Articles | Volume 17, issue 17
https://doi.org/10.5194/acp-17-10743-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-10743-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Gasoline aromatics: a critical determinant of urban secondary organic aerosol formation
Jianfei Peng
State Key Joint Laboratory of Environmental Simulation and
Pollution Control, College of Environmental Sciences and Engineering, Peking
University, Beijing 100871, China
now at: Department of Atmospheric Sciences, Texas A&M
University, College Station, TX 77843, USA
State Key Joint Laboratory of Environmental Simulation and
Pollution Control, College of Environmental Sciences and Engineering, Peking
University, Beijing 100871, China
Beijing Innovation Center for Engineering Science and Advanced
Technology, Peking University, Beijing 100871, China
Zhuofei Du
State Key Joint Laboratory of Environmental Simulation and
Pollution Control, College of Environmental Sciences and Engineering, Peking
University, Beijing 100871, China
Yinhui Wang
State Key Laboratory of Automotive Safety and Energy, Tsinghua
University, Beijing 100084, China
Jing Zheng
State Key Joint Laboratory of Environmental Simulation and
Pollution Control, College of Environmental Sciences and Engineering, Peking
University, Beijing 100871, China
Wenbin Zhang
State Key Laboratory of Automotive Safety and Energy, Tsinghua
University, Beijing 100084, China
Yudong Yang
State Key Joint Laboratory of Environmental Simulation and
Pollution Control, College of Environmental Sciences and Engineering, Peking
University, Beijing 100871, China
Yanhong Qin
State Key Joint Laboratory of Environmental Simulation and
Pollution Control, College of Environmental Sciences and Engineering, Peking
University, Beijing 100871, China
Rong Zheng
State Key Laboratory of Automotive Safety and Energy, Tsinghua
University, Beijing 100084, China
Yao Xiao
State Key Joint Laboratory of Environmental Simulation and
Pollution Control, College of Environmental Sciences and Engineering, Peking
University, Beijing 100871, China
Yusheng Wu
State Key Joint Laboratory of Environmental Simulation and
Pollution Control, College of Environmental Sciences and Engineering, Peking
University, Beijing 100871, China
Sihua Lu
State Key Joint Laboratory of Environmental Simulation and
Pollution Control, College of Environmental Sciences and Engineering, Peking
University, Beijing 100871, China
Zhijun Wu
State Key Joint Laboratory of Environmental Simulation and
Pollution Control, College of Environmental Sciences and Engineering, Peking
University, Beijing 100871, China
State Key Joint Laboratory of Environmental Simulation and
Pollution Control, College of Environmental Sciences and Engineering, Peking
University, Beijing 100871, China
Hongjun Mao
College of Environmental Sciences and Engineering, Nankai University,
Tianjin 300071, China
Shijin Shuai
CORRESPONDING AUTHOR
State Key Laboratory of Automotive Safety and Energy, Tsinghua
University, Beijing 100084, China
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59 citations as recorded by crossref.
