Articles | Volume 16, issue 2
Atmos. Chem. Phys., 16, 1161–1186, 2016
https://doi.org/10.5194/acp-16-1161-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Special issue: Marine trace gases and aerosols over tropical oceans (AMT/ACP...
Research article
02 Feb 2016
Research article
| 02 Feb 2016
Iodine's impact on tropospheric oxidants: a global model study in GEOS-Chem
T. Sherwen et al.
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Cited
71 citations as recorded by crossref.
- Global impacts of tropospheric halogens (Cl, Br, I) on oxidants and composition in GEOS-Chem T. Sherwen et al. 10.5194/acp-16-12239-2016
- Quantitative detection of iodine in the stratosphere T. Koenig et al. 10.1073/pnas.1916828117
- Influences of oceanic ozone deposition on tropospheric photochemistry R. Pound et al. 10.5194/acp-20-4227-2020
- Evidence for renoxification in the tropical marine boundary layer C. Reed et al. 10.5194/acp-17-4081-2017
- Marine iodine emissions in a changing world L. Carpenter et al. 10.1098/rspa.2020.0824
- Modelling the impacts of iodine chemistry on the northern Indian Ocean marine boundary layer A. Mahajan et al. 10.5194/acp-21-8437-2021
- Tropospheric Ozone Assessment Report: Assessment of global-scale model performance for global and regional ozone distributions, variability, and trends P. Young et al. 10.1525/elementa.265
- The potential role of kelp forests on iodine speciation in coastal seawater J. Gonzales et al. 10.1371/journal.pone.0180755
- Determination of the absorption cross sections of higher-order iodine oxides at 355 and 532 nm T. Lewis et al. 10.5194/acp-20-10865-2020
- Iodine chemistry in the chemistry–climate model SOCOL-AERv2-I A. Karagodin-Doyennel et al. 10.5194/gmd-14-6623-2021
- Climate changes modulated the history of Arctic iodine during the Last Glacial Cycle J. Corella et al. 10.1038/s41467-021-27642-5
- Observations of iodine oxide in the Indian Ocean marine boundary layer: A transect from the tropics to the high latitudes A. Mahajan et al. 10.1016/j.aeaoa.2019.100016
- Interferences in photolytic NO<sub>2</sub> measurements: explanation for an apparent missing oxidant? C. Reed et al. 10.5194/acp-16-4707-2016
- Improving the prediction of an atmospheric chemistry transport model using gradient-boosted regression trees P. Ivatt & M. Evans 10.5194/acp-20-8063-2020
- A Global Model for Iodine Speciation in the Upper Ocean M. Wadley et al. 10.1029/2019GB006467
- Parameterization retrieval of trace gas volume mixing ratios from Airborne MAX-DOAS B. Dix et al. 10.5194/amt-9-5655-2016
- Effects of Sea Salt Aerosol Emissions for Marine Cloud Brightening on Atmospheric Chemistry: Implications for Radiative Forcing H. Horowitz et al. 10.1029/2019GL085838
- An improved parameterisation of ozone dry deposition to the ocean and its impact in a global climate–chemistry model A. Luhar et al. 10.5194/acp-17-3749-2017
- Understanding Iodine Chemistry Over the Northern and Equatorial Indian Ocean A. Mahajan et al. 10.1029/2018JD029063
- Impacts of global NO<sub><i>x</i></sub> inversions on NO<sub>2</sub> and ozone simulations Z. Qu et al. 10.5194/acp-20-13109-2020
- Tropospheric Ozone Assessment Report A. Archibald et al. 10.1525/elementa.2020.034
- Direct field evidence of autocatalytic iodine release from atmospheric aerosol Y. Tham et al. 10.1073/pnas.2009951118
- Global Bromine- and Iodine-Mediated Tropospheric Ozone Loss Estimated Using the CHASER Chemical Transport Model T. Sekiya et al. 10.2151/sola.2020-037
