Articles | Volume 17, issue 3
https://doi.org/10.5194/acp-17-1673-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-1673-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
03 Feb 2017
Research article |
| 03 Feb 2017
Impact of biogenic very short-lived bromine on the Antarctic ozone hole during the 21st century
Rafael P. Fernandez
Department of Atmospheric Chemistry and Climate, Institute of Physical
Chemistry Rocasolano, CSIC, Madrid, 28006, Spain
National Research Council (CONICET), FCEN-UNCuyo, UNT-FRM, Mendoza,
5500, Argentina
Douglas E. Kinnison
Atmospheric Chemistry, Observations & Modelling Laboratory,
National Center for Atmospheric Research, Boulder, CO 80301, USA
Jean-Francois Lamarque
Atmospheric Chemistry, Observations & Modelling Laboratory,
National Center for Atmospheric Research, Boulder, CO 80301, USA
Simone Tilmes
Atmospheric Chemistry, Observations & Modelling Laboratory,
National Center for Atmospheric Research, Boulder, CO 80301, USA
Department of Atmospheric Chemistry and Climate, Institute of Physical
Chemistry Rocasolano, CSIC, Madrid, 28006, Spain
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36 citations as recorded by crossref.
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- Description and evaluation of the new UM–UKCA (vn11.0) Double Extended Stratospheric–Tropospheric (DEST vn1.0) scheme for comprehensive modelling of halogen chemistry in the stratosphere E. Bednarz et al. 10.5194/gmd-16-6187-2023
- Depletion of ozone and reservoir species of chlorine and nitrogen oxide in the lower Antarctic polar vortex measured from aircraft T. Jurkat et al. 10.1002/2017GL073270
- Natural short-lived halogens exert an indirect cooling effect on climate A. Saiz-Lopez et al. 10.1038/s41586-023-06119-z
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- Impacts of ocean biogeochemistry on atmospheric chemistry L. Tinel et al. 10.1525/elementa.2023.00032
- 200-year ice core bromine reconstruction at Dome C (Antarctica): observational and modelling results F. Burgay et al. 10.5194/tc-17-391-2023
- Arctic halogens reduce ozone in the northern mid-latitudes R. Fernandez et al. 10.1073/pnas.2401975121
- Brominated VSLS and their influence on ozone under a changing climate S. Falk et al. 10.5194/acp-17-11313-2017
- Delay in recovery of the Antarctic ozone hole from unexpected CFC-11 emissions S. Dhomse et al. 10.1038/s41467-019-13717-x
- Modeling the Effect of Potential Nitric Acid Removal During Convective Injection of Water Vapor Over the Central United States on the Chemical Composition of the Lower Stratosphere C. Clapp & J. Anderson 10.1029/2018JD029703
- The maintenance of elevated active chlorine levels in the Antarctic lower stratosphere through HCl null cycles R. Müller et al. 10.5194/acp-18-2985-2018
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- Rapid increase in atmospheric iodine levels in the North Atlantic since the mid-20th century C. Cuevas et al. 10.1038/s41467-018-03756-1
- The Chemistry of Mercury in the Stratosphere A. Saiz‐Lopez et al. 10.1029/2022GL097953
- Stratospheric Injection of Brominated Very Short‐Lived Substances: Aircraft Observations in the Western Pacific and Representation in Global Models P. Wales et al. 10.1029/2017JD027978
- Simulating the spread of disinfection by-products and anthropogenic bromoform emissions from ballast water discharge in Southeast Asia J. Maas et al. 10.5194/os-15-891-2019
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- Natural halogens buffer tropospheric ozone in a changing climate F. Iglesias-Suarez et al. 10.1038/s41558-019-0675-6
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- The relevance of reactions of the methyl peroxy radical (CH<sub>3</sub>O<sub>2</sub>) and methylhypochlorite (CH<sub>3</sub>OCl) for Antarctic chlorine activation and ozone loss A. Zafar et al. 10.1080/16000889.2018.1507391
- The influence of ocean halogen and sulfur emissions in the air quality of a coastal megacity: The case of Los Angeles M. Muñiz-Unamunzaga et al. 10.1016/j.scitotenv.2017.06.098
- Rapid increase in dichloromethane emissions from China inferred through atmospheric observations M. An et al. 10.1038/s41467-021-27592-y
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- Antarctic ozone hole modifies iodine geochemistry on the Antarctic Plateau A. Spolaor et al. 10.1038/s41467-021-26109-x
- Modeling the inorganic bromine partitioning in the tropical tropopause layer over the eastern and western Pacific Ocean M. Navarro et al. 10.5194/acp-17-9917-2017
- Probing the subtropical lowermost stratosphere and the tropical upper troposphere and tropopause layer for inorganic bromine B. Werner et al. 10.5194/acp-17-1161-2017
35 citations as recorded by crossref.
