Articles | Volume 16, issue 2
https://doi.org/10.5194/acp-16-1161-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-1161-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
02 Feb 2016
Research article |
| 02 Feb 2016
Iodine's impact on tropospheric oxidants: a global model study in GEOS-Chem
Wolfson Atmospheric Chemistry Laboratories (WACL), Department of Chemistry, University of York, York, YO10 5DD, UK
M. J. Evans
Wolfson Atmospheric Chemistry Laboratories (WACL), Department of Chemistry, University of York, York, YO10 5DD, UK
National Centre for Atmospheric Science (NCAS), University of York, York, YO10 5DD, UK
L. J. Carpenter
Wolfson Atmospheric Chemistry Laboratories (WACL), Department of Chemistry, University of York, York, YO10 5DD, UK
S. J. Andrews
Wolfson Atmospheric Chemistry Laboratories (WACL), Department of Chemistry, University of York, York, YO10 5DD, UK
R. T. Lidster
Wolfson Atmospheric Chemistry Laboratories (WACL), Department of Chemistry, University of York, York, YO10 5DD, UK
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO 80309-0215, USA
T. K. Koenig
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO 80309-0215, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309-021, USA
R. Sinreich
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO 80309-0215, USA
I. Ortega
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO 80309-0215, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309-021, USA
R. Volkamer
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO 80309-0215, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309-021, USA
A. Saiz-Lopez
Department of Atmospheric Chemistry and Climate, Institute of Physical Chemistry Rocasolano, CSIC, Madrid, 28006, Spain
C. Prados-Roman
Department of Atmospheric Chemistry and Climate, Institute of Physical Chemistry Rocasolano, CSIC, Madrid, 28006, Spain
A. S. Mahajan
Indian Institute of Tropical Meteorology, Maharashtra, 411008, India
C. Ordóñez
Met Office, FitzRoy Road, Exeter, EX1 3PB, UK
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- Modelling the impacts of iodine chemistry on the northern Indian Ocean marine boundary layer A. Mahajan et al. 10.5194/acp-21-8437-2021
- The potential role of kelp forests on iodine speciation in coastal seawater J. Gonzales et al. 10.1371/journal.pone.0180755
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- A Global Model for Iodine Speciation in the Upper Ocean M. Wadley et al. 10.1029/2019GB006467
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- Fundamental oxidation processes in the remote marine atmosphere investigated using the NO–NO2–O3 photostationary state S. Andersen et al. 10.5194/acp-22-15747-2022
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- Estimation of reactive inorganic iodine fluxes in the Indian and Southern Ocean marine boundary layer S. Inamdar et al. 10.5194/acp-20-12093-2020
- Characterisation of gaseous iodine species detection using the multi-scheme chemical ionisation inlet 2 with bromide and nitrate chemical ionisation methods X. He et al. 10.5194/amt-16-4461-2023
- Intercomparison of GEOS-Chem and CAM-chem tropospheric oxidant chemistry within the Community Earth System Model version 2 (CESM2) H. Lin et al. 10.5194/acp-24-8607-2024
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- Abiotic Emission of Volatile Organic Compounds from the Ocean Surface: Relationship to Seawater Composition S. Schneider et al. 10.1021/acsearthspacechem.4c00163
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- Theoretical treatment of IO–X (X = N2, CO, CO2, H2O) complexes S. Marzouk et al. 10.1039/D1CP05536D
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- Clumped‐Isotope Constraint on Upper‐Tropospheric Cooling During the Last Glacial Maximum A. Banerjee et al. 10.1029/2022AV000688
- Global budget of tropospheric ozone: Evaluating recent model advances with satellite (OMI), aircraft (IAGOS), and ozonesonde observations L. Hu et al. 10.1016/j.atmosenv.2017.08.036
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- Source Sector Mitigation of Solar Energy Generation Losses Attributable to Particulate Matter Pollution F. Yao & P. Palmer 10.1021/acs.est.2c01175
- Sensitivity of tropospheric ozone to halogen chemistry in the chemistry–climate model LMDZ-INCA vNMHC C. Caram et al. 10.5194/gmd-16-4041-2023
- Potential controls of isoprene in the surface ocean S. Hackenberg et al. 10.1002/2016GB005531
- Impacts of ocean biogeochemistry on atmospheric chemistry L. Tinel et al. 10.1525/elementa.2023.00032
- Alpine ice evidence of a three-fold increase in atmospheric iodine deposition since 1950 in Europe due to increasing oceanic emissions M. Legrand et al. 10.1073/pnas.1809867115
- Spatial and temporal variation of dissolved iodine in the eastern Arabian Sea A. Shaikh et al. 10.1016/j.marchem.2023.104322
- Global impacts of tropospheric halogens (Cl, Br, I) on oxidants and composition in GEOS-Chem T. Sherwen et al. 10.5194/acp-16-12239-2016
- Quantitative detection of iodine in the stratosphere T. Koenig et al. 10.1073/pnas.1916828117
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- Marine iodine emissions in a changing world L. Carpenter et al. 10.1098/rspa.2020.0824
- Tropospheric Ozone Assessment Report: Assessment of global-scale model performance for global and regional ozone distributions, variability, and trends P. Young et al. 10.1525/elementa.265
- Iodine Activation from Iodate Reduction in Aqueous Films via Photocatalyzed and Dark Reactions M. Reza et al. 10.1021/acsearthspacechem.4c00224
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- Key role of short-lived halogens on global atmospheric oxidation during historical periods A. Bossolasco et al. 10.1039/D4EA00141A
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102 citations as recorded by crossref.