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- Using an oxidation flow reactor to understand the effects of gasoline aromatics and ethanol levels on secondary aerosol formation N. Kuittinen et al. 10.1016/j.envres.2021.111453
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- Investigation of fluorine-promoted Pt-Re/Al2O3 catalysts in reforming of n-heptane E. Belopukhov et al. 10.1016/j.cattod.2021.06.016
- Refueling emission of volatile organic compounds from China 6 gasoline vehicles L. Sun et al. 10.1016/j.scitotenv.2021.147883
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- Primary organic gas emissions from gasoline vehicles in China: Factors, composition and trends L. Qi et al. 10.1016/j.envpol.2021.117984
- Effects of driving conditions on secondary aerosol formation from a GDI vehicle using an oxidation flow reactor N. Kuittinen et al. 10.1016/j.envpol.2021.117069
- Photochemical Transformation and Secondary Aerosol Formation Potential of Euro6 Gasoline and Diesel Passenger Car Exhaust Emissions O. Sippula et al. 10.2139/ssrn.4199864
- Tailpipe volatile organic compounds (VOCs) emissions from Chinese gasoline vehicles under different vehicle standards, fuel types, and driving conditions P. Liu et al. 10.1016/j.atmosenv.2024.120348
- Marked impacts of transient conditions on potential secondary organic aerosol production during rapid oxidation of gasoline exhausts J. Zhang et al. 10.1038/s41612-023-00385-4
- Aromatic compounds in a semi-urban site of western India: Seasonal variability and emission ratios L. Sahu et al. 10.1016/j.atmosres.2020.105114
- Secondary aerosol formation from a Chinese gasoline vehicle: Impacts of fuel (E10, gasoline) and driving conditions (idling, cruising) H. Wang et al. 10.1016/j.scitotenv.2021.148809
- Emission characteristics of intermediate volatility organic compounds from a Chinese gasoline engine under varied operating conditions: Influence of fuel, velocity, torque, rotational speed, and after-treatment device R. Tang et al. 10.1016/j.scitotenv.2023.167761
- Evaluating vehicular exhaust and evaporative emissions via VOC measurement in an underground parking garage Y. Wu et al. 10.1016/j.envpol.2023.122022
- Contrasting size-resolved hygroscopicity of fine particles derived by HTDMA and HR-ToF-AMS measurements between summer and winter in Beijing: the impacts of aerosol aging and local emissions X. Fan et al. 10.5194/acp-20-915-2020
- Ageing and hygroscopicity variation of black carbon particles in Beijing measured by a quasi-atmospheric aerosol evolution study (QUALITY) chamber J. Peng et al. 10.5194/acp-17-10333-2017
58 citations as recorded by crossref.
- Review of Chinese atmospheric science research over the past 70 years: Atmospheric physics and atmospheric environment T. Wang et al. 10.1007/s11430-019-9536-1
- Evaporative emission from China 5 and China 6 gasoline vehicles: Emission factors, profiles and future perspective Y. Liu et al. 10.1016/j.jclepro.2021.129861
- Comparison of primary aerosol emission and secondary aerosol formation from gasoline direct injection and port fuel injection vehicles Z. Du et al. 10.5194/acp-18-9011-2018
- Evaluating the relationships between aromatic and ethanol levels in gasoline on secondary aerosol formation from a gasoline direct injection vehicle P. Roth et al. 10.1016/j.scitotenv.2020.140333
- New Insights into the Radical Chemistry and Product Distribution in the OH-Initiated Oxidation of Benzene L. Xu et al. 10.1021/acs.est.0c04780
- Secondary Organic Aerosol Formation from Urban Roadside Air in Hong Kong T. Liu et al. 10.1021/acs.est.8b06587
- Evaluation of the Role of Lubricant Additives in Emission Control H. Shao et al. 10.3390/lubricants10120362
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- Potential dual effect of anthropogenic emissions on the formation of biogenic secondary organic aerosol (BSOA) E. Kari et al. 10.5194/acp-19-15651-2019
- Remarkable nucleation and growth of ultrafine particles from vehicular exhaust S. Guo et al. 10.1073/pnas.1916366117
- A comprehensive study on emission of volatile organic compounds for light duty gasoline passenger vehicles in China: Illustration of impact factors and renewal emissions of major compounds B. Li et al. 10.1016/j.envres.2020.110461
