Articles | Volume 15, issue 15
https://doi.org/10.5194/acp-15-8871-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-15-8871-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
13 Aug 2015
Research article |
| 13 Aug 2015
Examining the effects of anthropogenic emissions on isoprene-derived secondary organic aerosol formation during the 2013 Southern Oxidant and Aerosol Study (SOAS) at the Look Rock, Tennessee ground site
S. H. Budisulistiorini
Department of Environmental Sciences and Engineering, Gillings School of Global Public Health, The University of North Carolina at Chapel Hill, Chapel Hill, NC, USA
National Exposure Research Laboratory, US Environmental Protection Agency, Research Triangle Park, NC, USA
X. Li
Department of Environmental Sciences and Engineering, Gillings School of Global Public Health, The University of North Carolina at Chapel Hill, Chapel Hill, NC, USA
S. T. Bairai
Tennessee Valley Authority, Muscle Shoals, AL, USA
now at: Battelle, Pueblo, CO, USA
J. Renfro
National Park Service, Gatlinburg, TN, USA
Y. Liu
School of Engineering and Applied Sciences, Harvard University, Cambridge, MA USA
Y. J. Liu
School of Engineering and Applied Sciences, Harvard University, Cambridge, MA USA
K. A. McKinney
School of Engineering and Applied Sciences, Harvard University, Cambridge, MA USA
S. T. Martin
School of Engineering and Applied Sciences, Harvard University, Cambridge, MA USA
V. F. McNeill
Department of Chemical Engineering, Columbia University, New York, USA
H. O. T. Pye
National Exposure Research Laboratory, US Environmental Protection Agency, Research Triangle Park, NC, USA
School of Earth and Atmospheric Sciences, Georgia Institute of Technology, Atlanta, GA, USA
School of Chemical and Biomolecular Engineering, Georgia Institute of Technology, Atlanta, GA, USA
ICE-HT, Foundation for Research and Technology, Hellas, Patras, Greece
M. E. Neff
Department of Chemistry, University of Iowa, Iowa City, IA, USA
E. A. Stone
Department of Chemistry, University of Iowa, Iowa City, IA, USA
S. Mueller
Tennessee Valley Authority, Muscle Shoals, AL, USA
now at: Ensafe, Nashville, TN, USA
Department of Experimental Meteorology, Ludwig Maximilian University of Munich, Munich, Germany
S. L. Shaw
Electric Power Research Institute, Palo Alto, CA, USA
Z. Zhang
Department of Environmental Sciences and Engineering, Gillings School of Global Public Health, The University of North Carolina at Chapel Hill, Chapel Hill, NC, USA
A. Gold
Department of Environmental Sciences and Engineering, Gillings School of Global Public Health, The University of North Carolina at Chapel Hill, Chapel Hill, NC, USA
Department of Environmental Sciences and Engineering, Gillings School of Global Public Health, The University of North Carolina at Chapel Hill, Chapel Hill, NC, USA
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Short summary
Isoprene epoxydiols (IEPOX) are major gas-phase products from the atmospheric oxidation of isoprene that yield secondary organic aerosol (SOA) by reactive uptake onto acidic sulfate aerosol. We report a substantial contribution of IEPOX-derived SOA to the total fine aerosol collected during summer. IEPOX-derived SOA measured by online and offline mass spectrometry techniques is correlated with acidic sulfate aerosol, demonstrating the critical role of anthropogenic emissions in its formation.
Isoprene epoxydiols (IEPOX) are major gas-phase products from the atmospheric oxidation of...
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