Articles | Volume 16, issue 2
https://doi.org/10.5194/acp-16-1139-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-1139-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
02 Feb 2016
Research article |
| 02 Feb 2016
Wintertime aerosol chemical composition, volatility, and spatial variability in the greater London area
School of Chemical and Biomolecular Engineering, Georgia Institute of Technology, Atlanta, GA, USA
L. R. Williams
Aerodyne Research Inc., Billerica, MA, USA
D. E. Young
School of Earth, Atmospheric and Environmental Sciences, University of Manchester, Manchester, UK
now at: Department of Environmental Toxicology, University of California, Davis, CA, USA
J. D. Allan
School of Earth, Atmospheric and Environmental Sciences, University of Manchester, Manchester, UK
National Centre for Atmospheric Science, University of Manchester, Manchester, UK
School of Earth, Atmospheric and Environmental Sciences, University of Manchester, Manchester, UK
P. Massoli
Aerodyne Research Inc., Billerica, MA, USA
E. Fortner
Aerodyne Research Inc., Billerica, MA, USA
P. Chhabra
Aerodyne Research Inc., Billerica, MA, USA
now at: PerkinElmer Inc., Hopkinton, MA, USA
S. Herndon
Aerodyne Research Inc., Billerica, MA, USA
W. A. Brooks
Aerodyne Research Inc., Billerica, MA, USA
J. T. Jayne
Aerodyne Research Inc., Billerica, MA, USA
D. R. Worsnop
Aerodyne Research Inc., Billerica, MA, USA
A. C. Aiken
Earth and Environmental Sciences Division, Los Alamos National Laboratory, Los Alamos, NM, USA
S. Liu
Earth and Environmental Sciences Division, Los Alamos National Laboratory, Los Alamos, NM, USA
now at: Cooperative Institute for Research in the Environmental Sciences, University of Colorado, Boulder, CO, USA
K. Gorkowski
Earth and Environmental Sciences Division, Los Alamos National Laboratory, Los Alamos, NM, USA
now at: Center for Atmospheric Particle Studies, Carnegie Mellon University, Pittsburgh, PA, USA
M. K. Dubey
Earth and Environmental Sciences Division, Los Alamos National Laboratory, Los Alamos, NM, USA
Z. L. Fleming
Department of Chemistry, University of Leicester, Leicester, UK
National Centre for Atmospheric Science, University of Leicester, Leicester, UK
S. Visser
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen, Switzerland
A. S. H. Prévôt
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen, Switzerland
School of Chemical and Biomolecular Engineering, Georgia Institute of Technology, Atlanta, GA, USA
School of Earth and Atmospheric Sciences, Georgia Institute of Technology, Atlanta, GA, USA
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27 citations as recorded by crossref.
- Simulating secondary organic aerosol from missing diesel-related intermediate-volatility organic compound emissions during the Clean Air for London (ClearfLo) campaign R. Ots et al. 10.5194/acp-16-6453-2016
- Organic aerosol volatility and viscosity in the North China Plain: contrast between summer and winter W. Xu et al. 10.5194/acp-21-5463-2021
- Volatility measurement of atmospheric submicron aerosols in an urban atmosphere in southern China L. Cao et al. 10.5194/acp-18-1729-2018
- Summertime aerosol volatility measurements in Beijing, China W. Xu et al. 10.5194/acp-19-10205-2019
- Molecular-Size-Separated Brown Carbon Absorption for Biomass-Burning Aerosol at Multiple Field Sites R. Di Lorenzo et al. 10.1021/acs.est.6b06160
- Estimation of particulate organic nitrates from thermodenuder–aerosol mass spectrometer measurements in the North China Plain W. Xu et al. 10.5194/amt-14-3693-2021
