Articles | Volume 15, issue 9
https://doi.org/10.5194/acp-15-5243-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-15-5243-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
12 May 2015
Research article |
| 12 May 2015
Gas and aerosol carbon in California: comparison of measurements and model predictions in Pasadena and Bakersfield
K. R. Baker
CORRESPONDING AUTHOR
Office of Air Quality Planning and Standards, US Environmental Protection Agency, Research Triangle Park, NC, USA
A. G. Carlton
Dept. of Environmental Sciences, Rutgers University, New Brunswick, NJ, USA
T. E. Kleindienst
Office of Research and Development, US Environmental Protection Agency, Research Triangle Park, NC, USA
J. H. Offenberg
Office of Research and Development, US Environmental Protection Agency, Research Triangle Park, NC, USA
M. R. Beaver
Office of Research and Development, US Environmental Protection Agency, Research Triangle Park, NC, USA
D. R. Gentner
Department of Chemical and Environmental Engineering, Yale University, New Haven, CT, USA
A. H. Goldstein
Department of Civil and Environmental Engineering, University of California, Berkeley, CA, USA
P. L. Hayes
Département de Chimie, Université de Montréal, Montréal, Québec, Canada
J. L. Jimenez
Department of Chemistry & Biochemistry, and CIRES, University of Colorado, Boulder, Colorado, USA
J. B. Gilman
Chemical Sciences Division, Earth System Research Laboratory, National Oceanic and Atmospheric Administration, Boulder, CO, USA
J. A. de Gouw
Chemical Sciences Division, Earth System Research Laboratory, National Oceanic and Atmospheric Administration, Boulder, CO, USA
M. C. Woody
Office of Research and Development, US Environmental Protection Agency, Research Triangle Park, NC, USA
H. O. T. Pye
Office of Research and Development, US Environmental Protection Agency, Research Triangle Park, NC, USA
J. T. Kelly
Office of Air Quality Planning and Standards, US Environmental Protection Agency, Research Triangle Park, NC, USA
M. Lewandowski
Office of Research and Development, US Environmental Protection Agency, Research Triangle Park, NC, USA
Alion Science and Technology, Inc., Research Triangle Park, NC, USA
P. S. Stevens
Center for Research in Environmental Science, School of Public and Environmental Affairs and Department of Chemistry, Indiana University, Bloomington, IN, USA
W. H. Brune
Department of Meteorology, Pennsylvania State University, University Park, PA, USA
Y.-H. Lin
Department of Environmental Sciences and Engineering, Gillings School of Global Public Health, University of North Carolina at Chapel Hill, Chapel Hill, NC, USA
C. L. Rubitschun
Department of Environmental Sciences and Engineering, Gillings School of Global Public Health, University of North Carolina at Chapel Hill, Chapel Hill, NC, USA
J. D. Surratt
Department of Environmental Sciences and Engineering, Gillings School of Global Public Health, University of North Carolina at Chapel Hill, Chapel Hill, NC, USA
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36 citations as recorded by crossref.
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- Additional Benefits of Federal Air-Quality Rules: Model Estimates of Controllable Biogenic Secondary Organic Aerosol A. Carlton et al. 10.1021/acs.est.8b01869
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- Chemical transport model simulations of organic aerosol in southern California: model evaluation and gasoline and diesel source contributions S. Jathar et al. 10.5194/acp-17-4305-2017
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- Prediction of secondary organic aerosol from the multiphase reaction of gasoline vapor by using volatility–reactivity base lumping S. Han & M. Jang 10.5194/acp-22-625-2022
- Constraints on primary and secondary particulate carbon sources using chemical tracer and 14 C methods during CalNex-Bakersfield R. Sheesley et al. 10.1016/j.atmosenv.2017.07.025
- Modeling secondary organic aerosol formation from volatile chemical products E. Pennington et al. 10.5194/acp-21-18247-2021
- Simulating reactive nitrogen, carbon monoxide, and ozone in California during ARCTAS-CARB 2008 with high wildfire activity C. Cai et al. 10.1016/j.atmosenv.2015.12.031
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- Modeling the effects of pollutant emissions from large industrial complexes on benzene, toluene, and xylene concentrations in urban areas J. Bang et al. 10.5620/eht.e2017022
- Review of Urban Secondary Organic Aerosol Formation from Gasoline and Diesel Motor Vehicle Emissions D. Gentner et al. 10.1021/acs.est.6b04509
