Articles | Volume 14, issue 19
https://doi.org/10.5194/acp-14-10761-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-14-10761-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
13 Oct 2014
Research article |
| 13 Oct 2014
The influence of physical state on shikimic acid ozonolysis: a case for in situ microspectroscopy
S. S. Steimer
Swiss Federal Institute of Technology Zurich, Institute for Atmospheric and Climate Science, 8092 Zurich, Switzerland
Paul Scherrer Institute, Laboratory of Radio- and Environmental Chemistry, 5232 Villigen PSI, Switzerland
M. Lampimäki
now at: University of Helsinki, Viikki Teacher Training School, 00014 University of Helsinki, Finland
Paul Scherrer Institute, Laboratory of Radio- and Environmental Chemistry, 5232 Villigen PSI, Switzerland
Centro de Investigaciones Energéticas, Medioambientales y Tecnológicas, Department of the Environment, 28040 Madrid, Spain
G. Grzinic
University of Bern, Department of Chemistry and Biochemistry, 3012 Bern, Switzerland
Paul Scherrer Institute, Laboratory of Radio- and Environmental Chemistry, 5232 Villigen PSI, Switzerland
M. Ammann
Paul Scherrer Institute, Laboratory of Radio- and Environmental Chemistry, 5232 Villigen PSI, Switzerland
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Cited
40 citations as recorded by crossref.
- Humidity-Dependent Viscosity of Secondary Organic Aerosol from Ozonolysis of β-Caryophyllene: Measurements, Predictions, and Implications A. Maclean et al. https://doi.org/10.1021/acsearthspacechem.0c00296
- The persistence of a proxy for cooking emissions in megacities: a kinetic study of the ozonolysis of self-assembled films by simultaneous small and wide angle X-ray scattering (SAXS/WAXS) and Raman microscopy A. Milsom et al. https://doi.org/10.1039/D0FD00088D
- Possible Effects of Ozone Chemistry on the Phase Behavior of Skin Oil and Cooking Oil Films and Particles Indoors S. Xu et al. https://doi.org/10.1021/acsearthspacechem.2c00092
- Multiphase Chemistry at the Atmosphere–Biosphere Interface Influencing Climate and Public Health in the Anthropocene U. Pöschl & M. Shiraiwa https://doi.org/10.1021/cr500487s
- Measurements and Predictions of Binary Component Aerosol Particle Viscosity Y. Song et al. https://doi.org/10.1021/acs.jpca.6b07835
- Size-dependent chemical ageing of oleic acid aerosol under dry and humidified conditions S. Al-Kindi et al. https://doi.org/10.5194/acp-16-15561-2016
- Relative humidity-dependent viscosity of secondary organic material from toluene photo-oxidation and possible implications for organic particulate matter over megacities M. Song et al. https://doi.org/10.5194/acp-16-8817-2016
- Liquid–liquid phase separation and viscosity within secondary organic aerosol generated from diesel fuel vapors M. Song et al. https://doi.org/10.5194/acp-19-12515-2019
- Global Distribution of the Phase State and Mixing Times within Secondary Organic Aerosol Particles in the Troposphere Based on Room-Temperature Viscosity Measurements A. Maclean et al. https://doi.org/10.1021/acsearthspacechem.1c00296
- MIMiX: a Multipurpose In situ Microreactor system for X-ray microspectroscopy to mimic atmospheric aerosol processing J. Förster et al. https://doi.org/10.5194/amt-13-3717-2020
- Measuring Mass-Based Hygroscopicity of Atmospheric Particles through in Situ Imaging D. Piens et al. https://doi.org/10.1021/acs.est.6b00793
- Electrodynamic balance measurements of thermodynamic, kinetic, and optical aerosol properties inaccessible to bulk methods S. Steimer et al. https://doi.org/10.5194/amt-8-2397-2015
- Shikimic acid ozonolysis kinetics of the transition from liquid aqueous solution to highly viscous glass S. Steimer et al. https://doi.org/10.1039/C5CP04544D
- Probing the Heterogeneous Ozonolysis of Squalene Nanoparticles by Photoemission M. Jacobs et al. https://doi.org/10.1021/acs.jpca.6b09061
- A new hot-stage microscopy technique for measuring temperature-dependent viscosities of aerosol particles and its application to farnesene secondary organic aerosol K. Kiland et al. https://doi.org/10.5194/amt-15-5545-2022