- Experimental and model estimates of the contributions from biogenic monoterpenes and sesquiterpenes to secondary organic aerosol in the southeastern United States L. Xu et al. 10.5194/acp-18-12613-2018
- Impact of aging on the sources, volatility, and viscosity of organic aerosols in Chinese outflows T. Feng et al. 10.5194/acp-23-611-2023
- Characterization of organic nitrate constituents of secondary organic aerosol (SOA) from nitrate-radical-initiated oxidation of limonene using high-resolution chemical ionization mass spectrometry C. Faxon et al. 10.5194/acp-18-5467-2018
- Quantifying the volatility of organic aerosol in the southeastern US P. Saha et al. 10.5194/acp-17-501-2017
- Characterization of submicron aerosol volatility in the regional atmosphere in Southern China L. Cao et al. 10.1016/j.chemosphere.2019.124383
- Secondary Organic Aerosol (SOA) from Nitrate Radical Oxidation of Monoterpenes: Effects of Temperature, Dilution, and Humidity on Aerosol Formation, Mixing, and Evaporation C. Boyd et al. 10.1021/acs.est.7b01460
- Particle detection using the dual-vaporizer configuration of the soot particle Aerosol Mass Spectrometer (SP-AMS) A. Avery et al. 10.1080/02786826.2020.1844132
- Evaluation of a New Aerosol Chemical Speciation Monitor (ACSM) System at an Urban Site in Atlanta, GA: The Use of Capture Vaporizer and PM2.5 Inlet T. Joo et al. 10.1021/acsearthspacechem.1c00173
- Colloidal associations of major and trace elements in the snow pack across a 2800-km south-north gradient of western Siberia I. Krickov et al. 10.1016/j.chemgeo.2022.121090
- Extreme air pollution from residential solid fuel burning C. Lin et al. 10.1038/s41893-018-0125-x
- Chemical Characterization of Water-Soluble Organic Aerosol in Contrasting Rural and Urban Environments in the Southeastern United States L. Xu et al. 10.1021/acs.est.6b05002
- An omnipresent diversity and variability in the chemical composition of atmospheric functionalized organic aerosol J. Ditto et al. 10.1038/s42004-018-0074-3
- Overview of the French Operational Network for In Situ Observation of PM Chemical Composition and Sources in Urban Environments (CARA Program) O. Favez et al. 10.3390/atmos12020207
- Multivariate time series modelling for urban air quality H. Hajmohammadi & B. Heydecker 10.1016/j.uclim.2021.100834
- Oxidation of Substituted Catechols at the Air–Water Interface: Production of Carboxylic Acids, Quinones, and Polyphenols E. Pillar-Little & M. Guzman 10.1021/acs.est.7b00232
- Modelling carbonaceous aerosol from residential solid fuel burning with different assumptions for emissions R. Ots et al. 10.5194/acp-18-4497-2018
- Argon offline-AMS source apportionment of organic aerosol over yearly cycles for an urban, rural, and marine site in northern Europe C. Bozzetti et al. 10.5194/acp-17-117-2017
- A systematic re-evaluation of methods for quantification of bulk particle-phase organic nitrates using real-time aerosol mass spectrometry D. Day et al. 10.5194/amt-15-459-2022
- Organic aerosol in the summertime southeastern United States: components and their link to volatility distribution, oxidation state and hygroscopicity E. Kostenidou et al. 10.5194/acp-18-5799-2018
- Characterizing the volatility and mixing state of ambient fine particles in the summer and winter of urban Beijing L. Chen et al. 10.5194/acp-22-2293-2022
- Changes in Physicochemical Properties of Organic Aerosol During Photochemical Aging of Cooking and Burning Emissions W. Xu et al. 10.1029/2022JD037911
27 citations as recorded by crossref.
