Articles | Volume 15, issue 12
https://doi.org/10.5194/acp-15-7085-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-15-7085-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
30 Jun 2015
Research article |
| 30 Jun 2015
In situ vertical profiles of aerosol extinction, mass, and composition over the southeast United States during SENEX and SEAC4RS: observations of a modest aerosol enhancement aloft
N. L. Wagner
CORRESPONDING AUTHOR
NOAA Earth System Research Laboratory, 325 Broadway, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, USA
C. A. Brock
NOAA Earth System Research Laboratory, 325 Broadway, Boulder, CO 80305, USA
W. M. Angevine
NOAA Earth System Research Laboratory, 325 Broadway, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, USA
A. Beyersdorf
NASA Langley Research Center, MS 483, Hampton, VA 23681, USA
P. Campuzano-Jost
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO 80309, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO 80309, USA
J. A. de Gouw
NOAA Earth System Research Laboratory, 325 Broadway, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, USA
G. S. Diskin
NASA Langley Research Center, MS 483, Hampton, VA 23681, USA
T. D. Gordon
NOAA Earth System Research Laboratory, 325 Broadway, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, USA
M. G. Graus
NOAA Earth System Research Laboratory, 325 Broadway, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, USA
now at: Institute of Meteorology and Geophysics, University of Innsbruck, Austria
J. S. Holloway
NOAA Earth System Research Laboratory, 325 Broadway, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, USA
School of Earth {&} Atmospheric Sciences, Georgia Institute of Technology, Atlanta, GA 30332, USA
J. L. Jimenez
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO 80309, USA
D. A. Lack
NOAA Earth System Research Laboratory, 325 Broadway, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, USA
J. Liao
NOAA Earth System Research Laboratory, 325 Broadway, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, USA
X. Liu
School of Earth {&} Atmospheric Sciences, Georgia Institute of Technology, Atlanta, GA 30332, USA
M. Z. Markovic
NOAA Earth System Research Laboratory, 325 Broadway, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, USA
now at: Air Quality Research Division, Environment Canada, Toronto, ON, Canada
A. M. Middlebrook
NOAA Earth System Research Laboratory, 325 Broadway, Boulder, CO 80305, USA
T. Mikoviny
Oak Ridge Associated Universities (ORAU), Oak Ridge, TN, USA
J. Peischl
NOAA Earth System Research Laboratory, 325 Broadway, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, USA
A. E. Perring
NOAA Earth System Research Laboratory, 325 Broadway, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, USA
M. S. Richardson
NOAA Earth System Research Laboratory, 325 Broadway, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, USA
T. B. Ryerson
NOAA Earth System Research Laboratory, 325 Broadway, Boulder, CO 80305, USA
J. P. Schwarz
NOAA Earth System Research Laboratory, 325 Broadway, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, USA
C. Warneke
NOAA Earth System Research Laboratory, 325 Broadway, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, USA
NOAA Earth System Research Laboratory, 325 Broadway, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, USA
Institute for Atmospheric & Climate Science, Swiss Federal Institute of Technology, Zürich, Switzerland
A. Wisthaler
Institute for Ion Physics and Applied Physics, University of Innsbruck, Technikerstrasse 25, 6020 Innsbruck, Austria
L. D. Ziemba
NASA Langley Research Center, MS 483, Hampton, VA 23681, USA
D. M. Murphy
NOAA Earth System Research Laboratory, 325 Broadway, Boulder, CO 80305, USA
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40 citations as recorded by crossref.
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- The Weather Research and Forecasting Model: Overview, System Efforts, and Future Directions J. Powers et al. 10.1175/BAMS-D-15-00308.1
- Inconsistency of ammonium–sulfate aerosol ratios with thermodynamic models in the eastern US: a possible role of organic aerosol R. Silvern et al. 10.5194/acp-17-5107-2017
- Aerosol optical properties in the southeastern United States in summer – Part 1: Hygroscopic growth C. Brock et al. 10.5194/acp-16-4987-2016
- Drivers of cloud droplet number variability in the summertime in the southeastern United States A. Bougiatioti et al. 10.5194/acp-20-12163-2020
- Synthesis of the Southeast Atmosphere Studies: Investigating Fundamental Atmospheric Chemistry Questions A. Carlton et al. 10.1175/BAMS-D-16-0048.1
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- Limited impact of sulfate-driven chemistry on black carbon aerosol aging in power plant plumes M. Z. Markovic et al. 10.3934/environsci.2018.3.195
- Aerosol pH indicator and organosulfate detectability from aerosol mass spectrometry measurements M. Schueneman et al. 10.5194/amt-14-2237-2021
- Insights into atmospheric trace gases, aerosols, and transport processes at a high-altitude station (2623 m a.s.l.) in Northeast Asia Y. Shan et al. 10.1016/j.atmosenv.2024.120482
- Assessing the Challenges of Surface‐Level Aerosol Mass Estimates From Remote Sensing During the SEAC4RS and SEARCH Campaigns: Baseline Surface Observations and Remote Sensing in the Southeastern United States K. Kaku et al. 10.1029/2017JD028074