- Viscosity, Glass Formation, and Mixing Times within Secondary Organic Aerosol from Biomass Burning Phenolics K. Kiland et al. https://doi.org/10.1021/acsearthspacechem.3c00039
- Diffusion and reactivity in ultraviscous aerosol and the correlation with particle viscosity F. Marshall et al. https://doi.org/10.1039/C5SC03223G
- Diffusion of Organic Molecules as a Function of Temperature in a Sucrose Matrix (a Proxy for Secondary Organic Aerosol) K. Kiland et al. https://doi.org/10.1021/acs.jpclett.9b02182
- Study on the Mass transfer and hygroscopic behavior of glucose / ammonium sulfate aerosol droplets P. Chang & Z. Chen https://doi.org/10.1016/j.jaerosci.2024.106365
- Mass, charge, and radius of droplets in a linear quadrupole electrodynamic balance J. Davies https://doi.org/10.1080/02786826.2018.1559921
- Glass Formation Processes in Mixed Inorganic/Organic Aerosol Particles H. Dette & T. Koop https://doi.org/10.1021/jp5106967
- Particle-Phase Photosensitized Radical Production and Aerosol Aging P. Corral Arroyo et al. https://doi.org/10.1021/acs.est.8b00329
- Review of the bulk and surface chemistry of iron in atmospherically relevant systems containing humic-like substances H. Al-Abadleh https://doi.org/10.1039/C5RA03132J
- Amorphous phase state diagrams and viscosity of ternary aqueous organic/organic and inorganic/organic mixtures A. Marsh et al. https://doi.org/10.1039/C8CP00760H
- Microphysics of the aqueous bulk counters the water activity driven rate acceleration of bromide oxidation by ozone from 289–245 K J. Edebeli et al. https://doi.org/10.1039/C8EM00417J
- Elucidating the size distribution of p‑Phenylenediamine-Derived quinones in atmospheric particles K. Xia et al. https://doi.org/10.1016/j.envint.2025.109329
- The effect of viscosity and diffusion on the HO2 uptake by sucrose and secondary organic aerosol particles P. Lakey et al. https://doi.org/10.5194/acp-16-13035-2016
- Nitrate Photolysis in Mixed Sucrose–Nitrate–Sulfate Particles at Different Relative Humidities Z. Liang et al. https://doi.org/10.1021/acs.jpca.1c00669
- Imaging Molecular Reaction and Diffusion in Organic Aerosol Particles P. Alpert et al. https://doi.org/10.1017/S143192761801471X
- Secondary Organic Aerosol from Biomass Burning Phenolic Compounds and Nitrate Radicals can be Highly Viscous over a Wide Relative Humidity Range S. Nikkho et al. https://doi.org/10.1021/acs.est.4c06235
- Ozone uptake on glassy, semi-solid and liquid organic matter and the role of reactive oxygen intermediates in atmospheric aerosol chemistry T. Berkemeier et al. https://doi.org/10.1039/C6CP00634E
- Visualizing reaction and diffusion in xanthan gum aerosol particles exposed to ozone P. Alpert et al. https://doi.org/10.1039/C9CP03731D
- Phase Behavior and Viscosity in Biomass Burning Organic Aerosol and Climatic Impacts F. Gregson et al. https://doi.org/10.1021/acs.est.3c03231
- Photochemical degradation of iron(III) citrate/citric acid aerosol quantified with the combination of three complementary experimental techniques and a kinetic process model J. Dou et al. https://doi.org/10.5194/acp-21-315-2021
- Influence of particle viscosity on mass transfer and heterogeneous ozonolysis kinetics in aqueous–sucrose–maleic acid aerosol F. Marshall et al. https://doi.org/10.1039/C8CP01666F
- Ice nucleation imaged with X-ray spectro-microscopy P. Alpert et al. https://doi.org/10.1039/D1EA00077B
- Raman Spectroscopy of Isotopic Water Diffusion in Ultraviscous, Glassy, and Gel States in Aerosol by Use of Optical Tweezers J. Davies & K. Wilson https://doi.org/10.1021/acs.analchem.5b04315
- Viscosity and liquid–liquid phase separation in healthy and stressed plant SOA N. Smith et al. https://doi.org/10.1039/D0EA00020E
- Aerosol Hygroscopicity on A Single Particle Level Using Microscopic and Spectroscopic Techniques: A Review L. Wu & C. Ro https://doi.org/10.5572/ajae.2020.14.3.177
- Heterogeneous ozone oxidation of p-phenylenediamine antioxidants Z. Chen et al. https://doi.org/10.1016/j.jhazmat.2026.141745
40 citations as recorded by crossref.