- Halogen chemistry reduces tropospheric O<sub>3</sub> radiative forcing T. Sherwen et al. 10.5194/acp-17-1557-2017
- Importance of reactive halogens in the tropical marine atmosphere: a regional modelling study using WRF-Chem A. Badia et al. 10.5194/acp-19-3161-2019
- Quantifying Nitrate Formation Pathways in the Equatorial Pacific Atmosphere from the GEOTRACES Peru-Tahiti Transect T. Carter et al. 10.1021/acsearthspacechem.1c00072
- Influence of the Sea Surface Microlayer on Oceanic Iodine Emissions L. Tinel et al. 10.1021/acs.est.0c02736
- Senescence as the main driver of iodide release from a diverse range of marine phytoplankton H. Hepach et al. 10.5194/bg-17-2453-2020
- Spatial and Temporal Variability of Iodine in Aerosol J. Gómez Martín et al. 10.1029/2020JD034410
- Nighttime atmospheric chemistry of iodine A. Saiz-Lopez et al. 10.5194/acp-16-15593-2016
- Evaluating the impact of blowing-snow sea salt aerosol on springtime BrO and O<sub>3</sub> in the Arctic J. Huang et al. 10.5194/acp-20-7335-2020
- Estimation of reactive inorganic iodine fluxes in the Indian and Southern Ocean marine boundary layer S. Inamdar et al. 10.5194/acp-20-12093-2020
- GEOS-Chem High Performance (GCHP v11-02c): a next-generation implementation of the GEOS-Chem chemical transport model for massively parallel applications S. Eastham et al. 10.5194/gmd-11-2941-2018
- The role of chlorine in global tropospheric chemistry X. Wang et al. 10.5194/acp-19-3981-2019
- Ozone and carbon monoxide observations over open oceans on R/V <i>Mirai</i> from 67° S to 75° N during 2012 to 2017: testing global chemical reanalysis in terms of Arctic processes, low ozone levels at low latitudes, and pollution transport Y. Kanaya et al. 10.5194/acp-19-7233-2019
- Modeling the observed tropospheric BrO background: Importance of multiphase chemistry and implications for ozone, OH, and mercury J. Schmidt et al. 10.1002/2015JD024229
- Global impact of nitrate photolysis in sea-salt aerosol on NO<sub><i>x</i></sub>, OH, and O<sub>3</sub> in the marine boundary layer P. Kasibhatla et al. 10.5194/acp-18-11185-2018
- Regional Characteristics of Atmospheric Sulfate Formation in East Antarctica Imprinted on 17 O‐Excess Signature S. Ishino et al. 10.1029/2020JD033583
- Halogens in Seaweeds: Biological and Environmental Significance H. Al-Adilah et al. 10.3390/phycology2010009
- Iodine Catalyzed Ozone Destruction at the Texas Coast and Gulf of Mexico K. Tuite et al. 10.1029/2018GL078267
- Seasonal and geographical variability of nitryl chloride and its precursors in Northern Europe R. Sommariva et al. 10.1002/asl.844
- Effects of nutrient deficiency on the CH2I2, CH2ClI, and CH2BrI production in cultures of the temperate marine phytoplankton Bigelowiella natans M. Abe et al. 10.1016/j.marchem.2020.103765
- Rapid increase in atmospheric iodine levels in the North Atlantic since the mid-20th century C. Cuevas et al. 10.1038/s41467-018-03756-1
- Measurement of iodine species and sulfuric acid using bromide chemical ionization mass spectrometers M. Wang et al. 10.5194/amt-14-4187-2021
- Harmonized Emissions Component (HEMCO) 3.0 as a versatile emissions component for atmospheric models: application in the GEOS-Chem, NASA GEOS, WRF-GC, CESM2, NOAA GEFS-Aerosol, and NOAA UFS models H. Lin et al. 10.5194/gmd-14-5487-2021
- Coordinated Airborne Studies in the Tropics (CAST) N. Harris et al. 10.1175/BAMS-D-14-00290.1
