Articles | Volume 15, issue 8
https://doi.org/10.5194/acp-15-4063-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-15-4063-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
17 Apr 2015
Research article |
| 17 Apr 2015
On the derivation of particle nucleation rates from experimental formation rates
A. Kürten
Institute for Atmospheric and Environmental Sciences, Goethe University of Frankfurt, 60438 Frankfurt am Main, Germany
C. Williamson
Institute for Atmospheric and Environmental Sciences, Goethe University of Frankfurt, 60438 Frankfurt am Main, Germany
J. Almeida
CERN, 1211 Geneva, Switzerland
J. Kirkby
Institute for Atmospheric and Environmental Sciences, Goethe University of Frankfurt, 60438 Frankfurt am Main, Germany
CERN, 1211 Geneva, Switzerland
J. Curtius
Institute for Atmospheric and Environmental Sciences, Goethe University of Frankfurt, 60438 Frankfurt am Main, Germany
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- Global atmospheric particle formation from CERN CLOUD measurements E. Dunne et al. 10.1126/science.aaf2649
- Peroxy radical kinetics and new particle formation M. Schervish & N. Donahue 10.1039/D0EA00017E
- Effect of Relative Humidity on the Rate of New Particle Formation for Different VOCs A. Flueckiger & G. Petrucci 10.3390/atmos15040480
- Atmospheric new particle formation from the CERN CLOUD experiment J. Kirkby et al. 10.1038/s41561-023-01305-0
- Ion-induced nucleation of pure biogenic particles J. Kirkby et al. 10.1038/nature17953
- The ION‐CAGE Code: A Numerical Model for the Growth of Charged and Neutral Aerosols J. Svensmark et al. 10.1029/2020EA001142
- Estimation of atmospheric particle formation rates through an analytical formula: validation and application in Hyytiälä and Puijo, Finland E. Baranizadeh et al. 10.5194/acp-17-13361-2017
- What controls the observed size-dependency of the growth rates of sub-10 nm atmospheric particles? J. Kontkanen et al. 10.1039/D1EA00103E
- Reducing chemical complexity in representation of new-particle formation: evaluation of simplification approaches T. Olenius et al. 10.1039/D2EA00174H
- Extrapolating particle concentration along the size axis in the nanometer size range requires discrete rate equations T. Olenius et al. 10.1016/j.jaerosci.2015.07.004
- New particle formation in the sulfuric acid–dimethylamine–water system: reevaluation of CLOUD chamber measurements and comparison to an aerosol nucleation and growth model A. Kürten et al. 10.5194/acp-18-845-2018
- Formation and growth of sub-3-nm aerosol particles in experimental chambers L. Dada et al. 10.1038/s41596-019-0274-z
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- Aerosol formation and growth rates from chamber experiments using Kalman smoothing M. Ozon et al. 10.5194/acp-21-12595-2021
- Robust metric for quantifying the importance of stochastic effects on nanoparticle growth T. Olenius et al. 10.1038/s41598-018-32610-z
- Atmospheric new particle formation and growth: review of field observations V. Kerminen et al. 10.1088/1748-9326/aadf3c
- Current state of aerosol nucleation parameterizations for air-quality and climate modeling K. Semeniuk & A. Dastoor 10.1016/j.atmosenv.2018.01.039
- On Nucleation Pathways and Particle Size Distribution Evolutions in Stratospheric Aircraft Exhaust Plumes with H2SO4 Enhancement F. Yu et al. 10.1021/acs.est.3c08408
- Effect of ions on sulfuric acid‐water binary particle formation: 2. Experimental data and comparison with QC‐normalized classical nucleation theory J. Duplissy et al. 10.1002/2015JD023539
- New particle formation from sulfuric acid and ammonia: nucleation and growth model based on thermodynamics derived from CLOUD measurements for a wide range of conditions A. Kürten 10.5194/acp-19-5033-2019
- Exploring the potential of nano-Köhler theory to describe the growth of atmospheric molecular clusters by organic vapors using cluster kinetics simulations J. Kontkanen et al. 10.5194/acp-18-13733-2018
- In situ observation of new particle formation (NPF) in the tropical tropopause layer of the 2017 Asian monsoon anticyclone – Part 2: NPF inside ice clouds R. Weigel et al. 10.5194/acp-21-13455-2021
- Constraints on global aerosol number concentration, SO<sub>2</sub> and condensation sink in UKESM1 using ATom measurements A. Ranjithkumar et al. 10.5194/acp-21-4979-2021
- Contribution of new particle formation to the total aerosol concentration at the high‐altitude site Jungfraujoch (3580 m asl, Switzerland) J. Tröstl et al. 10.1002/2015JD024637
- H<sub>2</sub>SO<sub>4</sub> and particle production in a photolytic flow reactor: chemical modeling, cluster thermodynamics and contamination issues D. Hanson et al. 10.5194/acp-19-8999-2019
- Atmospheric Nanoparticle Survivability Reduction Due to Charge‐Induced Coagulation Scavenging Enhancement N. Mahfouz & N. Donahue 10.1029/2021GL092758
28 citations as recorded by crossref.