- Bromine from short-lived source gases in the extratropical northern hemispheric upper troposphere and lower stratosphere (UTLS) T. Keber et al. 10.5194/acp-20-4105-2020
- Modeling the Sources and Chemistry of Polar Tropospheric Halogens (Cl, Br, and I) Using the CAM‐Chem Global Chemistry‐Climate Model R. Fernandez et al. 10.1029/2019MS001655
- Description and evaluation of the new UM–UKCA (vn11.0) Double Extended Stratospheric–Tropospheric (DEST vn1.0) scheme for comprehensive modelling of halogen chemistry in the stratosphere E. Bednarz et al. 10.5194/gmd-16-6187-2023
- Depletion of ozone and reservoir species of chlorine and nitrogen oxide in the lower Antarctic polar vortex measured from aircraft T. Jurkat et al. 10.1002/2017GL073270
- Natural short-lived halogens exert an indirect cooling effect on climate A. Saiz-Lopez et al. 10.1038/s41586-023-06119-z
- Iodine chemistry in the chemistry–climate model SOCOL-AERv2-I A. Karagodin-Doyennel et al. 10.5194/gmd-14-6623-2021
- Impacts of ocean biogeochemistry on atmospheric chemistry L. Tinel et al. 10.1525/elementa.2023.00032
- 200-year ice core bromine reconstruction at Dome C (Antarctica): observational and modelling results F. Burgay et al. 10.5194/tc-17-391-2023
- Arctic halogens reduce ozone in the northern mid-latitudes R. Fernandez et al. 10.1073/pnas.2401975121
- Brominated VSLS and their influence on ozone under a changing climate S. Falk et al. 10.5194/acp-17-11313-2017
- Delay in recovery of the Antarctic ozone hole from unexpected CFC-11 emissions S. Dhomse et al. 10.1038/s41467-019-13717-x
- Modeling the Effect of Potential Nitric Acid Removal During Convective Injection of Water Vapor Over the Central United States on the Chemical Composition of the Lower Stratosphere C. Clapp & J. Anderson 10.1029/2018JD029703
- The maintenance of elevated active chlorine levels in the Antarctic lower stratosphere through HCl null cycles R. Müller et al. 10.5194/acp-18-2985-2018
- Global seasonal distribution of CH2Br2 and CHBr3 in the upper troposphere and lower stratosphere M. Jesswein et al. 10.5194/acp-22-15049-2022
- Seasonal impact of biogenic very short-lived bromocarbons on lowermost stratospheric ozone between 60° N and 60° S during the 21st century J. Barrera et al. 10.5194/acp-20-8083-2020
- A climatology of polar stratospheric cloud composition between 2002 and 2012 based on MIPAS/Envisat observations R. Spang et al. 10.5194/acp-18-5089-2018
- Rapid increase in atmospheric iodine levels in the North Atlantic since the mid-20th century C. Cuevas et al. 10.1038/s41467-018-03756-1
- The Chemistry of Mercury in the Stratosphere A. Saiz‐Lopez et al. 10.1029/2022GL097953
- Stratospheric Injection of Brominated Very Short‐Lived Substances: Aircraft Observations in the Western Pacific and Representation in Global Models P. Wales et al. 10.1029/2017JD027978
- Simulating the spread of disinfection by-products and anthropogenic bromoform emissions from ballast water discharge in Southeast Asia J. Maas et al. 10.5194/os-15-891-2019
- Transport of Asian surface pollutants to the global stratosphere from the Tibetan Plateau region during the Asian summer monsoon J. Bian et al. 10.1093/nsr/nwaa005
- Intercomparison Between Surrogate, Explicit, and Full Treatments of VSL Bromine Chemistry Within the CAM‐Chem Chemistry‐Climate Model R. Fernandez et al. 10.1029/2020GL091125
- Comparing the Effect of Anthropogenically Amplified Halogen Natural Emissions on Tropospheric Ozone Chemistry Between Pre‐Industrial and Present‐Day J. Barrera et al. 10.1029/2022JD038283
- Natural halogens buffer tropospheric ozone in a changing climate F. Iglesias-Suarez et al. 10.1038/s41558-019-0675-6
- Understanding atmospheric methane sub-seasonal variability over India Y. Tiwari et al. 10.1016/j.atmosenv.2019.117206
- Very short-lived halogens amplify ozone depletion trends in the tropical lower stratosphere J. Villamayor et al. 10.1038/s41558-023-01671-y
- Impacts of stratospheric sulfate geoengineering on tropospheric ozone L. Xia et al. 10.5194/acp-17-11913-2017
- The relevance of reactions of the methyl peroxy radical (CH<sub>3</sub>O<sub>2</sub>) and methylhypochlorite (CH<sub>3</sub>OCl) for Antarctic chlorine activation and ozone loss A. Zafar et al. 10.1080/16000889.2018.1507391
- The influence of ocean halogen and sulfur emissions in the air quality of a coastal megacity: The case of Los Angeles M. Muñiz-Unamunzaga et al. 10.1016/j.scitotenv.2017.06.098
- Rapid increase in dichloromethane emissions from China inferred through atmospheric observations M. An et al. 10.1038/s41467-021-27592-y
- The influence of iodine on the Antarctic stratospheric ozone hole C. Cuevas et al. 10.1073/pnas.2110864119
- Influence of emission inventory resolution on the modeled spatio-temporal distribution of air pollutants in Buenos Aires, Argentina, using WRF-Chem A. López-Noreña et al. 10.1016/j.atmosenv.2021.118839
- Physiological responses and altered halocarbon production in Phaeodactylum tricornutum after exposure to polystyrene microplastics X. Lang et al. 10.1016/j.ecoenv.2023.115702
- Antarctic ozone hole modifies iodine geochemistry on the Antarctic Plateau A. Spolaor et al. 10.1038/s41467-021-26109-x
- Modeling the inorganic bromine partitioning in the tropical tropopause layer over the eastern and western Pacific Ocean M. Navarro et al. 10.5194/acp-17-9917-2017
Latest update: 20 Nov 2024
Short summary
The inclusion of biogenic very-short lived bromine (VSLBr) in a chemistry-climate model produces an expansion of the ozone hole area of ~ 5 million km2, which is equivalent in magnitude to the recently estimated Antarctic ozone healing due to the reduction of anthropogenic CFCs and halons. The maximum Antarctic ozone hole depletion increases by up to 14 % when natural VSLBr are considered, but does not introduce a significant delay of the modelled ozone return date to 1980 October levels.
The inclusion of biogenic very-short lived bromine (VSLBr) in a chemistry-climate model produces...
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