Articles | Volume 17, issue 16
https://doi.org/10.5194/acp-17-10001-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-10001-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
25 Aug 2017
Research article |
| 25 Aug 2017
Modeling atmospheric mineral aerosol chemistry to predict heterogeneous photooxidation of SO2
Zechen Yu
Department of Environmental Engineering Sciences,
Engineering School of Sustainable Infrastructure and Environment, University
of Florida, P.O. Box 116450 Gainesville, FL 32611, USA
Department of Environmental Engineering Sciences,
Engineering School of Sustainable Infrastructure and Environment, University
of Florida, P.O. Box 116450 Gainesville, FL 32611, USA
Jiyeon Park
Department of Environmental Engineering Sciences,
Engineering School of Sustainable Infrastructure and Environment, University
of Florida, P.O. Box 116450 Gainesville, FL 32611, USA
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Cited
26 citations as recorded by crossref.
- Particle formation and surface processes on atmospheric aerosols: A review of applied quantum chemical calculations A. Leonardi et al. 10.1002/qua.26350
- Impact of mineral dust photocatalytic heterogeneous chemistry on the formation of the sulfate and nitrate: A modelling study over East Asia X. Li et al. 10.1016/j.atmosenv.2023.120166
- Ammonium nitrate promotes sulfate formation through uptake kinetic regime Y. Liu et al. 10.5194/acp-21-13269-2021
- Unveiling the Role of Carbonate Radical Anions in Dust‐Driven SO2 Oxidation Y. Liu et al. 10.1029/2023JD040017
- Photocatalytic Oxidation of SO2 by TiO2: Aerosol Formation and the Key Role of Gaseous Reactive Oxygen Species Y. Chen et al. 10.1021/acs.est.1c01608
- Vibrational spectroscopy as a probe of heterogeneities within geochemical thin films on macro, micro, and nanoscales D. Kim et al. 10.1039/D3RA05179J
- Photo-enhanced uptake of SO2 on Icelandic volcanic dusts J. Lasne et al. 10.1039/D1EA00094B
- Atmospheric Nitrate Formation through Oxidation by Carbonate Radical X. Fang et al. 10.1021/acsearthspacechem.1c00169
- Significant formation of sulfate aerosols contributed by the heterogeneous drivers of dust surface T. Wang et al. 10.5194/acp-22-13467-2022
- Atmospheric Processes of Aromatic Hydrocarbons in the Presence of Mineral Dust Particles in an Urban Environment Z. Yu & M. Jang 10.1021/acsearthspacechem.9b00195
- Simulation of SOA formation from the photooxidation of monoalkylbenzenes in the presence of aqueous aerosols containing electrolytes under various NO<sub><i>x</i></sub> levels C. Zhou et al. 10.5194/acp-19-5719-2019
- Acidity and the multiphase chemistry of atmospheric aqueous particles and clouds A. Tilgner et al. 10.5194/acp-21-13483-2021
- The evaluation on artificial neural networks (ANN) and multiple linear regressions (MLR) models for predicting SO2 concentration S. Shams et al. 10.1016/j.uclim.2021.100837
- A review on the heterogeneous oxidation of SO2 on solid atmospheric particles: Implications for sulfate formation in haze chemistry Q. Ma et al. 10.1080/10643389.2023.2190315
- Impact of flow velocity on the heterogeneous reaction of SO2 over Fe2O3 Y. Liu et al. 10.1016/j.atmosenv.2022.119491
- Seasonality in the Δ<sup>33</sup>S measured in urban aerosols highlights an additional oxidation pathway for atmospheric SO<sub>2</sub> D. Au Yang et al. 10.5194/acp-19-3779-2019
- Critical Roles of Surface-Enhanced Heterogeneous Oxidation of SO2 in Haze Chemistry: Review of Extended Pathways for Complex Air Pollution Z. Zhang et al. 10.1007/s40726-023-00287-2
- Roles of Sulfur Oxidation Pathways in the Variability in Stable Sulfur Isotopic Composition of Sulfate Aerosols at an Urban Site in Beijing, China M. Fan et al. 10.1021/acs.estlett.0c00623
- Effects of SO2 on NH4NO3 Photolysis: The Role of Reducibility and Acidic Products Q. Cao et al. 10.1021/acs.est.3c01082
- Atmospheric Chemistry of Oxalate: Insight Into the Role of Relative Humidity and Aerosol Acidity From High‐Resolution Observation C. Yang et al. 10.1029/2021JD035364
- Simulation of heterogeneous photooxidation of SO<sub>2</sub> and NO<sub><i>x</i></sub> in the presence of Gobi Desert dust particles under ambient sunlight Z. Yu & M. Jang 10.5194/acp-18-14609-2018
- Simulating the Impact of Long-Range-Transported Asian Mineral Dust on the Formation of Sulfate and Nitrate during the KORUS-AQ Campaign Z. Yu et al. 10.1021/acsearthspacechem.0c00074
- Research Progress on Heterogeneous Reactions of Pollutant Gases on the Surface of Atmospheric Mineral Particulate Matter in China F. Zheng et al. 10.3390/atmos13081283
- The high-resolution estimation of sulfur dioxide (SO2) concentration, health effect and monetary costs in Beijing Y. Wu et al. 10.1016/j.chemosphere.2019.125031
- Modeling of the Atmospheric Process of Cyanobacterial Toxins in Algal Aerosol V. Zorbas et al. 10.1021/acsearthspacechem.3c00050
- Ozone Concentration Forecasting Based on Artificial Intelligence Techniques: A Systematic Review A. Yafouz et al. 10.1007/s11270-021-04989-5
26 citations as recorded by crossref.