- Molecular understanding of new-particle formation from <i>α</i>-pinene between −50 and +25 °C M. Simon et al. 10.5194/acp-20-9183-2020
- Surface-active organic matter induces salt morphology transitions during new atmospheric particle formation and growth V. Daskalakis et al. 10.1039/C5RA09187J
- Global atmospheric particle formation from CERN CLOUD measurements E. Dunne et al. 10.1126/science.aaf2649
- Peroxy radical kinetics and new particle formation M. Schervish & N. Donahue 10.1039/D0EA00017E
- Effect of Relative Humidity on the Rate of New Particle Formation for Different VOCs A. Flueckiger & G. Petrucci 10.3390/atmos15040480
- Atmospheric new particle formation from the CERN CLOUD experiment J. Kirkby et al. 10.1038/s41561-023-01305-0
- Ion-induced nucleation of pure biogenic particles J. Kirkby et al. 10.1038/nature17953
- The ION‐CAGE Code: A Numerical Model for the Growth of Charged and Neutral Aerosols J. Svensmark et al. 10.1029/2020EA001142
- Estimation of atmospheric particle formation rates through an analytical formula: validation and application in Hyytiälä and Puijo, Finland E. Baranizadeh et al. 10.5194/acp-17-13361-2017
- What controls the observed size-dependency of the growth rates of sub-10 nm atmospheric particles? J. Kontkanen et al. 10.1039/D1EA00103E
- Reducing chemical complexity in representation of new-particle formation: evaluation of simplification approaches T. Olenius et al. 10.1039/D2EA00174H
- Extrapolating particle concentration along the size axis in the nanometer size range requires discrete rate equations T. Olenius et al. 10.1016/j.jaerosci.2015.07.004
- New particle formation in the sulfuric acid–dimethylamine–water system: reevaluation of CLOUD chamber measurements and comparison to an aerosol nucleation and growth model A. Kürten et al. 10.5194/acp-18-845-2018
- Formation and growth of sub-3-nm aerosol particles in experimental chambers L. Dada et al. 10.1038/s41596-019-0274-z
- Sources and sinks driving sulfuric acid concentrations in contrasting environments: implications on proxy calculations L. Dada et al. 10.5194/acp-20-11747-2020
- Aerosol formation and growth rates from chamber experiments using Kalman smoothing M. Ozon et al. 10.5194/acp-21-12595-2021
- Robust metric for quantifying the importance of stochastic effects on nanoparticle growth T. Olenius et al. 10.1038/s41598-018-32610-z
- Atmospheric new particle formation and growth: review of field observations V. Kerminen et al. 10.1088/1748-9326/aadf3c
- Current state of aerosol nucleation parameterizations for air-quality and climate modeling K. Semeniuk & A. Dastoor 10.1016/j.atmosenv.2018.01.039
- On Nucleation Pathways and Particle Size Distribution Evolutions in Stratospheric Aircraft Exhaust Plumes with H2SO4 Enhancement F. Yu et al. 10.1021/acs.est.3c08408
- Effect of ions on sulfuric acid‐water binary particle formation: 2. Experimental data and comparison with QC‐normalized classical nucleation theory J. Duplissy et al. 10.1002/2015JD023539
- New particle formation from sulfuric acid and ammonia: nucleation and growth model based on thermodynamics derived from CLOUD measurements for a wide range of conditions A. Kürten 10.5194/acp-19-5033-2019
- Exploring the potential of nano-Köhler theory to describe the growth of atmospheric molecular clusters by organic vapors using cluster kinetics simulations J. Kontkanen et al. 10.5194/acp-18-13733-2018
- In situ observation of new particle formation (NPF) in the tropical tropopause layer of the 2017 Asian monsoon anticyclone – Part 2: NPF inside ice clouds R. Weigel et al. 10.5194/acp-21-13455-2021
- Constraints on global aerosol number concentration, SO<sub>2</sub> and condensation sink in UKESM1 using ATom measurements A. Ranjithkumar et al. 10.5194/acp-21-4979-2021
- Contribution of new particle formation to the total aerosol concentration at the high‐altitude site Jungfraujoch (3580 m asl, Switzerland) J. Tröstl et al. 10.1002/2015JD024637
- H<sub>2</sub>SO<sub>4</sub> and particle production in a photolytic flow reactor: chemical modeling, cluster thermodynamics and contamination issues D. Hanson et al. 10.5194/acp-19-8999-2019
- Atmospheric Nanoparticle Survivability Reduction Due to Charge‐Induced Coagulation Scavenging Enhancement N. Mahfouz & N. Donahue 10.1029/2021GL092758
Saved (final revised paper)
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Latest update: 23 Apr 2024
Short summary
The manuscript provides insights into the calculation of new particle formation rates. Generally, formation rates are measured at a diameter which can be substantially larger than the critical size of the newly formed particles. In order to transform the formation rate to a smaller size, a correction needs to be applied. We present a new method to apply this correction which takes into account the effect of self-coagulation.
The manuscript provides insights into the calculation of new particle formation rates....
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