Articles | Volume 16, issue 3
https://doi.org/10.5194/acp-16-1747-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-1747-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
15 Feb 2016
Research article |
| 15 Feb 2016
Secondary organic aerosol formation from isoprene photooxidation during cloud condensation–evaporation cycles
L. Brégonzio-Rozier
CORRESPONDING AUTHOR
Laboratoire Interuniversitaire des Systèmes
Atmosphériques (LISA), UMR7583, CNRS,
Université Paris-Est-Créteil (UPEC) et Université Paris Diderot
(UPD), Institut Pierre Simon
Laplace (IPSL), Créteil, France
C. Giorio
Department of Chemistry, University of Cambridge,
Cambridge CB2 1EW, UK
Dipartimento di Scienze Chimiche, Università degli
Studi di Padova, Padova, 35131, Italy
F. Siekmann
Aix-Marseille Université, CNRS, LCE FRE 3416, 13331,
Marseille, France
E. Pangui
Laboratoire Interuniversitaire des Systèmes
Atmosphériques (LISA), UMR7583, CNRS,
Université Paris-Est-Créteil (UPEC) et Université Paris Diderot
(UPD), Institut Pierre Simon
Laplace (IPSL), Créteil, France
S. B. Morales
Laboratoire Interuniversitaire des Systèmes
Atmosphériques (LISA), UMR7583, CNRS,
Université Paris-Est-Créteil (UPEC) et Université Paris Diderot
(UPD), Institut Pierre Simon
Laplace (IPSL), Créteil, France
B. Temime-Roussel
Aix-Marseille Université, CNRS, LCE FRE 3416, 13331,
Marseille, France
A. Gratien
Laboratoire Interuniversitaire des Systèmes
Atmosphériques (LISA), UMR7583, CNRS,
Université Paris-Est-Créteil (UPEC) et Université Paris Diderot
(UPD), Institut Pierre Simon
Laplace (IPSL), Créteil, France
V. Michoud
Laboratoire Interuniversitaire des Systèmes
Atmosphériques (LISA), UMR7583, CNRS,
Université Paris-Est-Créteil (UPEC) et Université Paris Diderot
(UPD), Institut Pierre Simon
Laplace (IPSL), Créteil, France
M. Cazaunau
Laboratoire Interuniversitaire des Systèmes
Atmosphériques (LISA), UMR7583, CNRS,
Université Paris-Est-Créteil (UPEC) et Université Paris Diderot
(UPD), Institut Pierre Simon
Laplace (IPSL), Créteil, France
H. L. DeWitt
Aix-Marseille Université, CNRS, LCE FRE 3416, 13331,
Marseille, France
A. Tapparo
Dipartimento di Scienze Chimiche, Università degli
Studi di Padova, Padova, 35131, Italy
A. Monod
CORRESPONDING AUTHOR
Aix-Marseille Université, CNRS, LCE FRE 3416, 13331,
Marseille, France
J.-F. Doussin
Laboratoire Interuniversitaire des Systèmes
Atmosphériques (LISA), UMR7583, CNRS,
Université Paris-Est-Créteil (UPEC) et Université Paris Diderot
(UPD), Institut Pierre Simon
Laplace (IPSL), Créteil, France
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Cited
24 citations as recorded by crossref.
