Articles | Volume 15, issue 4
https://doi.org/10.5194/acp-15-2019-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-15-2019-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
24 Feb 2015
Research article |
| 24 Feb 2015
Contribution of liquid, NAT and ice particles to chlorine activation and ozone depletion in Antarctic winter and spring
Karlsruhe Institute of Technology, Steinbuch Centre for Computing (SCC), Karlsruhe, Germany
R. Müller
Research Centre Jülich GmbH, Institute of Energy and Climate Research – Stratosphere (IEK-7), Jülich, Germany
R. Ruhnke
Karlsruhe Institute of Technology, Institute for Meteorology and Climate Research (IMK), Karlsruhe, Germany
H. Fischer
Karlsruhe Institute of Technology, Institute for Meteorology and Climate Research (IMK), Karlsruhe, Germany
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27 citations as recorded by crossref.
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- The relevance of reactions of the methyl peroxy radical (CH<sub>3</sub>O<sub>2</sub>) and methylhypochlorite (CH<sub>3</sub>OCl) for Antarctic chlorine activation and ozone loss A. Zafar et al. 10.1080/16000889.2018.1507391
- Variability of water vapour in the Arctic stratosphere L. Thölix et al. 10.5194/acp-16-4307-2016
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- Proton Transfer Rates in Ionized Hydrogen Chloride–Water Clusters: A Direct Ab Initio Molecular Dynamics Study H. Tachikawa 10.1021/acs.jpca.7b05112
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- Electron-triggered chemistry in HNO3/H2O complexes J. Lengyel et al. 10.1039/C7CP01205E
- Linking uncertainty in simulated Arctic ozone loss to uncertainties in modelled tropical stratospheric water vapour L. Thölix et al. 10.5194/acp-18-15047-2018
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- The MIPAS/Envisat climatology (2002–2012) of polar stratospheric cloud volume density profiles M. Höpfner et al. 10.5194/amt-11-5901-2018
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27 citations as recorded by crossref.
- Evaluation of polar stratospheric clouds in the global chemistry–climate model SOCOLv3.1 by comparison with CALIPSO spaceborne lidar measurements M. Steiner et al. 10.5194/gmd-14-935-2021
- Earth’s atmosphere protects the biosphere from nearby supernovae T. Christoudias et al. 10.1038/s43247-024-01490-9
- Chemistry of NOx and HNO3 Molecules with Gas‐Phase Hydrated O.− and OH− Ions J. Lengyel et al. 10.1002/chem.202000322
- Statistical analysis of observations of polar stratospheric clouds with a lidar in Kiruna, northern Sweden P. Voelger & P. Dalin 10.5194/acp-23-5551-2023
- Polar Stratospheric Clouds: Satellite Observations, Processes, and Role in Ozone Depletion I. Tritscher et al. 10.1029/2020RG000702
- The impact of dehydration and extremely low HCl values in the Antarctic stratospheric vortex in mid-winter on ozone loss in spring Y. Zhang-Liu et al. 10.5194/acp-24-12557-2024
- The relevance of reactions of the methyl peroxy radical (CH<sub>3</sub>O<sub>2</sub>) and methylhypochlorite (CH<sub>3</sub>OCl) for Antarctic chlorine activation and ozone loss A. Zafar et al. 10.1080/16000889.2018.1507391
- Variability of water vapour in the Arctic stratosphere L. Thölix et al. 10.5194/acp-16-4307-2016
- Ozone depletion in the Arctic and Antarctic stratosphere induced by wildfire smoke A. Ansmann et al. 10.5194/acp-22-11701-2022
- A climatology of polar stratospheric cloud composition between 2002 and 2012 based on MIPAS/Envisat observations R. Spang et al. 10.5194/acp-18-5089-2018
- Australian wildfire smoke in the stratosphere: the decay phase in 2020/2021 and impact on ozone depletion K. Ohneiser et al. 10.5194/acp-22-7417-2022
- Record Low Arctic Stratospheric Ozone in Spring 2020: Measurements of Ground-Based Differential Optical Absorption Spectroscopy in Ny-Ålesund during 2017–2021 Q. Li et al. 10.3390/rs15194882
- The relationship between lower-stratospheric ozone at southern high latitudes and sea surface temperature in the East Asian marginal seas in austral spring W. Tian et al. 10.5194/acp-17-6705-2017
- A new method to detect and classify polar stratospheric nitric acid trihydrate clouds derived from radiative transfer simulations and its first application to airborne infrared limb emission observations C. Kalicinsky et al. 10.5194/amt-14-1893-2021
- Vortex-wide chlorine activation by a mesoscale PSC event in the Arctic winter of 2009/10 T. Wegner et al. 10.5194/acp-16-4569-2016
- Comparison of ECHAM5/MESSy Atmospheric Chemistry (EMAC) simulations of the Arctic winter 2009/2010 and 2010/2011 with Envisat/MIPAS and Aura/MLS observations F. Khosrawi et al. 10.5194/acp-18-8873-2018
- Proton Transfer Rates in Ionized Hydrogen Chloride–Water Clusters: A Direct Ab Initio Molecular Dynamics Study H. Tachikawa 10.1021/acs.jpca.7b05112
- Partitioning and budget of inorganic and organic chlorine species observed by MIPAS-B and TELIS in the Arctic in March 2011 G. Wetzel et al. 10.5194/acp-15-8065-2015
- Lagrangian simulation of ice particles and resulting dehydration in the polar winter stratosphere I. Tritscher et al. 10.5194/acp-19-543-2019
- Infrared transmittance spectra of polar stratospheric clouds M. Lecours et al. 10.1016/j.jqsrt.2022.108406
- Coupled Stratospheric Chemistry–Meteorology Data Assimilation. Part I: Physical Background and Coupled Modeling Aspects R. Ménard et al. 10.3390/atmos11020150
- Electron-triggered chemistry in HNO3/H2O complexes J. Lengyel et al. 10.1039/C7CP01205E
- Linking uncertainty in simulated Arctic ozone loss to uncertainties in modelled tropical stratospheric water vapour L. Thölix et al. 10.5194/acp-18-15047-2018
- Spatio-temporal variations of nitric acid total columns from 9 years of IASI measurements – a driver study G. Ronsmans et al. 10.5194/acp-18-4403-2018
- The MIPAS/Envisat climatology (2002–2012) of polar stratospheric cloud volume density profiles M. Höpfner et al. 10.5194/amt-11-5901-2018
- Paul J. Crutzen – a pioneer in Earth system science and a founding member of the journal Atmospheric Chemistry and Physics R. Müller et al. 10.5194/acp-23-15445-2023
- Exceptional loss in ozone in the Arctic winter/spring of 2019/2020 J. Kuttippurath et al. 10.5194/acp-21-14019-2021
Saved (final revised paper)
Saved (preprint)
Latest update: 21 Nov 2024
Short summary
We use multi-year simulations of the chemistry--climate model EMAC to investigate
the impact that the various types of PSCs have on Antarctic chlorine activation and ozone loss. Heterogeneous chemistry on liquid particles is responsible for more than 90% of the ozone depletion in Antarctic spring in the model simulations. In high southern latitudes, heterogeneous chemistry on ice particles causes only up to 5 DU of additional ozone depletion and chemistry on NAT particles less than 0.5 DU.
We use multi-year simulations of the chemistry--climate model EMAC to investigate
the impact...
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