Articles | Volume 16, issue 12
https://doi.org/10.5194/acp-16-7917-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-7917-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
29 Jun 2016
Research article |
| 29 Jun 2016
Rethinking the global secondary organic aerosol (SOA) budget: stronger production, faster removal, shorter lifetime
Alma Hodzic
CORRESPONDING AUTHOR
National Center for Atmospheric Research, Boulder, CO, USA
Prasad S. Kasibhatla
Nicholas School of the Environment, Duke University, Durham, USA
Duseong S. Jo
School of Earth and Environmental Science, Seoul National University, Seoul, Republic of Korea
Christopher D. Cappa
Department of Civil and Environmental Engineering, University of California, Davis, CA, USA
Jose L. Jimenez
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO, USA
Sasha Madronich
National Center for Atmospheric Research, Boulder, CO, USA
Rokjin J. Park
School of Earth and Environmental Science, Seoul National University, Seoul, Republic of Korea
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Short summary
The global budget and spatial distribution of secondary organic aerosol (SOA) are highly uncertain in chemistry-climate models, which reflects our inability to characterize all phases of the OA lifecycle. We have performed global model simulations with the newly proposed formation and removal processes (photolysis and heterogeneous chemistry) and shown that SOA is a far more dynamic system, with 4 times stronger production rates and more efficient removal mechanisms, than assumed in models.
The global budget and spatial distribution of secondary organic aerosol (SOA) are highly...
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