Articles | Volume 16, issue 12
https://doi.org/10.5194/acp-16-7623-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-7623-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
23 Jun 2016
Research article |
| 23 Jun 2016
The lifetime of nitrogen oxides in an isoprene-dominated forest
Paul S. Romer
Department of Chemistry, University of California at Berkeley, Berkeley, CA, USA
Kaitlin C. Duffey
Department of Chemistry, University of California at Berkeley, Berkeley, CA, USA
Paul J. Wooldridge
Department of Chemistry, University of California at Berkeley, Berkeley, CA, USA
Hannah M. Allen
Department of Chemistry, Reed College, Portland, OR, USA
Division of Chemistry and Chemical Engineering, California Institute of Technology, Pasadena, CA, USA
Benjamin R. Ayres
Department of Chemistry, Reed College, Portland, OR, USA
Steven S. Brown
Chemical Sciences Division, Earth System Research Laboratory, National Oceanic and Atmospheric Administration, Boulder, CO, USA
William H. Brune
Department of Meteorology, Pennsylvania State University, University Park, PA, USA
John D. Crounse
Division of Geological and Planetary Sciences, California Institute of Technology, Pasadena, CA, USA
Joost de Gouw
Chemical Sciences Division, Earth System Research Laboratory, National Oceanic and Atmospheric Administration, Boulder, CO, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO, USA
Danielle C. Draper
Department of Chemistry, Reed College, Portland, OR, USA
Department of Chemistry, University of California, Irvine, CA, USA
Philip A. Feiner
Department of Meteorology, Pennsylvania State University, University Park, PA, USA
Juliane L. Fry
Department of Chemistry, Reed College, Portland, OR, USA
Allen H. Goldstein
Department of Civil and Environmental Engineering, University of California at Berkeley, Berkeley, CA, USA
Department of Environmental Science, Policy and Management, University of California at Berkeley, Berkeley, CA, USA
Abigail Koss
Chemical Sciences Division, Earth System Research Laboratory, National Oceanic and Atmospheric Administration, Boulder, CO, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO, USA
Pawel K. Misztal
Department of Environmental Science, Policy and Management, University of California at Berkeley, Berkeley, CA, USA
Tran B. Nguyen
Division of Geological and Planetary Sciences, California Institute of Technology, Pasadena, CA, USA
Department of Environmental Toxicology, University of California, Davis, CA, USA
Kevin Olson
Department of Environmental Science, Policy and Management, University of California at Berkeley, Berkeley, CA, USA
Alex P. Teng
Division of Geological and Planetary Sciences, California Institute of Technology, Pasadena, CA, USA
Paul O. Wennberg
Division of Geological and Planetary Sciences, California Institute of Technology, Pasadena, CA, USA
Division of Engineering and Applied Science, California Institute of Technology, Pasadena, CA, USA
Robert J. Wild
Chemical Sciences Division, Earth System Research Laboratory, National Oceanic and Atmospheric Administration, Boulder, CO, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO, USA
Li Zhang
Department of Meteorology, Pennsylvania State University, University Park, PA, USA
Department of Chemistry, University of California at Berkeley, Berkeley, CA, USA
Department of Earth and Planetary Sciences, University of California at Berkeley, Berkeley, CA, USA
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61 citations as recorded by crossref.
