Articles | Volume 16, issue 2
https://doi.org/10.5194/acp-16-675-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-675-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
21 Jan 2016
Research article |
| 21 Jan 2016
Formation of secondary aerosols from gasoline vehicle exhaust when mixing with SO2
T. Liu
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
University of Chinese Academy of Sciences, Beijing 100049, China
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
University of Chinese Academy of Sciences, Beijing 100049, China
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
X. Fu
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
University of Chinese Academy of Sciences, Beijing 100049, China
F. Bernard
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
Chemical Sciences Division, NOAA Earth System Research Laboratory, Boulder, Colorado 80305, USA
Z. Zhang
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
University of Chinese Academy of Sciences, Beijing 100049, China
S. Lü
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
University of Chinese Academy of Sciences, Beijing 100049, China
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
University of Chinese Academy of Sciences, Beijing 100049, China
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science & Engineering, Fudan University, Shanghai 200433, China
Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China
Division of Environment, Hong Kong University of Science & Technology, Clear Water Bay, Kowloon, Hong Kong, China
P. Peng
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
G. Sheng
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
J. Fu
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
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Cited
61 citations as recorded by crossref.
- Rate constant and secondary organic aerosol formation from the gas-phase reaction of eugenol with hydroxyl radicals C. Liu et al. 10.5194/acp-19-2001-2019
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- Novel Method for Determining Internal Combustion Engine Dysfunctions on Platform as a Service T. Harach et al. 10.3390/s23010477
- Comparison between idling and cruising gasoline vehicles in primary emissions and secondary organic aerosol formation during photochemical ageing Y. Zhang et al. 10.1016/j.scitotenv.2020.137934
- Effects of OH radical and SO2 concentrations on photochemical reactions of mixed anthropogenic organic gases J. Li et al. 10.5194/acp-22-10489-2022
- Review of Smog Chamber Research Trends J. Kim et al. 10.5572/KOSAE.2023.39.5.866
- Synergistic Effects of SO2 and NH3 Coexistence on SOA Formation from Gasoline Evaporative Emissions T. Chen et al. 10.1021/acs.est.3c01921
- Effect of NOx and SO2 on the photooxidation of methylglyoxal: Implications in secondary aerosol formation S. Wang et al. 10.1016/j.jes.2020.02.011
- Surprisingly long lifetime of methacrolein oxide, an isoprene derived Criegee intermediate, under humid conditions Y. Lin et al. 10.1038/s42004-021-00451-z
- The Roles of N, S, and O in Molecular Absorption Features of Brown Carbon in PM2.5 in a Typical Semi‐Arid Megacity in Northwestern China Y. Zeng et al. 10.1029/2021JD034791
- Assessing the influence of environmental conditions on secondary organic aerosol formation from a typical biomass burning compound X. Jiang et al. 10.1016/j.jes.2021.08.016
- Elevated production of NH 4 NO 3 from the photochemical processing of vehicle exhaust: Implications for air quality in the Seoul Metropolitan Region M. Link et al. 10.1016/j.atmosenv.2017.02.031
- Sensitivity of Nitrate Aerosol Production to Vehicular Emissions in an Urban Street M. Kim 10.3390/atmos10040212
- PM2.5-bound polycyclic aromatic hydrocarbons (PAHs) and their derivatives (nitrated-PAHs and oxygenated-PAHs) in a road tunnel located in Qingdao, China: Characteristics, sources and emission factors T. Zhao et al. 10.1016/j.scitotenv.2020.137521
- Promoting mechanism of N-doped single-walled carbon nanotubes for O2 dissociation and SO2 oxidation Y. Chen et al. 10.1016/j.apsusc.2017.10.137
