Articles | Volume 15, issue 22
https://doi.org/10.5194/acp-15-12989-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-15-12989-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
24 Nov 2015
Research article |
| 24 Nov 2015
Impact of gas-to-particle partitioning approaches on the simulated radiative effects of biogenic secondary organic aerosol
School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, UK
D. V. Spracklen
School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, UK
J. R. Pierce
Department of Atmospheric Science, Colorado State University, Ft. Collins, CO, USA
I. Riipinen
Department of Applied Environmental Science & Bolin Centre for Climate Research, Stockholm University, 10691 Stockholm, Sweden
S. D. D'Andrea
Department of Atmospheric Science, Colorado State University, Ft. Collins, CO, USA
School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, UK
K. S. Carslaw
School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, UK
P. M. Forster
School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, UK
P. Artaxo
Institute of Physics, University of São Paulo, São Paulo, Brazil
M. Kulmala
Department of Physics, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
L. V. Rizzo
Department of Earth and Exact Sciences, Institute of Environmental, Chemical and Pharmaceutics Sciences, Federal University of São Paulo, UNIFESP, Diadema, Brazil
E. Swietlicki
Division of Nuclear Physics, Lund University, P.O. Box 118, 221 00 Lund, Sweden
Centre for Environmental and Climate Research, Lund University, P.O. Box 118, 221 00 Lund, Sweden
G. W. Mann
School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, UK
National Centre for Atmospheric Science, University of Leeds, Leeds, LS2 9JT, UK
K. J. Pringle
School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, UK
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31 citations as recorded by crossref.
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- Enhanced global primary production by biogenic aerosol via diffuse radiation fertilization A. Rap et al. 10.1038/s41561-018-0208-3
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- Nonequilibrium Behavior in Isoprene Secondary Organic Aerosol Y. Chen et al. 10.1021/acs.est.3c03532
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- Morphology and Viscosity Changes after Reactive Uptake of Isoprene Epoxydiols in Submicrometer Phase Separated Particles with Secondary Organic Aerosol Formed from Different Volatile Organic Compounds Z. Lei et al. 10.1021/acsearthspacechem.1c00156
- Can semi-volatile organic aerosols lead to fewer cloud particles? C. Gao et al. 10.5194/acp-18-14243-2018
- Aircraft observations of the chemical composition and aging of aerosol in the Manaus urban plume during GoAmazon 2014/5 J. Shilling et al. 10.5194/acp-18-10773-2018
- Phase state of ambient aerosol linked with water uptake and chemical aging in the southeastern US A. Pajunoja et al. 10.5194/acp-16-11163-2016
- Photochemical Aging Alters Secondary Organic Aerosol Partitioning Behavior J. Shilling et al. 10.1021/acsearthspacechem.9b00248
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- Causes and importance of new particle formation in the present‐day and preindustrial atmospheres H. Gordon et al. 10.1002/2017JD026844
- Decrease in sulfate aerosol light backscattering by reactive uptake of isoprene epoxydiols C. Dubois et al. 10.1039/D0CP05468B
- Impact on short-lived climate forcers (SLCFs) from a realistic land-use change scenario via changes in biogenic emissions C. Scott et al. 10.1039/C7FD00028F
- Multiple new-particle growth pathways observed at the US DOE Southern Great Plains field site A. Hodshire et al. 10.5194/acp-16-9321-2016
- NMVOC emissions and their formation into secondary organic aerosols over India using WRF-Chem model S. Azmi et al. 10.1016/j.atmosenv.2022.119254
- Design and application of a novel integrated microsampling system for simultaneous collection of gas- and particle-phase semivolatile organic compounds T. Xu et al. 10.1016/j.atmosenv.2016.11.022
- Open questions on atmospheric nanoparticle growth T. Yli-Juuti et al. 10.1038/s42004-020-00339-4
- Current State of Atmospheric Aerosol Thermodynamics and Mass Transfer Modeling: A Review K. Semeniuk & A. Dastoor 10.3390/atmos11020156
- Growth Kinetics and Size Distribution Dynamics of Viscous Secondary Organic Aerosol R. Zaveri et al. 10.1021/acs.est.7b04623
- Ozonolysis Chemistry and Phase Behavior of 1-Octen-3-ol-Derived Secondary Organic Aerosol K. Fischer et al. 10.1021/acsearthspacechem.0c00092
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- The Influence of Absolute Mass Loading of Secondary Organic Aerosols on Their Phase State S. Jain et al. 10.3390/atmos9040131
- The roles of volatile organic compound deposition and oxidation mechanisms in determining secondary organic aerosol production: a global perspective using the UKCA chemistry–climate model (vn8.4) J. Kelly et al. 10.5194/gmd-12-2539-2019
- Changes in biodiversity impact atmospheric chemistry and climate through plant volatiles and particles A. Sanaei et al. 10.1038/s43247-023-01113-9
- The direct and indirect radiative effects of biogenic secondary organic aerosol C. Scott et al. 10.5194/acp-14-447-2014
30 citations as recorded by crossref.
