Articles | Volume 17, issue 2
https://doi.org/10.5194/acp-17-1571-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-1571-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
31 Jan 2017
Research article |
| 31 Jan 2017
Uptake of nitric acid, ammonia, and organics in orographic clouds: mass spectrometric analyses of droplet residual and interstitial aerosol particles
Johannes Schneider
CORRESPONDING AUTHOR
Particle Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Stephan Mertes
Leibniz Institute for Tropospheric Research, 04318 Leipzig, Germany
Dominik van Pinxteren
Leibniz Institute for Tropospheric Research, 04318 Leipzig, Germany
Hartmut Herrmann
Leibniz Institute for Tropospheric Research, 04318 Leipzig, Germany
Stephan Borrmann
Particle Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
Institute for Atmospheric Physics, Johannes Gutenberg University, 55128 Mainz, Germany
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- Stage-resolved in-cloud scavenging of submicron and BC-containing particles: A case study Y. Yang et al. 10.1016/j.atmosenv.2020.117883
- Box Model Intercomparison of Cloud Chemistry M. Barth et al. 10.1029/2021JD035486
- In situ chemical composition measurement of individual cloud residue particles at a mountain site, southern China Q. Lin et al. 10.5194/acp-17-8473-2017
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- A systematic re-evaluation of methods for quantification of bulk particle-phase organic nitrates using real-time aerosol mass spectrometry D. Day et al. 10.5194/amt-15-459-2022
- In-cloud scavenging of chemically segregated particle types by individual particle observation Y. Yang et al. 10.1016/j.apgeochem.2023.105657
- In Situ Observation of Multiphase Oxidation-Driven Secondary Organic Aerosol Formation during Cloud Processing at a Mountain Site in Southern China M. Gao et al. 10.1021/acs.estlett.3c00331
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- Observations on aerosol optical properties and scavenging during cloud events A. Ruuskanen et al. 10.5194/acp-21-1683-2021
- Mass spectrometric measurements of ambient ions and estimation of gaseous sulfuric acid in the free troposphere and lowermost stratosphere during the CAFE-EU/BLUESKY campaign M. Zauner-Wieczorek et al. 10.5194/acp-22-11781-2022
- Enrichment of submicron sea-salt-containing particles in small cloud droplets based on single-particle mass spectrometry Q. Lin et al. 10.5194/acp-19-10469-2019
- Aircraft-based observations of isoprene-epoxydiol-derived secondary organic aerosol (IEPOX-SOA) in the tropical upper troposphere over the Amazon region C. Schulz et al. 10.5194/acp-18-14979-2018
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- Comparison of acidity and chemical composition of summertime cloud water and aerosol at an alpine site in Northwest China: Implications for the neutral property of clouds in the free troposphere M. Shen et al. 10.1016/j.scitotenv.2024.171775
- Observed below-Cloud and Cloud Interstitial Submicron Aerosol Chemical and Physical Properties at Whiteface Mountain, New York, during August 2017 J. Zhang et al. 10.1021/acsearthspacechem.9b00117
Latest update: 29 Jun 2024
Short summary
We analyzed the composition of cloud droplet residuals and of aerosol particles sampled on a mountaintop site. The data show that about 85 % of the submicron aerosol mass partitions into the cloud phase, and that the uptake of soluble compounds (nitric acid, ammonia, and organic gases) from the gas phase into the cloud droplets is very effective. This will lead to a redistribution of these compounds among the aerosol particles and thereby to a more uniform aerosol after cloud evaporation.
We analyzed the composition of cloud droplet residuals and of aerosol particles sampled on a...
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