- Simulating secondary organic aerosol from missing diesel-related intermediate-volatility organic compound emissions during the Clean Air for London (ClearfLo) campaign R. Ots et al. 10.5194/acp-16-6453-2016
- Organic aerosol volatility and viscosity in the North China Plain: contrast between summer and winter W. Xu et al. 10.5194/acp-21-5463-2021
- Volatility measurement of atmospheric submicron aerosols in an urban atmosphere in southern China L. Cao et al. 10.5194/acp-18-1729-2018
- Summertime aerosol volatility measurements in Beijing, China W. Xu et al. 10.5194/acp-19-10205-2019
- Molecular-Size-Separated Brown Carbon Absorption for Biomass-Burning Aerosol at Multiple Field Sites R. Di Lorenzo et al. 10.1021/acs.est.6b06160
- Estimation of particulate organic nitrates from thermodenuder–aerosol mass spectrometer measurements in the North China Plain W. Xu et al. 10.5194/amt-14-3693-2021
- Experimental and model estimates of the contributions from biogenic monoterpenes and sesquiterpenes to secondary organic aerosol in the southeastern United States L. Xu et al. 10.5194/acp-18-12613-2018
- Impact of aging on the sources, volatility, and viscosity of organic aerosols in Chinese outflows T. Feng et al. 10.5194/acp-23-611-2023
- Characterization of organic nitrate constituents of secondary organic aerosol (SOA) from nitrate-radical-initiated oxidation of limonene using high-resolution chemical ionization mass spectrometry C. Faxon et al. 10.5194/acp-18-5467-2018
- Quantifying the volatility of organic aerosol in the southeastern US P. Saha et al. 10.5194/acp-17-501-2017
- Characterization of submicron aerosol volatility in the regional atmosphere in Southern China L. Cao et al. 10.1016/j.chemosphere.2019.124383
- Secondary Organic Aerosol (SOA) from Nitrate Radical Oxidation of Monoterpenes: Effects of Temperature, Dilution, and Humidity on Aerosol Formation, Mixing, and Evaporation C. Boyd et al. 10.1021/acs.est.7b01460
- Particle detection using the dual-vaporizer configuration of the soot particle Aerosol Mass Spectrometer (SP-AMS) A. Avery et al. 10.1080/02786826.2020.1844132
- Evaluation of a New Aerosol Chemical Speciation Monitor (ACSM) System at an Urban Site in Atlanta, GA: The Use of Capture Vaporizer and PM2.5 Inlet T. Joo et al. 10.1021/acsearthspacechem.1c00173
- Colloidal associations of major and trace elements in the snow pack across a 2800-km south-north gradient of western Siberia I. Krickov et al. 10.1016/j.chemgeo.2022.121090
- Extreme air pollution from residential solid fuel burning C. Lin et al. 10.1038/s41893-018-0125-x
- Chemical Characterization of Water-Soluble Organic Aerosol in Contrasting Rural and Urban Environments in the Southeastern United States L. Xu et al. 10.1021/acs.est.6b05002
- An omnipresent diversity and variability in the chemical composition of atmospheric functionalized organic aerosol J. Ditto et al. 10.1038/s42004-018-0074-3
- Overview of the French Operational Network for In Situ Observation of PM Chemical Composition and Sources in Urban Environments (CARA Program) O. Favez et al. 10.3390/atmos12020207
- Multivariate time series modelling for urban air quality H. Hajmohammadi & B. Heydecker 10.1016/j.uclim.2021.100834
- Oxidation of Substituted Catechols at the Air–Water Interface: Production of Carboxylic Acids, Quinones, and Polyphenols E. Pillar-Little & M. Guzman 10.1021/acs.est.7b00232
- Modelling carbonaceous aerosol from residential solid fuel burning with different assumptions for emissions R. Ots et al. 10.5194/acp-18-4497-2018
- Argon offline-AMS source apportionment of organic aerosol over yearly cycles for an urban, rural, and marine site in northern Europe C. Bozzetti et al. 10.5194/acp-17-117-2017
- A systematic re-evaluation of methods for quantification of bulk particle-phase organic nitrates using real-time aerosol mass spectrometry D. Day et al. 10.5194/amt-15-459-2022
- Organic aerosol in the summertime southeastern United States: components and their link to volatility distribution, oxidation state and hygroscopicity E. Kostenidou et al. 10.5194/acp-18-5799-2018
- Characterizing the volatility and mixing state of ambient fine particles in the summer and winter of urban Beijing L. Chen et al. 10.5194/acp-22-2293-2022
- Changes in Physicochemical Properties of Organic Aerosol During Photochemical Aging of Cooking and Burning Emissions W. Xu et al. 10.1029/2022JD037911
Saved (preprint)
Latest update: 20 Apr 2024
Short summary
We investigate the spatial distribution of submicron aerosol in the greater London area as part of the Clean Air for London (ClearfLo) project in winter 2012. Although the concentrations of organic aerosol (OA) are similar between a rural and an urban site, the OA sources are different. We also examine the volatility of submicron aerosol at the rural site and find that the non-volatile organics have similar sources or have undergone similar chemical processing as refractory black carbon.
We investigate the spatial distribution of submicron aerosol in the greater London area as part...
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