- Nitroaromatic Compounds from Secondary Nitrate Formation and Biomass Burning Are Major Proinflammatory Components in Organic Aerosols in Guangzhou: A Bioassay Combining High-Resolution Mass Spectrometry Analysis Q. Zhang et al. 10.1021/acs.est.3c04983
- Photooxidation of cyclohexene in the presence of SO<sub>2</sub>: SOA yield and chemical composition S. Liu et al. 10.5194/acp-17-13329-2017
- Characteristics and aging of traffic-derived particles in a highway tunnel at a coastal city in southern China C. Hou et al. 10.1016/j.scitotenv.2017.11.165
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- Seasonal concentration distribution of PM1.0 and PM2.5 and a risk assessment of bound trace metals in Harbin, China: Effect of the species distribution of heavy metals and heat supply K. Wang et al. 10.1038/s41598-020-65187-7
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- Kinetics of the Gas-Phase Reactions of syn- and anti-CH3CHOO Criegee Intermediate Conformers with SO2 as a Function of Temperature and Pressure R. Lade et al. 10.1021/acs.jpca.4c00199
- Significant Production of Secondary Organic Aerosol from Emissions of Heated Cooking Oils T. Liu et al. 10.1021/acs.estlett.7b00530
- Formation mechanism of secondary organic aerosol from ozonolysis of gasoline vehicle exhaust B. Yang et al. 10.1016/j.envpol.2017.12.048
- Determination of atmospheric sulphur dioxide and sulphuric acid traces by indirect flame atomic absorption method S. Kapitány et al. 10.1016/j.microc.2020.104853
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- Investigation of the spatially varying relationships of PM2.5 with meteorology, topography, and emissions over China in 2015 by using modified geographically weighted regression Q. Yang et al. 10.1016/j.envpol.2020.114257
- Effects of NOx, SO2 and RH on the SOA formation from cyclohexene photooxidation S. Liu et al. 10.1016/j.chemosphere.2018.10.180
- Secondary organic aerosol formation from the OH-initiated oxidation of guaiacol under different experimental conditions C. Liu et al. 10.1016/j.atmosenv.2019.03.021
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- Effects of SO<sub>2</sub> on optical properties of secondary organic aerosol generated from photooxidation of toluene under different relative humidity conditions W. Zhang et al. 10.5194/acp-20-4477-2020
- Effect of nitrogen oxides (NO and NO 2 ) and toluene on SO 2 photooxidation, nucleation and growth: A smog chamber study K. Li et al. 10.1016/j.atmosres.2017.03.017
- Spatial variation in lag structure in the short-term effects of air pollution on mortality in seven major South Korean cities, 2006–2013 H. Kim et al. 10.1016/j.envint.2018.09.004
- Formation, features and controlling strategies of severe haze-fog pollutions in China H. Fu & J. Chen 10.1016/j.scitotenv.2016.10.201
- Effect of PdSx on Sulfur Resistance of Pd-Based Catalysts for CO Oxidation C. Qian et al. 10.1021/acs.iecr.2c04098
- Effects of the emergency control measures in Beijing on air quality improvement J. Tian et al. 10.1016/j.apr.2018.10.005
- Applications of environmental mass spectrometry in atmospheric haze chemistry T. Chen et al. 10.1016/j.trac.2024.117614
- Influence of metal-mediated aerosol-phase oxidation on secondary organic aerosol formation from the ozonolysis and OH-oxidation of α-pinene B. Chu et al. 10.1038/srep40311
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- Significant source of secondary aerosol: formation from gasoline evaporative emissions in the presence of SO<sub>2</sub> and NH<sub>3</sub> T. Chen et al. 10.5194/acp-19-8063-2019
- Application of VUV-PIMS coupled with GC-MS in chemical characterization, identification and comparative analysis of organic components in both vehicular-derived SOA and haze particles P. Zhang et al. 10.1016/j.atmosenv.2017.06.013
- Primary and secondary organic aerosol from heated cooking oil emissions T. Liu et al. 10.5194/acp-18-11363-2018
- Molecular Characterization of Organosulfur Compounds in Biodiesel and Diesel Fuel Secondary Organic Aerosol S. Blair et al. 10.1021/acs.est.6b03304
- Pollution characteristics and sources of environmentally persistent free radicals and oxidation potential in fine particulate matter related to city lockdown (CLD) in Xi'an, China D. Ainur et al. 10.1016/j.envres.2022.112899