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- Contrasting Reactive Organic Carbon Observations in the Southeast United States (SOAS) and Southern California (CalNex) C. Heald et al. 10.1021/acs.est.0c05027
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- Rapid hydrolysis of tertiary isoprene nitrate efficiently removes NO x from the atmosphere K. Vasquez et al. 10.1073/pnas.2017442117
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- Characterization of organic nitrogen in aerosols at a forest site in the southern Appalachian Mountains X. Chen et al. 10.5194/acp-18-6829-2018
- The production and hydrolysis of organic nitrates from OH radical oxidation of <i>β</i>-ocimene A. Morales et al. 10.5194/acp-21-129-2021
- Gas-Phase Oxidation Rates and Products of 1,2-Dihydroxy Isoprene K. Bates et al. 10.1021/acs.est.1c04177
- Variable effects of spatial resolution on modeling of nitrogen oxides C. Li et al. 10.5194/acp-23-3031-2023
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- Identifying NOx Sources in Arequipa, Peru Using Nitrogen Isotopes in Particulate Nitrate G. Michalski et al. 10.3389/fenvs.2022.916738
- Quantifying the transboundary contribution of nitrogen oxides to UK air quality E. Stirling et al. 10.1002/asl.955
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- Field Measurement of Alkyl Nitrates in the Atmosphere C. Li et al. 10.6023/A23100460
- Efficient Nighttime Biogenic SOA Formation in a Polluted Residual Layer R. Zaveri et al. 10.1029/2019JD031583
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- Development of a Solar-Induced Fluorescence─Canopy Conductance Model and Its Application to Stomatal Reactive Nitrogen Deposition E. Delaria et al. 10.1021/acsearthspacechem.1c00260
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- Comprehensive isoprene and terpene gas-phase chemistry improves simulated surface ozone in the southeastern US R. Schwantes et al. 10.5194/acp-20-3739-2020
- Differences in BVOC oxidation and SOA formation above and below the forest canopy B. Schulze et al. 10.5194/acp-17-1805-2017
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- Large uncertainties in global hydroxyl projections tied to fate of reactive nitrogen and carbon L. Murray et al. 10.1073/pnas.2115204118
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- Air quality observations onboard commercial and targeted Zeppelin flights in Germany – a platform for high-resolution trace-gas and aerosol measurements within the planetary boundary layer R. Tillmann et al. 10.5194/amt-15-3827-2022
- A top-down assessment using OMI NO<sub>2</sub> suggests an underestimate in the NO<sub><i>x</i></sub> emissions inventory in Seoul, South Korea, during KORUS-AQ D. Goldberg et al. 10.5194/acp-19-1801-2019
- Secondary organic aerosol (SOA) yields from NO<sub>3</sub> radical + isoprene based on nighttime aircraft power plant plume transects J. Fry et al. 10.5194/acp-18-11663-2018
- Measurement of NO<sub><i>x</i></sub> and NO<sub><i>y</i></sub> with a thermal dissociation cavity ring-down spectrometer (TD-CRDS): instrument characterisation and first deployment N. Friedrich et al. 10.5194/amt-13-5739-2020
- A comprehensive organic nitrate chemistry: insights into the lifetime of atmospheric organic nitrates A. Zare et al. 10.5194/acp-18-15419-2018
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- Synthesis of the Southeast Atmosphere Studies: Investigating Fundamental Atmospheric Chemistry Questions A. Carlton et al. 10.1175/BAMS-D-16-0048.1
- Chemistry and deposition in the Model of Atmospheric composition at Global and Regional scales using Inversion Techniques for Trace gas Emissions (MAGRITTE v1.1) – Part 1: Chemical mechanism J. Müller et al. 10.5194/gmd-12-2307-2019
- Sensitivity of Tropospheric Ozone Over the Southeast USA to Dry Deposition C. Baublitz et al. 10.1029/2020GL087158
- Investigation of the limonene photooxidation by OH at different NO concentrations in the atmospheric simulation chamber SAPHIR (Simulation of Atmospheric PHotochemistry In a large Reaction Chamber) J. Pang et al. 10.5194/acp-22-8497-2022
- Comparison of Airborne Reactive Nitrogen Measurements During WINTER T. Sparks et al. 10.1029/2019JD030700
- Transboundary atmospheric pollution in Southeast Asia: current methods, limitations and future developments Q. Chen & D. Taylor 10.1080/10643389.2018.1493337
- Methyl, Ethyl, and Propyl Nitrates: Global Distribution and Impacts on Reactive Nitrogen in Remote Marine Environments J. Fisher et al. 10.1029/2018JD029046
- Importance of biogenic volatile organic compounds to acyl peroxy nitrates (APN) production in the southeastern US during SOAS 2013 S. Toma et al. 10.5194/acp-19-1867-2019
- NOx Lifetime and NOy Partitioning During WINTER H. Kenagy et al. 10.1029/2018JD028736
- Organic nitrate chemistry and its implications for nitrogen budgets in an isoprene- and monoterpene-rich atmosphere: constraints from aircraft (SEAC<sup>4</sup>RS) and ground-based (SOAS) observations in the Southeast US J. Fisher et al. 10.5194/acp-16-5969-2016
60 citations as recorded by crossref.