- Multiphase Photochemistry of Pyruvic Acid under Atmospheric Conditions A. Reed Harris et al. 10.1021/acs.jpca.7b01107
- Chemical Equilibria and Kinetics in Aqueous Solutions of Zymonic Acid R. Perkins et al. 10.1021/acs.jpca.6b10526
- Spectral- and size-resolved mass absorption efficiency of mineral dust aerosols in the shortwave spectrum: a simulation chamber study L. Caponi et al. 10.5194/acp-17-7175-2017
- Photochemical Synthesis of Oligomeric Amphiphiles from Alkyl Oxoacids in Aqueous Environments R. Rapf et al. 10.1021/jacs.7b01707
- Modeling organic aerosol over Europe in summer conditions with the VBS-GECKO parameterization: sensitivity to secondary organic compound properties and IVOC (intermediate-volatility organic compound) emissions V. Lannuque et al. 10.5194/acp-20-4905-2020
- Formation of Metal–Cyanide Complexes in Deliquescent Airborne Particles: A New Possible Sink for HCN in Urban Environments C. Giorio et al. 10.1021/acs.est.7b03123
- Large contribution to secondary organic aerosol from isoprene cloud chemistry H. Lamkaddam et al. 10.1126/sciadv.abe2952
- Mechanistic Description of Photochemical Oligomer Formation from Aqueous Pyruvic Acid R. Rapf et al. 10.1021/acs.jpca.7b03310
- Current State of Atmospheric Aerosol Thermodynamics and Mass Transfer Modeling: A Review K. Semeniuk & A. Dastoor 10.3390/atmos11020156
- Chemical characteristics of cloud water and the impacts on aerosol properties at a subtropical mountain site in Hong Kong SAR T. Li et al. 10.5194/acp-20-391-2020
- Measurement report: Impact of cloud processes on secondary organic aerosols at a forested mountain site in southeastern China Z. Zhang et al. 10.5194/acp-24-8473-2024
- Cloud Processing of Secondary Organic Aerosol from Isoprene and Methacrolein Photooxidation C. Giorio et al. 10.1021/acs.jpca.7b05933
- Observed and CMIP6-model-simulated organic aerosol response to drought in the contiguous United States during summertime W. Li & Y. Wang 10.5194/acp-24-9339-2024
- Humidity impact on photo-catalytic degradation: Adsorption behavior simulations and catalytic reaction mechanisms for main gaseous pollutants in papermaking industry Z. Lin et al. 10.1016/j.jclepro.2019.118863
- CLEPS 1.0: A new protocol for cloud aqueous phase oxidation of VOC mechanisms C. Mouchel-Vallon et al. 10.5194/gmd-10-1339-2017
- Comparison of Measurement-Based Methodologies to Apportion Secondary Organic Carbon (SOC) in PM2.5: A Review of Recent Studies D. Srivastava et al. 10.3390/atmos9110452
- Development of a protocol for the auto-generation of explicit aqueous-phase oxidation schemes of organic compounds P. Bräuer et al. 10.5194/acp-19-9209-2019
- An evaluation of global organic aerosol schemes using airborne observations S. Pai et al. 10.5194/acp-20-2637-2020
- Alternative Carbon Sources for Isoprene Emission V. de Souza et al. 10.1016/j.tplants.2018.09.012
- Methylamine’s Effects on Methylglyoxal-Containing Aerosol: Chemical, Physical, and Optical Changes D. De Haan et al. 10.1021/acsearthspacechem.9b00103
- Photo-catalytic degradation of mixed gaseous HCHO and C6H6 in paper mills: Experimental and theoretical study on the adsorption behavior simulation and catalytic reaction mechanism Z. Lin et al. 10.1016/j.jhazmat.2019.121779
- Recent advances in understanding secondary organic aerosol: Implications for global climate forcing M. Shrivastava et al. 10.1002/2016RG000540
- Kinetic and Mechanistic Study of the Reactions of NO3 Radicals with Unsaturated Aldehydes: 2-Butenal, 2-Methyl-2-butenal, and 3-Methyl-2-butenal B. Picquet-Varrault et al. 10.1021/acs.jpca.2c04216
- Aqueous-phase mechanism for secondary organic aerosol formation from isoprene: application to the southeast United States and co-benefit of SO<sub>2</sub> emission controls E. Marais et al. 10.5194/acp-16-1603-2016
23 citations as recorded by crossref.
