Discontinuities in hygroscopic growth below and above water saturation for
laboratory surrogates of oligomers in organic atmospheric aerosols

Hodas, Natasha; Zuend, Andreas; Schilling, Katherine; Berkemeier, Thomas; Shiraiwa, Manabu; Flagan, Richard C.; Seinfeld, John H.

doi:10.5194/acp-16-12767-2016

Articles | Volume 16, issue 19

https://doi.org/10.5194/acp-16-12767-2016

© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

https://doi.org/10.5194/acp-16-12767-2016

© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

Articles | Volume 16, issue 19

Research article

|

13 Oct 2016

Research article |

| 13 Oct 2016

Discontinuities in hygroscopic growth below and above water saturation for laboratory surrogates of oligomers in organic atmospheric aerosols

Natasha Hodas, Andreas Zuend, Katherine Schilling, Thomas Berkemeier, Manabu Shiraiwa, Richard C. Flagan, and John H. Seinfeld

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2,403	1,248	132	3,783	129	179

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Views and downloads (calculated since 28 Apr 2016)

Month	HTML	PDF	XML	Total
Apr 2016	132	50	1	183
May 2016	73	38	3	114
Jun 2016	22	17	0	39
Jul 2016	9	5	1	15
Aug 2016	15	6	1	22
Sep 2016	3	3	0	6
Oct 2016	123	54	5	182
Nov 2016	21	14	5	40
Dec 2016	15	5	0	20
Jan 2017	32	12	4	48
Feb 2017	26	7	0	33
Mar 2017	45	19	3	67
Apr 2017	36	19	1	56
May 2017	34	19	2	55
Jun 2017	29	10	2	41
Jul 2017	19	10	1	30
Aug 2017	12	11	0	23
Sep 2017	17	12	1	30
Oct 2017	18	9	1	28
Nov 2017	17	9	2	28
Dec 2017	10	8	1	19
Jan 2018	14	8	0	22
Feb 2018	15	12	1	28
Mar 2018	12	6	1	19
Apr 2018	11	9	2	22
May 2018	12	8	6	26
Jun 2018	7	10	1	18
Jul 2018	9	11	0	20
Aug 2018	21	5	0	26
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Oct 2018	19	9	3	31
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Dec 2019	5	7	0	12
Jan 2020	12	5	0	17
Feb 2020	6	5	2	13
Mar 2020	7	3	1	11
Apr 2020	5	3	0	8
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Jan 2021	15	12	0	27
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Jul 2021	11	13	1	25
Aug 2021	9	7	0	16
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Oct 2021	10	46	0	56
Nov 2021	24	30	0	54
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Jan 2022	14	10	1	25
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Apr 2022	9	8	1	18
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Jan 2023	18	22	2	42
Feb 2023	14	8	0	22
Mar 2023	19	9	0	28
Apr 2023	6	6	0	12
May 2023	32	6	0	38
Jun 2023	49	10	1	60
Jul 2023	35	5	1	41
Aug 2023	45	7	3	55
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Oct 2023	42	9	1	52
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Jan 2024	44	8	1	53
Feb 2024	41	8	0	49
Mar 2024	47	18	5	70
Apr 2024	43	14	4	61
May 2024	18	16	2	36
Jun 2024	16	11	2	29
Jul 2024	13	16	2	31
Aug 2024	26	10	1	37
Sep 2024	16	2	0	18
Oct 2024	19	5	0	24
Nov 2024	19	10	2	31
Dec 2024	11	16	3	30
Jan 2025	15	12	1	28
Feb 2025	38	10	6	54
Mar 2025	16	13	0	29
Apr 2025	20	19	3	42
May 2025	30	2	3	35
Jun 2025	45	14	1	60
Jul 2025	35	14	1	50
Aug 2025	33	10	0	43
Sep 2025	50	9	2	61
Oct 2025	21	22	2	45
Nov 2025	28	25	4	57
Dec 2025	2	5	0	7

Cumulative views and downloads (calculated since 28 Apr 2016)

Month	HTML	PDF	XML	Total
Apr 2016	132	50	1	183
May 2016	73	38	3	114
Jun 2016	22	17	0	39
Jul 2016	9	5	1	15
Aug 2016	15	6	1	22
Sep 2016	3	3	0	6
Oct 2016	123	54	5	182
Nov 2016	21	14	5	40
Dec 2016	15	5	0	20
Jan 2017	32	12	4	48
Feb 2017	26	7	0	33
Mar 2017	45	19	3	67
Apr 2017	36	19	1	56
May 2017	34	19	2	55
Jun 2017	29	10	2	41
Jul 2017	19	10	1	30
Aug 2017	12	11	0	23
Sep 2017	17	12	1	30
Oct 2017	18	9	1	28
Nov 2017	17	9	2	28
Dec 2017	10	8	1	19
Jan 2018	14	8	0	22
Feb 2018	15	12	1	28
Mar 2018	12	6	1	19
Apr 2018	11	9	2	22
May 2018	12	8	6	26
Jun 2018	7	10	1	18
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Aug 2018	21	5	0	26
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Oct 2018	19	9	3	31
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May 2021	15	11	1	27
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Aug 2021	9	7	0	16
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Nov 2022	18	7	0	25
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Jan 2023	18	22	2	42
Feb 2023	14	8	0	22
Mar 2023	19	9	0	28
Apr 2023	6	6	0	12
May 2023	32	6	0	38
Jun 2023	49	10	1	60
Jul 2023	35	5	1	41
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Oct 2023	42	9	1	52
Nov 2023	24	3	0	27
Dec 2023	42	8	3	53
Jan 2024	44	8	1	53
Feb 2024	41	8	0	49
Mar 2024	47	18	5	70
Apr 2024	43	14	4	61
May 2024	18	16	2	36
Jun 2024	16	11	2	29
Jul 2024	13	16	2	31
Aug 2024	26	10	1	37
Sep 2024	16	2	0	18
Oct 2024	19	5	0	24
Nov 2024	19	10	2	31
Dec 2024	11	16	3	30
Jan 2025	15	12	1	28
Feb 2025	38	10	6	54
Mar 2025	16	13	0	29
Apr 2025	20	19	3	42
May 2025	30	2	3	35
Jun 2025	45	14	1	60
Jul 2025	35	14	1	50
Aug 2025	33	10	0	43
Sep 2025	50	9	2	61
Oct 2025	21	22	2	45
Nov 2025	28	25	4	57
Dec 2025	2	5	0	7

Latest update: 06 Dec 2025

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Discontinuities in apparent hygroscopicity below and above water saturation have been observed for organic and mixed organic-inorganic aerosol particles in both laboratory studies and in the ambient atmosphere. This work explores the extent to which such discontinuities are influenced by organic component molecular mass and viscosity, non-ideal thermodynamic interactions between aerosol components, and the combination of these factors.