- Simulation of organic nitrates in Pearl River Delta in 2006 and the chemical impact on ozone production X. Chen et al. 10.1007/s11430-017-9115-5
- Alkyl nitrates in the boreal forest: formation via the NO<sub>3</sub>-, OH- and O<sub>3</sub>-induced oxidation of biogenic volatile organic compounds and ambient lifetimes J. Liebmann et al. 10.5194/acp-19-10391-2019
- Contrasting Reactive Organic Carbon Observations in the Southeast United States (SOAS) and Southern California (CalNex) C. Heald et al. 10.1021/acs.est.0c05027
- Leaf Stomatal Control over Acyl Peroxynitrate Dry Deposition to Trees B. Place et al. 10.1021/acsearthspacechem.0c00152
- Rapid hydrolysis of tertiary isoprene nitrate efficiently removes NO x from the atmosphere K. Vasquez et al. 10.1073/pnas.2017442117
- Evaluation of isoprene nitrate chemistry in detailed chemical mechanisms A. Mayhew et al. 10.5194/acp-22-14783-2022
- Impact of NO<sub><i>x</i></sub> on secondary organic aerosol (SOA) formation from <i>α</i>-pinene and <i>β</i>-pinene photooxidation: the role of highly oxygenated organic nitrates I. Pullinen et al. 10.5194/acp-20-10125-2020
- Characterization of organic nitrogen in aerosols at a forest site in the southern Appalachian Mountains X. Chen et al. 10.5194/acp-18-6829-2018
- The production and hydrolysis of organic nitrates from OH radical oxidation of <i>β</i>-ocimene A. Morales et al. 10.5194/acp-21-129-2021
- Gas-Phase Oxidation Rates and Products of 1,2-Dihydroxy Isoprene K. Bates et al. 10.1021/acs.est.1c04177
- Variable effects of spatial resolution on modeling of nitrogen oxides C. Li et al. 10.5194/acp-23-3031-2023
- Leaf Stomatal Uptake of Alkyl Nitrates B. Place et al. 10.1021/acs.estlett.1c00793
- Identifying NOx Sources in Arequipa, Peru Using Nitrogen Isotopes in Particulate Nitrate G. Michalski et al. 10.3389/fenvs.2022.916738
- Quantifying the transboundary contribution of nitrogen oxides to UK air quality E. Stirling et al. 10.1002/asl.955
- Mobile monitoring of urban air quality at high spatial resolution by low-cost sensors: impacts of COVID-19 pandemic lockdown S. Wang et al. 10.5194/acp-21-7199-2021
- Metal-free catalysis on the reactions of nitric acid with aliphatic aldehydes: A new potential source of organic nitrates F. Bai et al. 10.1016/j.atmosenv.2023.119673
- Observation and modeling of organic nitrates on a suburban site in southwest China C. Li et al. 10.1016/j.scitotenv.2022.160287
- Interrelation between Dynamics of Gas Composition and Meteorological Parameters in the Region of Tomsk P. Antokhin et al. 10.1134/S1024856020060044
- Southeast Atmosphere Studies: learning from model-observation syntheses J. Mao et al. 10.5194/acp-18-2615-2018
- The acid-catalyzed hydrolysis of an <i>α</i>-pinene-derived organic nitrate: kinetics, products, reaction mechanisms, and atmospheric impact J. Rindelaub et al. 10.5194/acp-16-15425-2016
- i<sub>N</sub>RACM: incorporating <sup>15</sup>N into the Regional Atmospheric Chemistry Mechanism (RACM) for assessing the role photochemistry plays in controlling the isotopic composition of NO<sub><i>x</i></sub>, NO<sub><i>y</i></sub>, and atmospheric nitrate H. Fang et al. 10.5194/gmd-14-5001-2021
- Field Measurement of Alkyl Nitrates in the Atmosphere C. Li et al. 10.6023/A23100460
- Efficient Nighttime Biogenic SOA Formation in a Polluted Residual Layer R. Zaveri et al. 10.1029/2019JD031583