- Spatial and temporal variation of particulate matter and gaseous pollutants in China during 2014–2016 R. Li et al. 10.1016/j.atmosenv.2017.05.008
- Evolution of light absorption properties during photochemical aging of straw open burning aerosols Z. Fang et al. 10.1016/j.scitotenv.2022.156431
- Recent advances in understanding secondary organic aerosol: Implications for global climate forcing M. Shrivastava et al. 10.1002/2016RG000540
- The spatiotemporal variation and key factors of SO2 in 336 cities across China R. Li et al. 10.1016/j.jclepro.2018.11.062
- How aging process changes characteristics of vehicle emissions? A review H. Liu et al. 10.1080/10643389.2019.1669402
- Restricted Anthropogenic Activities and Improved Urban Air Quality in China: Evidence from Real-Time and Remotely Sensed Datasets Using Air Quality Zonal Modeling S. Rahaman et al. 10.3390/atmos13060961
- Formation of secondary organic aerosols from the ozonolysis of dihydrofurans Y. Diaz-de-Mera et al. 10.5194/acp-17-2347-2017
- Intermediate-volatility aromatic hydrocarbons from the rubber products industry in China Z. Zhang et al. 10.1016/j.scitotenv.2023.165583
- Secondary Organic Aerosol Formation from Urban Roadside Air in Hong Kong T. Liu et al. 10.1021/acs.est.8b06587
- Thermal effects on dispersion of secondary inorganic aerosols in an urban street canyon S. Lee et al. 10.1016/j.uclim.2022.101375
- Air pollution characteristics in China during 2015–2016: Spatiotemporal variations and key meteorological factors R. Li et al. 10.1016/j.scitotenv.2018.08.181
- Secondary organic aerosol formation from photo-oxidation of toluene with NO x and SO 2 : Chamber simulation with purified air versus urban ambient air as matrix W. Deng et al. 10.1016/j.atmosenv.2016.11.047
- Primary emissions and secondary production of organic aerosols from heated animal fats L. Zhou et al. 10.1016/j.scitotenv.2021.148638
- Criegee intermediates and their impacts on the troposphere M. Khan et al. 10.1039/C7EM00585G
- Comparative study of PM10-bound heavy metals and PAHs during six years in a Chinese megacity: Compositions, sources, and source-specific risks Q. Xue et al. 10.1016/j.ecoenv.2019.109740
61 citations as recorded by crossref.
- Rate constant and secondary organic aerosol formation from the gas-phase reaction of eugenol with hydroxyl radicals C. Liu et al. 10.5194/acp-19-2001-2019
- Effects of NO<sub><i>x</i></sub> and SO<sub>2</sub> on the secondary organic aerosol formation from photooxidation of <i>α</i>-pinene and limonene D. Zhao et al. 10.5194/acp-18-1611-2018
- Novel Method for Determining Internal Combustion Engine Dysfunctions on Platform as a Service T. Harach et al. 10.3390/s23010477
- Comparison between idling and cruising gasoline vehicles in primary emissions and secondary organic aerosol formation during photochemical ageing Y. Zhang et al. 10.1016/j.scitotenv.2020.137934
- Effects of OH radical and SO2 concentrations on photochemical reactions of mixed anthropogenic organic gases J. Li et al. 10.5194/acp-22-10489-2022
- Review of Smog Chamber Research Trends J. Kim et al. 10.5572/KOSAE.2023.39.5.866
- Synergistic Effects of SO2 and NH3 Coexistence on SOA Formation from Gasoline Evaporative Emissions T. Chen et al. 10.1021/acs.est.3c01921
- Effect of NOx and SO2 on the photooxidation of methylglyoxal: Implications in secondary aerosol formation S. Wang et al. 10.1016/j.jes.2020.02.011
- Surprisingly long lifetime of methacrolein oxide, an isoprene derived Criegee intermediate, under humid conditions Y. Lin et al. 10.1038/s42004-021-00451-z
- The Roles of N, S, and O in Molecular Absorption Features of Brown Carbon in PM2.5 in a Typical Semi‐Arid Megacity in Northwestern China Y. Zeng et al. 10.1029/2021JD034791
- Assessing the influence of environmental conditions on secondary organic aerosol formation from a typical biomass burning compound X. Jiang et al. 10.1016/j.jes.2021.08.016
- Elevated production of NH 4 NO 3 from the photochemical processing of vehicle exhaust: Implications for air quality in the Seoul Metropolitan Region M. Link et al. 10.1016/j.atmosenv.2017.02.031
- Sensitivity of Nitrate Aerosol Production to Vehicular Emissions in an Urban Street M. Kim 10.3390/atmos10040212