- Particle formation and surface processes on atmospheric aerosols: A review of applied quantum chemical calculations A. Leonardi et al. 10.1002/qua.26350
- Impact of mineral dust photocatalytic heterogeneous chemistry on the formation of the sulfate and nitrate: A modelling study over East Asia X. Li et al. 10.1016/j.atmosenv.2023.120166
- Ammonium nitrate promotes sulfate formation through uptake kinetic regime Y. Liu et al. 10.5194/acp-21-13269-2021
- Unveiling the Role of Carbonate Radical Anions in Dust‐Driven SO2 Oxidation Y. Liu et al. 10.1029/2023JD040017
- Photocatalytic Oxidation of SO2 by TiO2: Aerosol Formation and the Key Role of Gaseous Reactive Oxygen Species Y. Chen et al. 10.1021/acs.est.1c01608
- Vibrational spectroscopy as a probe of heterogeneities within geochemical thin films on macro, micro, and nanoscales D. Kim et al. 10.1039/D3RA05179J
- Photo-enhanced uptake of SO2 on Icelandic volcanic dusts J. Lasne et al. 10.1039/D1EA00094B
- Atmospheric Nitrate Formation through Oxidation by Carbonate Radical X. Fang et al. 10.1021/acsearthspacechem.1c00169
- Significant formation of sulfate aerosols contributed by the heterogeneous drivers of dust surface T. Wang et al. 10.5194/acp-22-13467-2022
- Atmospheric Processes of Aromatic Hydrocarbons in the Presence of Mineral Dust Particles in an Urban Environment Z. Yu & M. Jang 10.1021/acsearthspacechem.9b00195
- Simulation of SOA formation from the photooxidation of monoalkylbenzenes in the presence of aqueous aerosols containing electrolytes under various NO<sub><i>x</i></sub> levels C. Zhou et al. 10.5194/acp-19-5719-2019
- Acidity and the multiphase chemistry of atmospheric aqueous particles and clouds A. Tilgner et al. 10.5194/acp-21-13483-2021
- The evaluation on artificial neural networks (ANN) and multiple linear regressions (MLR) models for predicting SO2 concentration S. Shams et al. 10.1016/j.uclim.2021.100837
- A review on the heterogeneous oxidation of SO2 on solid atmospheric particles: Implications for sulfate formation in haze chemistry Q. Ma et al. 10.1080/10643389.2023.2190315
- Impact of flow velocity on the heterogeneous reaction of SO2 over Fe2O3 Y. Liu et al. 10.1016/j.atmosenv.2022.119491
- Seasonality in the Δ<sup>33</sup>S measured in urban aerosols highlights an additional oxidation pathway for atmospheric SO<sub>2</sub> D. Au Yang et al. 10.5194/acp-19-3779-2019
- Critical Roles of Surface-Enhanced Heterogeneous Oxidation of SO2 in Haze Chemistry: Review of Extended Pathways for Complex Air Pollution Z. Zhang et al. 10.1007/s40726-023-00287-2
- Roles of Sulfur Oxidation Pathways in the Variability in Stable Sulfur Isotopic Composition of Sulfate Aerosols at an Urban Site in Beijing, China M. Fan et al. 10.1021/acs.estlett.0c00623
- Effects of SO2 on NH4NO3 Photolysis: The Role of Reducibility and Acidic Products Q. Cao et al. 10.1021/acs.est.3c01082
- Atmospheric Chemistry of Oxalate: Insight Into the Role of Relative Humidity and Aerosol Acidity From High‐Resolution Observation C. Yang et al. 10.1029/2021JD035364
- Simulation of heterogeneous photooxidation of SO<sub>2</sub> and NO<sub><i>x</i></sub> in the presence of Gobi Desert dust particles under ambient sunlight Z. Yu & M. Jang 10.5194/acp-18-14609-2018
- Simulating the Impact of Long-Range-Transported Asian Mineral Dust on the Formation of Sulfate and Nitrate during the KORUS-AQ Campaign Z. Yu et al. 10.1021/acsearthspacechem.0c00074
- Research Progress on Heterogeneous Reactions of Pollutant Gases on the Surface of Atmospheric Mineral Particulate Matter in China F. Zheng et al. 10.3390/atmos13081283
- The high-resolution estimation of sulfur dioxide (SO2) concentration, health effect and monetary costs in Beijing Y. Wu et al. 10.1016/j.chemosphere.2019.125031
- Modeling of the Atmospheric Process of Cyanobacterial Toxins in Algal Aerosol V. Zorbas et al. 10.1021/acsearthspacechem.3c00050
- Ozone Concentration Forecasting Based on Artificial Intelligence Techniques: A Systematic Review A. Yafouz et al. 10.1007/s11270-021-04989-5
Latest update: 18 Apr 2024
Short summary
Mineral dust is an important sink for sulfur dioxide that can be oxidized and further influence the acidification of particles as well as cloud formation. In this study, a model was developed to capture the importance of mineral dust on sulfate formation in various environments. The results suggest that the oxidation of sulfur dioxide is greatly promoted in the presence of dust particles. Our model is helpful to enhance the accuracy of sulfate formation predicted.
Mineral dust is an important sink for sulfur dioxide that can be oxidized and further influence...
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