- Effects of short chain aromatics in gasoline on GDI engine combustion and emissions Z. He et al. 10.1016/j.fuel.2021.120725
- Photochemical transformation and secondary aerosol formation potential of Euro6 gasoline and diesel passenger car exhaust emissions A. Hartikainen et al. 10.1016/j.jaerosci.2023.106159
- Using an oxidation flow reactor to understand the effects of gasoline aromatics and ethanol levels on secondary aerosol formation N. Kuittinen et al. 10.1016/j.envres.2021.111453
- Catalyzed Gasoline Particulate Filters Reduce Secondary Organic Aerosol Production from Gasoline Direct Injection Vehicles P. Roth et al. 10.1021/acs.est.8b06418
- Evaluation of the chemical composition of gas- and particle-phase products of aromatic oxidation A. Mehra et al. 10.5194/acp-20-9783-2020
- Towards zero pollution vehicles by advanced fuels and exhaust aftertreatment technologies S. Saarikoski et al. 10.1016/j.envpol.2024.123665
- Influence of Inorganic Gases on Formation and Chemical Composition of Monoaromatic Hydrocarbons Secondary Organic Aerosol J. XU & M. HUANG 10.1016/S1872-2040(20)60008-1
- Performance Analysis of New Continue FCC Bench Scale: Modified HS-FCC Integrated with Riser in Producing Bio-Hydrocarbon C. Widiawaty et al. 10.2139/ssrn.3950080
- Source–Receptor Relationship Revealed by the Halted Traffic and Aggravated Haze in Beijing during the COVID-19 Lockdown Z. Lv et al. 10.1021/acs.est.0c04941
- Suppression of anthropogenic secondary organic aerosol formation by isoprene K. Li et al. 10.1038/s41612-022-00233-x
- Toxicological responses in human airway epithelial cells (BEAS-2B) exposed to particulate matter emissions from gasoline fuels with varying aromatic and ethanol levels C. Ahmed et al. 10.1016/j.scitotenv.2019.135732
- Characteristics of volatile organic compounds and secondary organic aerosol pollution in different functional areas of petrochemical industrial cities in Northwest China Y. Yang et al. 10.1016/j.scitotenv.2022.159903
- Highly efficient adsorption of benzothiophene from model fuel on a metal-organic framework modified with dodeca-tungstophosphoric acid L. Ullah et al. 10.1016/j.cej.2018.12.141
- Characterization of single scattering albedo and chemical components of aged toluene secondary organic aerosol Z. Feng et al. 10.1016/j.apr.2019.07.005
- Chemical characterization and source identification of PM<sub>2.5</sub> at multiple sites in the Beijing–Tianjin–Hebei region, China X. Huang et al. 10.5194/acp-17-12941-2017
- Multiphase interactions between sulfur dioxide and secondary organic aerosol from the photooxidation of toluene: Reactivity and sulfate formation Q. Ye et al. 10.1016/j.scitotenv.2023.168736
- Formation kinetics and mechanisms of ozone and secondary organic aerosols from photochemical oxidation of different aromatic hydrocarbons: dependence on NO<sub><i>x</i></sub> and organic substituents H. Luo et al. 10.5194/acp-21-7567-2021
- Investigation of fluorine-promoted Pt-Re/Al2O3 catalysts in reforming of n-heptane E. Belopukhov et al. 10.1016/j.cattod.2021.06.016
- Refueling emission of volatile organic compounds from China 6 gasoline vehicles L. Sun et al. 10.1016/j.scitotenv.2021.147883
- Tunnel measurements reveal significant reduction in traffic-related light-absorbing aerosol emissions in China C. Ho et al. 10.1016/j.scitotenv.2022.159212
- Effects of fuel composition and vehicle operating temperature on in vitro toxicity of exhaust emissions H. Hakkarainen et al. 10.1039/D3EA00136A
- Secondary Organic and Inorganic Aerosol Formation from a GDI Vehicle under Different Driving Conditions W. Peng et al. 10.3390/atmos13030433
- Intermediate and high ethanol blends reduce secondary organic aerosol formation from gasoline direct injection vehicles P. Roth et al. 10.1016/j.atmosenv.2019.117064
- Vehicular non-exhaust particulate emissions in Chinese megacities: Source profiles, real-world emission factors, and inventories J. Zhang et al. 10.1016/j.envpol.2020.115268
- Isobaric Vapor–Liquid Equilibria for Binary Mixtures of Gamma-Valerolactone + Toluene M. Al-Lami et al. 10.1021/acs.jced.0c00791
