Articles | Volume 16, issue 19
https://doi.org/10.5194/acp-16-12793-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-12793-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Observation of new particle formation and measurement of sulfuric acid, ammonia, amines and highly oxidized organic molecules at a rural site in central Germany
Andreas Kürten
CORRESPONDING AUTHOR
Institute for Atmospheric and Environmental Sciences, Goethe
University Frankfurt, Frankfurt am Main, Germany
Anton Bergen
Institute for Atmospheric and Environmental Sciences, Goethe
University Frankfurt, Frankfurt am Main, Germany
Martin Heinritzi
Institute for Atmospheric and Environmental Sciences, Goethe
University Frankfurt, Frankfurt am Main, Germany
Markus Leiminger
Institute for Atmospheric and Environmental Sciences, Goethe
University Frankfurt, Frankfurt am Main, Germany
Verena Lorenz
Institute for Atmospheric and Environmental Sciences, Goethe
University Frankfurt, Frankfurt am Main, Germany
Felix Piel
Institute for Atmospheric and Environmental Sciences, Goethe
University Frankfurt, Frankfurt am Main, Germany
Mario Simon
Institute for Atmospheric and Environmental Sciences, Goethe
University Frankfurt, Frankfurt am Main, Germany
Robert Sitals
Institute for Atmospheric and Environmental Sciences, Goethe
University Frankfurt, Frankfurt am Main, Germany
Andrea C. Wagner
Institute for Atmospheric and Environmental Sciences, Goethe
University Frankfurt, Frankfurt am Main, Germany
Joachim Curtius
Institute for Atmospheric and Environmental Sciences, Goethe
University Frankfurt, Frankfurt am Main, Germany
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Cited
72 citations as recorded by crossref.
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- Impacts of Mixed Gaseous and Particulate Pollutants on Secondary Particle Formation during Ozonolysis of Butyl Vinyl Ether P. Zhang et al. 10.1021/acs.est.9b07650
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72 citations as recorded by crossref.
- Hydration motifs of ammonium bisulfate clusters of relevance to atmospheric new particle formation Y. Yang & C. Johnson 10.1039/C8FD00206A
- Enhancing Potential of Trimethylamine Oxide on Atmospheric Particle Formation N. Myllys et al. 10.3390/atmos11010035
- Characteristics and sources of aerosol aminiums over the eastern coast of China: insights from the integrated observations in a coastal city, adjacent island and surrounding marginal seas S. Zhou et al. 10.5194/acp-19-10447-2019
- Impacts of Mixed Gaseous and Particulate Pollutants on Secondary Particle Formation during Ozonolysis of Butyl Vinyl Ether P. Zhang et al. 10.1021/acs.est.9b07650
- Observations of Gas-Phase Alkylamines at a Coastal Site in the East Mediterranean Atmosphere E. Tzitzikalaki et al. 10.3390/atmos12111454
- Characteristics and sources of amine-containing particles in the urban atmosphere of Liaocheng, a seriously polluted city in North China during the COVID-19 outbreak Z. Li et al. 10.1016/j.envpol.2021.117887
- Perspective on the Recent Measurements of Reduced Nitrogen Compounds in the Atmosphere S. Lee 10.3389/fenvs.2022.868534
- New Particle Formation and Growth Mechanisms in Highly Polluted Environments H. Yu et al. 10.1007/s40726-017-0067-3
- Enigma of Urban Gaseous Oxygenated Organic Molecules: Precursor Type, Role of NOx, and Degree of Oxygenation L. Tian et al. 10.1021/acs.est.2c05047
- Exploring atmospheric free-radical chemistry in China: the self-cleansing capacity and the formation of secondary air pollution K. Lu et al. 10.1093/nsr/nwy073
- Emissions of volatile organic compounds from Norway spruce and potential atmospheric impacts H. Hakola et al. 10.3389/ffgc.2023.1116414
- Box modelling of gas-phase atmospheric iodine chemical reactivity in case of a nuclear accident C. Fortin et al. 10.1016/j.atmosenv.2019.116838
- Integrated experimental and theoretical approach to probe the synergistic effect of ammonia in methanesulfonic acid reactions with small alkylamines V. Perraud et al. 10.1039/C9EM00431A
- Nonagricultural emissions enhance dimethylamine and modulate urban atmospheric nucleation Y. Chang et al. 10.1016/j.scib.2023.05.033
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- The synergistic role of sulfuric acid, ammonia and organics in particle formation over an agricultural land L. Dada et al. 10.1039/D3EA00065F