- Humidity-Dependent Viscosity of Secondary Organic Aerosol from Ozonolysis of β-Caryophyllene: Measurements, Predictions, and Implications A. Maclean et al. https://doi.org/10.1021/acsearthspacechem.0c00296
- The persistence of a proxy for cooking emissions in megacities: a kinetic study of the ozonolysis of self-assembled films by simultaneous small and wide angle X-ray scattering (SAXS/WAXS) and Raman microscopy A. Milsom et al. https://doi.org/10.1039/D0FD00088D
- Possible Effects of Ozone Chemistry on the Phase Behavior of Skin Oil and Cooking Oil Films and Particles Indoors S. Xu et al. https://doi.org/10.1021/acsearthspacechem.2c00092
- Multiphase Chemistry at the Atmosphere–Biosphere Interface Influencing Climate and Public Health in the Anthropocene U. Pöschl & M. Shiraiwa https://doi.org/10.1021/cr500487s
- Measurements and Predictions of Binary Component Aerosol Particle Viscosity Y. Song et al. https://doi.org/10.1021/acs.jpca.6b07835
- Size-dependent chemical ageing of oleic acid aerosol under dry and humidified conditions S. Al-Kindi et al. https://doi.org/10.5194/acp-16-15561-2016
- Relative humidity-dependent viscosity of secondary organic material from toluene photo-oxidation and possible implications for organic particulate matter over megacities M. Song et al. https://doi.org/10.5194/acp-16-8817-2016
- Liquid–liquid phase separation and viscosity within secondary organic aerosol generated from diesel fuel vapors M. Song et al. https://doi.org/10.5194/acp-19-12515-2019
- Global Distribution of the Phase State and Mixing Times within Secondary Organic Aerosol Particles in the Troposphere Based on Room-Temperature Viscosity Measurements A. Maclean et al. https://doi.org/10.1021/acsearthspacechem.1c00296
- MIMiX: a Multipurpose In situ Microreactor system for X-ray microspectroscopy to mimic atmospheric aerosol processing J. Förster et al. https://doi.org/10.5194/amt-13-3717-2020
- Measuring Mass-Based Hygroscopicity of Atmospheric Particles through in Situ Imaging D. Piens et al. https://doi.org/10.1021/acs.est.6b00793
- Electrodynamic balance measurements of thermodynamic, kinetic, and optical aerosol properties inaccessible to bulk methods S. Steimer et al. https://doi.org/10.5194/amt-8-2397-2015
- Shikimic acid ozonolysis kinetics of the transition from liquid aqueous solution to highly viscous glass S. Steimer et al. https://doi.org/10.1039/C5CP04544D
- Probing the Heterogeneous Ozonolysis of Squalene Nanoparticles by Photoemission M. Jacobs et al. https://doi.org/10.1021/acs.jpca.6b09061
- A new hot-stage microscopy technique for measuring temperature-dependent viscosities of aerosol particles and its application to farnesene secondary organic aerosol K. Kiland et al. https://doi.org/10.5194/amt-15-5545-2022
- Viscosity, Glass Formation, and Mixing Times within Secondary Organic Aerosol from Biomass Burning Phenolics K. Kiland et al. https://doi.org/10.1021/acsearthspacechem.3c00039
- Diffusion and reactivity in ultraviscous aerosol and the correlation with particle viscosity F. Marshall et al. https://doi.org/10.1039/C5SC03223G
- Diffusion of Organic Molecules as a Function of Temperature in a Sucrose Matrix (a Proxy for Secondary Organic Aerosol) K. Kiland et al. https://doi.org/10.1021/acs.jpclett.9b02182
- Study on the Mass transfer and hygroscopic behavior of glucose / ammonium sulfate aerosol droplets P. Chang & Z. Chen https://doi.org/10.1016/j.jaerosci.2024.106365
