Articles | Volume 16, issue 24
https://doi.org/10.5194/acp-16-15545-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-15545-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
16 Dec 2016
Research article |
| 16 Dec 2016
Organic aerosol source apportionment in London 2013 with ME-2: exploring the solution space with annual and seasonal analysis
Ernesto Reyes-Villegas
School of Earth, Atmospheric and Environmental Sciences, The
University of Manchester, Manchester, M13 9PL, UK
David C. Green
School of Biomedical and Health Sciences, King's College London,
London, UK
Max Priestman
School of Biomedical and Health Sciences, King's College London,
London, UK
Francesco Canonaco
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen PSI, Switzerland
School of Earth, Atmospheric and Environmental Sciences, The
University of Manchester, Manchester, M13 9PL, UK
André S. H. Prévôt
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen PSI, Switzerland
James D. Allan
CORRESPONDING AUTHOR
School of Earth, Atmospheric and Environmental Sciences, The
University of Manchester, Manchester, M13 9PL, UK
National Centre for Atmospheric Science, The University of
Manchester, Manchester, M13 9PL, UK
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Cited
34 citations as recorded by crossref.
- Comparison of Atmospheric Monocarboxylic and Dicarboxylic Acids in Xi’ an, China, for Source Apportionment of Organic Aerosols L. Wu et al. 10.1007/s11270-020-04675-y
- Impact of anthropogenic and biogenic sources on the seasonal variation in the molecular composition of urban organic aerosols: a field and laboratory study using ultra-high-resolution mass spectrometry K. Daellenbach et al. 10.5194/acp-19-5973-2019
- Assessing the Impact of Non-Exhaust Emissions on the Asthmatic Airway (IONA) Protocol for a Randomised Three-Exposure Crossover Study J. Scales et al. 10.3390/ijerph21070895
- Primary emissions versus secondary formation of fine particulate matter in the most polluted city (Shijiazhuang) in North China R. Huang et al. 10.5194/acp-19-2283-2019
- Measurement report: On the contribution of long-distance transport to the secondary aerosol formation and aging H. Zhong et al. 10.5194/acp-22-9513-2022
- Chemical characteristics and sources of nitrogen-containing organic compounds at a regional site in the North China Plain during the transition period of autumn and winter M. Wang et al. 10.1016/j.scitotenv.2021.151451
- Simulating organic aerosol in Delhi with WRF-Chem using the volatility-basis-set approach: exploring model uncertainty with a Gaussian process emulator E. Reyes-Villegas et al. 10.5194/acp-23-5763-2023
- From outdoor to indoor air pollution source apportionment: Answers to ten challenging questions D. Saraga et al. 10.1016/j.trac.2024.117821
- Simultaneous aerosol mass spectrometry and chemical ionisation mass spectrometry measurements during a biomass burning event in the UK: insights into nitrate chemistry E. Reyes-Villegas et al. 10.5194/acp-18-4093-2018
- Sources and processes that control the submicron organic aerosol composition in an urban Mediterranean environment (Athens): a high temporal-resolution chemical composition measurement study I. Stavroulas et al. 10.5194/acp-19-901-2019
- Mass spectral characterization of secondary organic aerosol from urban cooking and vehicular sources W. Zhu et al. 10.5194/acp-21-15065-2021
- Source apportionment of submicron organic aerosol collected from Atlanta, Georgia, during 2014–2015 using the aerosol chemical speciation monitor (ACSM) W. Rattanavaraha et al. 10.1016/j.atmosenv.2017.07.055
- International airport emissions and their impact on local air quality: chemical speciation of ambient aerosols at Madrid–Barajas Airport during the AVIATOR campaign S. Alzahrani et al. 10.5194/acp-24-9045-2024
- Real-time chemical characterization of primary and aged biomass burning aerosols derived from sub-Saharan African biomass fuels in smoldering fires M. James et al. 10.1039/D4EA00110A
- Annual exposure to polycyclic aromatic hydrocarbons in urban environments linked to wintertime wood-burning episodes I. Tsiodra et al. 10.5194/acp-21-17865-2021
- The effect of the averaging period for PMF analysis of aerosol mass spectrometer measurements during offline applications C. Vasilakopoulou et al. 10.5194/amt-15-6419-2022
- Time-dependent source apportionment of submicron organic aerosol for a rural site in an alpine valley using a rolling positive matrix factorisation (PMF) window G. Chen et al. 10.5194/acp-21-15081-2021
- A new method for long-term source apportionment with time-dependent factor profiles and uncertainty assessment using SoFi Pro: application to 1 year of organic aerosol data F. Canonaco et al. 10.5194/amt-14-923-2021
- Wintertime aerosol dominated by solid-fuel-burning emissions across Ireland: insight into the spatial and chemical variation in submicron aerosol C. Lin et al. 10.5194/acp-19-14091-2019