- Aerosol Optical Thickness: Organic Composition, Associated Particle Water, and Aloft Extinction A. Christiansen et al. 10.1021/acsearthspacechem.8b00163
- Southeast Atmosphere Studies: learning from model-observation syntheses J. Mao et al. 10.5194/acp-18-2615-2018
- Free tropospheric aerosols at the Mt. Bachelor Observatory: more oxidized and higher sulfate content compared to boundary layer aerosols S. Zhou et al. 10.5194/acp-19-1571-2019
- Evaluation of Stratospheric Intrusions and Biomass Burning Plumes on the Vertical Distribution of Tropospheric Ozone Over the Midwestern United States J. Wilkins et al. 10.1029/2020JD032454
- Ground‐based High Spectral Resolution Lidar observation of aerosol vertical distribution in the summertime Southeast United States J. Reid et al. 10.1002/2016JD025798
- A study of the impact of spatial resolution on the estimation of particle matter concentration from the aerosol optical depth retrieved from satellite observations L. Mei et al. 10.1080/01431161.2019.1601279
- Formaldehyde production from isoprene oxidation across NO<sub><i>x</i></sub> regimes G. Wolfe et al. 10.5194/acp-16-2597-2016
- Enhanced formation of isoprene‐derived organic aerosol in sulfur‐rich power plant plumes during Southeast Nexus L. Xu et al. 10.1002/2016JD025156
- Is there an aerosol signature of chemical cloud processing? B. Ervens et al. 10.5194/acp-18-16099-2018
- Characterization of the Real Part of Dry Aerosol Refractive Index Over North America From the Surface to 12 km A. Aldhaif et al. 10.1029/2018JD028504
- Observational evidence for pollution‐influenced selective uptake contributing to biogenic secondary organic aerosols in the southeastern U.S. J. Liu et al. 10.1002/2017GL074665
- Vapor-Pressure Pathways Initiate but Hydrolysis Products Dominate the Aerosol Estimated from Organic Nitrates A. Zare et al. 10.1021/acsearthspacechem.9b00067
- Sources and Secondary Production of Organic Aerosols in the Northeastern United States during WINTER J. Schroder et al. 10.1029/2018JD028475
- Glyoxal yield from isoprene oxidation and relation to formaldehyde: chemical mechanism, constraints from SENEX aircraft observations, and interpretation of OMI satellite data C. Chan Miller et al. 10.5194/acp-17-8725-2017
- Identifying chemical aerosol signatures using optical suborbital observations: how much can optical properties tell us about aerosol composition? M. Kacenelenbogen et al. 10.5194/acp-22-3713-2022
- Recent advances in understanding secondary organic aerosol: Implications for global climate forcing M. Shrivastava et al. 10.1002/2016RG000540
- Long-term observational constraints of organic aerosol dependence on inorganic species in the southeast US Y. Zheng et al. 10.5194/acp-20-13091-2020
- Summertime tropospheric ozone enhancement associated with a cold front passage due to stratosphere‐to‐troposphere transport and biomass burning: Simultaneous ground‐based lidar and airborne measurements S. Kuang et al. 10.1002/2016JD026078
- Biogenic emissions and land–atmosphere interactions as drivers of the daytime evolution of secondary organic aerosol in the southeastern US J. Nagori et al. 10.5194/acp-19-701-2019
- Evaluating the Impacts of Cloud Processing on Resuspended Aerosol Particles After Cloud Evaporation Using a Particle‐Resolved Model Y. Yao et al. 10.1029/2021JD034992
- Aqueous-phase mechanism for secondary organic aerosol formation from isoprene: application to the southeast United States and co-benefit of SO<sub>2</sub> emission controls E. Marais et al. 10.5194/acp-16-1603-2016
- Transport and chemistry of isoprene and its oxidation products in deep convective clouds R. Bardakov et al. 10.1080/16000889.2021.1979856
- Aerosol optical properties in the southeastern United States in summer – Part 2: Sensitivity of aerosol optical depth to relative humidity and aerosol parameters C. Brock et al. 10.5194/acp-16-5009-2016
- The Present and Future of Secondary Organic Aerosol Direct Forcing on Climate K. Tsigaridis & M. Kanakidou 10.1007/s40641-018-0092-3
- The impacts of aerosol loading, composition, and water uptake on aerosol extinction variability in the Baltimore–Washington, D.C. region A. Beyersdorf et al. 10.5194/acp-16-1003-2016
- Planning, implementation, and scientific goals of the Studies of Emissions and Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC4RS) field mission O. Toon et al. 10.1002/2015JD024297
- Towards a satellite formaldehyde – in situ hybrid estimate for organic aerosol abundance J. Liao et al. 10.5194/acp-19-2765-2019
- Comparison of the aerosol optical properties and size distribution retrieved by sun photometer with in situ measurements at midlatitude A. Chauvigné et al. 10.5194/amt-9-4569-2016
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Short summary
This paper investigates the summertime vertical profile of aerosol over the southeastern US using in situ measurements collected from aircraft. We use a vertical mixing model and measurements of CO to predict the vertical profile of aerosol that we would expect from vertical mixing alone and compare with the observed aerosol profile. We found a modest enhancement of aerosol in the cloudy transition layer during shallow cumulus convection and attribute the enhancement to local aerosol formation.
This paper investigates the summertime vertical profile of aerosol over the southeastern US...
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