- PM2.5-bound polycyclic aromatic hydrocarbons (PAHs) and their derivatives (nitrated-PAHs and oxygenated-PAHs) in a road tunnel located in Qingdao, China: Characteristics, sources and emission factors T. Zhao et al. 10.1016/j.scitotenv.2020.137521
- Promoting mechanism of N-doped single-walled carbon nanotubes for O2 dissociation and SO2 oxidation Y. Chen et al. 10.1016/j.apsusc.2017.10.137
- Nitroaromatic Compounds from Secondary Nitrate Formation and Biomass Burning Are Major Proinflammatory Components in Organic Aerosols in Guangzhou: A Bioassay Combining High-Resolution Mass Spectrometry Analysis Q. Zhang et al. 10.1021/acs.est.3c04983
- Photooxidation of cyclohexene in the presence of SO<sub>2</sub>: SOA yield and chemical composition S. Liu et al. 10.5194/acp-17-13329-2017
- Characteristics and aging of traffic-derived particles in a highway tunnel at a coastal city in southern China C. Hou et al. 10.1016/j.scitotenv.2017.11.165
- SO2 measurements in a clean coastal environment of the southwestern Europe: Sources, transport and influence in the formation of secondary aerosols J. Adame et al. 10.1016/j.scitotenv.2020.137075
- Formation of secondary aerosols from the ozonolysis of styrene: Effect of SO2 and H2O Y. Díaz-de-Mera et al. 10.1016/j.atmosenv.2017.10.011
- Seasonal concentration distribution of PM1.0 and PM2.5 and a risk assessment of bound trace metals in Harbin, China: Effect of the species distribution of heavy metals and heat supply K. Wang et al. 10.1038/s41598-020-65187-7
- Tropospheric volatile organic compounds in China H. Guo et al. 10.1016/j.scitotenv.2016.09.116
- Kinetics of the Gas-Phase Reactions of syn- and anti-CH3CHOO Criegee Intermediate Conformers with SO2 as a Function of Temperature and Pressure R. Lade et al. 10.1021/acs.jpca.4c00199
- Significant Production of Secondary Organic Aerosol from Emissions of Heated Cooking Oils T. Liu et al. 10.1021/acs.estlett.7b00530
- Formation mechanism of secondary organic aerosol from ozonolysis of gasoline vehicle exhaust B. Yang et al. 10.1016/j.envpol.2017.12.048
- Determination of atmospheric sulphur dioxide and sulphuric acid traces by indirect flame atomic absorption method S. Kapitány et al. 10.1016/j.microc.2020.104853
- Single-particle Raman spectroscopy for studying physical and chemical processes of atmospheric particles Z. Liang et al. 10.5194/acp-22-3017-2022
- Enhancement of secondary organic aerosol formation and its oxidation state by SO<sub>2</sub> during photooxidation of 2-methoxyphenol C. Liu et al. 10.5194/acp-19-2687-2019
- Investigation of the spatially varying relationships of PM2.5 with meteorology, topography, and emissions over China in 2015 by using modified geographically weighted regression Q. Yang et al. 10.1016/j.envpol.2020.114257
- Effects of NOx, SO2 and RH on the SOA formation from cyclohexene photooxidation S. Liu et al. 10.1016/j.chemosphere.2018.10.180
- Secondary organic aerosol formation from the OH-initiated oxidation of guaiacol under different experimental conditions C. Liu et al. 10.1016/j.atmosenv.2019.03.021
- SO<sub>2</sub> and NH<sub>3</sub> emissions enhance organosulfur compounds and fine particle formation from the photooxidation of a typical aromatic hydrocarbon Z. Yang et al. 10.5194/acp-21-7963-2021
- Effects of SO<sub>2</sub> on optical properties of secondary organic aerosol generated from photooxidation of toluene under different relative humidity conditions W. Zhang et al. 10.5194/acp-20-4477-2020
- Effect of nitrogen oxides (NO and NO 2 ) and toluene on SO 2 photooxidation, nucleation and growth: A smog chamber study K. Li et al. 10.1016/j.atmosres.2017.03.017
- Spatial variation in lag structure in the short-term effects of air pollution on mortality in seven major South Korean cities, 2006–2013 H. Kim et al. 10.1016/j.envint.2018.09.004
- Formation, features and controlling strategies of severe haze-fog pollutions in China H. Fu & J. Chen 10.1016/j.scitotenv.2016.10.201
- Effect of PdSx on Sulfur Resistance of Pd-Based Catalysts for CO Oxidation C. Qian et al. 10.1021/acs.iecr.2c04098
- Effects of the emergency control measures in Beijing on air quality improvement J. Tian et al. 10.1016/j.apr.2018.10.005
