Articles | Volume 15, issue 15
https://doi.org/10.5194/acp-15-8975-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-15-8975-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
13 Aug 2015
Research article |
| 13 Aug 2015
Hygroscopic and phase separation properties of ammonium sulfate/organics/water ternary solutions
M. A. Zawadowicz
Massachusetts Institute of Technology, Cambridge, Massachusetts, USA
S. R. Proud
Massachusetts Institute of Technology, Cambridge, Massachusetts, USA
University of Copenhagen, Copenhagen, Denmark
S. S. Seppalainen
Massachusetts Institute of Technology, Cambridge, Massachusetts, USA
D. J. Cziczo
CORRESPONDING AUTHOR
Massachusetts Institute of Technology, Cambridge, Massachusetts, USA
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- Stability assessment of organic sulfur and organosulfate compounds in filter samples for quantification by Fourier- transform infrared spectroscopy M. Anunciado et al. 10.5194/amt-16-3515-2023
- Direct observations of organic aerosols in common wintertime hazes in North China: insights into direct emissions from Chinese residential stoves S. Chen et al. 10.5194/acp-17-1259-2017
- Hygroscopicity of organic surrogate compounds from biomass burning and their effect on the efflorescence of ammonium sulfate in mixed aerosol particles T. Lei et al. 10.5194/acp-18-1045-2018
- Exploring the inorganic composition of the Asian Tropopause Aerosol Layer using medium-duration balloon flights H. Vernier et al. 10.5194/acp-22-12675-2022
- Measurement report: Water diffusion in single suspended phase-separated aerosols Y. Tong et al. 10.5194/acp-24-2937-2024
- Hygroscopic Behavior of Ammonium Sulfate, Ammonium Nitrate, and their Mixture Particles L. Wu et al. 10.5572/ajae.2019.13.3.196
- Current State of Atmospheric Aerosol Thermodynamics and Mass Transfer Modeling: A Review K. Semeniuk & A. Dastoor 10.3390/atmos11020156
- Effect of mixing structure on the water uptake of mixtures of ammonium sulfate and phthalic acid particles W. Wang et al. 10.5194/acp-21-2179-2021
- Vapor-phase grafting of a model aminosilane compound to Al2O3, ZnO, and TiO2 surfaces prepared by atomic layer deposition V. Rozyyev et al. 10.1016/j.apsusc.2021.149996
- Single-Particle Time-of-Flight Mass Spectrometry Utilizing a Femtosecond Desorption and Ionization Laser M. Zawadowicz et al. 10.1021/acs.analchem.5b03158
- Increased Aerosol Extinction Efficiency Hinders Visibility Improvement in Eastern China J. Liu et al. 10.1029/2020GL090167
- Ice nucleation ability of ammonium sulfate aerosol particles internally mixed with secondary organics B. Bertozzi et al. 10.5194/acp-21-10779-2021
- Organic Coating Reduces Hygroscopic Growth of Phase-Separated Aerosol Particles W. Li et al. 10.1021/acs.est.1c05901
- Liquid–Liquid Phase Separation in Single Suspended Aerosol Microdroplets Y. Tong & A. Ye 10.1021/acs.analchem.2c05605
- Estimation of the Growth and Dissolution Kinetics of Ammonium Bicarbonate in Aqueous Ammonia Solutions from Batch Crystallization Experiments. 2. The Effect of Sulfate Impurity F. Milella & M. Mazzotti 10.1021/acs.cgd.9b01315
- Aerosol Hygroscopicity on A Single Particle Level Using Microscopic and Spectroscopic Techniques: A Review L. Wu & C. Ro 10.5572/ajae.2020.14.3.177
- A review of experimental techniques for aerosol hygroscopicity studies M. Tang et al. 10.5194/acp-19-12631-2019
- Solid organic-coated ammonium sulfate particles at high relative humidity in the summertime Arctic atmosphere R. Kirpes et al. 10.1073/pnas.2104496119
- Chemical reaction between sodium pyruvate and ammonium sulfate in aerosol particles and resultant sodium sulfate efflorescence H. Yang et al. 10.1016/j.chemosphere.2018.10.062
19 citations as recorded by crossref.