- Theoretical treatment of IO–X (X = N2, CO, CO2, H2O) complexes S. Marzouk et al. 10.1039/D1CP05536D
- Global modeling of tropospheric iodine aerosol T. Sherwen et al. 10.1002/2016GL070062
- Oxidation of iodide to iodate by cultures of marine ammonia-oxidising bacteria C. Hughes et al. 10.1016/j.marchem.2021.104000
- A machine-learning-based global sea-surface iodide distribution T. Sherwen et al. 10.5194/essd-11-1239-2019
- Global budget of atmospheric 129I during 2007–2010 estimated by a chemical transport model: GEARN–FDM M. Kadowaki et al. 10.1016/j.aeaoa.2020.100098
- Global tropospheric halogen (Cl, Br, I) chemistry and its impact on oxidants X. Wang et al. 10.5194/acp-21-13973-2021
- Global sea-surface iodide observations, 1967–2018 R. Chance et al. 10.1038/s41597-019-0288-y
- Impact of uncertainties in inorganic chemical rate constants on tropospheric composition and ozone radiative forcing B. Newsome & M. Evans 10.5194/acp-17-14333-2017
- The Global Budget of Atmospheric Methanol: New Constraints on Secondary, Oceanic, and Terrestrial Sources K. Bates et al. 10.1029/2020JD033439
- Influence of bromine and iodine chemistry on annual, seasonal, diurnal, and background ozone: CMAQ simulations over the Northern Hemisphere G. Sarwar et al. 10.1016/j.atmosenv.2019.06.020
- Box modelling of gas-phase atmospheric iodine chemical reactivity in case of a nuclear accident C. Fortin et al. 10.1016/j.atmosenv.2019.116838
- Threshold Photoelectron Spectroscopy of IO and HOI D. Schleier et al. 10.1002/cphc.201900813
- Global simulation of tropospheric chemistry at 12.5 km resolution: performance and evaluation of the GEOS-Chem chemical module (v10-1) within the NASA GEOS Earth system model (GEOS-5 ESM) L. Hu et al. 10.5194/gmd-11-4603-2018
- Chemical Interactions Between Ship‐Originated Air Pollutants and Ocean‐Emitted Halogens Q. Li et al. 10.1029/2020JD034175
- Global budget of tropospheric ozone: Evaluating recent model advances with satellite (OMI), aircraft (IAGOS), and ozonesonde observations L. Hu et al. 10.1016/j.atmosenv.2017.08.036
- A gas-to-particle conversion mechanism helps to explain atmospheric particle formation through clustering of iodine oxides J. Gómez Martín et al. 10.1038/s41467-020-18252-8
- Ozone depletion due to dust release of iodine in the free troposphere T. Koenig et al. 10.1126/sciadv.abj6544
- Impacts of bromine and iodine chemistry on tropospheric OH and HO<sub>2</sub>: comparing observations with box and global model perspectives D. Stone et al. 10.5194/acp-18-3541-2018
- Potential controls of isoprene in the surface ocean S. Hackenberg et al. 10.1002/2016GB005531
- Alpine ice evidence of a three-fold increase in atmospheric iodine deposition since 1950 in Europe due to increasing oceanic emissions M. Legrand et al. 10.1073/pnas.1809867115
- Technical note: Examining ozone deposition over seawater G. Sarwar et al. 10.1016/j.atmosenv.2016.06.072
- Effects of halogens on European air-quality T. Sherwen et al. 10.1039/C7FD00026J
- Role of Iodine Recycling on Sea‐Salt Aerosols in the Global Marine Boundary Layer Q. Li et al. 10.1029/2021GL097567
- Atmospheric ethanol in London and the potential impacts of future fuel formulations R. Dunmore et al. 10.1039/C5FD00190K
- A nocturnal atmospheric loss of CH2I2 in the remote marine boundary layer L. Carpenter et al. 10.1007/s10874-015-9320-6
69 citations as recorded by crossref.