- Important role of aromatic hydrocarbons in SOA formation from unburned gasoline vapor T. Chen et al. 10.1016/j.atmosenv.2019.01.001
- Optical properties of vehicular brown carbon emissions: Road tunnel and chassis dynamometer tests C. Ho et al. 10.1016/j.envpol.2023.121037
- Characterization, mixing state, and evolution of single particles in a megacity of Sichuan Basin, southwest China J. Zhang et al. 10.1016/j.atmosres.2018.03.014
- Emission Reduction of Traffic-Related Light-Absorbing Aerosols in a Megacity in China: A Case Study Via Tunnel Measurements C. Ho et al. 10.2139/ssrn.4164413
- Effects of Ammonia Mitigation on Secondary Organic Aerosol and Ammonium Nitrate Particle Formation in Photochemical Reacted Gasoline Vehicle Exhausts H. Hagino & R. Uchida 10.3390/atmos15091061
- Characteristics of Volatile Organic Compounds and Their Contribution to Secondary Organic Aerosols during the High O3 Period in a Central Industry City in China D. Yao et al. 10.3390/atmos13101625
- Nonlinear and lagged effects of VOCs on SOA and O3 and multi-model validated control strategy for VOC sources R. Wang et al. 10.1016/j.scitotenv.2023.164113
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- Brake wear-derived particles: Single-particle mass spectral signatures and real-world emissions J. Liu et al. 10.1016/j.ese.2023.100240
- Modelling molecular composition of SOA from toluene photo-oxidation at urban and street scales K. Sartelet et al. 10.1039/D4EA00049H
- Measurement report: Distinct emissions and volatility distribution of intermediate-volatility organic compounds from on-road Chinese gasoline vehicles: implication of high secondary organic aerosol formation potential R. Tang et al. 10.5194/acp-21-2569-2021
- Primary organic gas emissions from gasoline vehicles in China: Factors, composition and trends L. Qi et al. 10.1016/j.envpol.2021.117984
- Effects of driving conditions on secondary aerosol formation from a GDI vehicle using an oxidation flow reactor N. Kuittinen et al. 10.1016/j.envpol.2021.117069
- Photochemical Transformation and Secondary Aerosol Formation Potential of Euro6 Gasoline and Diesel Passenger Car Exhaust Emissions O. Sippula et al. 10.2139/ssrn.4199864
- Tailpipe volatile organic compounds (VOCs) emissions from Chinese gasoline vehicles under different vehicle standards, fuel types, and driving conditions P. Liu et al. 10.1016/j.atmosenv.2024.120348
- Marked impacts of transient conditions on potential secondary organic aerosol production during rapid oxidation of gasoline exhausts J. Zhang et al. 10.1038/s41612-023-00385-4
- Aromatic compounds in a semi-urban site of western India: Seasonal variability and emission ratios L. Sahu et al. 10.1016/j.atmosres.2020.105114
- Secondary aerosol formation from a Chinese gasoline vehicle: Impacts of fuel (E10, gasoline) and driving conditions (idling, cruising) H. Wang et al. 10.1016/j.scitotenv.2021.148809
- Emission characteristics of intermediate volatility organic compounds from a Chinese gasoline engine under varied operating conditions: Influence of fuel, velocity, torque, rotational speed, and after-treatment device R. Tang et al. 10.1016/j.scitotenv.2023.167761
- Evaluating vehicular exhaust and evaporative emissions via VOC measurement in an underground parking garage Y. Wu et al. 10.1016/j.envpol.2023.122022
- Contrasting size-resolved hygroscopicity of fine particles derived by HTDMA and HR-ToF-AMS measurements between summer and winter in Beijing: the impacts of aerosol aging and local emissions X. Fan et al. 10.5194/acp-20-915-2020
Latest update: 15 Nov 2024
Short summary
Through an environmental chamber approach, we find that a small increase in aromatic content in gasoline fuel will result in a large enhancement in the secondary organic aerosol formation from vehicle exhaust. The higher emissions of both monocyclic and polycyclic aromatic organic compounds from the high-aromatic fuel played an essential role. Our findings highlight the importance of more stringent regulation of gasoline aromatic content for air quality in urban areas.
Through an environmental chamber approach, we find that a small increase in aromatic content in...
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