Articles | Volume 14, issue 21
https://doi.org/10.5194/acp-14-11853-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-14-11853-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Biogenic SOA formation through gas-phase oxidation and gas-to-particle partitioning – a comparison between process models of varying complexity
E. Hermansson
CORRESPONDING AUTHOR
Division of Nuclear Physics, Lund University, P.O. Box 118, 221 00, Lund, Sweden
Centre for Environmental and Climate Research, Lund University, P.O. Box 118, 221 00, Lund, Sweden
P. Roldin
Division of Nuclear Physics, Lund University, P.O. Box 118, 221 00, Lund, Sweden
Department of Physics, P.O. Box 64, 00014 University of Helsinki, Helsinki, Finland
A. Rusanen
Department of Physics, P.O. Box 64, 00014 University of Helsinki, Helsinki, Finland
D. Mogensen
Department of Physics, P.O. Box 64, 00014 University of Helsinki, Helsinki, Finland
N. Kivekäs
Division of Nuclear Physics, Lund University, P.O. Box 118, 221 00, Lund, Sweden
now at: Atmospheric Composition, Finnish Meteorological Institute, P.O. Box 503, 00101, Helsinki, Finland
R. Väänänen
Department of Physics, P.O. Box 64, 00014 University of Helsinki, Helsinki, Finland
M. Boy
Department of Physics, P.O. Box 64, 00014 University of Helsinki, Helsinki, Finland
E. Swietlicki
Division of Nuclear Physics, Lund University, P.O. Box 118, 221 00, Lund, Sweden
Centre for Environmental and Climate Research, Lund University, P.O. Box 118, 221 00, Lund, Sweden
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Cited
8 citations as recorded by crossref.
- Online chemical characterization of atmospheric fine secondary aerosols and organic nitrates in summer Nanjing, China J. Xian et al. https://doi.org/10.1016/j.atmosres.2023.106783
- Simulation of atmospheric organic aerosol using its volatility–oxygen-content distribution during the PEGASOS 2012 campaign E. Karnezi et al. https://doi.org/10.5194/acp-18-10759-2018
- Modelling the contribution of biogenic volatile organic compounds to new particle formation in the Jülich plant atmosphere chamber P. Roldin et al. https://doi.org/10.5194/acp-15-10777-2015
- Modeling the role of highly oxidized multifunctional organic molecules for the growth of new particles over the boreal forest region E. Öström et al. https://doi.org/10.5194/acp-17-8887-2017
- Sources, seasonality, and trends of southeast US aerosol: an integrated analysis of surface, aircraft, and satellite observations with the GEOS-Chem chemical transport model P. Kim et al. https://doi.org/10.5194/acp-15-10411-2015
- A parameterisation for the co-condensation of semi-volatile organics into multiple aerosol particle modes M. Crooks et al. https://doi.org/10.5194/gmd-11-3261-2018
- Multi-year statistical and modeling analysis of submicrometer aerosol number size distributions at a rain forest site in Amazonia L. Varanda Rizzo et al. https://doi.org/10.5194/acp-18-10255-2018
- Interactions between the atmosphere, cryosphere, and ecosystems at northern high latitudes M. Boy et al. https://doi.org/10.5194/acp-19-2015-2019
8 citations as recorded by crossref.
- Online chemical characterization of atmospheric fine secondary aerosols and organic nitrates in summer Nanjing, China J. Xian et al. https://doi.org/10.1016/j.atmosres.2023.106783
- Simulation of atmospheric organic aerosol using its volatility–oxygen-content distribution during the PEGASOS 2012 campaign E. Karnezi et al. https://doi.org/10.5194/acp-18-10759-2018
- Modelling the contribution of biogenic volatile organic compounds to new particle formation in the Jülich plant atmosphere chamber P. Roldin et al. https://doi.org/10.5194/acp-15-10777-2015
- Modeling the role of highly oxidized multifunctional organic molecules for the growth of new particles over the boreal forest region E. Öström et al. https://doi.org/10.5194/acp-17-8887-2017
- Sources, seasonality, and trends of southeast US aerosol: an integrated analysis of surface, aircraft, and satellite observations with the GEOS-Chem chemical transport model P. Kim et al. https://doi.org/10.5194/acp-15-10411-2015
- A parameterisation for the co-condensation of semi-volatile organics into multiple aerosol particle modes M. Crooks et al. https://doi.org/10.5194/gmd-11-3261-2018
- Multi-year statistical and modeling analysis of submicrometer aerosol number size distributions at a rain forest site in Amazonia L. Varanda Rizzo et al. https://doi.org/10.5194/acp-18-10255-2018
- Interactions between the atmosphere, cryosphere, and ecosystems at northern high latitudes M. Boy et al. https://doi.org/10.5194/acp-19-2015-2019
Saved (final revised paper)
Latest update: 24 Jun 2026
Short summary
Secondary organic aerosols (SOA), produced through oxidation processes, constitute a large part of the global organic aerosol load and affect the climate. We found that the modeled mass of SOA was highly dependent on how the oxidation processes were explained in models. The results indicated that it was especially important to get the volatility distribution of the products from the first oxidation step right and that fragmentation during the oxidation process played an important role.
Secondary organic aerosols (SOA), produced through oxidation processes, constitute a large part...
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