Articles | Volume 16, issue 2
https://doi.org/10.5194/acp-16-1161-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-1161-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Iodine's impact on tropospheric oxidants: a global model study in GEOS-Chem
Wolfson Atmospheric Chemistry Laboratories (WACL), Department of Chemistry, University of York, York, YO10 5DD, UK
M. J. Evans
Wolfson Atmospheric Chemistry Laboratories (WACL), Department of Chemistry, University of York, York, YO10 5DD, UK
National Centre for Atmospheric Science (NCAS), University of York, York, YO10 5DD, UK
L. J. Carpenter
Wolfson Atmospheric Chemistry Laboratories (WACL), Department of Chemistry, University of York, York, YO10 5DD, UK
S. J. Andrews
Wolfson Atmospheric Chemistry Laboratories (WACL), Department of Chemistry, University of York, York, YO10 5DD, UK
R. T. Lidster
Wolfson Atmospheric Chemistry Laboratories (WACL), Department of Chemistry, University of York, York, YO10 5DD, UK
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO 80309-0215, USA
T. K. Koenig
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO 80309-0215, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309-021, USA
R. Sinreich
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO 80309-0215, USA
I. Ortega
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO 80309-0215, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309-021, USA
R. Volkamer
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO 80309-0215, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309-021, USA
A. Saiz-Lopez
Department of Atmospheric Chemistry and Climate, Institute of Physical Chemistry Rocasolano, CSIC, Madrid, 28006, Spain
C. Prados-Roman
Department of Atmospheric Chemistry and Climate, Institute of Physical Chemistry Rocasolano, CSIC, Madrid, 28006, Spain
A. S. Mahajan
Indian Institute of Tropical Meteorology, Maharashtra, 411008, India
C. Ordóñez
Met Office, FitzRoy Road, Exeter, EX1 3PB, UK
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- Potential controls of isoprene in the surface ocean S. Hackenberg et al. 10.1002/2016GB005531
- Impacts of ocean biogeochemistry on atmospheric chemistry L. Tinel et al. 10.1525/elementa.2023.00032
- Alpine ice evidence of a three-fold increase in atmospheric iodine deposition since 1950 in Europe due to increasing oceanic emissions M. Legrand et al. 10.1073/pnas.1809867115
- Spatial and temporal variation of dissolved iodine in the eastern Arabian Sea A. Shaikh et al. 10.1016/j.marchem.2023.104322
- Global impacts of tropospheric halogens (Cl, Br, I) on oxidants and composition in GEOS-Chem T. Sherwen et al. 10.5194/acp-16-12239-2016
- Quantitative detection of iodine in the stratosphere T. Koenig et al. 10.1073/pnas.1916828117
- Influences of oceanic ozone deposition on tropospheric photochemistry R. Pound et al. 10.5194/acp-20-4227-2020
- Marine iodine emissions in a changing world L. Carpenter et al. 10.1098/rspa.2020.0824
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Using a global chemical transport model (GEOS-Chem) with additional iodine emissions, chemistry, and deposition we show that iodine is responsible for ~ 9 % of global ozone loss but has negligible impacts on global OH. Uncertainties are large in the chemistry and emissions and future research is needed in both. Measurements of iodine species (especially HOI) would be useful. We believe iodine chemistry should be considered in future chemistry-climate and in air quality modelling.
Using a global chemical transport model (GEOS-Chem) with additional iodine emissions, chemistry,...
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