- Highly Oxygenated Organic Molecules (HOM) from Gas-Phase Autoxidation Involving Peroxy Radicals: A Key Contributor to Atmospheric Aerosol F. Bianchi et al. 10.1021/acs.chemrev.8b00395
- Measurement report: Contribution of atmospheric new particle formation to ultrafine particle concentration, cloud condensation nuclei, and radiative forcing – results from 5-year observations in central Europe J. Sun et al. 10.5194/acp-24-10667-2024
- Particle number size distributions and formation and growth rates of different new particle formation types of a megacity in China L. Dai et al. 10.1016/j.jes.2022.07.029
- Organic aerosol source apportionment in Zurich using an extractive electrospray ionization time-of-flight mass spectrometer (EESI-TOF-MS) – Part 1: Biogenic influences and day–night chemistry in summer G. Stefenelli et al. 10.5194/acp-19-14825-2019
- Role of Iodine-Assisted Aerosol Particle Formation in Antarctica C. Xavier et al. 10.1021/acs.est.3c09103
- Constraints on the Role of Laplace Pressure in Multiphase Reactions and Viscosity of Organic Aerosols S. Petters 10.1029/2022GL098959
- Quantifying New Sources of Ambient Organic Aerosol and Their Roles in Particle Growth Using Oxygenated Organic Molecule (OOM) Tracers Y. Zhao et al. 10.1021/acs.estlett.4c00536
- Heterogeneous uptake of ammonia and dimethylamine into sulfuric and oxalic acid particles M. Sauerwein & C. Chan 10.5194/acp-17-6323-2017
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- New particle formation in the sulfuric acid–dimethylamine–water system: reevaluation of CLOUD chamber measurements and comparison to an aerosol nucleation and growth model A. Kürten et al. 10.5194/acp-18-845-2018
- Amines in boreal forest air at SMEAR II station in Finland M. Hemmilä et al. 10.5194/acp-18-6367-2018
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- Nitrate Radicals Suppress Biogenic New Particle Formation from Monoterpene Oxidation D. Li et al. 10.1021/acs.est.3c07958
- Atmospheric new particle formation from sulfuric acid and amines in a Chinese megacity L. Yao et al. 10.1126/science.aao4839
- Quantitation of 11 alkylamines in atmospheric samples: separating structural isomers by ion chromatography B. Place et al. 10.5194/amt-10-1061-2017
- Direct Link between Structure and Hydration in Ammonium and Aminium Bisulfate Clusters Implicated in Atmospheric New Particle Formation Y. Yang et al. 10.1021/acs.jpclett.8b02500
- Atmospheric clusters to nanoparticles: Recent progress and challenges in closing the gap in chemical composition J. Smith et al. 10.1016/j.jaerosci.2020.105733
- Role of Criegee intermediates in the formation of sulfuric acid at a Mediterranean (Cape Corsica) site under influence of biogenic emissions A. Kukui et al. 10.5194/acp-21-13333-2021
- Synergistic HNO3–H2SO4–NH3 upper tropospheric particle formation M. Wang et al. 10.1038/s41586-022-04605-4
- Contribution of Atmospheric Oxygenated Organic Compounds to Particle Growth in an Urban Environment X. Qiao et al. 10.1021/acs.est.1c02095
- Responses of gaseous sulfuric acid and particulate sulfate to reduced SO2 concentration: A perspective from long-term measurements in Beijing X. Li et al. 10.1016/j.scitotenv.2020.137700
- Iodine oxoacids and their roles in sub-3 nm particle growth in polluted urban environments Y. Zhang et al. 10.5194/acp-24-1873-2024
- Measurement report: Insights into the chemical composition and origin of molecular clusters and potential precursor molecules present in the free troposphere over the southern Indian Ocean: observations from the Maïdo Observatory (2150 m a.s.l., Réunion) R. Salignat et al. 10.5194/acp-24-3785-2024
- Relative humidity effect on the formation of highly oxidized molecules and new particles during monoterpene oxidation X. Li et al. 10.5194/acp-19-1555-2019
- New Particle Formation in the Atmosphere: From Molecular Clusters to Global Climate S. Lee et al. 10.1029/2018JD029356
- Competitive Uptake of Dimethylamine and Trimethylamine against Ammonia on Acidic Particles in Marine Atmospheres D. Chen et al. 10.1021/acs.est.1c08713
- Dimethylamine in cloud water: a case study over the northwest Atlantic Ocean A. Corral et al. 10.1039/D2EA00117A
- Simultaneous determination of nine atmospheric amines and six inorganic ions by non-suppressed ion chromatography using acetonitrile and 18-crown-6 as eluent additive H. Feng et al. 10.1016/j.chroma.2020.461234
