Articles | Volume 16, issue 22
https://doi.org/10.5194/acp-16-14515-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-14515-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
23 Nov 2016
Research article |
| 23 Nov 2016
Morphology and mixing of black carbon particles collected in central California during the CARES field study
Department of Chemistry, University of the Pacific, Stockton, CA
95211, USA
Rachel E. O'Brien
Department of Chemistry, University of the Pacific, Stockton, CA
95211, USA
Chemical Sciences Division, Lawrence Berkeley National
Laboratory, Berkeley, CA 94720, USA
present address: Department of Civil and Environmental Engineering,
Massachusetts Institute of Technology, Cambridge, MA 02139,
USA
Peter A. Alpert
Institute for Terrestrial and
Planetary Atmospheres, School of Marine and Atmospheric Sciences,
Stony Brook University, Stony Brook, NY 11794, USA
present address: CNRS, UMR5256, IRCELYON, Institut de
Recherches sur la Catalyse et l'Environnement de Lyon,
Villeurbanne 69626, France
Stephen T. Kelly
Chemical Sciences Division, Lawrence Berkeley National
Laboratory, Berkeley, CA 94720, USA
present address: Carl Zeiss X-ray
Microscopy Inc., Pleasanton, CA 94588, USA
Don Q. Pham
Department of Chemistry, University of the Pacific, Stockton, CA
95211, USA
Mary K. Gilles
Chemical Sciences Division, Lawrence Berkeley National
Laboratory, Berkeley, CA 94720, USA
Daniel A. Knopf
Institute for Terrestrial and
Planetary Atmospheres, School of Marine and Atmospheric Sciences,
Stony Brook University, Stony Brook, NY 11794, USA
Alexander Laskin
Pacific Northwest National Laboratory, W. R. Wiley Environmental
Molecular Sciences Laboratory, Richland, WA 99354, USA
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- Aircraft soot from conventional fuels and biofuels during ground idle and climb-out conditions: Electron microscopy and X-ray micro-spectroscopy A. Liati et al. 10.1016/j.envpol.2019.01.078
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- The effects of morphology, mobility size, and secondary organic aerosol (SOA) material coating on the ice nucleation activity of black carbon in the cirrus regime C. Zhang et al. 10.5194/acp-20-13957-2020
42 citations as recorded by crossref.
- Condensed-phase biogenic–anthropogenic interactions with implications for cold cloud formation J. Charnawskas et al. 10.1039/C7FD00010C
- Structural Collapse and Coating Composition Changes of Soot Particles During Long‐Range Transport J. Zhang et al. 10.1029/2023JD038871
- The Role of Organic Aerosol in Atmospheric Ice Nucleation: A Review D. Knopf et al. 10.1021/acsearthspacechem.7b00120
- Markedly different impacts of primary emissions and secondary aerosol formation on aerosol mixing states revealed by simultaneous measurements of CCNC, H(/V)TDMA, and SP2 J. Tao et al. 10.5194/acp-24-9131-2024
- Constructing Shapes and Mixing Structures of Black Carbon Particles With Applications to Optical Calculations Y. Wang et al. 10.1029/2021JD034620
- Quantifying black carbon light absorption enhancement with a novel statistical approach C. Wu et al. 10.5194/acp-18-289-2018
- Quantitative capabilities of STXM to measure spatially resolved organic volume fractions of mixed organic ∕ inorganic particles M. Fraund et al. 10.5194/amt-12-1619-2019
- The diverse chemical mixing state of aerosol particles in the southeastern United States A. Bondy et al. 10.5194/acp-18-12595-2018
- Influences of Primary Emission and Secondary Coating Formation on the Particle Diversity and Mixing State of Black Carbon Particles A. Lee et al. 10.1021/acs.est.9b03064
- Mixing State of Black Carbon Particles in Asian Outflow Observed at a Remote Site in Taiwan in the Spring of 2017 C. Sun et al. 10.1029/2020JD032526
- Impact of dry intrusion events on the composition and mixing state of particles during the winter Aerosol and Cloud Experiment in the Eastern North Atlantic (ACE-ENA) J. Tomlin et al. 10.5194/acp-21-18123-2021
- Ice nucleation abilities of soot particles determined with the Horizontal Ice Nucleation Chamber F. Mahrt et al. 10.5194/acp-18-13363-2018
- Coupling Effect of Elemental Carbon and Organic Carbon on the Changes of Optical Properties and Oxidative Potential of Soot Particles under Visible Light R. Tang et al. 10.1021/acs.est.4c09217
- Chemical characterization of microplastic particles formed in airborne waste discharged from sewer pipe repairs B. Peterson et al. 10.1039/D3EM00193H
- Microscopic Observations of Core‐Shell Particle Structure and Implications for Atmospheric Aerosol Remote Sensing F. Unga et al. 10.1029/2018JD028602
- Liquid-liquid phase separation reduces radiative absorption by aged black carbon aerosols J. Zhang et al. 10.1038/s43247-022-00462-1