- NASA GEOS Composition Forecast Modeling System GEOS‐CF v1.0: Stratospheric Composition K. Knowland et al. 10.1029/2021MS002852
- Evidence for renoxification in the tropical marine boundary layer C. Reed et al. 10.5194/acp-17-4081-2017
- Modelling the impacts of iodine chemistry on the northern Indian Ocean marine boundary layer A. Mahajan et al. 10.5194/acp-21-8437-2021
- The potential role of kelp forests on iodine speciation in coastal seawater J. Gonzales et al. 10.1371/journal.pone.0180755
- Determination of the absorption cross sections of higher-order iodine oxides at 355 and 532 nm T. Lewis et al. 10.5194/acp-20-10865-2020
- Iodine chemistry in the chemistry–climate model SOCOL-AERv2-I A. Karagodin-Doyennel et al. 10.5194/gmd-14-6623-2021
- Climate changes modulated the history of Arctic iodine during the Last Glacial Cycle J. Corella et al. 10.1038/s41467-021-27642-5
- Observations of iodine oxide in the Indian Ocean marine boundary layer: A transect from the tropics to the high latitudes A. Mahajan et al. 10.1016/j.aeaoa.2019.100016
- Improving the prediction of an atmospheric chemistry transport model using gradient-boosted regression trees P. Ivatt & M. Evans 10.5194/acp-20-8063-2020
- Potential deterioration of ozone pollution in coastal areas caused by marine-emitted halogens: A case study in the Guangdong-Hong Kong-Macao Greater Bay Area S. Fan & Y. Li 10.1016/j.scitotenv.2022.160456
- A Global Model for Iodine Speciation in the Upper Ocean M. Wadley et al. 10.1029/2019GB006467
- Parameterization retrieval of trace gas volume mixing ratios from Airborne MAX-DOAS B. Dix et al. 10.5194/amt-9-5655-2016
- Fundamental oxidation processes in the remote marine atmosphere investigated using the NO–NO2–O3 photostationary state S. Andersen et al. 10.5194/acp-22-15747-2022
- Field Evidence of Nocturnal Multiphase Production of Iodic Acid D. Li et al. 10.1021/acs.estlett.4c00244
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- Impacts of global NOx inversions on NO2 and ozone simulations Z. Qu et al. 10.5194/acp-20-13109-2020
- Direct field evidence of autocatalytic iodine release from atmospheric aerosol Y. Tham et al. 10.1073/pnas.2009951118
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- Influence of the Sea Surface Microlayer on Oceanic Iodine Emissions L. Tinel et al. 10.1021/acs.est.0c02736
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- Nighttime atmospheric chemistry of iodine A. Saiz-Lopez et al. 10.5194/acp-16-15593-2016
- Evaluating the impact of blowing-snow sea salt aerosol on springtime BrO and O3 in the Arctic J. Huang et al. 10.5194/acp-20-7335-2020
- Estimation of reactive inorganic iodine fluxes in the Indian and Southern Ocean marine boundary layer S. Inamdar et al. 10.5194/acp-20-12093-2020
- Characterisation of gaseous iodine species detection using the multi-scheme chemical ionisation inlet 2 with bromide and nitrate chemical ionisation methods X. He et al. 10.5194/amt-16-4461-2023
- Intercomparison of GEOS-Chem and CAM-chem tropospheric oxidant chemistry within the Community Earth System Model version 2 (CESM2) H. Lin et al. 10.5194/acp-24-8607-2024
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- Regional Characteristics of Atmospheric Sulfate Formation in East Antarctica Imprinted on 17O‐Excess Signature S. Ishino et al. 10.1029/2020JD033583
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- Abiotic Emission of Volatile Organic Compounds from the Ocean Surface: Relationship to Seawater Composition S. Schneider et al. 10.1021/acsearthspacechem.4c00163
- Rapid increase in atmospheric iodine levels in the North Atlantic since the mid-20th century C. Cuevas et al. 10.1038/s41467-018-03756-1
- Measurement of iodine species and sulfuric acid using bromide chemical ionization mass spectrometers M. Wang et al. 10.5194/amt-14-4187-2021