- Applications of environmental mass spectrometry in atmospheric haze chemistry T. Chen et al. 10.1016/j.trac.2024.117614
- Influence of metal-mediated aerosol-phase oxidation on secondary organic aerosol formation from the ozonolysis and OH-oxidation of α-pinene B. Chu et al. 10.1038/srep40311
- Differences of the oxidation process and secondary organic aerosol formation at low and high precursor concentrations T. Chen et al. 10.1016/j.jes.2018.11.011
- Significant source of secondary aerosol: formation from gasoline evaporative emissions in the presence of SO<sub>2</sub> and NH<sub>3</sub> T. Chen et al. 10.5194/acp-19-8063-2019
- Application of VUV-PIMS coupled with GC-MS in chemical characterization, identification and comparative analysis of organic components in both vehicular-derived SOA and haze particles P. Zhang et al. 10.1016/j.atmosenv.2017.06.013
- Primary and secondary organic aerosol from heated cooking oil emissions T. Liu et al. 10.5194/acp-18-11363-2018
- Molecular Characterization of Organosulfur Compounds in Biodiesel and Diesel Fuel Secondary Organic Aerosol S. Blair et al. 10.1021/acs.est.6b03304
- Pollution characteristics and sources of environmentally persistent free radicals and oxidation potential in fine particulate matter related to city lockdown (CLD) in Xi'an, China D. Ainur et al. 10.1016/j.envres.2022.112899
- Spatial and temporal variation of particulate matter and gaseous pollutants in China during 2014–2016 R. Li et al. 10.1016/j.atmosenv.2017.05.008
- Evolution of light absorption properties during photochemical aging of straw open burning aerosols Z. Fang et al. 10.1016/j.scitotenv.2022.156431
- Recent advances in understanding secondary organic aerosol: Implications for global climate forcing M. Shrivastava et al. 10.1002/2016RG000540
- The spatiotemporal variation and key factors of SO2 in 336 cities across China R. Li et al. 10.1016/j.jclepro.2018.11.062
- How aging process changes characteristics of vehicle emissions? A review H. Liu et al. 10.1080/10643389.2019.1669402
- Restricted Anthropogenic Activities and Improved Urban Air Quality in China: Evidence from Real-Time and Remotely Sensed Datasets Using Air Quality Zonal Modeling S. Rahaman et al. 10.3390/atmos13060961
- Formation of secondary organic aerosols from the ozonolysis of dihydrofurans Y. Diaz-de-Mera et al. 10.5194/acp-17-2347-2017
- Intermediate-volatility aromatic hydrocarbons from the rubber products industry in China Z. Zhang et al. 10.1016/j.scitotenv.2023.165583
- Secondary Organic Aerosol Formation from Urban Roadside Air in Hong Kong T. Liu et al. 10.1021/acs.est.8b06587
- Thermal effects on dispersion of secondary inorganic aerosols in an urban street canyon S. Lee et al. 10.1016/j.uclim.2022.101375
- Air pollution characteristics in China during 2015–2016: Spatiotemporal variations and key meteorological factors R. Li et al. 10.1016/j.scitotenv.2018.08.181
- Secondary organic aerosol formation from photo-oxidation of toluene with NO x and SO 2 : Chamber simulation with purified air versus urban ambient air as matrix W. Deng et al. 10.1016/j.atmosenv.2016.11.047
- Primary emissions and secondary production of organic aerosols from heated animal fats L. Zhou et al. 10.1016/j.scitotenv.2021.148638
- Criegee intermediates and their impacts on the troposphere M. Khan et al. 10.1039/C7EM00585G
- Comparative study of PM10-bound heavy metals and PAHs during six years in a Chinese megacity: Compositions, sources, and source-specific risks Q. Xue et al. 10.1016/j.ecoenv.2019.109740
Saved (preprint)
Latest update: 23 Apr 2024
Short summary
The formation of SOA and sulfate aerosols from the photooxidation of gasoline vehicle exhaust (GVE) when mixing with SO2 was investigated in a smog chamber. We found that the presence of GVE enhanced the conversion of SO2 to sulfate predominantly through reactions with stabilized Criegee intermediates. On the other hand, the elevated particle acidity enhanced the SOA production from GVE. This study indicated that SO2 and GVE could enhance each other in forming secondary aerosols.
The formation of SOA and sulfate aerosols from the photooxidation of gasoline vehicle exhaust...
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