- Assessment of the impacts of aromatic VOC emissions and yields of SOA on SOA concentrations with the air quality model RAMS-CMAQ J. Li et al. 10.1016/j.atmosenv.2017.03.035
- Criteria pollutant impacts of volatile chemical products informed by near-field modelling M. Qin et al. 10.1038/s41893-020-00614-1
- EURODELTA III exercise: An evaluation of air quality models’ capacity to reproduce the carbonaceous aerosol M. Mircea et al. 10.1016/j.aeaoa.2019.100018
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- Simulation of organic aerosol formation during the CalNex study: updated mobile emissions and secondary organic aerosol parameterization for intermediate-volatility organic compounds Q. Lu et al. 10.5194/acp-20-4313-2020
- Simulating secondary organic aerosol in a regional air quality model using the statistical oxidation model – Part 2: Assessing the influence of vapor wall losses C. Cappa et al. 10.5194/acp-16-3041-2016
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- On the implications of aerosol liquid water and phase separation for organic aerosol mass H. Pye et al. 10.5194/acp-17-343-2017
- Volatile Chemical Product Enhancements to Criteria Pollutants in the United States K. Seltzer et al. 10.1021/acs.est.1c04298
- Modeling regional air quality and climate: improving organic aerosol and aerosol activation processes in WRF/Chem version 3.7.1 K. Yahya et al. 10.5194/gmd-10-2333-2017
- Comprehensive organic emission profiles for gasoline, diesel, and gas-turbine engines including intermediate and semi-volatile organic compound emissions Q. Lu et al. 10.5194/acp-18-17637-2018
- Characterization of organic aerosol across the global remote troposphere: a comparison of ATom measurements and global chemistry models A. Hodzic et al. 10.5194/acp-20-4607-2020
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- Gas Phase Oxidation of Campholenic Aldehyde and Solution Phase Reactivity of its Epoxide Derivative W. Thomas et al. 10.1021/acs.jpca.6b08642
- Quantification of the sources and composition of particulate matter by field-deployable mass spectrometry: implications for air quality and public health P. Hayes 10.1039/C6AN02378A
- WRF-Chem simulation of aerosol seasonal variability in the San Joaquin Valley L. Wu et al. 10.5194/acp-17-7291-2017
- Predicting wildfire particulate matter and hypothetical re-emission of radiological Cs-137 contamination incidents K. Baker et al. 10.1016/j.scitotenv.2021.148872
36 citations as recorded by crossref.
- Urban particulate matter pollution: a tale of five cities S. Pandis et al. 10.1039/C5FD00212E
- Influence of biomass burning vapor wall loss correction on modeling organic aerosols in Europe by CAMx v6.50 J. Jiang et al. 10.5194/gmd-14-1681-2021
- Additional Benefits of Federal Air-Quality Rules: Model Estimates of Controllable Biogenic Secondary Organic Aerosol A. Carlton et al. 10.1021/acs.est.8b01869
- Simulating the impact of gas-wall partitioning on SOA formation using the explicit gas mechanism integrated with aqueous reactions containing electrolytes S. Han & M. Jang 10.1016/j.scitotenv.2020.141360
- Toxicological effects of fresh and aged gasoline exhaust particles in Hong Kong Y. Lau et al. 10.1016/j.jhazmat.2022.129846
- Mapping Modeled Exposure of Wildland Fire Smoke for Human Health Studies in California P. Koman et al. 10.3390/atmos10060308
- Chemical transport model simulations of organic aerosol in southern California: model evaluation and gasoline and diesel source contributions S. Jathar et al. 10.5194/acp-17-4305-2017
- Simulating secondary organic aerosol in a regional air quality model using the statistical oxidation model – Part 3: Assessing the influence of semi-volatile and intermediate-volatility organic compounds and NO<sub><i>x</i></sub> A. Akherati et al. 10.5194/acp-19-4561-2019
- Prediction of secondary organic aerosol from the multiphase reaction of gasoline vapor by using volatility–reactivity base lumping S. Han & M. Jang 10.5194/acp-22-625-2022
- Constraints on primary and secondary particulate carbon sources using chemical tracer and 14 C methods during CalNex-Bakersfield R. Sheesley et al. 10.1016/j.atmosenv.2017.07.025
- Modeling secondary organic aerosol formation from volatile chemical products E. Pennington et al. 10.5194/acp-21-18247-2021
- Simulating reactive nitrogen, carbon monoxide, and ozone in California during ARCTAS-CARB 2008 with high wildfire activity C. Cai et al. 10.1016/j.atmosenv.2015.12.031