- Multiphase Photochemistry of Pyruvic Acid under Atmospheric Conditions A. Reed Harris et al. 10.1021/acs.jpca.7b01107
- Chemical Equilibria and Kinetics in Aqueous Solutions of Zymonic Acid R. Perkins et al. 10.1021/acs.jpca.6b10526
- Spectral- and size-resolved mass absorption efficiency of mineral dust aerosols in the shortwave spectrum: a simulation chamber study L. Caponi et al. 10.5194/acp-17-7175-2017
- Photochemical Synthesis of Oligomeric Amphiphiles from Alkyl Oxoacids in Aqueous Environments R. Rapf et al. 10.1021/jacs.7b01707
- Modeling organic aerosol over Europe in summer conditions with the VBS-GECKO parameterization: sensitivity to secondary organic compound properties and IVOC (intermediate-volatility organic compound) emissions V. Lannuque et al. 10.5194/acp-20-4905-2020
- Formation of Metal–Cyanide Complexes in Deliquescent Airborne Particles: A New Possible Sink for HCN in Urban Environments C. Giorio et al. 10.1021/acs.est.7b03123
- Large contribution to secondary organic aerosol from isoprene cloud chemistry H. Lamkaddam et al. 10.1126/sciadv.abe2952
- Mechanistic Description of Photochemical Oligomer Formation from Aqueous Pyruvic Acid R. Rapf et al. 10.1021/acs.jpca.7b03310
- Current State of Atmospheric Aerosol Thermodynamics and Mass Transfer Modeling: A Review K. Semeniuk & A. Dastoor 10.3390/atmos11020156
- Chemical characteristics of cloud water and the impacts on aerosol properties at a subtropical mountain site in Hong Kong SAR T. Li et al. 10.5194/acp-20-391-2020
- Measurement report: Impact of cloud processes on secondary organic aerosols at a forested mountain site in southeastern China Z. Zhang et al. 10.5194/acp-24-8473-2024
- Cloud Processing of Secondary Organic Aerosol from Isoprene and Methacrolein Photooxidation C. Giorio et al. 10.1021/acs.jpca.7b05933
- Observed and CMIP6-model-simulated organic aerosol response to drought in the contiguous United States during summertime W. Li & Y. Wang 10.5194/acp-24-9339-2024
- Humidity impact on photo-catalytic degradation: Adsorption behavior simulations and catalytic reaction mechanisms for main gaseous pollutants in papermaking industry Z. Lin et al. 10.1016/j.jclepro.2019.118863
- CLEPS 1.0: A new protocol for cloud aqueous phase oxidation of VOC mechanisms C. Mouchel-Vallon et al. 10.5194/gmd-10-1339-2017
- Comparison of Measurement-Based Methodologies to Apportion Secondary Organic Carbon (SOC) in PM2.5: A Review of Recent Studies D. Srivastava et al. 10.3390/atmos9110452
- Development of a protocol for the auto-generation of explicit aqueous-phase oxidation schemes of organic compounds P. Bräuer et al. 10.5194/acp-19-9209-2019
- An evaluation of global organic aerosol schemes using airborne observations S. Pai et al. 10.5194/acp-20-2637-2020
- Alternative Carbon Sources for Isoprene Emission V. de Souza et al. 10.1016/j.tplants.2018.09.012
- Methylamine’s Effects on Methylglyoxal-Containing Aerosol: Chemical, Physical, and Optical Changes D. De Haan et al. 10.1021/acsearthspacechem.9b00103
- Photo-catalytic degradation of mixed gaseous HCHO and C6H6 in paper mills: Experimental and theoretical study on the adsorption behavior simulation and catalytic reaction mechanism Z. Lin et al. 10.1016/j.jhazmat.2019.121779
- Recent advances in understanding secondary organic aerosol: Implications for global climate forcing M. Shrivastava et al. 10.1002/2016RG000540
- Kinetic and Mechanistic Study of the Reactions of NO3 Radicals with Unsaturated Aldehydes: 2-Butenal, 2-Methyl-2-butenal, and 3-Methyl-2-butenal B. Picquet-Varrault et al. 10.1021/acs.jpca.2c04216
Saved (preprint)
Latest update: 13 Dec 2024
Short summary
The impact of cloud events on isoprene secondary organic aerosol (SOA) formation has been studied from an isoprene/ NOx/light system in an atmospheric simulation chamber. aqSOA formation can be linked to water soluble volatile organic compounds' dissolution in the aqueous phase and to further aqueous phase reactions. Cloud-induced SOA formation is experimentally demonstrated in this study, thus highlighting the importance of aqueous multiphase systems in atmospheric SOA formation estimations.
The impact of cloud events on isoprene secondary organic aerosol (SOA) formation has been...
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