- Particle-Phase Diffusion Modulates Partitioning of Semivolatile Organic Compounds to Aged Secondary Organic Aerosol R. Zaveri et al. 10.1021/acs.est.9b05514
- Aerosol characteristics at the Southern Great Plains site during the HI-SCALE campaign J. Liu et al. 10.5194/acp-21-5101-2021
- Atmospheric nanoparticle growth D. Stolzenburg et al. 10.1103/RevModPhys.95.045002
- Modeling the role of highly oxidized multifunctional organic molecules for the growth of new particles over the boreal forest region E. Öström et al. 10.5194/acp-17-8887-2017
- Enhanced global primary production by biogenic aerosol via diffuse radiation fertilization A. Rap et al. 10.1038/s41561-018-0208-3
- Biogenic volatile organic compounds from 14 landscape woody species: Tree species selection in the construction of urban greenspace with forest healthcare effects J. Wu et al. 10.1016/j.jenvman.2021.113761
- Rapid growth of anthropogenic organic nanoparticles greatly alters cloud life cycle in the Amazon rainforest R. Zaveri et al. 10.1126/sciadv.abj0329
- MATRIX-VBS (v1.0): implementing an evolving organic aerosol volatility in an aerosol microphysics model C. Gao et al. 10.5194/gmd-10-751-2017
- Nonequilibrium Behavior in Isoprene Secondary Organic Aerosol Y. Chen et al. 10.1021/acs.est.3c03532
- The impact of biogenic, anthropogenic, and biomass burning volatile organic compound emissions on regional and seasonal variations in secondary organic aerosol J. Kelly et al. 10.5194/acp-18-7393-2018
- Morphology and Viscosity Changes after Reactive Uptake of Isoprene Epoxydiols in Submicrometer Phase Separated Particles with Secondary Organic Aerosol Formed from Different Volatile Organic Compounds Z. Lei et al. 10.1021/acsearthspacechem.1c00156
- Can semi-volatile organic aerosols lead to fewer cloud particles? C. Gao et al. 10.5194/acp-18-14243-2018
- Aircraft observations of the chemical composition and aging of aerosol in the Manaus urban plume during GoAmazon 2014/5 J. Shilling et al. 10.5194/acp-18-10773-2018
- Phase state of ambient aerosol linked with water uptake and chemical aging in the southeastern US A. Pajunoja et al. 10.5194/acp-16-11163-2016
- Photochemical Aging Alters Secondary Organic Aerosol Partitioning Behavior J. Shilling et al. 10.1021/acsearthspacechem.9b00248
- Gas-phase kinetics modifies the CCN activity of a biogenic SOA A. Vizenor & A. Asa-Awuku 10.1039/C8CP00075A
- Causes and importance of new particle formation in the present‐day and preindustrial atmospheres H. Gordon et al. 10.1002/2017JD026844
- Decrease in sulfate aerosol light backscattering by reactive uptake of isoprene epoxydiols C. Dubois et al. 10.1039/D0CP05468B
- Impact on short-lived climate forcers (SLCFs) from a realistic land-use change scenario via changes in biogenic emissions C. Scott et al. 10.1039/C7FD00028F
- Multiple new-particle growth pathways observed at the US DOE Southern Great Plains field site A. Hodshire et al. 10.5194/acp-16-9321-2016
- NMVOC emissions and their formation into secondary organic aerosols over India using WRF-Chem model S. Azmi et al. 10.1016/j.atmosenv.2022.119254
- Design and application of a novel integrated microsampling system for simultaneous collection of gas- and particle-phase semivolatile organic compounds T. Xu et al. 10.1016/j.atmosenv.2016.11.022
- Open questions on atmospheric nanoparticle growth T. Yli-Juuti et al. 10.1038/s42004-020-00339-4
- Current State of Atmospheric Aerosol Thermodynamics and Mass Transfer Modeling: A Review K. Semeniuk & A. Dastoor 10.3390/atmos11020156
- Growth Kinetics and Size Distribution Dynamics of Viscous Secondary Organic Aerosol R. Zaveri et al. 10.1021/acs.est.7b04623
- Ozonolysis Chemistry and Phase Behavior of 1-Octen-3-ol-Derived Secondary Organic Aerosol K. Fischer et al. 10.1021/acsearthspacechem.0c00092
- A global model perturbed parameter ensemble study of secondary organic aerosol formation K. Sengupta et al. 10.5194/acp-21-2693-2021
- The Influence of Absolute Mass Loading of Secondary Organic Aerosols on Their Phase State S. Jain et al. 10.3390/atmos9040131
- The roles of volatile organic compound deposition and oxidation mechanisms in determining secondary organic aerosol production: a global perspective using the UKCA chemistry–climate model (vn8.4) J. Kelly et al. 10.5194/gmd-12-2539-2019
- Changes in biodiversity impact atmospheric chemistry and climate through plant volatiles and particles A. Sanaei et al. 10.1038/s43247-023-01113-9
1 citations as recorded by crossref.
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Latest update: 21 Nov 2024
Short summary
To understand the radiative effects of biogenic secondary organic aerosol (SOA) it is necessary to consider the manner in which it is distributed across the existing aerosol size distribution. We explore the importance of the approach taken by global-scale models to do this, when calculating the direct radiative effect (DRE) & first aerosol indirect effect (AIE) due to biogenic SOA. This choice has little effect on the DRE, but a substantial impact on the magnitude and even sign of the first AIE
To understand the radiative effects of biogenic secondary organic aerosol (SOA) it is necessary...
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