- Measurement of ammonia, amines and iodine compounds using protonated water cluster chemical ionization mass spectrometry J. Pfeifer et al. 10.5194/amt-13-2501-2020
- A high-transmission axial ion mobility classifier for mass–mobility measurements of atmospheric ions M. Leiminger et al. 10.5194/amt-15-3705-2022
- Driving parameters of biogenic volatile organic compounds and consequences on new particle formation observed at an eastern Mediterranean background site C. Debevec et al. 10.5194/acp-18-14297-2018
- Seasonal variation in oxygenated organic molecules in urban Beijing and their contribution to secondary organic aerosol Y. Guo et al. 10.5194/acp-22-10077-2022
- A new advance in the pollution profile, transformation process, and contribution to aerosol formation and aging of atmospheric amines X. Shen et al. 10.1039/D2EA00167E
- A predictive model for salt nanoparticle formation using heterodimer stability calculations S. Chee et al. 10.5194/acp-21-11637-2021
- A nitrate ion chemical-ionization atmospheric-pressure-interface time-of-flight mass spectrometer (NO3− ToFCIMS) sensitivity study S. Alage et al. 10.5194/amt-17-4709-2024
- Self-Catalytic Reaction of SO3 and NH3 To Produce Sulfamic Acid and Its Implication to Atmospheric Particle Formation H. Li et al. 10.1021/jacs.8b04928
- Gas-phase catalytic hydration of I2O5 in the polluted coastal regions: Reaction mechanisms and atmospheric implications Y. Liang et al. 10.1016/j.jes.2021.09.028
- Wintertime new particle formation and its contribution to cloud condensation nuclei in the Northeastern United States F. Yu et al. 10.5194/acp-20-2591-2020
- The effect of meteorological conditions and atmospheric composition in the occurrence and development of new particle formation (NPF) events in Europe D. Bousiotis et al. 10.5194/acp-21-3345-2021
- Measurement Report: Wintertime new particle formation in the rural area of the North China Plain – influencing factors and possible formation mechanism J. Hong et al. 10.5194/acp-23-5699-2023
- Guanidine: A Highly Efficient Stabilizer in Atmospheric New-Particle Formation N. Myllys et al. 10.1021/acs.jpca.8b02507
- Formation of nighttime sulfuric acid from the ozonolysis of alkenes in Beijing Y. Guo et al. 10.5194/acp-21-5499-2021
- Large Increases in Primary Trimethylaminium and Secondary Dimethylaminium in Atmospheric Particles Associated With Cyclonic Eddies in the Northwest Pacific Ocean Q. Hu et al. 10.1029/2018JD028836
- Fast Evolution of Sulfuric Acid Aerosol Activated by External Fields for Enhanced Emission Control Z. Yang et al. 10.1021/acs.est.9b06191
- Nonagricultural Emissions Dominate Urban Atmospheric Amines as Revealed by Mobile Measurements Y. Chang et al. 10.1029/2021GL097640
- Investigation of the Reaction Mechanism and Kinetics of Iodic Acid with OH Radical Using Quantum Chemistry S. Khanniche et al. 10.1021/acsearthspacechem.7b00038
- Detection of atmospheric gaseous amines and amides by a high-resolution time-of-flight chemical ionization mass spectrometer with protonated ethanol reagent ions L. Yao et al. 10.5194/acp-16-14527-2016
- Measurement report: Urban ammonia and amines in Houston, Texas L. Tiszenkel et al. 10.5194/acp-24-11351-2024
- Limited Role of Malonic Acid in Sulfuric Acid–Dimethylamine New Particle Formation S. Fomete et al. 10.1021/acsomega.3c01643
- Resolving Atmospheric Oxygenated Organic Molecules in Urban Beijing Using Online Ultrahigh-Resolution Chemical Ionization Mass Spectrometry Y. Yuan et al. 10.1021/acs.est.4c04214
- Vertical characterization of highly oxygenated molecules (HOMs) below and above a boreal forest canopy Q. Zha et al. 10.5194/acp-18-17437-2018
Latest update: 06 Nov 2024
Short summary
Field measurements were conducted at a rural site in central Germany close to dairy farms to investigate if there is a connection between new particle formation and the presence of amines. A variety of trace gases were measured in addition to amines, like sulfuric acid, ammonia and highly oxygenated organic molecules (HOM). The results indicate that amines are very likely involved in the growth of aerosol particles and probably also in the nucleation process, although HOM could be relevant, too.
Field measurements were conducted at a rural site in central Germany close to dairy farms to...
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