- Global impacts of tropospheric halogens (Cl, Br, I) on oxidants and composition in GEOS-Chem T. Sherwen et al. 10.5194/acp-16-12239-2016
- Quantitative detection of iodine in the stratosphere T. Koenig et al. 10.1073/pnas.1916828117
- Influences of oceanic ozone deposition on tropospheric photochemistry R. Pound et al. 10.5194/acp-20-4227-2020
- Evidence for renoxification in the tropical marine boundary layer C. Reed et al. 10.5194/acp-17-4081-2017
- Marine iodine emissions in a changing world L. Carpenter et al. 10.1098/rspa.2020.0824
- Modelling the impacts of iodine chemistry on the northern Indian Ocean marine boundary layer A. Mahajan et al. 10.5194/acp-21-8437-2021
- Tropospheric Ozone Assessment Report: Assessment of global-scale model performance for global and regional ozone distributions, variability, and trends P. Young et al. 10.1525/elementa.265
- The potential role of kelp forests on iodine speciation in coastal seawater J. Gonzales et al. 10.1371/journal.pone.0180755
- Determination of the absorption cross sections of higher-order iodine oxides at 355 and 532 nm T. Lewis et al. 10.5194/acp-20-10865-2020
- Iodine chemistry in the chemistry–climate model SOCOL-AERv2-I A. Karagodin-Doyennel et al. 10.5194/gmd-14-6623-2021
- Climate changes modulated the history of Arctic iodine during the Last Glacial Cycle J. Corella et al. 10.1038/s41467-021-27642-5
- Observations of iodine oxide in the Indian Ocean marine boundary layer: A transect from the tropics to the high latitudes A. Mahajan et al. 10.1016/j.aeaoa.2019.100016
- Interferences in photolytic NO<sub>2</sub> measurements: explanation for an apparent missing oxidant? C. Reed et al. 10.5194/acp-16-4707-2016
- Improving the prediction of an atmospheric chemistry transport model using gradient-boosted regression trees P. Ivatt & M. Evans 10.5194/acp-20-8063-2020
- A Global Model for Iodine Speciation in the Upper Ocean M. Wadley et al. 10.1029/2019GB006467
- Parameterization retrieval of trace gas volume mixing ratios from Airborne MAX-DOAS B. Dix et al. 10.5194/amt-9-5655-2016
- Effects of Sea Salt Aerosol Emissions for Marine Cloud Brightening on Atmospheric Chemistry: Implications for Radiative Forcing H. Horowitz et al. 10.1029/2019GL085838
- An improved parameterisation of ozone dry deposition to the ocean and its impact in a global climate–chemistry model A. Luhar et al. 10.5194/acp-17-3749-2017
- Understanding Iodine Chemistry Over the Northern and Equatorial Indian Ocean A. Mahajan et al. 10.1029/2018JD029063
- Impacts of global NO<sub><i>x</i></sub> inversions on NO<sub>2</sub> and ozone simulations Z. Qu et al. 10.5194/acp-20-13109-2020
- Tropospheric Ozone Assessment Report A. Archibald et al. 10.1525/elementa.2020.034
- Direct field evidence of autocatalytic iodine release from atmospheric aerosol Y. Tham et al. 10.1073/pnas.2009951118
- Global Bromine- and Iodine-Mediated Tropospheric Ozone Loss Estimated Using the CHASER Chemical Transport Model T. Sekiya et al. 10.2151/sola.2020-037
- Halogen chemistry reduces tropospheric O<sub>3</sub> radiative forcing T. Sherwen et al. 10.5194/acp-17-1557-2017
- Importance of reactive halogens in the tropical marine atmosphere: a regional modelling study using WRF-Chem A. Badia et al. 10.5194/acp-19-3161-2019
- Quantifying Nitrate Formation Pathways in the Equatorial Pacific Atmosphere from the GEOTRACES Peru-Tahiti Transect T. Carter et al. 10.1021/acsearthspacechem.1c00072
