Articles | Volume 15, issue 18
https://doi.org/10.5194/acp-15-10281-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Special issue:
https://doi.org/10.5194/acp-15-10281-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Constraining black carbon aerosol over Asia using OMI aerosol absorption optical depth and the adjoint of GEOS-Chem
L. Zhang
Department of Mechanical Engineering, University of Colorado, Boulder, CO, USA
Global Systems Division, Earth System Research Laboratory, NOAA, Boulder, CO, USA
D. K. Henze
CORRESPONDING AUTHOR
Department of Mechanical Engineering, University of Colorado, Boulder, CO, USA
G. A. Grell
Global Systems Division, Earth System Research Laboratory, NOAA, Boulder, CO, USA
G. R. Carmichael
Department of Chemical and Biochemical Engineering, University of Iowa, Iowa City, IA, USA
N. Bousserez
Department of Mechanical Engineering, University of Colorado, Boulder, CO, USA
Q. Zhang
Center for Earth System Science, Tsinghua University, Beijing, China
O. Torres
NASA Goddard Space Flight Center, Greenbelt, MD, USA
C. Ahn
Science Systems and Applications, Inc., Lanham, MD, USA
Z. Lu
Energy Systems Division, Argonne National Laboratory, Argonne, IL, USA
J. Cao
Key Lab of Aerosol Chemistry & Physics, Institute of Earth Environment, Chinese Academy of Sciences, Xi'an, China
Y. Mao
Department of Atmospheric and Oceanic Sciences, University of California, Los Angeles, CA, USA
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, China
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Saved (final revised paper)
Latest update: 21 Nov 2024
Short summary
We attempt to reduce uncertainties in BC emissions and improve BC model simulations by developing top-down, spatially resolved, estimates of BC emissions through assimilation of OMI observations of aerosol absorption optical depth (AAOD) with the GEOS-Chem model and its adjoint for April and October of 2006. Despite the limitations and uncertainties, using OMI AAOD to constrain BC sources we are able to improve model representation of BC distributions, particularly over China.
We attempt to reduce uncertainties in BC emissions and improve BC model simulations by...
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