- The changing role of organic nitrates in the removal and transport of NO<sub><i>x</i></sub> P. Romer Present et al. 10.5194/acp-20-267-2020
- Changes to simulated global atmospheric composition resulting from recent revisions to isoprene oxidation chemistry M. Khan et al. 10.1016/j.atmosenv.2020.117914
- Development of a Solar-Induced Fluorescence─Canopy Conductance Model and Its Application to Stomatal Reactive Nitrogen Deposition E. Delaria et al. 10.1021/acsearthspacechem.1c00260
- Decadal changes in summertime reactive oxidized nitrogen and surface ozone over the Southeast United States J. Li et al. 10.5194/acp-18-2341-2018
- Comprehensive isoprene and terpene gas-phase chemistry improves simulated surface ozone in the southeastern US R. Schwantes et al. 10.5194/acp-20-3739-2020
- Differences in BVOC oxidation and SOA formation above and below the forest canopy B. Schulze et al. 10.5194/acp-17-1805-2017
- Laboratory measurements of stomatal NO<sub>2</sub> deposition to native California trees and the role of forests in the NO<sub>x</sub> cycle E. Delaria et al. 10.5194/acp-20-14023-2020
- Large uncertainties in global hydroxyl projections tied to fate of reactive nitrogen and carbon L. Murray et al. 10.1073/pnas.2115204118
- Influence of urban pollution on the production of organic particulate matter from isoprene epoxydiols in central Amazonia S. de Sá et al. 10.5194/acp-17-6611-2017
- The important contribution of secondary formation and biomass burning to oxidized organic nitrogen (OON) in a polluted urban area: insights from in situ measurements of a chemical ionization mass spectrometer (CIMS) Y. Cai et al. 10.5194/acp-23-8855-2023
- A model-based analysis of foliar NO<sub><i>x</i></sub> deposition E. Delaria & R. Cohen 10.5194/acp-20-2123-2020
- Measurements of Atmosphere–Biosphere Exchange of Oxidized Nitrogen and Implications for the Chemistry of Atmospheric NOx E. Delaria & R. Cohen 10.1021/acs.accounts.3c00090
- Characteristics of HONO and its impact on O3 formation in the Seoul Metropolitan Area during the Korea-US Air Quality study J. Gil et al. 10.1016/j.atmosenv.2020.118182
- Observational Evidence of Unknown NOx Source and Its Perturbation of Oxidative Capacity in Bermuda's Marine Boundary Layer Y. Wang et al. 10.1029/2023JD039582
- A new model mechanism for atmospheric oxidation of isoprene: global effects on oxidants, nitrogen oxides, organic products, and secondary organic aerosol K. Bates & D. Jacob 10.5194/acp-19-9613-2019
- Ambient Measurements of Highly Oxidized Gas-Phase Molecules during the Southern Oxidant and Aerosol Study (SOAS) 2013 P. Massoli et al. 10.1021/acsearthspacechem.8b00028
- Evidence of precedent wind role on controlling PM1 wet scavenging of aerosols during monsoon rain events L. Yang et al. 10.1016/j.atmosenv.2018.12.041
- Effects of temperature-dependent NO<sub><i>x</i></sub> emissions on continental ozone production P. Romer et al. 10.5194/acp-18-2601-2018
- Reactive nitrogen around the Arabian Peninsula and in the Mediterranean Sea during the 2017 AQABA ship campaign N. Friedrich et al. 10.5194/acp-21-7473-2021
- Volatile Methyl Siloxane Atmospheric Oxidation Mechanism from a Theoretical Perspective─How is the Siloxanol Formed? M. Alton et al. 10.1021/acs.jpca.3c06287
- Evaluation of Novel Routes for NOx Formation in Remote Regions C. Ye et al. 10.1021/acs.est.6b06441
- Unambiguous identification of N-containing oxygenated organic molecules using a chemical-ionization Orbitrap (CI-Orbitrap) in an eastern Chinese megacity Y. Lu et al. 10.5194/acp-23-3233-2023