- Influence of the Sea Surface Microlayer on Oceanic Iodine Emissions L. Tinel et al. 10.1021/acs.est.0c02736
- Senescence as the main driver of iodide release from a diverse range of marine phytoplankton H. Hepach et al. 10.5194/bg-17-2453-2020
- Spatial and Temporal Variability of Iodine in Aerosol J. Gómez Martín et al. 10.1029/2020JD034410
- Nighttime atmospheric chemistry of iodine A. Saiz-Lopez et al. 10.5194/acp-16-15593-2016
- Evaluating the impact of blowing-snow sea salt aerosol on springtime BrO and O<sub>3</sub> in the Arctic J. Huang et al. 10.5194/acp-20-7335-2020
- Estimation of reactive inorganic iodine fluxes in the Indian and Southern Ocean marine boundary layer S. Inamdar et al. 10.5194/acp-20-12093-2020
- GEOS-Chem High Performance (GCHP v11-02c): a next-generation implementation of the GEOS-Chem chemical transport model for massively parallel applications S. Eastham et al. 10.5194/gmd-11-2941-2018
- The role of chlorine in global tropospheric chemistry X. Wang et al. 10.5194/acp-19-3981-2019
- Ozone and carbon monoxide observations over open oceans on R/V <i>Mirai</i> from 67° S to 75° N during 2012 to 2017: testing global chemical reanalysis in terms of Arctic processes, low ozone levels at low latitudes, and pollution transport Y. Kanaya et al. 10.5194/acp-19-7233-2019
- Modeling the observed tropospheric BrO background: Importance of multiphase chemistry and implications for ozone, OH, and mercury J. Schmidt et al. 10.1002/2015JD024229
- Global impact of nitrate photolysis in sea-salt aerosol on NO<sub><i>x</i></sub>, OH, and O<sub>3</sub> in the marine boundary layer P. Kasibhatla et al. 10.5194/acp-18-11185-2018
- Regional Characteristics of Atmospheric Sulfate Formation in East Antarctica Imprinted on 17 O‐Excess Signature S. Ishino et al. 10.1029/2020JD033583
- Halogens in Seaweeds: Biological and Environmental Significance H. Al-Adilah et al. 10.3390/phycology2010009
- Iodine Catalyzed Ozone Destruction at the Texas Coast and Gulf of Mexico K. Tuite et al. 10.1029/2018GL078267
- Seasonal and geographical variability of nitryl chloride and its precursors in Northern Europe R. Sommariva et al. 10.1002/asl.844
- Effects of nutrient deficiency on the CH2I2, CH2ClI, and CH2BrI production in cultures of the temperate marine phytoplankton Bigelowiella natans M. Abe et al. 10.1016/j.marchem.2020.103765
- Rapid increase in atmospheric iodine levels in the North Atlantic since the mid-20th century C. Cuevas et al. 10.1038/s41467-018-03756-1
- Measurement of iodine species and sulfuric acid using bromide chemical ionization mass spectrometers M. Wang et al. 10.5194/amt-14-4187-2021
- Harmonized Emissions Component (HEMCO) 3.0 as a versatile emissions component for atmospheric models: application in the GEOS-Chem, NASA GEOS, WRF-GC, CESM2, NOAA GEFS-Aerosol, and NOAA UFS models H. Lin et al. 10.5194/gmd-14-5487-2021
- Coordinated Airborne Studies in the Tropics (CAST) N. Harris et al. 10.1175/BAMS-D-14-00290.1
- Theoretical treatment of IO–X (X = N2, CO, CO2, H2O) complexes S. Marzouk et al. 10.1039/D1CP05536D
- Global modeling of tropospheric iodine aerosol T. Sherwen et al. 10.1002/2016GL070062
- Oxidation of iodide to iodate by cultures of marine ammonia-oxidising bacteria C. Hughes et al. 10.1016/j.marchem.2021.104000
- A machine-learning-based global sea-surface iodide distribution T. Sherwen et al. 10.5194/essd-11-1239-2019