- A cleaner approach for high-efficiency regeneration of base and precious metals from waste printed circuit boards through stepwise oxido-acidic and thiocyanate leaching M. Rezaee et al. 10.1016/j.chemosphere.2022.134283
- Stability assessment of organic sulfur and organosulfate compounds in filter samples for quantification by Fourier- transform infrared spectroscopy M. Anunciado et al. 10.5194/amt-16-3515-2023
- Direct observations of organic aerosols in common wintertime hazes in North China: insights into direct emissions from Chinese residential stoves S. Chen et al. 10.5194/acp-17-1259-2017
- Hygroscopicity of organic surrogate compounds from biomass burning and their effect on the efflorescence of ammonium sulfate in mixed aerosol particles T. Lei et al. 10.5194/acp-18-1045-2018
- Exploring the inorganic composition of the Asian Tropopause Aerosol Layer using medium-duration balloon flights H. Vernier et al. 10.5194/acp-22-12675-2022
- Measurement report: Water diffusion in single suspended phase-separated aerosols Y. Tong et al. 10.5194/acp-24-2937-2024
- Hygroscopic Behavior of Ammonium Sulfate, Ammonium Nitrate, and their Mixture Particles L. Wu et al. 10.5572/ajae.2019.13.3.196
- Current State of Atmospheric Aerosol Thermodynamics and Mass Transfer Modeling: A Review K. Semeniuk & A. Dastoor 10.3390/atmos11020156
- Effect of mixing structure on the water uptake of mixtures of ammonium sulfate and phthalic acid particles W. Wang et al. 10.5194/acp-21-2179-2021
- Vapor-phase grafting of a model aminosilane compound to Al2O3, ZnO, and TiO2 surfaces prepared by atomic layer deposition V. Rozyyev et al. 10.1016/j.apsusc.2021.149996
- Single-Particle Time-of-Flight Mass Spectrometry Utilizing a Femtosecond Desorption and Ionization Laser M. Zawadowicz et al. 10.1021/acs.analchem.5b03158
- Increased Aerosol Extinction Efficiency Hinders Visibility Improvement in Eastern China J. Liu et al. 10.1029/2020GL090167
- Ice nucleation ability of ammonium sulfate aerosol particles internally mixed with secondary organics B. Bertozzi et al. 10.5194/acp-21-10779-2021
- Organic Coating Reduces Hygroscopic Growth of Phase-Separated Aerosol Particles W. Li et al. 10.1021/acs.est.1c05901
- Liquid–Liquid Phase Separation in Single Suspended Aerosol Microdroplets Y. Tong & A. Ye 10.1021/acs.analchem.2c05605
- Estimation of the Growth and Dissolution Kinetics of Ammonium Bicarbonate in Aqueous Ammonia Solutions from Batch Crystallization Experiments. 2. The Effect of Sulfate Impurity F. Milella & M. Mazzotti 10.1021/acs.cgd.9b01315
- Aerosol Hygroscopicity on A Single Particle Level Using Microscopic and Spectroscopic Techniques: A Review L. Wu & C. Ro 10.5572/ajae.2020.14.3.177
- A review of experimental techniques for aerosol hygroscopicity studies M. Tang et al. 10.5194/acp-19-12631-2019
- Solid organic-coated ammonium sulfate particles at high relative humidity in the summertime Arctic atmosphere R. Kirpes et al. 10.1073/pnas.2104496119
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Latest update: 20 Apr 2024
Short summary
This work investigates hygroscopic properties of internally mixed organic/inorganic aerosol particles. Aerosol particles containing organic and inorganic components can phase separate under certain relative humidity conditions, creating particles with an inorganic core and an organic shell. This paper explores whether water uptake from gaseous phase still occurs in such phase-separated systems. It finds that phase separation does not inhibit water uptake for the five systems that were studied.
This work investigates hygroscopic properties of internally mixed organic/inorganic aerosol...
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