- Air quality observations onboard commercial and targeted Zeppelin flights in Germany – a platform for high-resolution trace-gas and aerosol measurements within the planetary boundary layer R. Tillmann et al. 10.5194/amt-15-3827-2022
- A top-down assessment using OMI NO<sub>2</sub> suggests an underestimate in the NO<sub><i>x</i></sub> emissions inventory in Seoul, South Korea, during KORUS-AQ D. Goldberg et al. 10.5194/acp-19-1801-2019
- Secondary organic aerosol (SOA) yields from NO<sub>3</sub> radical + isoprene based on nighttime aircraft power plant plume transects J. Fry et al. 10.5194/acp-18-11663-2018
- Measurement of NO<sub><i>x</i></sub> and NO<sub><i>y</i></sub> with a thermal dissociation cavity ring-down spectrometer (TD-CRDS): instrument characterisation and first deployment N. Friedrich et al. 10.5194/amt-13-5739-2020
- A comprehensive organic nitrate chemistry: insights into the lifetime of atmospheric organic nitrates A. Zare et al. 10.5194/acp-18-15419-2018
- Vapor-Pressure Pathways Initiate but Hydrolysis Products Dominate the Aerosol Estimated from Organic Nitrates A. Zare et al. 10.1021/acsearthspacechem.9b00067
- Synthesis of the Southeast Atmosphere Studies: Investigating Fundamental Atmospheric Chemistry Questions A. Carlton et al. 10.1175/BAMS-D-16-0048.1
- Chemistry and deposition in the Model of Atmospheric composition at Global and Regional scales using Inversion Techniques for Trace gas Emissions (MAGRITTE v1.1) – Part 1: Chemical mechanism J. Müller et al. 10.5194/gmd-12-2307-2019
- Sensitivity of Tropospheric Ozone Over the Southeast USA to Dry Deposition C. Baublitz et al. 10.1029/2020GL087158
- Investigation of the limonene photooxidation by OH at different NO concentrations in the atmospheric simulation chamber SAPHIR (Simulation of Atmospheric PHotochemistry In a large Reaction Chamber) J. Pang et al. 10.5194/acp-22-8497-2022
- Comparison of Airborne Reactive Nitrogen Measurements During WINTER T. Sparks et al. 10.1029/2019JD030700
- Transboundary atmospheric pollution in Southeast Asia: current methods, limitations and future developments Q. Chen & D. Taylor 10.1080/10643389.2018.1493337
- Methyl, Ethyl, and Propyl Nitrates: Global Distribution and Impacts on Reactive Nitrogen in Remote Marine Environments J. Fisher et al. 10.1029/2018JD029046
- Importance of biogenic volatile organic compounds to acyl peroxy nitrates (APN) production in the southeastern US during SOAS 2013 S. Toma et al. 10.5194/acp-19-1867-2019
- NOx Lifetime and NOy Partitioning During WINTER H. Kenagy et al. 10.1029/2018JD028736
1 citations as recorded by crossref.
Saved (preprint)
Discussed (final revised paper)
Latest update: 18 Apr 2024
Short summary
The lifetime of nitrogen oxides (NOx) is evaluated by analysis of field measurements from the southeastern United States. At warm temperatures in the daytime boundary layer, NOx interconverts rapidly with both PAN and alkyl and multifunctional nitrates (RONO2), and the relevant lifetime is the combined lifetime of these three classes. We find that the production of RONO2, followed by hydrolysis to produce nitric acid, is the dominant pathway for NOx removal in an isoprene dominated forest.
The lifetime of nitrogen oxides (NOx) is evaluated by analysis of field measurements from the...
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