- Source apportionment resolved by time of day for improved deconvolution of primary source contributions to air pollution S. Bhandari et al. 10.5194/amt-15-6051-2022
- Six-year source apportionment of submicron organic aerosols from near-continuous highly time-resolved measurements at SIRTA (Paris area, France) Y. Zhang et al. 10.5194/acp-19-14755-2019
- Technical note: A new approach to discriminate different black carbon sources by utilising fullerene and metals in positive matrix factorisation analysis of high-resolution soot particle aerosol mass spectrometer data Z. Bibi et al. 10.5194/acp-21-10763-2021
- Improved source apportionment of organic aerosols in complex urban air pollution using the multilinear engine (ME-2) Q. Zhu et al. 10.5194/amt-11-1049-2018
- Measurement report: Fourteen months of real-time characterisation of the submicronic aerosol and its atmospheric dynamics at the Marseille–Longchamp supersite B. Chazeau et al. 10.5194/acp-21-7293-2021
- Exploration of PM<sub>2.5</sub> sources on the regional scale in the Pearl River Delta based on ME-2 modeling X. Huang et al. 10.5194/acp-18-11563-2018
- Organic aerosol source apportionment by using rolling positive matrix factorization: Application to a Mediterranean coastal city B. Chazeau et al. 10.1016/j.aeaoa.2022.100176
- Total carbon and benzo(a)pyrene in particulate matter over a Polish urban site – A combined effect of major anthropogenic sources and air mass transport P. Siudek 10.1016/j.apr.2018.01.001
- A novel probabilistic source apportionment approach: Bayesian auto-correlated matrix factorization A. Rusanen et al. 10.5194/amt-17-1251-2024
- Online Chemical Characterization of Food-Cooking Organic Aerosols: Implications for Source Apportionment E. Reyes-Villegas et al. 10.1021/acs.est.7b06278
- A searchable database and mass spectral comparison tool for the Aerosol Mass Spectrometer (AMS) and the Aerosol Chemical Speciation Monitor (ACSM) S. Jeon et al. 10.5194/amt-16-6075-2023
- Chemical Characterization and Source Apportionment of Organic Aerosols in the Coastal City of Chennai, India: Impact of Marine Air Masses on Aerosol Chemical Composition and Potential for Secondary Organic Aerosol Formation S. Kommula et al. 10.1021/acsearthspacechem.1c00276
- Molecular tracers, mass spectral tracers and oxidation of organic aerosols emitted from cooking and fossil fuel burning sources C. Liang et al. 10.1016/j.scitotenv.2023.161635
- Long-term trends in particulate matter from wood burning in the United Kingdom: Dependence on weather and social factors A. Font et al. 10.1016/j.envpol.2022.120105
- Secondary organic aerosol formation in China from urban-lifestyle sources: Vehicle exhaust and cooking emission Z. Zhang et al. 10.1016/j.scitotenv.2022.159340
34 citations as recorded by crossref.
- Comparison of Atmospheric Monocarboxylic and Dicarboxylic Acids in Xi’ an, China, for Source Apportionment of Organic Aerosols L. Wu et al. 10.1007/s11270-020-04675-y
- Impact of anthropogenic and biogenic sources on the seasonal variation in the molecular composition of urban organic aerosols: a field and laboratory study using ultra-high-resolution mass spectrometry K. Daellenbach et al. 10.5194/acp-19-5973-2019
- Assessing the Impact of Non-Exhaust Emissions on the Asthmatic Airway (IONA) Protocol for a Randomised Three-Exposure Crossover Study J. Scales et al. 10.3390/ijerph21070895
- Primary emissions versus secondary formation of fine particulate matter in the most polluted city (Shijiazhuang) in North China R. Huang et al. 10.5194/acp-19-2283-2019
- Measurement report: On the contribution of long-distance transport to the secondary aerosol formation and aging H. Zhong et al. 10.5194/acp-22-9513-2022
- Chemical characteristics and sources of nitrogen-containing organic compounds at a regional site in the North China Plain during the transition period of autumn and winter M. Wang et al. 10.1016/j.scitotenv.2021.151451
- Simulating organic aerosol in Delhi with WRF-Chem using the volatility-basis-set approach: exploring model uncertainty with a Gaussian process emulator E. Reyes-Villegas et al. 10.5194/acp-23-5763-2023
- From outdoor to indoor air pollution source apportionment: Answers to ten challenging questions D. Saraga et al. 10.1016/j.trac.2024.117821
- Simultaneous aerosol mass spectrometry and chemical ionisation mass spectrometry measurements during a biomass burning event in the UK: insights into nitrate chemistry E. Reyes-Villegas et al. 10.5194/acp-18-4093-2018
- Sources and processes that control the submicron organic aerosol composition in an urban Mediterranean environment (Athens): a high temporal-resolution chemical composition measurement study I. Stavroulas et al. 10.5194/acp-19-901-2019
- Mass spectral characterization of secondary organic aerosol from urban cooking and vehicular sources W. Zhu et al. 10.5194/acp-21-15065-2021