- Global budget of atmospheric 129I during 2007–2010 estimated by a chemical transport model: GEARN–FDM M. Kadowaki et al. 10.1016/j.aeaoa.2020.100098
- Global tropospheric halogen (Cl, Br, I) chemistry and its impact on oxidants X. Wang et al. 10.5194/acp-21-13973-2021
- Global sea-surface iodide observations, 1967–2018 R. Chance et al. 10.1038/s41597-019-0288-y
- Impact of uncertainties in inorganic chemical rate constants on tropospheric composition and ozone radiative forcing B. Newsome & M. Evans 10.5194/acp-17-14333-2017
- The Global Budget of Atmospheric Methanol: New Constraints on Secondary, Oceanic, and Terrestrial Sources K. Bates et al. 10.1029/2020JD033439
- Influence of bromine and iodine chemistry on annual, seasonal, diurnal, and background ozone: CMAQ simulations over the Northern Hemisphere G. Sarwar et al. 10.1016/j.atmosenv.2019.06.020
- Box modelling of gas-phase atmospheric iodine chemical reactivity in case of a nuclear accident C. Fortin et al. 10.1016/j.atmosenv.2019.116838
- Threshold Photoelectron Spectroscopy of IO and HOI D. Schleier et al. 10.1002/cphc.201900813
- Global simulation of tropospheric chemistry at 12.5 km resolution: performance and evaluation of the GEOS-Chem chemical module (v10-1) within the NASA GEOS Earth system model (GEOS-5 ESM) L. Hu et al. 10.5194/gmd-11-4603-2018
- Chemical Interactions Between Ship‐Originated Air Pollutants and Ocean‐Emitted Halogens Q. Li et al. 10.1029/2020JD034175
- Global budget of tropospheric ozone: Evaluating recent model advances with satellite (OMI), aircraft (IAGOS), and ozonesonde observations L. Hu et al. 10.1016/j.atmosenv.2017.08.036
- A gas-to-particle conversion mechanism helps to explain atmospheric particle formation through clustering of iodine oxides J. Gómez Martín et al. 10.1038/s41467-020-18252-8
- Ozone depletion due to dust release of iodine in the free troposphere T. Koenig et al. 10.1126/sciadv.abj6544
- Impacts of bromine and iodine chemistry on tropospheric OH and HO<sub>2</sub>: comparing observations with box and global model perspectives D. Stone et al. 10.5194/acp-18-3541-2018
- Potential controls of isoprene in the surface ocean S. Hackenberg et al. 10.1002/2016GB005531
- Alpine ice evidence of a three-fold increase in atmospheric iodine deposition since 1950 in Europe due to increasing oceanic emissions M. Legrand et al. 10.1073/pnas.1809867115
- Technical note: Examining ozone deposition over seawater G. Sarwar et al. 10.1016/j.atmosenv.2016.06.072
- Effects of halogens on European air-quality T. Sherwen et al. 10.1039/C7FD00026J
- Role of Iodine Recycling on Sea‐Salt Aerosols in the Global Marine Boundary Layer Q. Li et al. 10.1029/2021GL097567
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Using a global chemical transport model (GEOS-Chem) with additional iodine emissions, chemistry, and deposition we show that iodine is responsible for ~ 9 % of global ozone loss but has negligible impacts on global OH. Uncertainties are large in the chemistry and emissions and future research is needed in both. Measurements of iodine species (especially HOI) would be useful. We believe iodine chemistry should be considered in future chemistry-climate and in air quality modelling.
Using a global chemical transport model (GEOS-Chem) with additional iodine emissions, chemistry,...
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