- Chemical Imaging of Fine Mode Atmospheric Particles Collected from a Research Aircraft over Agricultural Fields J. Tomlin et al. 10.1021/acsearthspacechem.0c00172
- Micro-spectroscopic and freezing characterization of ice-nucleating particles collected in the marine boundary layer in the eastern North Atlantic D. Knopf et al. 10.5194/acp-22-5377-2022
- Internally mixed black carbon in the Indo-Gangetic Plain and its effect on absorption enhancement N. Thamban et al. 10.1016/j.atmosres.2017.07.007
- Determination of equivalent black carbon mass concentration from aerosol light absorption using variable mass absorption cross section W. Zhao et al. 10.5194/amt-14-1319-2021
- Monthly and Diurnal Variation of the Concentrations of Aerosol Surface Area in Fukuoka, Japan, Measured by Diffusion Charging Method M. Kiriya et al. 10.3390/atmos8070114
- Technical note: Mismeasurement of the core-shell structure of black carbon-containing ambient aerosols by SP2 measurements G. Zhao et al. 10.1016/j.atmosenv.2020.117885
- Role of black carbon mass size distribution in the direct aerosol radiative forcing G. Zhao et al. 10.5194/acp-19-13175-2019
- Chemical Imaging of Atmospheric Particles A. Laskin et al. 10.1021/acs.accounts.9b00396
- Aerosol Composition, Mixing State, and Phase State of Free Tropospheric Particles and Their Role in Ice Cloud Formation N. Lata et al. 10.1021/acsearthspacechem.1c00315
- Mixing state evolution of agglomerating particles in an aerosol chamber: Comparison of measurements and particle-resolved simulations C. Shou et al. 10.1080/02786826.2019.1661959
- Aging induced changes in ice nucleation activity of combustion aerosol as determined by near edge X-ray absorption fine structure (NEXAFS) spectroscopy F. Mahrt et al. 10.1039/C9EM00525K
- Radiative absorption enhancements by black carbon controlled by particle-to-particle heterogeneity in composition L. Fierce et al. 10.1073/pnas.1919723117
- Characterization and morphological analysis of individual aerosol of PM10 in urban area of Lucknow, India S. Bharti et al. 10.1016/j.micron.2017.09.004
- Phase Behavior of Internal Mixtures of Hydrocarbon-like Primary Organic Aerosol and Secondary Aerosol Based on Their Differences in Oxygen-to-Carbon Ratios F. Mahrt et al. 10.1021/acs.est.1c07691
- Mixing state of black carbon at different atmospheres in north and southwest China G. Zhao et al. 10.5194/acp-22-10861-2022
- An evaluation of three methods for measuring black carbon in Alert, Canada S. Sharma et al. 10.5194/acp-17-15225-2017
- Variability in the mass absorption cross section of black carbon (BC) aerosols is driven by BC internal mixing state at a central European background site (Melpitz, Germany) in winter J. Yuan et al. 10.5194/acp-21-635-2021
- Scaling Laws for Light Absorption Enhancement Due to Nonrefractory Coating of Atmospheric Black Carbon Aerosol R. Chakrabarty & W. Heinson 10.1103/PhysRevLett.121.218701
- The Impact of Cloud Processing on the Ice Nucleation Abilities of Soot Particles at Cirrus Temperatures F. Mahrt et al. 10.1029/2019JD030922
- Aircraft soot from conventional fuels and biofuels during ground idle and climb-out conditions: Electron microscopy and X-ray micro-spectroscopy A. Liati et al. 10.1016/j.envpol.2019.01.078
- Long term variation of microphysical properties of black carbon in Beijing derived from observation and machine learning K. Hu et al. 10.1088/1748-9326/ad4618
- Aerosol Mixing State: Measurements, Modeling, and Impacts N. Riemer et al. 10.1029/2018RG000615
- Oxidation Potential Reduction of Carbon Nanomaterials during Atmospheric-Relevant Aging: Role of Surface Coating H. Jiang et al. 10.1021/acs.est.9b02062
- Chemical composition and morphological analysis of atmospheric particles from an intensive bonfire burning festival J. Tomlin et al. 10.1039/D2EA00037G
- Lifecycle of light-absorbing carbonaceous aerosols in the atmosphere D. Liu et al. 10.1038/s41612-020-00145-8
- The effects of morphology, mobility size, and secondary organic aerosol (SOA) material coating on the ice nucleation activity of black carbon in the cirrus regime C. Zhang et al. 10.5194/acp-20-13957-2020
Discussed (final revised paper)
Latest update: 25 Dec 2024
Short summary
Atmospheric black carbon (BC), commonly known as soot, is an important constituent of the earth that imparts a warming similar to that of carbon dioxide. However, BC is much shorter lived and has uncertain warming due to its mixture with other solid and liquid components. Here, advanced microscopic methods have provided a detailed look at thousands of BC particles sampled from central California; these measurements will lead towards a better understanding of the effects that BC has on climate.
Atmospheric black carbon (BC), commonly known as soot, is an important constituent of the earth...
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