- Source apportionment of submicron organic aerosol collected from Atlanta, Georgia, during 2014–2015 using the aerosol chemical speciation monitor (ACSM) W. Rattanavaraha et al. 10.1016/j.atmosenv.2017.07.055
- International airport emissions and their impact on local air quality: chemical speciation of ambient aerosols at Madrid–Barajas Airport during the AVIATOR campaign S. Alzahrani et al. 10.5194/acp-24-9045-2024
- Real-time chemical characterization of primary and aged biomass burning aerosols derived from sub-Saharan African biomass fuels in smoldering fires M. James et al. 10.1039/D4EA00110A
- Annual exposure to polycyclic aromatic hydrocarbons in urban environments linked to wintertime wood-burning episodes I. Tsiodra et al. 10.5194/acp-21-17865-2021
- The effect of the averaging period for PMF analysis of aerosol mass spectrometer measurements during offline applications C. Vasilakopoulou et al. 10.5194/amt-15-6419-2022
- Time-dependent source apportionment of submicron organic aerosol for a rural site in an alpine valley using a rolling positive matrix factorisation (PMF) window G. Chen et al. 10.5194/acp-21-15081-2021
- A new method for long-term source apportionment with time-dependent factor profiles and uncertainty assessment using SoFi Pro: application to 1 year of organic aerosol data F. Canonaco et al. 10.5194/amt-14-923-2021
- Wintertime aerosol dominated by solid-fuel-burning emissions across Ireland: insight into the spatial and chemical variation in submicron aerosol C. Lin et al. 10.5194/acp-19-14091-2019
- Source apportionment resolved by time of day for improved deconvolution of primary source contributions to air pollution S. Bhandari et al. 10.5194/amt-15-6051-2022
- Six-year source apportionment of submicron organic aerosols from near-continuous highly time-resolved measurements at SIRTA (Paris area, France) Y. Zhang et al. 10.5194/acp-19-14755-2019
- Technical note: A new approach to discriminate different black carbon sources by utilising fullerene and metals in positive matrix factorisation analysis of high-resolution soot particle aerosol mass spectrometer data Z. Bibi et al. 10.5194/acp-21-10763-2021
- Improved source apportionment of organic aerosols in complex urban air pollution using the multilinear engine (ME-2) Q. Zhu et al. 10.5194/amt-11-1049-2018
- Measurement report: Fourteen months of real-time characterisation of the submicronic aerosol and its atmospheric dynamics at the Marseille–Longchamp supersite B. Chazeau et al. 10.5194/acp-21-7293-2021
- Exploration of PM<sub>2.5</sub> sources on the regional scale in the Pearl River Delta based on ME-2 modeling X. Huang et al. 10.5194/acp-18-11563-2018
- Organic aerosol source apportionment by using rolling positive matrix factorization: Application to a Mediterranean coastal city B. Chazeau et al. 10.1016/j.aeaoa.2022.100176
- Total carbon and benzo(a)pyrene in particulate matter over a Polish urban site – A combined effect of major anthropogenic sources and air mass transport P. Siudek 10.1016/j.apr.2018.01.001
- A novel probabilistic source apportionment approach: Bayesian auto-correlated matrix factorization A. Rusanen et al. 10.5194/amt-17-1251-2024
- Online Chemical Characterization of Food-Cooking Organic Aerosols: Implications for Source Apportionment E. Reyes-Villegas et al. 10.1021/acs.est.7b06278
- A searchable database and mass spectral comparison tool for the Aerosol Mass Spectrometer (AMS) and the Aerosol Chemical Speciation Monitor (ACSM) S. Jeon et al. 10.5194/amt-16-6075-2023
- Chemical Characterization and Source Apportionment of Organic Aerosols in the Coastal City of Chennai, India: Impact of Marine Air Masses on Aerosol Chemical Composition and Potential for Secondary Organic Aerosol Formation S. Kommula et al. 10.1021/acsearthspacechem.1c00276
- Molecular tracers, mass spectral tracers and oxidation of organic aerosols emitted from cooking and fossil fuel burning sources C. Liang et al. 10.1016/j.scitotenv.2023.161635
- Long-term trends in particulate matter from wood burning in the United Kingdom: Dependence on weather and social factors A. Font et al. 10.1016/j.envpol.2022.120105
- Secondary organic aerosol formation in China from urban-lifestyle sources: Vehicle exhaust and cooking emission Z. Zhang et al. 10.1016/j.scitotenv.2022.159340
Discussed (preprint)
Latest update: 14 Dec 2024
Short summary
For the first time in the UK, an Aerosol Chemical Speciation Monitor was used to measure aerosol concentrations in London in March–December 2013, with further organic aerosol (OA) source apportionment using the ME-2 factorization tool. Five OA sources were identified: biomass burning OA, hydrocarbon-like OA, cooking OA, semivolatile oxygenated OA and low-volatility oxygenated OA. This information can be used to take future action on the respective legislation in order to improve the air quality.
For the first time in the UK, an Aerosol Chemical Speciation Monitor was used to measure aerosol...
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