- Mass, charge, and radius of droplets in a linear quadrupole electrodynamic balance J. Davies https://doi.org/10.1080/02786826.2018.1559921
- Glass Formation Processes in Mixed Inorganic/Organic Aerosol Particles H. Dette & T. Koop https://doi.org/10.1021/jp5106967
- Particle-Phase Photosensitized Radical Production and Aerosol Aging P. Corral Arroyo et al. https://doi.org/10.1021/acs.est.8b00329
- Review of the bulk and surface chemistry of iron in atmospherically relevant systems containing humic-like substances H. Al-Abadleh https://doi.org/10.1039/C5RA03132J
- Amorphous phase state diagrams and viscosity of ternary aqueous organic/organic and inorganic/organic mixtures A. Marsh et al. https://doi.org/10.1039/C8CP00760H
- Microphysics of the aqueous bulk counters the water activity driven rate acceleration of bromide oxidation by ozone from 289–245 K J. Edebeli et al. https://doi.org/10.1039/C8EM00417J
- Elucidating the size distribution of p‑Phenylenediamine-Derived quinones in atmospheric particles K. Xia et al. https://doi.org/10.1016/j.envint.2025.109329
- The effect of viscosity and diffusion on the HO2 uptake by sucrose and secondary organic aerosol particles P. Lakey et al. https://doi.org/10.5194/acp-16-13035-2016
- Nitrate Photolysis in Mixed Sucrose–Nitrate–Sulfate Particles at Different Relative Humidities Z. Liang et al. https://doi.org/10.1021/acs.jpca.1c00669
- Imaging Molecular Reaction and Diffusion in Organic Aerosol Particles P. Alpert et al. https://doi.org/10.1017/S143192761801471X
- Secondary Organic Aerosol from Biomass Burning Phenolic Compounds and Nitrate Radicals can be Highly Viscous over a Wide Relative Humidity Range S. Nikkho et al. https://doi.org/10.1021/acs.est.4c06235
- Ozone uptake on glassy, semi-solid and liquid organic matter and the role of reactive oxygen intermediates in atmospheric aerosol chemistry T. Berkemeier et al. https://doi.org/10.1039/C6CP00634E
- Visualizing reaction and diffusion in xanthan gum aerosol particles exposed to ozone P. Alpert et al. https://doi.org/10.1039/C9CP03731D
- Phase Behavior and Viscosity in Biomass Burning Organic Aerosol and Climatic Impacts F. Gregson et al. https://doi.org/10.1021/acs.est.3c03231
- Photochemical degradation of iron(III) citrate/citric acid aerosol quantified with the combination of three complementary experimental techniques and a kinetic process model J. Dou et al. https://doi.org/10.5194/acp-21-315-2021
- Influence of particle viscosity on mass transfer and heterogeneous ozonolysis kinetics in aqueous–sucrose–maleic acid aerosol F. Marshall et al. https://doi.org/10.1039/C8CP01666F
- Ice nucleation imaged with X-ray spectro-microscopy P. Alpert et al. https://doi.org/10.1039/D1EA00077B
- Raman Spectroscopy of Isotopic Water Diffusion in Ultraviscous, Glassy, and Gel States in Aerosol by Use of Optical Tweezers J. Davies & K. Wilson https://doi.org/10.1021/acs.analchem.5b04315
- Viscosity and liquid–liquid phase separation in healthy and stressed plant SOA N. Smith et al. https://doi.org/10.1039/D0EA00020E
- Aerosol Hygroscopicity on A Single Particle Level Using Microscopic and Spectroscopic Techniques: A Review L. Wu & C. Ro https://doi.org/10.5572/ajae.2020.14.3.177
- Heterogeneous ozone oxidation of p-phenylenediamine antioxidants Z. Chen et al. https://doi.org/10.1016/j.jhazmat.2026.141745
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