- Real-time measurements of secondary organic aerosol formation and aging from ambient air in an oxidation flow reactor in the Los Angeles area A. Ortega et al. 10.5194/acp-16-7411-2016
- Gasoline cars produce more carbonaceous particulate matter than modern filter-equipped diesel cars S. Platt et al. 10.1038/s41598-017-03714-9
- Modeling the effects of pollutant emissions from large industrial complexes on benzene, toluene, and xylene concentrations in urban areas J. Bang et al. 10.5620/eht.e2017022
- Review of Urban Secondary Organic Aerosol Formation from Gasoline and Diesel Motor Vehicle Emissions D. Gentner et al. 10.1021/acs.est.6b04509
- Assessment of the impacts of aromatic VOC emissions and yields of SOA on SOA concentrations with the air quality model RAMS-CMAQ J. Li et al. 10.1016/j.atmosenv.2017.03.035
- Criteria pollutant impacts of volatile chemical products informed by near-field modelling M. Qin et al. 10.1038/s41893-020-00614-1
- EURODELTA III exercise: An evaluation of air quality models’ capacity to reproduce the carbonaceous aerosol M. Mircea et al. 10.1016/j.aeaoa.2019.100018
- Semivolatile POA and parameterized total combustion SOA in CMAQv5.2: impacts on source strength and partitioning B. Murphy et al. 10.5194/acp-17-11107-2017
- Simulation of organic aerosol formation during the CalNex study: updated mobile emissions and secondary organic aerosol parameterization for intermediate-volatility organic compounds Q. Lu et al. 10.5194/acp-20-4313-2020
- Simulating secondary organic aerosol in a regional air quality model using the statistical oxidation model – Part 2: Assessing the influence of vapor wall losses C. Cappa et al. 10.5194/acp-16-3041-2016
- Using wildland fire smoke modeling data in gerontological health research (California, 2007–2018) P. Koman et al. 10.1016/j.scitotenv.2022.156403
- CAMx–UNIPAR simulation of secondary organic aerosol mass formed from multiphase reactions of hydrocarbons under the Central Valley urban atmospheres of California Y. Jo et al. 10.5194/acp-24-487-2024
- Reflecting on progress since the 2005 NARSTO emissions inventory report M. Day et al. 10.1080/10962247.2019.1629363
- Reactive organic carbon emissions from volatile chemical products K. Seltzer et al. 10.5194/acp-21-5079-2021
- On the implications of aerosol liquid water and phase separation for organic aerosol mass H. Pye et al. 10.5194/acp-17-343-2017
- Volatile Chemical Product Enhancements to Criteria Pollutants in the United States K. Seltzer et al. 10.1021/acs.est.1c04298
- Modeling regional air quality and climate: improving organic aerosol and aerosol activation processes in WRF/Chem version 3.7.1 K. Yahya et al. 10.5194/gmd-10-2333-2017
- Comprehensive organic emission profiles for gasoline, diesel, and gas-turbine engines including intermediate and semi-volatile organic compound emissions Q. Lu et al. 10.5194/acp-18-17637-2018
- Characterization of organic aerosol across the global remote troposphere: a comparison of ATom measurements and global chemistry models A. Hodzic et al. 10.5194/acp-20-4607-2020
- Understanding sources of organic aerosol during CalNex-2010 using the CMAQ-VBS M. Woody et al. 10.5194/acp-16-4081-2016
- Gas Phase Oxidation of Campholenic Aldehyde and Solution Phase Reactivity of its Epoxide Derivative W. Thomas et al. 10.1021/acs.jpca.6b08642
- Quantification of the sources and composition of particulate matter by field-deployable mass spectrometry: implications for air quality and public health P. Hayes 10.1039/C6AN02378A
- WRF-Chem simulation of aerosol seasonal variability in the San Joaquin Valley L. Wu et al. 10.5194/acp-17-7291-2017
- Predicting wildfire particulate matter and hypothetical re-emission of radiological Cs-137 contamination incidents K. Baker et al. 10.1016/j.scitotenv.2021.148872
Saved (final revised paper)
Latest update: 04 Nov 2024
Short summary
This work details the evaluation of PM2.5 carbon, VOC precursors, and OH estimated by the CMAQ photochemical transport model using routine and special measurements from the 2010 CalNex field study. Here, CMAQ and most recent emissions inventory (2011 NEI) are used to generate model PM2.5 OC estimates that are examined in novel ways including primary vs. secondary formation, fossil vs. contemporary carbon, OH and HO2 evaluation, and the relationship between key VOC precursors and SOC tracers.
This work details the evaluation of PM2.5 carbon, VOC precursors, and OH estimated by the CMAQ...
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