- Harmonized Emissions Component (HEMCO) 3.0 as a versatile emissions component for atmospheric models: application in the GEOS-Chem, NASA GEOS, WRF-GC, CESM2, NOAA GEFS-Aerosol, and NOAA UFS models H. Lin et al. 10.5194/gmd-14-5487-2021
- Theoretical treatment of IO–X (X = N2, CO, CO2, H2O) complexes S. Marzouk et al. 10.1039/D1CP05536D
- Opinion: Stratospheric ozone – depletion, recovery and new challenges M. Chipperfield & S. Bekki 10.5194/acp-24-2783-2024
- A machine-learning-based global sea-surface iodide distribution T. Sherwen et al. 10.5194/essd-11-1239-2019
- Distinguishing Surface and Bulk Reactivity: Concentration-Dependent Kinetics of Iodide Oxidation by Ozone in Microdroplets A. Prophet et al. 10.1021/acs.jpca.4c05129
- Global tropospheric halogen (Cl, Br, I) chemistry and its impact on oxidants X. Wang et al. 10.5194/acp-21-13973-2021
- Global sea-surface iodide observations, 1967–2018 R. Chance et al. 10.1038/s41597-019-0288-y
- Influence of bromine and iodine chemistry on annual, seasonal, diurnal, and background ozone: CMAQ simulations over the Northern Hemisphere G. Sarwar et al. 10.1016/j.atmosenv.2019.06.020
- Clumped‐Isotope Constraint on Upper‐Tropospheric Cooling During the Last Glacial Maximum A. Banerjee et al. 10.1029/2022AV000688
- Global budget of tropospheric ozone: Evaluating recent model advances with satellite (OMI), aircraft (IAGOS), and ozonesonde observations L. Hu et al. 10.1016/j.atmosenv.2017.08.036
- How do Cl concentrations matter for the simulation of CH4 and δ13C(CH4) and estimation of the CH4 budget through atmospheric inversions? J. Thanwerdas et al. 10.5194/acp-22-15489-2022
- Source Sector Mitigation of Solar Energy Generation Losses Attributable to Particulate Matter Pollution F. Yao & P. Palmer 10.1021/acs.est.2c01175
- Sensitivity of tropospheric ozone to halogen chemistry in the chemistry–climate model LMDZ-INCA vNMHC C. Caram et al. 10.5194/gmd-16-4041-2023
- Potential controls of isoprene in the surface ocean S. Hackenberg et al. 10.1002/2016GB005531
- Impacts of ocean biogeochemistry on atmospheric chemistry L. Tinel et al. 10.1525/elementa.2023.00032
- Alpine ice evidence of a three-fold increase in atmospheric iodine deposition since 1950 in Europe due to increasing oceanic emissions M. Legrand et al. 10.1073/pnas.1809867115
- Spatial and temporal variation of dissolved iodine in the eastern Arabian Sea A. Shaikh et al. 10.1016/j.marchem.2023.104322
- Global impacts of tropospheric halogens (Cl, Br, I) on oxidants and composition in GEOS-Chem T. Sherwen et al. 10.5194/acp-16-12239-2016
- Quantitative detection of iodine in the stratosphere T. Koenig et al. 10.1073/pnas.1916828117
- Influences of oceanic ozone deposition on tropospheric photochemistry R. Pound et al. 10.5194/acp-20-4227-2020
- Marine iodine emissions in a changing world L. Carpenter et al. 10.1098/rspa.2020.0824
- Tropospheric Ozone Assessment Report: Assessment of global-scale model performance for global and regional ozone distributions, variability, and trends P. Young et al. 10.1525/elementa.265
- Iodine Activation from Iodate Reduction in Aqueous Films via Photocatalyzed and Dark Reactions M. Reza et al. 10.1021/acsearthspacechem.4c00224
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Using a global chemical transport model (GEOS-Chem) with additional iodine emissions, chemistry, and deposition we show that iodine is responsible for ~ 9 % of global ozone loss but has negligible impacts on global OH. Uncertainties are large in the chemistry and emissions and future research is needed in both. Measurements of iodine species (especially HOI) would be useful. We believe iodine chemistry should be considered in future chemistry-climate and in air quality modelling.
Using a global chemical transport model (GEOS-Chem) with additional iodine emissions, chemistry,...
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