
Switzerland
André S. H. Prévôt
CORRESPONDING AUTHOR
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen PSI, Switzerland
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Latest update: 14 Dec 2024
Short summary
Most studies use a single Ångström exponent for wood burning (αWB) and traffic (αTR) emissions in the Aethalometer model, used for source apportionment of black carbon, derived from previous work. However, accurate determination of the α values is currently lacking. Comparing radiocarbon measurements (14C) with the Aehtalometer model, good agreement was found, indicating that the Aethalometer model reproduces reasonably well the 14C results using our best estimate of a single αWB and αTR.
Most studies use a single Ångström exponent for wood burning (αWB) and traffic (αTR) emissions...
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