Articles | Volume 15, issue 22
https://doi.org/10.5194/acp-15-12989-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-15-12989-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
24 Nov 2015
Research article |
| 24 Nov 2015
Impact of gas-to-particle partitioning approaches on the simulated radiative effects of biogenic secondary organic aerosol
School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, UK
D. V. Spracklen
School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, UK
J. R. Pierce
Department of Atmospheric Science, Colorado State University, Ft. Collins, CO, USA
I. Riipinen
Department of Applied Environmental Science & Bolin Centre for Climate Research, Stockholm University, 10691 Stockholm, Sweden
S. D. D'Andrea
Department of Atmospheric Science, Colorado State University, Ft. Collins, CO, USA
School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, UK
K. S. Carslaw
School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, UK
P. M. Forster
School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, UK
P. Artaxo
Institute of Physics, University of São Paulo, São Paulo, Brazil
M. Kulmala
Department of Physics, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
L. V. Rizzo
Department of Earth and Exact Sciences, Institute of Environmental, Chemical and Pharmaceutics Sciences, Federal University of São Paulo, UNIFESP, Diadema, Brazil
E. Swietlicki
Division of Nuclear Physics, Lund University, P.O. Box 118, 221 00 Lund, Sweden
Centre for Environmental and Climate Research, Lund University, P.O. Box 118, 221 00 Lund, Sweden
G. W. Mann
School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, UK
National Centre for Atmospheric Science, University of Leeds, Leeds, LS2 9JT, UK
K. J. Pringle
School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, UK
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Latest update: 06 Dec 2025
Short summary
To understand the radiative effects of biogenic secondary organic aerosol (SOA) it is necessary to consider the manner in which it is distributed across the existing aerosol size distribution. We explore the importance of the approach taken by global-scale models to do this, when calculating the direct radiative effect (DRE) & first aerosol indirect effect (AIE) due to biogenic SOA. This choice has little effect on the DRE, but a substantial impact on the magnitude and even sign of the first AIE
To understand the radiative effects of biogenic secondary organic aerosol (SOA) it is necessary...
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